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Sounak Mukherjee

Publications and source records attributed to Sounak Mukherjee.

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A defect in diamond with millisecond-scale spin relaxation time at room temperature

Spin defects in diamond are promising platforms for quantum sensing. The longest electron spin relaxation times ($T_1$) at room temperature for solid-state defects are observed in nitrogen vacancy centers in diamond, which can reach 6.67 ms, and substitutional nitrogen ("P1 centers") in diamond, which exhibit a $T_1$ of 2 ms. No other solid-state defect has exhibited millisecond-scale spin relaxation times at room temperature thus far. Here, we characterize the spin properties of the WAR5 defect in diamond with pulsed electron spin resonance. The observed $T_1$ is one of the longest for solid-state spin defects: 0.97(27) ms at room temperature and 14.38(19) min at 4 K. The observed coherence time ($T_2$) is 246(7) $μ$s, which can be extended to 6.49(34) ms at 4 K with dynamical decoupling. Furthermore, we demonstrate optical spin polarization with a range of wavelengths from 405 nm to 500 nm and propose potential zero-phonon line candidates.

cond-mat.mtrl-sci

Design and Fabrication of Robust Hybrid Photonic Crystal Cavities

Heterogeneously integrated hybrid photonic crystal cavities enable strong light-matter interactions with solid-state, optically addressable quantum memories. A key challenge to realizing high quality factor (Q) hybrid photonic crystals is the reduced index contrast on the substrate compared to suspended devices in air. This challenge is particularly acute for color centers in diamond because of diamond's high refractive index, which leads to increased scattering loss into the substrate. Here we develop a design methodology for hybrid photonic crystals utilizing a detailed understanding of substrate-mediated loss, which incorporates sensitivity to fabrication errors as a critical parameter. Using this methodology we design robust, high-Q, GaAs-on-diamond photonic crystal cavities, and by optimizing our fabrication procedure we experimentally realize cavities with Q approaching 30,000 at a resonance wavelength of 955 nm.

physics.optics

An instructional lab apparatus for quantum experiments with single nitrogen-vacancy centers in diamond

Hands-on experimental experience with quantum systems in the undergraduate physics curriculum provides students with a deeper understanding of quantum physics and equips them for the fast-growing quantum science industry. Here we present an experimental apparatus for performing quantum experiments with single nitrogen-vacancy (NV) centers in diamond. This apparatus is capable of basic experiments such as single-qubit initialization, rotation, and measurement, as well as more advanced experiments investigating electron-nuclear spin interactions. We describe the basic physics of the NV center and give examples of potential experiments that can be performed with this apparatus. We also discuss the options and inherent trade-offs associated with the choice of diamond samples and hardware. The apparatus described here enables students to write their own experimental control and data analysis software from scratch all within a single semester of a typical lab course, as well as to inspect the optical components and inner workings of the apparatus. We hope that this work can serve as a standalone resource for any institution that would like to integrate a quantum instructional lab into its undergraduate physics and engineering curriculum.

quant-ph

A telecom O-band emitter in diamond

Color centers in diamond are promising platforms for quantum technologies. Most color centers in diamond discovered thus far emit in the visible or near-infrared wavelength range, which are incompatible with long-distance fiber communication and unfavorable for imaging in biological tissues. Here, we report the experimental observation of a new color center that emits in the telecom O-band, which we observe in silicon-doped bulk single crystal diamonds and microdiamonds. Combining absorption and photoluminescence measurements, we identify a zero-phonon line at 1221 nm and phonon replicas separated by 42 meV. Using transient absorption spectroscopy, we measure an excited state lifetime of around 270 ps and observe a long-lived baseline that may arise from intersystem crossing to another spin manifold.

cond-mat.mtrl-sci

Single-shot measurement of space varying polarization state of light through interferometric quantification of geometric phase

Light beam carrying spatially varying state of polarization generates space varying Pancharatnam-Berry geometric phase while propagating through homogeneous anisotropic medium. We show that determination of such space varying geometric phase provides a unique way to quantify the space varying polarization state of light using a single-shot interferometric measurement. We demonstrate this concept in a Mach-Zehnder interferometric arrangement using a linearly polarized reference light beam, where full information on the spatially varying polarization state is successfully recovered by quantifying the space varying geometric phase and the contrast of interference. The proposed method enables single-shot measurement of any space varying polarization state of light from the measured interference pattern with a polarized reference beam. This approach shows considerable potential for instantaneous mapping of complex space varying polarization of light in diverse applications, such as astronomy, biomedical imaging, nanophotonics, etc., where high precision and near real-time measurement of spatial polarization patterns are desirable.

physics.optics