arXiv subjects

Srujan Meesala

Publications and source records attributed to Srujan Meesala.

At least 19 recordsLinked to original sources

arXiv2025

Purcell-enhanced spin-phonon coupling with a single color center

The radiative properties of atoms are inherently linked to their surrounding environment. Placing an electromagnetic resonator around atoms can enhance spontaneous emission, as shown by Purcell in the 1940s. This approach is now routinely used in quantum computing and communication to channel photons emitted by atoms into well-defined modes and control atom-photon interactions. For solid-state artificial atoms, such as color-centers, the host lattice introduces an acoustic environment, allowing excited atoms to relax by emitting phonons. Here we observe the acoustic Purcell effect by constructing a specially engineered, microwave-frequency nanomechanical resonator around a color-center spin qubit in diamond. Using a co-localized optical mode of the structure that strongly couples to the color-center's excited state, we perform single-photon-level laser spectroscopy at milliKelvin temperatures and observe ten-fold faster spin relaxation when the spin qubit is tuned into resonance with a 12 GHz acoustic mode. Additionally, we use the color-center as an atomic-scale probe to measure the broadband phonon spectrum of the nanostructure up to a frequency of 28 GHz. Our work establishes a new regime of control for quantum defects in solids and paves the way for interconnects between atomic-scale quantum memories and qubits encoded in acoustic and superconducting devices.

quant-ph↗

arXiv2024

Microwave-Optical Entanglement from Pulse-pumped Electro-optomechanics

Entangling microwave and optical photons is one of the promising ways to realize quantum transduction through quantum teleportation. This paper investigates the entanglement of microwave-optical photon pairs generated from an electro-optomechanical system driven by a blue-detuned pulsed Gaussian pump. The photon pairs are obtained through weak parametric-down-conversion, and their temporal correlation is revealed by the second-order correlation function. We then study the discrete variable entanglement encoded in the time bin degree of freedom, where entanglement is identified by Bell inequality violation. Furthermore, we estimate the laser-induced heating and show that the pulse-pumped system features lower heating effects while maintaining a reasonable coincidence photon counting rate.

quant-ph↗

arXiv2024

High-Efficiency Low-Noise Optomechanical Crystal Photon-Phonon Transducers

Optomechanical crystals (OMCs) enable coherent interactions between optical photons and microwave acoustic phonons, and represent a platform for implementing quantum transduction between microwave and optical signals. Optical absorption-induced thermal noise at cryogenic (millikelvin) temperatures is one of the primary limitations of performance for OMC-based quantum transducers. Here, we address this challenge with a two-dimensional silicon OMC resonator that is side-coupled to a mechanically detached optical waveguide, realizing a six-fold reduction in the heating rate of the acoustic resonator compared to prior state-of-the-art, while operating in a regime of high optomechanical-backaction and millikelvin base temperature. This reduced heating translates into a demonstrated phonon-to-photon conversion efficiency of 93.1 $\pm$ 0.8% at an added noise of 0.25 $\pm$ 0.01 quanta, representing a significant advance toward quantum-limited microwave-optical frequency conversion and optically-controlled quantum acoustic memories.

physics.optics↗

arXiv2024

Acceptor-induced bulk dielectric loss in superconducting circuits on silicon

The performance of superconducting quantum circuits is primarily limited by dielectric loss due to interactions with two-level systems (TLS). State-of-the-art circuits with engineered material interfaces are approaching a limit where dielectric loss from bulk substrates plays an important role. However, a microscopic understanding of dielectric loss in crystalline substrates is still lacking. In this work, we show that boron acceptors in silicon constitute a strongly coupled TLS bath for superconducting circuits. We discuss how the electronic structure of boron acceptors leads to an effective TLS response in silicon. We sweep the boron concentration in silicon and demonstrate the bulk dielectric loss limit from boron acceptors. We show that boron-induced dielectric loss can be reduced in a magnetic field due to the spin-orbit structure of boron. This work provides the first detailed microscopic description of a TLS bath for superconducting circuits, and demonstrates the need for ultrahigh purity substrates for next-generation superconducting quantum processors.

quant-ph↗

arXiv2023

Quantum entanglement between optical and microwave photonic qubits

Entanglement is an extraordinary feature of quantum mechanics. Sources of entangled optical photons were essential to test the foundations of quantum physics through violations of Bell's inequalities. More recently, entangled many-body states have been realized via strong non-linear interactions in microwave circuits with superconducting qubits. Here we demonstrate a chip-scale source of entangled optical and microwave photonic qubits. Our device platform integrates a piezo-optomechanical transducer with a superconducting resonator which is robust under optical illumination. We drive a photon-pair generation process and employ a dual-rail encoding intrinsic to our system to prepare entangled states of microwave and optical photons. We place a lower bound on the fidelity of the entangled state by measuring microwave and optical photons in two orthogonal bases. This entanglement source can directly interface telecom wavelength time-bin qubits and GHz frequency superconducting qubits, two well-established platforms for quantum communication and computation, respectively.

quant-ph↗

arXiv2023

In-situ tuning of optomechanical crystals with nano-oxidation

Optomechanical crystals are a promising device platform for quantum transduction and sensing. Precise targeting of the optical and acoustic resonance frequencies of these devices is crucial for future advances on these fronts. However, fabrication disorder in these wavelength-scale nanoscale devices typically leads to inhomogeneous resonance frequencies. Here we achieve in-situ, selective frequency tuning of optical and acoustic resonances in silicon optomechanical crystals via electric field-induced nano-oxidation using an atomic-force microscope. Our method can achieve a tuning range >2 nm (0.13%) for the optical resonance wavelength in the telecom C-band, and >60 MHz (1.2%) for the acoustic resonance frequency at 5 GHz. The tuning resolution of 1.1 nm for the optical wavelength, and $150$ kHz for the acoustic frequency allows us to spectrally align multiple optomechanical crystal resonators using optimal oxidation patterns determined via an inverse design protocol. Our results establish a method for precise post-fabrication tuning of optomechancical crystals. This technique can enable coupled optomechanical resonator arrays, scalable resonant optomechanical circuits, and frequency matching of microwave-optical quantum transducers.

physics.optics↗

arXiv2023

High Q-factor diamond optomechanical resonators with silicon vacancy centers at millikelvin temperatures

Phonons are envisioned as coherent intermediaries between different types of quantum systems. Engineered nanoscale devices such as optomechanical crystals (OMCs) provide a platform to utilize phonons as quantum information carriers. Here we demonstrate OMCs in diamond designed for strong interactions between phonons and a silicon vacancy (SiV) spin. Using optical measurements at millikelvin temperatures, we measure a linewidth of 13 kHz (Q-factor of ~440,000) for 6 GHz acoustic modes, a record for diamond in the GHz frequency range and within an order of magnitude of state-of-the-art linewidths for OMCs in silicon. We investigate SiV optical and spin properties in these devices and outline a path towards a coherent spin-phonon interface.

physics.optics↗

arXiv2023

Design of an ultra-low mode volume piezo-optomechanical quantum transducer

Coherent transduction of quantum states from the microwave to the optical domain can play a key role in quantum networking and distributed quantum computing. We present the design of a piezo-optomechanical device formed in a hybrid lithium niobate on silicon platform, that is suitable for microwave-to-optical quantum transduction. Our design is based on acoustic hybridization of an ultra-low mode volume piezoacoustic cavity with an optomechanical crystal cavity. The strong piezoelectric nature of lithium niobate allows us to mediate transduction via an acoustic mode which only minimally interacts with the lithium niobate, and is predominantly silicon-like, with very low electrical and acoustic loss. We estimate that this transducer can realize an intrinsic conversion efficiency of up to 35% with <0.5 added noise quanta when resonantly coupled to a superconducting transmon qubit and operated in pulsed mode at 10 kHz repetition rate. The performance improvement gained in such hybrid lithium niobate-silicon transducers make them suitable for heralded entanglement of qubits between superconducting quantum processors connected by optical fiber links.

quant-ph↗

arXiv2023

Non-classical microwave-optical photon pair generation with a chip-scale transducer

Modern computing and communication technologies such as supercomputers and the internet are based on optically connected networks of microwave frequency information processors. In recent years, an analogous architecture has emerged for quantum networks with optically distributed entanglement between remote superconducting quantum processors, a leading platform for quantum computing. Here we report an important milestone towards such networks by observing non-classical correlations between photons in an optical link and a superconducting electrical circuit. We generate such states of light through a spontaneous parametric down-conversion (SPDC) process in a chip-scale piezo-optomechanical transducer. The non-classical nature of the emitted light is verified by observing anti-bunching in the microwave state conditioned on detection of an optical photon. Such a transducer can be readily connected to a superconducting quantum processor, and serve as a key building block for optical quantum networks of microwave frequency qubits.

quant-ph↗

arXiv2020

Magnetic Field Fingerprinting of Integrated Circuit Activity with a Quantum Diamond Microscope

Current density distributions in active integrated circuits (ICs) result in patterns of magnetic fields that contain structural and functional information about the IC. Magnetic fields pass through standard materials used by the semiconductor industry and provide a powerful means to fingerprint IC activity for security and failure analysis applications. Here, we demonstrate high spatial resolution, wide field-of-view, vector magnetic field imaging of static (DC) magnetic field emanations from an IC in different active states using a Quantum Diamond Microscope (QDM). The QDM employs a dense layer of fluorescent nitrogen-vacancy (NV) quantum defects near the surface of a transparent diamond substrate placed on the IC to image magnetic fields. We show that QDM imaging achieves simultaneous $\sim10$ $μ$m resolution of all three vector magnetic field components over the 3.7 mm $\times$ 3.7 mm field-of-view of the diamond. We study activity arising from spatially-dependent current flow in both intact and decapsulated field-programmable gate arrays (FPGAs); and find that QDM images can determine pre-programmed IC active states with high fidelity using machine-learning classification methods.

quant-ph↗

arXiv2019

Coherent Acoustic Control of a Single Silicon Vacancy Spin in Diamond

Phonons are considered to be universal quantum transducers due to their ability to couple to a wide variety of quantum systems. Among these systems, solid-state point defect spins are known for being long-lived optically accessible quantum memories. Recently, it has been shown that inversion-symmetric defects in diamond, such as the negatively charged silicon vacancy center (SiV), feature spin qubits that are highly susceptible to strain. Here, we leverage this strain response to achieve coherent and low-power acoustic control of a single SiV spin, and perform acoustically driven Ramsey interferometry of a single spin. Our results demonstrate a novel and efficient method of spin control for these systems, offering a path towards strong spin-phonon coupling and phonon-mediated hybrid quantum systems.

quant-ph↗

arXiv2019

Quantum interference of electromechanically stabilized emitters in nanophotonic devices

Photon-mediated coupling between distant matter qubits may enable secure communication over long distances, the implementation of distributed quantum computing schemes, and the exploration of new regimes of many-body quantum dynamics. Nanophotonic devices coupled to solid-state quantum emitters represent a promising approach towards realization of these goals, as they combine strong light-matter interaction and high photon collection efficiencies. However, the scalability of these approaches is limited by the frequency mismatch between solid-state emitters and the instability of their optical transitions. Here we present a nano-electromechanical platform for stabilization and tuning of optical transitions of silicon-vacancy (SiV) color centers in diamond nanophotonic devices by dynamically controlling their strain environments. This strain-based tuning scheme has sufficient range and bandwidth to alleviate the spectral mismatch between individual SiV centers. Using strain, we ensure overlap between color center optical transitions and observe an entangled superradiant state by measuring correlations of photons collected from the diamond waveguide. This platform for tuning spectrally stable color centers in nanophotonic waveguides and resonators constitutes an important step towards a scalable quantum network.

physics.app-ph↗

arXiv2018

Spectral alignment of single-photon emitters in diamond using strain gradient

Solid-state single-photon emitters are attractive for realization of integrated quantum systems due to their experimental convenience and scalability. Unfortunately, however, their complex mesoscopic environments cause photons from different emitters to be spectrally distinguishable. Here we demonstrate spectral alignment of two solid-state single-photon emitters by utilizing the strain gradient. Multiple germanium vacancy (GeV) color centers in diamond are created in fabricated diamond microcantilevers using focused ion beam implantation. The strain response of the electronic energy levels of the GeV is measured by inducing an electrically controlled strain in the device. Leveraging the large strain gradient, we tune two GeVs in the spot to emit at the same optical wavelength. Simultaneous resonant excitation of two spectrally aligned GeVs is demonstrated using a narrow linewidth laser. This strain gradient tuning can be used to realize spectrally identical quantum emitters for on-chip integrated quantum systems.

cond-mat.mes-hall↗

arXiv2018

Controlling the coherence of a diamond spin qubit through strain engineering

The uncontrolled interaction of a quantum system with its environment is detrimental for quantum coherence. In the context of solid-state qubits, techniques to mitigate the impact of fluctuating electric and magnetic fields from the environment are well-developed. In contrast, suppression of decoherence from thermal lattice vibrations is typically achieved only by lowering the temperature of operation. Here, we use a nano-electro-mechanical system (NEMS) to mitigate the effect of thermal phonons on a solid-state quantum emitter without changing the system temperature. We study the silicon-vacancy (SiV) colour centre in diamond which has optical and spin transitions that are highly sensitive to phonons. First, we show that its electronic orbitals are highly susceptible to local strain, leading to its high sensitivity to phonons. By controlling the strain environment, we manipulate the electronic levels of the emitter to probe, control, and eventually, suppress its interaction with the thermal phonon bath. Strain control allows for both an impressive range of optical tunability and significantly improved spin coherence. Finally, our findings indicate that it may be possible to achieve strong coupling between the SiV spin and single phonons, which can lead to the realisation of phonon-mediated quantum gates and nonlinear quantum phononics.

quant-ph↗

arXiv2018

Strain engineering of the silicon-vacancy center in diamond

We control the electronic structure of the silicon-vacancy (SiV) color-center in diamond by changing its static strain environment with a nano-electro-mechanical system. This allows deterministic and local tuning of SiV optical and spin transition frequencies over a wide range, an essential step towards multi-qubit networks. In the process, we infer the strain Hamiltonian of the SiV revealing large strain susceptibilities of order 1 PHz/strain for the electronic orbital states. We identify regimes where the spin-orbit interaction results in a large strain suseptibility of order 100 THz/strain for spin transitions, and propose an experiment where the SiV spin is strongly coupled to a nanomechanical resonator.

quant-ph↗

arXiv2017

A fiber-coupled diamond quantum nanophotonic interface

Color centers in diamond provide a promising platform for quantum optics in the solid state, with coherent optical transitions and long-lived electron and nuclear spins. Building upon recent demonstrations of nanophotonic waveguides and optical cavities in single-crystal diamond, we now demonstrate on-chip diamond nanophotonics with a high efficiency fiber-optical interface, achieving > 90% power coupling at visible wavelengths. We use this approach to demonstrate a bright source of narrowband single photons, based on a silicon-vacancy color center embedded within a waveguide-coupled diamond photonic crystal cavity. Our fiber-coupled diamond quantum nanophotonic interface results in a high flux of coherent single photons into a single mode fiber, enabling new possibilities for realizing quantum networks that interface multiple emitters, both on-chip and separated by long distances.

cond-mat.mes-hall↗

arXiv2016

Diamond optomechanical crystals

Cavity-optomechanical systems realized in single-crystal diamond are poised to benefit from its extraordinary material properties, including low mechanical dissipation and a wide optical transparency window. Diamond is also rich in optically active defects, such as the nitrogen-vacancy (NV) and silicon-vacancy (SiV) centers, which behave as atom-like systems in the solid state. Predictions and observations of coherent coupling of the NV electronic spin to phonons via lattice strain has motivated the development of diamond nanomechanical devices aimed at realization of hybrid quantum systems, in which phonons provide an interface with diamond spins. In this work, we demonstrate diamond optomechanical crystals (OMCs), a device platform to enable such applications, wherein the co-localization of ~ 200 THz photons and few to 10 GHz phonons in a quasi-periodic diamond nanostructure leads to coupling of an optical cavity field to a mechanical mode via radiation pressure. In contrast to other material systems, diamond OMCs operating in the resolved-sideband regime possess large intracavity photon capacity (> 10$^5$) and sufficient optomechanical coupling rates to reach a cooperativity of ~ 20 at room temperature, allowing for the observation of optomechanically induced transparency and the realization of large amplitude optomechanical self-oscillations.

cond-mat.mes-hall↗

arXiv2015

Enhanced strain coupling of nitrogen vacancy spins to nanoscale diamond cantilevers

Nitrogen vacancy (NV) centers can couple to confined phonons in diamond mechanical resonators via the effect of lattice strain on their energy levels. Access to the strong spin-phonon coupling regime with this system requires resonators with nanoscale dimensions in order to overcome the weak strain response of the NV ground state spin sublevels. In this work, we study NVs in diamond cantilevers with lateral dimensions of a few hundred nm. Coupling of the NV ground state spin to the mechanical mode is detected in electron spin resonance (ESR), and its temporal dynamics are measured via spin echo. Our small mechanical mode volume leads to a 10-100X enhancement in spin-phonon coupling strength over previous NV-strain coupling demonstrations. This is an important step towards strong spin-phonon coupling, which can enable phonon-mediated quantum information processing and quantum metrology.

quant-ph↗