arXiv subjects

Stéphane Auffret

Publications and source records attributed to Stéphane Auffret.

At least 19 recordsLinked to original sources

arXiv2025

Dzyaloshinskii-Moriya interaction chirality reversal with ferromagnetic thickness

In ultrathin ferromagnetic films sandwiched between two distinct heavy metal layers or between a heavy metal and an oxide layer, the Dzyaloshinskii-Moriya interaction (DMI) is of interfacial origin. Its chirality and strength are determined by the properties of the adjacent heavy metals and the degree of oxidation at the interfaces. Here, we demonstrate that the DMI chirality can change solely with variations in the thickness of the ferromagnetic layer - an effect that has not been experimentally studied in details or explained until now. Our experimental observation in the trilayer system Ta/FeCoB/TaOx is supported by ab initio calculations: they reveal that variations in orbital filling and inter-atomic distances at the interface, driven by the structural relaxations in the ultrathin regime, lead to an inversion of DMI chirality. We hence propose a new degree of freedom to tune DMI chirality and the associated chiral spin textures by tailoring crystal structure e.g. using strain or surface acoustic waves.

cond-mat.mtrl-sci↗

arXiv2025

Low-Noise Nanoscale Vortex Sensor for Out-of-Plane Magnetic Field Detection

This study investigates a vortex sensor based on a nanoscale (sub-100 nm) magnetic tunnel junction (MTJ) with a strong shape anisotropy, designed for sensitivity to the out-of-plane magnetic field component ($H_z$). The sensor comprises a free layer with a vortex configuration and a perpendicularly magnetized reference layer, which provides a reproducible and linear response when excited by a perpendicular magnetic field. Experimental measurements and micromagnetic simulations were combined to systematically assess the influence of structural parameters, specifically aspect ratio and defect landscape, on key sensor performance metrics, including dynamic range, sensitivity, and detectivity. The out-of-plane vortex sensor demonstrates a significantly improved dynamic range exceeding 200 mT, compared to the 40-80 mT typical of conventional in-plane vortex sensors. Frequency-dependent noise measurements reveal that the sensor exhibits low intrinsic noise, along with improved detectivity and resolution. This performance is ascribed to the field-dependent expansion and contraction of the vortex core, which reduces Barkhausen-type noise caused by defect-induced pinning potentials. Moreover, the sub-100\,nm lateral dimensions of the sensor enable scalable array integration, providing further enhancements in noise and detectivity through collective averaging. These results underscore the potential of this sensor architecture for advanced magnetic field sensing applications requiring a wide dynamic range and high measurement accuracy at the same time.

cond-mat.mes-hall↗

arXiv2025

Entropy-Assisted Nanosecond stochastic operation in perpendicular superparamagnetic tunnel junctions

We demonstrate a good agreement between mean dwell times measured in 50~nm diameter, perpendicularly magnetized superparamagnetic tunnel junctions (SMTJ), and theoretical predictions based on Langer's theory. Due to a large entropic contribution, the theory yields Arrhenius prefactors in the femtosecond range for the measured junctions, in stark contrast to the typically assumed value of 1~ns. Thanks to the low prefactors, and fine-tuning of the perpendicular magnetic anisotropy, we report measured mean dwell times as low as 2.7~ns under an in-plane applied field at negligible bias voltage. Under a perpendicular applied field, we predict a Meyer-Neldel compensation phenomenon, whereby the prefactor scales like an exponential of the activation energy, in line with the exponential dependence of the measured dwell time on the field. We further predict the occurrence of (sub)nanosecond dwell times as a function of effective anisotropy and junction diameter at zero bias voltage. These findings pave the way towards the development of ultrafast, low-power, unconventional computing schemes operating by leveraging thermal noise in perpendicular SMTJs, which can be scaled down below 20~nm.

cond-mat.mtrl-sci↗

arXiv2024

Fast current-induced skyrmion motion in synthetic antiferromagnets

Magnetic skyrmions are topological magnetic textures that hold great promise as nanoscale bits of information in memory and logic devices. Although room-temperature ferromagnetic skyrmions and their current-induced manipulation have been demonstrated, their velocity has been limited to about 100 meters per second. In addition, their dynamics are perturbed by the skyrmion Hall effect, a motion transverse to the current direction caused by the skyrmion topological charge. Here, we show that skyrmions in compensated synthetic antiferromagnets can be moved by current along the current direction at velocities of up to 900 meters per second. This can be explained by the cancellation of the net topological charge leading to a vanishing skyrmion Hall effect. Our results open an important path toward the realization of logic and memory devices based on the fast manipulation of skyrmions in tracks.

cond-mat.mes-hall↗

arXiv2023

Spiking Dynamics in Dual Free Layer Perpendicular Magnetic Tunnel Junctions

Spintronic devices have recently attracted a lot of attention in the field of unconventional computing due to their non-volatility for short and long term memory, non-linear fast response and relatively small footprint. Here we report how voltage driven magnetization dynamics of dual free layer perpendicular magnetic tunnel junctions enable to emulate spiking neurons in hardware. The output spiking rate was controlled by varying the dc bias voltage across the device. The field-free operation of this two terminal device and its robustness against an externally applied magnetic field make it a suitable candidate to mimic neuron response in a dense Neural Network (NN). The small energy consumption of the device (4-16 pJ/spike) and its scalability are important benefits for embedded applications. This compact perpendicular magnetic tunnel junction structure could finally bring spiking neural networks (SNN) to sub-100nm size elements.

physics.app-ph↗

arXiv2023

Control of skyrmion chirality in Ta/FeCoB/TaOx trilayers by TaOx oxidation and FeCoB thickness

Skyrmions are magnetic bubbles with nontrivial topology envisioned as data bits for ultrafast and power-efficient spintronic memory and logic devices. They may be stabilized in heavy-metal/ferromagnetic/oxide trilayer systems. The skyrmion chirality is then determined by the sign of the interfacial Dzyaloshinskii-Moriya interaction (DMI). Nevertheless, for apparently identical systems, there is some controversy about the DMI sign. Here, we show that the degree of oxidation of the top interface and the thickness of the ferromagnetic layer play a major role. Using Brillouin light-scattering measurements in Ta/Fe-Co-B/TaOx trilayers, we demonstrate a sign change of the DMI with the degree of oxidation of the Fe-Co-B/TaOx interface. Using polar magneto-optical Kerr effect microscopy, we consistently observe a reversal of the direction of current-induced motion of skyrmions with the oxidation level of TaOx; this is attributed to their chirality reversal. In addition, a second chirality reversal is observed when changing the Fe-Co-B thickness, probably due to the proximity of the two Fe-Co-B interfaces in the ultrathin case. By properly tuning the chirality of the skyrmion, spin-transfer and spin-orbit torques combine constructively to enhance the skyrmion velocity. These observations thus allow us to envision an optimization of the material parameters to produce highly mobile skyrmions. Moreover, this chirality control enables a versatile manipulation of skyrmions and paves the way towards multidirectional devices.

cond-mat.mtrl-sci↗

arXiv2022

Gate-controlled skyrmion and domain wall chirality

Magnetic skyrmions are localized chiral spin textures, which offer great promise to store and process information at the nanoscale. In the presence of asymmetric exchange interactions, their chirality, which governs their dynamics, is generally considered as an intrinsic parameter set during the sample deposition. In this work, we experimentally demonstrate that a gate voltage can control this key parameter. We probe the chirality of skyrmions and chiral domain walls by observing the direction of their current-induced motion and show that a gate voltage can reverse it. This local and dynamical reversal of the chirality is due to a sign inversion of the interfacial Dzyaloshinskii-Moriya interaction that we attribute to ionic migration of oxygen under gate voltage. Micromagnetic simulations show that the chirality reversal is a continuous transformation, in which the skyrmion is conserved. This control of chirality with 2 - 3 V gate voltage can be used for skyrmion-based logic devices, yielding new functionalities.

cond-mat.mes-hall↗

arXiv2021

Imprint from ferromagnetic skyrmions in an antiferromagnet via exchange bias

Magnetic skyrmions are topological spin textures holding great potential as nanoscale information carriers. Recently, skyrmions have been predicted in antiferromagnets, with key advantages in terms of stability, size, and dynamical properties over their ferromagnetic analogs. However, their experimental demonstration is still lacking. Here, we show the imprint from ferromagnetic skyrmions into a thin film of an IrMn antiferromagnet, at room temperature and zero external magnetic field, using exchange-bias. Using high-spatial-resolution x-ray magnetic circular dichroism photoemission electron microscopy (XMCD-PEEM), we observed the imprinted spin textures within the IrMn from the XMCD signal of the uncompensated Mn spins at the interface with the ferromagnet. This result opens up a path for logic and memory devices based on skyrmion manipulation in antiferromagnets.

cond-mat.mtrl-sci↗

arXiv2020

Electric field control of interfacial Dzyaloshinskii-Moriya interaction in Pt/Co/AlO$_x$ thin films

We studied electric field modification of magnetic properties in a Pt/Co/AlO$_x$ trilayer via magneto-optical Kerr microscopy. We observed the spontaneous formation of labyrinthine magnetic domain structure due to thermally activated domain nucleation and propagation under zero applied magnetic field. A variation of the period of the labyrinthine structure under electric field is observed as well as saturation magnetization and magnetic anisotropy variations. Using an analytical formula of the stripe equilibrium width we estimate the variation of the interfacial Dzyaloshinskii-Moriya interaction under electric field as function of the exchange stiffness constant.

cond-mat.mtrl-sci↗

arXiv2019

Mapping different skyrmion phases in double wedges of Ta/FeCoB(tFeCoB)/Ta(tTa)Ox

Skyrmions are chiral magnetic textures that have immense potential for applications in spintronic devices. However, their formation is quite challenging and necessitates a subtle balance of the magnetic interactions at play. Here, we study Ta/FeCoB/TaOx trilayer using crossed double wedges i.e. thickness gradients of FeCoB and of top Ta, which is subsequently oxidized leading to an oxidation gradient. This enabled us to observe micron-sized skyrmions in the vicinity of different transition regions of the sample: from perpendicular magnetic anisotropy to paramagnetic phase and also from perpendicular to in-plane magnetic anisotropy. These observations can be explained by the isolated bubble model taking into account the different energy contributions at play namely anisotropy, exchange, Dzyaloshinskii-Moriya, dipolar and Zeeman. We also qualitatively compare the current-induced motion of skyrmions obtained in different transition regions. Our study not only provides an effective means to form skyrmions by tuning the interfacial magnetic properties but also highlights the differences pertaining to the skyrmions observed in different transition zones, which is extremely crucial for any envisaged application.

cond-mat.mtrl-sci↗

arXiv2019

Current-Driven Skyrmion Dynamics and Drive-Dependent Skyrmion Hall Effect in an Ultrathin Film

Magnetic skyrmions are chiral spin textures that hold great promise as nanoscale information carriers. Since their first observation at room temperature, progress has been made in their current-induced manipulation, with fast motion reported in stray-field-coupled multilayers. However, the complex spin textures with hybrid chiralities and large power dissipation in these multilayers limit their practical implementation and the fundamental understanding of their dynamics. Here, we report on the current-driven motion of Néel skyrmions with diameters in the 100-nm range in an ultrathin Pt/Co/MgO trilayer. We find that these skyrmions can be driven at a speed of 100 m/s and exhibit a drive-dependent skyrmion Hall effect, which is accounted for by the effect of pinning. Our experiments are well substantiated by an analytical model of the skyrmion dynamics as well as by micromagnetic simulations including material inhomogeneities. This good agreement is enabled by the simple skyrmion spin structure in our system and a thorough characterization of its static and dynamical properties.

cond-mat.mes-hall↗

arXiv2018

Creation of Magnetic Skyrmion Bubble Lattices by Ultrafast Laser in Ultrathin Films

Magnetic skyrmions are topologically nontrivial spin textures which hold great promise as stable information carriers in spintronic devices at the nanoscale. One of the major challenges for developing novel skyrmion-based memory and logic devices is fast and controlled creation of magnetic skyrmions at ambient conditions. Here we demonstrate the single ultrafast (35-fs) laser pulse-induced generation of skyrmion bubbles and skyrmion bubble lattices from a ferromagnetic state in sputtered ultrathin magnetic films at room temperature. The skyrmion bubble density increases with the laser fluence in a controlled way, and it finally becomes saturated, forming disordered hexagonal lattices. Moreover, we present that the skyrmion bubble lattice configuration leads to enhanced topological stability as compared to isolated skyrmions, suggesting its promising use in data storage. Our findings shed light on the optical approach to the skyrmion bubble lattice in commonly accessible materials, paving the road toward the emerging skyrmion-based memory and synaptic devices.

cond-mat.mtrl-sci↗

arXiv2018

Large voltage tuning of Dzyaloshinskii-Moriya Interaction: a route towards dynamic control of skyrmion chirality

Electric control of magnetism is a prerequisite for efficient and low power spintronic devices. More specifically, in heavy metal/ ferromagnet/ insulator heterostructures, voltage gating has been shown to locally and dynamically tune magnetic properties like interface anisotropy and saturation magnetization. However, its effect on interfacial Dzyaloshinskii-Moriya Interaction (DMI), which is crucial for the stability of magnetic skyrmions, has been challenging to achieve and has not been reported yet for ultrathin films. Here, we demonstrate 130% variation of DMI with electric field in Ta/FeCoB/TaOx trilayers through Brillouin Light Spectroscopy (BLS). Using polar- Magneto-Optical-Kerr-Effect microscopy, we further show a monotonic variation of DMI and skyrmionic bubble size with electric field, with an unprecedented efficiency. We anticipate through our observations that a sign reversal of DMI with electric field is possible, leading to a chirality switch. This dynamic manipulation of DMI establishes an additional degree of control to engineer programmable skyrmion based memory or logic devices.

cond-mat.mtrl-sci↗

arXiv2017

Magnetic skyrmions in confined geometries : effect of the magnetic field and the disorder

We report on the effect of the lateral confinement and a perpendicular magnetic field on isolated room-temperature magnetic skyrmions in sputtered Pt/Co/MgO nanotracks and nanodots. We show that the skyrmions size can be easily tuned by playing on the lateral dimensions of the nanostructures and by using external magnetic field amplitudes of a few mT, which allow to reach sub-100 nm diameters. Our XMCD-PEEM observations also highlight the important role of the pinning on the skyrmions size and stability under an out-of-plane magnetic field. Micromagnetic simulations reveal that the effect of local pinning can be well accounted for by considering the thin film grain structure with local anisotropy variations and reproduce well the dependence of the skyrmion diameter on the magnetic field and the geometry.

cond-mat.mes-hall↗

arXiv2016

Room temperature chiral magnetic skyrmion in ultrathin magnetic nanostructures

Magnetic skyrmions are chiral spin structures with a whirling configuration. Their topological properties, nanometer size and the fact that they can be moved by small current densities have opened a new paradigm for the manipulation of magnetisation at the nanoscale. To date, chiral skyrmion structures have been experimentally demonstrated only in bulk materials and in epitaxial ultrathin films and under external magnetic field or at low temperature. Here, we report on the observation of stable skyrmions in sputtered ultrathin Pt/Co/MgO nanostructures, at room temperature and zero applied magnetic field. We use high lateral resolution X-ray magnetic circular dichroism microscopy to image their chiral Néel internal structure which we explain as due to the large strength of the Dzyaloshinskii-Moriya interaction as revealed by spin wave spectroscopy measurements. Our results are substantiated by micromagnetic simulations and numerical models, which allow the identification of the physical mechanisms governing the size and stability of the skyrmions.

cond-mat.mtrl-sci↗

arXiv2014

Chirality-induced asymmetric magnetic nucleation in Pt/Co/AlOx ultrathin microstructures

The nucleation of reversed magnetic domains in Pt/Co/AlO$_{x}$ microstructures with perpendicular anisotropy was studied experimentally in the presence of an in-plane magnetic field. For large enough in-plane field, nucleation was observed preferentially at an edge of the sample normal to this field. The position at which nucleation takes place was observed to depend in a chiral way on the initial magnetization and applied field directions. An explanation of these results is proposed, based on the existence of a sizable Dzyaloshinskii-Moriya interaction in this sample. Another consequence of this interaction is that the energy of domain walls can become negative for in-plane fields smaller than the effective anisotropy field.

cond-mat.mtrl-sci↗

arXiv2014

Ultrafast magnetization switching by spin-orbit torques

Spin-orbit torques induced by spin Hall and interfacial effects in heavy metal/ferromagnetic bilayers allow for a switching geometry based on in-plane current injection. Using this geometry, we demonstrate deterministic magnetization reversal by current pulses ranging from 180~ps to ms in Pt/Co/AlOx dots with lateral dimensions of 90~nm. We characterize the switching probability and critical current $I_c$ as function of pulse length, amplitude, and external field. Our data evidence two distinct regimes: a short-time intrinsic regime, where $I_c$ scales linearly with the inverse of the pulse length, and a long-time thermally assisted regime where $I_c$ varies weakly. Both regimes are consistent with magnetization reversal proceeding by nucleation and fast propagation of domains. We find that $I_c$ is a factor 3-4 smaller compared to a single domain model and that the incubation time is negligibly small, which is a hallmark feature of spin-orbit torques.

cond-mat.mes-hall↗

arXiv2013

Symmetry and magnitude of spin-orbit torques in ferromagnetic heterostructures

Current-induced spin torques are of great interest to manipulate the orientation of nanomagnets without applying external magnetic fields. They find direct application in non-volatile data storage and logic devices, and provide insight into fundamental processes related to the interdependence between charge and spin transport. Recent demonstrations of magnetization switching induced by in-plane current injection in ferromagnetic heterostructures have drawn attention to a class of spin torques based on orbital-to-spin momentum transfer, which is alternative to pure spin transfer torque (STT) between noncollinear magnetic layers and amenable to more diversified device functions. Due to the limited number of studies, however, there is still no consensus on the symmetry, magnitude, and origin of spin-orbit torques (SOTs). Here we report on the quantitative vector measurement of SOTs in Pt/Co/AlO trilayers using harmonic analysis of the anomalous and planar Hall effects as a function of the applied current and magnetization direction. We provide an all-purpose scheme to measure the amplitude and direction of SOTs for any arbitrary orientation of the magnetization, including corrections due to the interplay of Hall and thermoelectric effects. Based on general space and time inversion symmetry arguments, we show that asymmetric heterostructures allow for two different SOTs having odd and even behavior with respect to magnetization reversal. Our results reveal a scenario that goes beyond established models of the Rashba and spin Hall contributions to SOTs. The even SOT is STT-like but stronger than expected from the spin Hall effect in Pt. The odd SOT is composed of a constant field-like term and an additional component, which is strongly anisotropic and does not correspond to a simple Rashba field.

cond-mat.mes-hall↗