arXiv subjects

Srinivas Raghu

Publications and source records attributed to Srinivas Raghu.

At least 37 records · Page 2Linked to original sources

arXiv2022

Random singlet-like phase of disordered Hubbard chains

Local moment formation is ubiquitous in disordered semiconductors such as Si:P, where it is observed both in the metallic and the insulating regimes. Here, we focus on local moment behavior in disordered insulators, which arises from short-ranged, repulsive electron-electron interactions. Using density matrix renormalization group and strong-disorder renormalization group methods, we study paradigmatic models of interacting insulators: one dimensional Hubbard chains with quenched randomness. In chains with either random fermion hoppings or random chemical potentials, both at and away from half-filling, we find exponential decay of charge and fermion 2-point correlations but power-law decay of spin correlations that are indicative of the random singlet phase. The numerical results can be understood qualitatively by appealing to the large-interaction limit of the Hubbard chain, in which a remarkably simple picture emerges.

cond-mat.str-el↗

arXiv2022

Character of the "normal state" of the nickelate superconductors

The occurrence of superconductivity in proximity to various strongly correlated phases of matter has drawn extensive focus on their normal state properties, to develop an understanding of the state from which superconductivity emerges. The recent finding of superconductivity in layered nickelates raises similar interests. However, transport measurements of doped infinite-layer nickelate thin films have been hampered by materials limitations of these metastable compounds - in particular, a relatively high density of extended defects. Here, by moving to a substrate (LaAlO$_{3}$)$_{0.3}$(Sr$_{2}$TaAlO$_{6}$)$_{0.7}$ which better stabilizes the growth and reduction conditions, we can synthesize the doping series of Nd$_{1-x}$Sr$_{x}$NiO$_{2}$ essentially free from extended defects. This enables the first examination of the 'intrinsic' temperature and doping dependent evolution of the transport properties. The normal state resistivity exhibits a low-temperature upturn in the underdoped regime, linear behavior near optimal doping, and quadratic temperature dependence for overdoping. This is strikingly similar to the copper oxides, despite key distinctions - namely the absence of an insulating parent compound, multiband electronic structure, and a Mott-Hubbard orbital alignment rather than the charge-transfer insulator of the copper oxides. These results suggest an underlying universality in the emergent electronic properties of both superconducting families.

cond-mat.supr-con↗

arXiv2021

The Hubbard Model

The repulsive Hubbard model has been immensely useful in understanding strongly correlated electron systems, and serves as the paradigmatic model of the field. Despite its simplicity, it exhibits a strikingly rich phenomenology which is reminiscent of that observed in quantum materials. Nevertheless, much of its phase diagram remains controversial. Here, we review a subset of what is known about the Hubbard model, based on exact results or controlled approximate solutions in various limits, for which there is a suitable small parameter. Our primary focus is on the ground state properties of the system on various lattices in two spatial dimensions, although both lower and higher dimensions are discussed as well. Finally, we highlight some of the important outstanding open questions.

cond-mat.str-el↗

arXiv2021

Low-density superconductivity in SrTiO$_3$ bounded by the adiabatic criterion

SrTiO$_3$ exhibits superconductivity for carrier densities $10^{19}-10^{21}$ cm$^{-3}$. Across this range, the Fermi level traverses a number of vibrational modes in the system, making it ideal for studying dilute superconductivity. We use high-resolution planar-tunneling spectroscopy to probe chemically-doped SrTiO$_3$ across the superconducting dome. The over-doped superconducting boundary aligns, with surprising precision, to the Fermi energy crossing the Debye energy. Superconductivity emerges with decreasing density, maintaining throughout the Bardeen-Cooper-Schrieffer (BCS) gap to transition-temperature ratio, despite being in the anti-adiabatic regime. At lowest superconducting densities, the lone remaining adiabatic phonon van Hove singularity is the soft transverse-optic mode, associated with the ferroelectric instability. We suggest a scenario for pairing mediated by this mode in the presence of spin-orbit coupling, which naturally accounts for the superconducting dome and BCS ratio.

cond-mat.supr-con↗

arXiv2021

Universal behavior of the bosonic metallic ground state in a two-dimensional superconductor

Anomalous metallic behavior, marked by a saturating finite resistivity much lower than the Drude estimate, has been observed in a wide range of two-dimensional superconductors. Utilizing the electrostatically gated LaAlO3/SrTiO3 interface as a versatile platform for superconductor-metal quantum phase transitions, we probe variations in the gate, magnetic field, and temperature to construct a phase diagram crossing from superconductor, anomalous metal, vortex liquid, to Drude metal states, combining longitudinal and Hall resistivity measurements. We find that the anomalous metal phases induced by gating and magnetic field, although differing in symmetry, are connected in the phase diagram and exhibit similar magnetic field response approaching zero temperature. Namely, within a finite regime of the anomalous metal state, the longitudinal resistivity linearly depends on field while the Hall resistivity diminishes, indicating an emergent particle-hole symmetry. The universal behavior highlights the uniqueness of the quantum bosonic metallic state, distinct from bosonic insulators and vortex liquids.

cond-mat.supr-con↗

arXiv2020

Robust $d_{x^2-y^2}$-wave superconductivity of infinite-layer nickelates

Motivated by the recent observation of superconductivity in strontium doped NdNiO$_2$, we study the superconducting instabilities in this system from various vantage points. Starting with first-principles calculations, we construct two distinct tight-binding models, a simpler single-orbital as well as a three-orbital model, both of which capture the key low energy degrees of freedom to varying degree of accuracy. We study superconductivity in both models using the random phase approximation (RPA). We then analyze the problem at stronger coupling, and study the dominant pairing instability in the associated t-J model limit. In all instances, the dominant pairing tendency is in the $d_{x^2-y^2}$ channel, analogous to the cuprate superconductors.

cond-mat.supr-con↗

arXiv2019

Two dimensional non-Fermi liquid metals: a solvable large N limit

Significant effort has been devoted to the study of "non-Fermi liquid" (NFL) metals: gapless conducting systems that lack a quasiparticle description. One class of NFL metals involves a finite density of fermions interacting with soft order parameter fluctuations near a quantum critical point. The problem has been extensively studied in a large N limit (N corresponding to the number of fermion flavors) where universal behavior can be obtained by solving a set of coupled saddle-point equations. However a remarkable study by S.-S.~Lee revealed the breakdown of such approximations in two spatial dimensions. We show that an alternate approach, in which the fermions belong to the fundamental representation of a global SU(N) flavor symmetry, while the order parameter fields transform under the adjoint representation (a "matrix large N" theory), yields a tractable large N limit. At low energies, the system consists of an overdamped boson with dynamical exponent $z=3$ coupled to a non-Fermi liquid with self energy $Σ(ω) \sim ω^{2/3}$, consistent with previous studies.

cond-mat.str-el↗

arXiv2018

Composite fermion Hall conductivity and the half-filled Landau level

We consider the Hall conductivity of composite fermions in the theory of Halperin, Lee, and Read (HLR). We present a fully quantum mechanical numerical calculation that shows, under suitable conditions, the HLR theory exhibits a particle-hole symmetric dc electrical Hall response in the presence of quenched disorder. Remarkably, this response of the HLR theory remains robust even when the disorder range is of the order of the Fermi wavelength. We find that deviations from particle-hole symmetric response can appear in the ac Hall conductivity at frequencies sufficiently large compared to the inverse system size. Our results agree with a recent semi-classical analysis by Wang et al., Phys. Rev. X 7, 031029 (2017) and complement the arguments based on the fully quantum-mechanical model by Kumar et al., Phys. Rev. B 98, 11505 (2018). These results provide further evidence that the HLR theory is compatible with an emergent particle-hole symmetry.

cond-mat.str-el↗

arXiv2018

The density and disorder tuned superconductor-metal transition in two dimensions

Quantum ground states which arise at atomically controlled oxide interfaces provide an opportunity to address key questions in condensed matter physics, including the nature of two-dimensional (2D) metallic behaviour often observed adjacent to superconductivity. At the superconducting LaAlO3/SrTiO3 interface, a metallic ground state emerges upon the collapse of superconductivity with field-effect gating. Strikingly, such metallicity is accompanied with a pseudogap. Here, we utilize independent control of carrier density and disorder of the interfacial superconductor using dual electrostatic gates, which enables the comprehensive examination of the electronic phase diagram approaching zero temperature. We find that the pseudogap corresponds to precursor pairing, and the onset of long-range phase coherence forms a 2D superconducting dome as a function of the dual gate voltages. The gate-tuned superconductor-metal transitions are driven by macroscopic phase fluctuations of Josephson coupled superconducting puddles.

cond-mat.supr-con↗

arXiv2018

Superconducting tunneling spectroscopy of spin-orbit coupling and orbital depairing in Nb:SrTiO$_3$

We have examined the intrinsic spin-orbit coupling (SOC) and orbital depairing in thin films of Nb-doped SrTiO$_3$ by superconducting tunneling spectroscopy. The orbital depairing is geometrically suppressed in the two-dimensional limit, enabling a quantitative evaluation of the Fermi level spin-orbit scattering using Maki's theory. The response of the superconducting gap under in-plane magnetic fields demonstrates short spin-orbit scattering times $τ_{so} \leq 1.1$ ps. Analysis of the orbital depairing indicates that the heavy electron band contributes significantly to pairing. These results suggest that the intrinsic spin-orbit scattering time in SrTiO$_3$ is comparable to those associated with Rashba effects in SrTiO$_3$ interfacial conducting layers and can be considered significant in all forms of superconductivity in SrTiO$_3$.

cond-mat.supr-con↗

arXiv2017

Polaronic behavior in a weak coupling superconductor

The nature of superconductivity in the dilute semiconductor SrTiO$_3$ has remained an open question for more than 50 years. The extremely low carrier densities ($10^{18}$ - $10^{20}$ cm$^{-3}$) at which superconductivity occurs suggests an unconventional origin of superconductivity outside of the adiabatic limit on which the Bardeen-Cooper-Schrieffer (BCS) and Migdal-Eliashberg (ME) theories are based. We take advantage of a newly developed method for engineering band alignments at oxide interfaces and access the electronic structure of Nb-doped SrTiO$_3$ using high resolution tunneling spectroscopy. We observe strong coupling to the highest energy longitudinal optic (LO) phonon branch and estimate the doping evolution of the dimensionless electron-phonon interaction strength ($λ$). Upon cooling below the superconducting transition temperature ($T_{\mathrm{c}}$), we observe a single superconducting gap corresponding to the weak-coupling limit of BCS theory, indicating an order of magnitude smaller coupling ($λ_{\textrm{BCS}} \approx 0.1$). These results suggest that despite the strong normal state interaction with electrons, the highest LO phonon does not provide a dominant contribution to pairing. They further demonstrate that SrTiO$_3$ is an ideal system to probe superconductivity over a wide range of carrier density, adiabatic parameter, and electron-phonon coupling strength.

cond-mat.supr-con↗

arXiv2017

Two dimensional metallic phases from disordered QED$_3$

Metallic phases have been observed in several disordered two dimensional (2d) systems, including thin films near superconductor-insulator transitions and quantum Hall systems near plateau transitions. The existence of 2d metallic phases at zero temperature generally requires an interplay of disorder and interaction effects. Consequently, experimental observations of 2d metallic behavior have largely defied explanation. We formulate a general stability criterion for strongly interacting, massless Dirac fermions against disorder, which describe metallic ground states with vanishing density of states. We show that (2+1)-dimensional quantum electrodynamics (QED$_3$) with a large, even number of fermion flavors remains metallic in the presence of weak scalar potential disorder due to the dynamic screening of disorder by gauge fluctuations. We also show that QED$_3$ with weak mass disorder exhibits a stable, dirty metallic phase in which both interactions and disorder play important roles.

cond-mat.str-el↗

arXiv2016

Non-Fermi liquid Superconductivity: Eliashberg versus the Renormalization Group

We address the problem of superconductivity for non-Fermi liquids using two commonly adopted, yet apparently distinct methods: 1) the renormalization group (RG) and 2) Eliashberg theory. The extent to which both methods yield consistent solutions for the low energy behavior of quantum metals has remained unclear. We show that the perturbative RG beta function for the 4-Fermi coupling can be explicitly derived from the linearized Eliashberg equations, under the assumption that quantum corrections are approximately local across energy scales. We apply our analysis to the test case of phonon mediated superconductivity and show the consistency of both the Eliashberg and RG treatments. We next study superconductivity near a class of quantum critical points and find a transition between superconductivity and a "naked" metallic quantum critical point with finite, critical BCS couplings. We speculate on the applications of our theory to the phenomenology of unconventional metals.

cond-mat.str-el↗

arXiv2015

Band-structure effects on superconductivity in Hubbard models

We study the influence of the band structure on the symmetry and superconducting transition temperature in the (solvable) weak-coupling limit of the repulsive Hubbard model. Among other results we find: 1) As a function of increasing nematicity, starting from the square lattice (zero nematicity) limit where nodal d-wave state is strongly preferred, there is a smooth evolution to the quasi-1D limit, where a striking near-degeneracy is found between a p-wave- and a d-wave-type paired states with accidental nodes on the quasi-one-dimensional Fermi surfaces---a situation which may be relevant to the Bechgaard salts. 2) In a bilayer system, we find a phase transition as a function of increasing bilayer coupling from a d-wave to an $s_{\pm}$-wave state reminiscent of the iron-based superconductors. 3) When an antinodal gap is produced by charge-density-wave order, not only is the pairing scale reduced, but the symmetry of the pairs switches from $d_{x^2-y^2} to $d_{xy}$; in the context of the cuprates, this suggests that were the pseudo-gap entirely due to a competing order, this would likely cause a corresponding symmetry change of the superconducting order (which is not seen in experiment).

cond-mat.supr-con↗

arXiv2015

Metallic quantum critical points with finite BCS couplings

We study the fate of superconductivity in the vicinity of a class of metallic quantum critical points obtained by coupling a Fermi surface to a critical boson. In such systems there is a competition between the enhanced pairing tendency due to the presence of long-range attractive interactions near criticality, and the suppression of superconductivity due to the destruction of the Landau quasiparticles. We show that there are regimes in which these two effects offset one another, resulting in a novel non-Fermi liquid fixed point with finite, scale invariant, BCS coupling. While these interactions lead to substantial superconducting fluctuations, they do not drive the system into a superconducting ground state. The metallic quantum critical fixed points are connected to the superconducting regime by a continuous phase transition. These results are established using a controlled expansion in the deviation from d=3 spatial dimensions, as well as in a large number N of internal flavors. We discuss the possible relevance of our findings to the phenomenon of superconducting domes condensing out of a non-Fermi liquid normal state near quantum critical points.

cond-mat.str-el↗

arXiv2014

Suppression of spontaneous currents in Sr$_2$RuO$_4$ by surface disorder

A major challenge to the chiral $p$-wave hypothesis for the pairing symmetry of the unconventional superconductor Sr$_2$RuO$_4$ is the null result of sensitive scanning magnetometry experiments designed to detect the expected spontaneous charge currents. Motivated by junction tunneling conductance measurements which indicate the quenching of superconductivity at the surfaces of even high-purity samples, we examine the spontaneous currents in a chiral $p$-wave superconductor near a normal metal / superconductor interface using the lattice Bogoliubov-de Gennes equations and Ginzburg-Landau theory, and find that the edge current is suppressed by more than an order of magnitude compared to previous estimates. These calculations demonstrate that interface details can have a quantitatively meaningful effect on the expectations for magnetometry experiments.

cond-mat.supr-con↗

arXiv2013

Tunable Coupling of Two-Dimensional Superconductors in Bilayer SrTiO3 Heterostructures

Interlayer coupling effects between high mobility two-dimensional superconductors are studied in bilayer delta-doped SrTiO3 heterostructures. By tuning the undoped SrTiO3 spacer layer between the dopant planes, clear tunable coupling is demonstrated in the variation of the sheet carrier density, Hall mobility, superconducting transition temperature, and the temperature- and angle-dependences of the superconducting upper critical field. Systematic variation is found between one effective (merged) two-dimensional superconductor to two decoupled two-dimensional superconductors. In the intermediate coupled regime, a crossover is observed due to coupling arising from inter-sub-band interactions.

cond-mat.supr-con↗

arXiv2013

Spin-Orbit Coupling in LaAlO$_3$/SrTiO$_3$ interfaces: Magnetism and Orbital Ordering

The combination of Rashba spin-orbit coupling and electron correlations can induce unusual phenomena in the metallic interface between SrTiO$_3$ and LaAlO$_3$. We consider effects of Rashba spin-orbit coupling at this interface in the context of the recent observation of anisotropic magnetism. Firstly, we show how Rashba spin-orbit coupling in a system near a band-edge can account for the observed magnetic anisotropy. Secondly, we investigate the coupling between in-plane magnetic-moment anisotropy and nematicity in the form of an orbital imbalance between d$_{xz}$ / d$_{yz}$ orbitals. We estimate this coupling to be substantial in the low electron density regime. Such an orbital ordering can affect magneto transport.

cond-mat.str-el↗