arXiv subjects

Srijit Bhattacharya

Publications and source records attributed to Srijit Bhattacharya.

At least 19 recordsLinked to original sources

arXiv2025

Unraveling the anomaly in the production of $^{60}$Fe nucleus in massive stars

The production of $^{60}$Fe is crucial for nucleosynthesis in massive stars and supernovae. In this work, by using the microscopic EP+IPM (exact pairing plus the independent-particle model) for the nuclear level density (NLD) and extended EP+PDM (exact pairing plus phonon damping model) for the $γ$-ray strength function (gSF), we re-evaluate the substantial enhancement of $^{60}$Fe production recently reported in {\it A. Spyrou et al., Nat. Comm. {\bf 15}, 9608 (2024)}, which was attributed to an unexpectedly large Maxwellian-averaged cross section (MACS). Our analysis demonstrates that this enhancement indeed originates from the choice of NLD, which, despite being constrained to reproduce the total NLD and gSF data, lacks a reliable spin dependence, a critical input for Hauser-Feshbach calculations of nuclear reaction rate. In contrast, our predictions yield a significantly lower MACS, calling the claimed enhancement into question. In particular, our approach highlights the microscopic nature of the low-energy enhancement of the gSF, the so-called upbend resonance, which arises from strong particle-particle ($pp$) and hole-hole ($hh$) excitations that emerge only at finite temperature, thereby further reinsisting on the invalidity of the Brink-Axel hypothesis in this low-energy region. Overall, our study reopens the question on the long-standing problem of $^{60}$Fe production in massive stars.

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arXiv2025

Analysis of (p,$γ$) capture cross-sections relevant to p-process using TALYS for A=75-110

The proton capture (p, $γ$) cross-sections for eight different atomic nuclei in the mass region A=75-110 were calculated within the nuclear reaction model code TALYS. For all the reactions, we tested different combinations of inputs for level density (l.d) parameter and gamma strength function ($γ_{sf}$). Finally, it was observed that application of hybrid input in TALYS (macroscopic l.d and microscopic or semi-microscopic $γ_{sf}$ or in abbreviation mac-mic) resulted successful agreement of theoretical prediction with the existing experimental data. Isospin correction was also incorporated in a few cases which improved the matching if the centre of mass energy reaches the threshold energy of the opening of (p,n) channel. The corresponding thermonuclear reaction rates were calculated for all the nuclei and some discrepancies were found with the prediction of the NON-SMOKER code. Using the particular mac-mic input combination, the cross-section and reaction rate for the nuclei $^{92}$Nb and $^{92}$Mo are calculated within TALYS. These two nuclei lack experimental data but are highly important for understanding early solar system processes. This is a rare attempt to explain the p-capture cross-section of different p-nuclei (A=75-110 range) with similar set of input combinations in TALYS, which may help to remove the uncertainty generated due to the variation of input parameters within nuclear statistical model code

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arXiv2024

Measurement of the Hoyle State Radiative Transition Width

The radiative decay of the Hoyle state is the doorway to the production of heavier elements in stellar environment. Here we report, an exclusive measurement of electric quadruple (E$_2$) transitions of the Hoyle state to the ground state of $^{12}$C through the $^{12}$C(p, p$^\prime$$γ$$γ$)$^{12}$C reaction. Triple coincidence measurement yields a value of radiative branching ratio $Γ_{rad}$/$Γ$ = 4.01 (30) $\times$ 10$^{-4}$. The result has been corroborated by an independent experiment based on the complete kinematical measurement $via.$ $^{12}$C(p, p$^\prime$)$^{12}$C reaction ($Γ_{rad}$/$Γ$ = 4.04 (30) $\times$ 10$^{-4}$). Using our results together with the currently adopted values of $Γ_π$(E$_0$)/$Γ$ and $Γ_π$($E_0$), the radiative width of the Hoyle state is found to be 3.75 (40) $\times$ 10$^{-3}$ eV. We emphasize here that our result is not in agreement with 34 $\%$ increase in the radiative decay width of the Hoyle state measured recently but consistent with the currently adopted value.

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arXiv2021

Enhanced symmetry energy bears universality of the r-process

The abundance of about half of the stable nuclei heavier than iron via the rapid neutron capture process or $r$-process is intimately related to the competition between neutron capture and $β$-decay rates, which ultimately depends on the binding energy of neutron-rich nuclei. The well-known Bethe-Weizsäcker semi-empirical mass formula\cite{weiz,bethe} describes the binding energy of ground states -- i.e. nuclei with temperatures of $T\approx0$ MeV -- with the symmetry energy parameter converging between $23-27$ MeV for heavy nuclei. Here we find an unexpected enhancement of the symmetry energy at higher temperatures, $T\approx0.7-1.0$ MeV, from the available data of giant dipole resonances built on excited states. Although these are likely the temperatures where seed elements are created -- during the cooling down of the ejecta following neutron-star mergers\cite{mergersnucleo} or collapsars\cite{collapsar} -- the fact that the symmetry energy remains constant between $T\approx0.7-1.0$ MeV, suggests a similar trend down to $T\approx0.5$ MeV, where neutron-capture may start occurring. Calculations using this relatively larger symmetry energy yield a reduction of the binding energy per nucleon for heavy neutron-rich nuclei and inhibits radiative neutron-capture rates. This results in a substantial close in of the neutron dripline -- where nuclei become unbound -- which elucidates the long sought universality of heavy-element abundances through the $r$-process; as inferred from the similar abundances found in extremely metal-poor stars and the Sun.

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arXiv2018

Experimental signature of collective enhancement in nuclear level density

We present a probable experimental signature of collective enhancement in the nuclear level density (NLD) by measuring the neutron and the giant dipole resonance (GDR) $γ$ rays emitted from the rare earth $^{169}$Tm compound nucleus populated at 26.1 MeV excitation energy. An enhanced yield is observed in both neutron and $γ$ ray spectra corresponding to the same excitation energy in the daughter nuclei. The enhancement could only be reproduced by including a collective enhancement factor in the Fermi gas model of NLD to explain the neutron and GDR spectra simultaneously. The experimental results show that the relative enhancement factor is of the order of 10 and the fadeout occurs at $\sim$ 14 MeV excitation energy, much before the commonly accepted transition from deformed to spherical shape. We also explain how the collective enhancement contribution changes the inverse level density parameter ($k$) from 8 to 9.5 MeV observed recently in several deformed nuclei.

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arXiv2017

Experimental Determination of $η$/$s$ for Finite Nuclear Matter

We present, for the first time, simultaneous determination of shear viscosity ($η$) and entropy density ($s$) and thus, $η/s$ for equilibrated nuclear systems from $A$ $\sim$ 30 to $A$ $\sim$ 208 at different temperatures. At finite temperature, $η$ is estimated by utilizing the $γ$ decay of the isovector giant dipole resonance populated via fusion evaporation reaction, while $s$ is evaluated from the nuclear level density parameter (${a}$) and nuclear temperature ($T$), determined precisely by the simultaneous measurements of the evaporated neutron energy spectra and the compound nuclear angular momenta. The transport parameter $η$ and the thermodynamic parameter $s$ both increase with temperature resulting in a mild decrease of $η$/$s$ with temperature. The extracted $η$/$s$ is also found to be independent of the neutron-proton asymmetry at a given temperature. Interestingly, the measured $η$/$s$ values are comparable to that of the high-temperature quark-gluon plasma, pointing towards the fact that strong fluidity may be the universal feature of the strong interaction of many-body quantum systems.

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arXiv2017

Signature of clustering in quantum many body systems probed by the giant dipole resonance

The present experimental study illustrates how large deformations attained by nuclei due to cluster formation are perceived through the giant dipole resonance (GDR) strength function. The high energy GDR $γ$-rays have been measured from $^{32}$S at different angular momenta ($J$) but similar temperatures in the reactions $^{4}$He(E$_{lab}$=45MeV) + $^{28}$Si and $^{20}$Ne(E$_{lab}$=145MeV) + $^{12}$C. The experimental data at lower J ($\sim$ 10$\hbar$) suggests a normal deformation, similar to the ground state value, showing no potential signature of clustering. However, it is found that the GDR lineshape is fragmented into two prominent peaks at high J ($\sim$ 20$\hbar$) providing a direct measurement of the large deformation developed in the nucleus. The observed lineshape is also completely different from the ones seen for Jacobi shape transition at high $J$ pointing towards the formation of cluster structure in super-deformed states of $^{32}$S at such high spin. Thus, the GDR can be regarded as a unique tool to study cluster formation at high excitation energies and angular momenta.

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arXiv2015

Experimental investigation on the temperature dependence of the nuclear level density parameter

The effect of temperature (T) and angular momentum (J) on the inverse level density parameter (k) has been studied by populating the compound nucleus $^{97}$Tc in the reaction $^{4}$He + $^{93}$Nb at four incident beam energies of 28, 35, 42 and 50 MeV. For all the four energies, the value of k decreases with increasing J. The T dependence of k has been compared for two angular momentum windows with different theoretical predictions as well as with FTBCS1 calculation which takes into account the quasiparticle-number fluctuations in the pairing field. Interestingly, the experimental data are in good agreement with the theoretical calculations at higher J but deviate from all the calculations at lower J.

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arXiv2014

Examination of level density prescriptions in the interpretation of high energy gamma-ray spectra

High energy $γ$-ray spectra measured by our group involving the compound nuclei (CN) $^{63}$Cu at excitation energy ($E^*$) $\sim$ 36 MeV with average angular momentum ($J$) = 12 - 17 $\hbar$, $^{97}$Tc at $E^* \sim$ 29 - 50 MeV with $J$ = 12 - 14 $\hbar$, $^{113}$Sb at $E^*$ = 109 MeV and 121 MeV with $J$ = 49 - 59 $\hbar$ and $^{201}$Tl at $E^*$ = 39.5, 47.5 MeV with $J$ = 18 - 24 $\hbar$ have been analyzed utilizing the level density prescriptions of (i)Ignatyuk, Smirenkin and Tishin (IST), (ii)Budtz-Jorgensen and Knitter (BJK), and (iii) Kataria, Ramamurthy and Kapoor (KRK). These three prescriptions have been tested for correct statistical model description of high energy $γ$-rays in the light of extracting the giant dipole resonance (GDR) parameters at low excitation energy and spin where shell effects might play an important role as well as at high excitation energy where shell effects have melted. Interestingly, only the IST level density prescription could explain the high energy $γ$-ray spectra with reasonable GDR parameters for all the four nuclei.

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arXiv2014

Probing the critical behavior in the evolution of GDR width at very low temperatures in A~100 mass region

The influence of giant dipole resonance (GDR) induced quadrupole moment on GDR width at low temperatures is investigated experimentally by measuring GDR width systematically in the unexplored temperature range $T$=0.8-1.5 MeV, for the first time, in $A$ $\sim$ 100 mass region. The measured GDR widths, using alpha induced fusion reaction, for $^{97}$Tc confirm that the GDR width remains constant at the ground state value up to a critical temperature and increases sharply thereafter with increase in $T$. The data have been compared with the adiabatic Thermal Shape Fluctuation Model (TSFM), phenomenological Critical Temperature Fluctuation Model (CTFM) and microscopic Phonon Damping Model (PDM). Interestingly, CTFM and PDM give similar results and agree with the data, whereas the TSFM differs significantly even after incorporating the shell effects.

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arXiv2013

Giant dipole resonance width and the universality of the Critical Temperature included Fluctuation Model

The universality of the Critical Temperature included Fluctuation Model (CTFM) in explaining the evolution of the giant dipole resonance (GDR) width as a function of angular momentum is examined in the light of recent experimental data on $^{144}$Sm and $^{152}$Gd. We compare both the data sets with the phenomenological formula based on the CTFM and the thermal shape fluctuation model (pTSFM). The CTFM describes both the data sets reasonably well using the actual ground state GDR width ($Γ_0$) values, whereas, the pTSFM describes the $^{144}$Sm data well but is unable to explain the $^{152}$Gd data using a single value of $Γ_0$ for two excitation energies. These interesting results clearly indicate that the phenomenological CTFM can be used universally to describe the evolution of the GDR width with both angular momentum and temperature in the entire mass region. Moreover, it should provide new insights into the modification of the TSFM.

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arXiv2013

Neutron response of the LAMBDA spectrometer and neutron interaction length in BaF2

We report on the neutron response of the LAMBDA spectrometer developed earlier for high-energy gamma-ray measurement. The energy dependent neutron detection efficiency of the spectrometer has been measured using the time-of-flight (TOF) technique and compared with that of an organic liquid scintillator based neutron detector (BC501A). The extracted efficiencies have also been compared with those obtained from Monte Carlo GEANT4 simulation. We have also measured the average interaction length of neutrons in the BaF2 crystal in a separate experiment, in order to determine the TOF energy resolution. Finally, the LAMBDA spectrometer has been tested in an in-beam-experiment by measuring neutron energy spectra in the 4He + 93Nb reaction to extract nuclear level density parameters. Nuclear level density parameters obtained by the LAMBDA spectrometer were found to be consistent with those obtained by the BC501A neutron detector, indicating that the spectrometer can be efficiently used as a neutron detector to measure the nuclear level density parameter.

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arXiv2013

Giant dipole resonance width as a probe for nuclear deformation at finite excitation

The systematic study of the correlation between the experimental giant dipole resonance (GDR) width and the average deformation <β> of the nucleus at finite excitation is presented for the mass region A ~ 59 to 208. We show that the width of the GDR (Γ) and the quadrupole deformation of the nucleus do not follow a linear relation, as predicted earlier, due to the GDR induced quadrupole moment and the correlation also depends on the mass of the nuclei. The different empirical values of <β> extracted from the experimental GDR width match exceptionally well with the thermal shape fluctuation model. As a result, this universal correlation between <β> and Γprovides a direct experimental probe to determine the nuclear deformation at finite temperature and angular momentum in the entire mass region.

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arXiv2012

Onset of deformation at $N = 112$ in Bi nuclei

The high spin states in $^{195}$Bi has been studied by $γ$-ray spectroscopic method using the $^{181}$Ta($^{20}$Ne, 6n) fusion evaporation reaction at 130 MeV. The $γγ$ coincidence data were taken using an array of 8 clover HPGe detectors. The spin and parity assignments of the excited states have been made from the measured directional correlation from oriented states (DCO) ratios and integrated polarization asymmetry (IPDCO) ratios. The results show, for the first time, the evidence of a rotational like band based on a 13/2$^+$ band head in this nucleus, indicating the onset of deformation at neutron number $N = 112$ for the Bismuth isotopes. The results obtained were found to be consistent with the prediction of the total Routhian surface calculations using Woods Saxon potential. The same calculations also predict a change in shape from oblate to triaxial in $^{195}$Bi at high rotational frequency.

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arXiv2011

Measurement of Giant Dipole Resonance width at low temperature: A new experimental perspective

The systematic evolution of the giant dipole resonance (GDR) width in the temperature region of 0.9 ~ 1.4 MeV has been measured experimentally for 119Sb using alpha induced fusion reaction and employing the LAMBDA high energy photon spectrometer. The temperatures have been precisely determined by simultaneously extracting the vital level density parameter from the neutron evaporation spectrum and the angular momentum from gamma multiplicity filter using a realistic approach. The systematic trend of the data seems to disagree with the thermal shape fluctuation model (TSFM). The model predicts the gradual increase of GDR width from its ground state value for T > 0 MeV whereas the measured GDR widths appear to remain constant at the ground state value till T ~ 1 MeV and increase thereafter indicating towards a failure of the adiabatic assumption of the model at low temperature.

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arXiv2010

A realistic technique for selection of angular momenta from hot nuclei: A case study with 4He + 115In \to 119Sb at E_Lab = 35 MeV

A rather new approach employing Monte Carlo GEANT simulation for converting the experimentally measured fold distribution to angular momentum distribution has been described. The technique has been successfully utilized to measure the angular momentum of the compound nucleus formed in the reaction 4He + 115In --> 119Sb at E_Lab = 35 MeV. A 50 element gamma multiplicity filter, fabricated in-house, was used to measure experimentally the required fold distribution. The present method has been compared with the other ones exiting in the literature and relative merits have been discussed.

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arXiv2010

Coherent bremsstrahlung and GDR width from 252Cf cold fission

The energy spectrum of the high energy gamma-rays in coincidence with the prompt gamma rays has been measured for the spontaneous fission of 252Cf. The nucleus-nucleus coherent bremsstrahlung of the accelerating fission fragments is observed and the result has been substantiated with a theoretical calculation based on the coulomb acceleration model. The width of the giant dipole resonance (GDR) decay from the excited fission fragments has been extracted for the first time and compared with the thermal shape fluctuation model (TSFM) in the liquid drop formalism. The extracted GDR width is significantly smaller than the predictions of TSFM.

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arXiv2010

Extreme nuclear shapes examined via Giant Dipole Resonance lineshapes in hot light mass system

The influence of alpha clustering on nuclear reaction dynamics is investigated using the giant dipole resonance (GDR) lineshape studies in the reactions 20Ne (Elab=145,160 MeV) + 12C and 20Ne (Elab=160 MeV) + 27Al, populating 32S and 47V, respectively. The GDR lineshapes from the two systems are remarkably different from each other. Whereas, the non alpha-like 47V undergoes Jacobi shape transition and matches exceptionally well with the theoretical GDR lineshape estimated under the framework rotating liquid drop model (RLDM) and thermal shape fluctuation model (TSFM) signifying shape equilibration, for alpha cluster 32S an extended prolate kind of shape is observed. This unusual deformation, seen directly via -decay for the first time, is predicted to be due to the formation of orbiting di-nuclear configuration or molecular structure of 16O+ 16O in 32S superdeformed band.

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