arXiv subjects

Stefan Ostermann

Publications and source records attributed to Stefan Ostermann.

34 records · Page 2Linked to original sources

arXiv2023

Programmable Simulations of Molecules and Materials with Reconfigurable Quantum Processors

Simulations of quantum chemistry and quantum materials are believed to be among the most important potential applications of quantum information processors, but realizing practical quantum advantage for such problems is challenging. Here, we introduce a simulation framework for strongly correlated quantum systems that can be represented by model spin Hamiltonians. Our approach leverages reconfigurable qubit architectures to programmably simulate real-time dynamics and introduces an algorithm for extracting chemically relevant spectral properties via classical co-processing of quantum measurement results. We develop a digital-analog simulation toolbox for efficient Hamiltonian time evolution utilizing digital Floquet engineering and hardware-optimized multi-qubit operations to accurately realize complex spin-spin interactions, and as an example present an implementation proposal based on Rydberg atom arrays. Then, we show how detailed spectral information can be extracted from these dynamics through snapshot measurements and single-ancilla control, enabling the evaluation of excitation energies and finite-temperature susceptibilities from a single-dataset. To illustrate the approach, we show how this method can be used to compute key properties of a polynuclear transition-metal catalyst and 2D magnetic materials.

quant-ph↗

arXiv2023

Chirality Dependent Photon Transport and Helical Superradiance

Chirality, or handedness, is a geometrical property denoting a lack of mirror symmetry. Chirality is ubiquitous in nature and is associated with the non-reciprocal interactions observed in complex systems ranging from biomolecules to topological materials. Here, we demonstrate that chiral arrangements of dipole-coupled atoms or molecules can facilitate the unidirectional transport of helical photonic excitations without breaking time-reversal symmetry. We show that such helicity dependent transport stems from an emergent spin-orbit coupling induced by the chiral geometry, which results in nontrivial topological properties. We also examine the effects of collective dissipation and find that many-body coherences lead to helicity dependent photon emission: an effect we call helical superradiance. Our results demonstrate an intimate connection between chirality, topology, and photon helicity that may contribute to molecular photodynamics in nature and could be probed with near-term quantum simulators.

quant-ph↗

arXiv2023

Dynamic population of multiexcitation subradiant states in incoherently excited atomic arrays

The deterministic generation of multiexcitation subradiant states proves to be challenging. Here, we present a viable path towards their transient generation in finite-sized ordered arrays of dipole-dipole coupled quantum emitters, based on incoherent driving of the atomic ensemble. In particular, we show that a maximal coupling to long-lived subradiant states is achieved if only half of the atoms are initially excited. We characterize the nature of the resulting states by calculating the dynamic fluorescence spectrum of the emitted light. Finally, we elucidate the role of coherent interactions during the decay process of sufficiently dense atomic arrays, which result in a coherently driven radiation burst that leads to a subsequent reduction of the chances to prepare multiexcitation subradiant states.

quant-ph↗

arXiv2023

Crystalline Phases of Laser-Driven Dipolar Bose-Einstein Condensates

Although crystallization is a ubiquitous phenomenon in nature, crystal formation and melting still remain fascinating processes with several open questions yet to be addressed. In this work, we study the emergent crystallization of a laser-driven dipolar Bose-Einstein condensate due to the interplay between long-range magnetic and effectively infinite-range light-induced interactions. The competition between these two interactions results in a collective excitation spectrum with two roton minima that introduce two different length scales at which crystalline order can emerge. In addition to the formation of regular crystals with simple periodic patterns due to the softening of one of the rotons, we find that both rotons can also soften simultaneously, resulting in the formation of exotic, complex periodic or aperiodic density patterns. We also demonstrate dynamic state-preparation schemes for achieving all the found crystalline ground states for experimentally relevant and feasible parameter regimes

cond-mat.quant-gas↗

arXiv2022

Characterizing superradiant dynamics in atomic arrays via a cumulant expansion approach

Ordered atomic arrays with subwavelength lattice spacing emit light collectively. For fully inverted atomic arrays, this results in an initial burst of radiation and a fast build up of coherences between the atoms at initial times. Based on a cumulant expansion of the equations of motion, we derive exact analytical expressions for the emission properties and numerically analyze the full many-body problem resulting in the collective decay process for unprecedented system sizes of up to a few hundred atoms. We benchmark the cumulant expansion approach and show that it correctly captures the cooperative dynamics resulting in superradiance. For fully inverted arrays, this allows us to extract the scaling of the superradiant peak with particle number. For partially excited arrays where no coherences are shared among atoms, we also determine the critical number of excitations required for the emergence of superradiance in one- and two-dimensional geometries. In addition, we study the robustness of superradiance in the case of non-unit filling and position disorder.

quant-ph↗

arXiv2022

Optimized geometries for cooperative photon storage in an impurity coupled to a two-dimensional atomic array

The collective modes of two-dimensional ordered atomic arrays can modify the radiative environment of embedded atomic impurities. We analyze the role of the lattice geometry on the impurity's emission linewidth by comparing the effective impurity decay rate obtained for all non-centered Bravais lattices and an additional honeycomb lattice. We demonstrate that the lattice geometry plays a crucial role in determining the effective decay rate for the impurity. In particular, we find that the minimal effective decay rate appears in lattices where the number of the impurity's nearest neighbours is maximal and the number of distinct distances among nearest neighbours is minimal. We further show that, in the choice between interstitial and substitutional placement of the impurity, the former always wins by exhibiting a lower decay rate and longer photon storage. For interstitial placements, we determine the optimal impurity position in the lattice plane, which is not necessarily found in the center of the lattice plaquette.

quant-ph↗

arXiv2022

Superglass formation in an atomic BEC with competing long-range interactions

The complex dynamical phases of quantum systems are dictated by atomic interactions that usually evoke an emergent periodic order. Here, we study a quantum many-body system with two competing and substantially different long-range interaction potentials where the dynamical instability towards density order can give way to a superglass phase, i. e., a superfluid disordered amorphous solid, which exhibits local density modulations but no long-range periodic order. We consider a two-dimensional BEC in the Rydberg-dressing regime coupled to an optical standing wave resonator. The dynamic pattern formation in this system is governed by the competition between the two involved interaction potentials: repulsive soft-core interactions arising due to Rydberg dressing and infinite-range sign changing interactions induced by the cavity photons. The superglass phase is found when the two interaction potentials introduce incommensurate length scales. The dynamic formation of this peculiar phase without any externally added disorder is driven by quantum fluctuations and can be attributed to frustration induced by the two competing interaction energies and length scales.

cond-mat.quant-gas↗

arXiv2020

Many-Body Phases of a Planar Bose-Einstein Condensate with Cavity-Induced Spin-Orbit Coupling

We explore the many-body phases of a two-dimensional Bose-Einstein condensate with cavity-mediated dynamic spin-orbit coupling. By the help of two transverse non-interfering, counterpropagating pump lasers and a single standing-wave cavity mode, two degenerate Zeeman sub-levels of the quantum gas are Raman coupled in a double-$Λ$-configuration. Beyond a critical pump strength the cavity mode is populated via coherent superradiant Raman scattering from the two pump lasers, leading to the appearance of a dynamical spin-orbit coupling for the atoms. We identify three quantum phases with distinct atomic and photonic properties: the normal ``homogeneous'' phase, the superradiant ``spin-helix'' phase, and the superradiant ``supersolid spin-density-wave'' phase. The latter exhibits an emergent periodic atomic density distribution with an orthorhombic centered rectangular-lattice structure due to the interplay between the coherent photon scattering into the resonator and the collision-induced momentum coupling. The transverse lattice spacing of the emergent crystal is set by the dynamic spin-orbit coupling.

cond-mat.quant-gas↗

arXiv2019

Unraveling the quantum nature of atomic self-ordering in a ring cavity

Atomic self-ordering to a crystalline phase in optical resonators is a consequence of the intriguing non-linear dynamics of strongly coupled atom motion and photons. Generally the resulting phase diagrams and atomic states can be largely understood on a mean-field level. However, close to the phase transition point, quantum fluctuations and atom-field entanglement play a key role and initiate the symmetry breaking. Here we propose a modified ring cavity geometry, in which the asymmetry imposed by a tilted pump beam reveals clear signatures of quantum dynamics even in a larger regime around the phase transition point. Quantum fluctuations become visible both in the dynamic and steady-state properties. Most strikingly we can identify a regime where a mean-field approximation predicts a runaway instability, while in the full quantum model the quantum fluctuations of the light field modes stabilize uniform atomic motion. The proposed geometry thus allows to unveil the "quantumness" of atomic self-ordering via experimentally directly accessible quantities.

quant-ph↗

arXiv2019

Antiferromagnetic self-ordering of a Fermi gas in a ring cavity

We explore the density and spin self-ordering of driven spin-$1/2$ collisionless fermionic atoms coupled to the electromagnetic fields of a ring resonator. The two spin states are two-photon Raman-coupled via a pair of degenerate counterpropagating cavity modes and two transverse pump fields. In this one-dimensional configuration the coupled atom-field system possesses a continuous $U(1)$ translational symmetry and a discrete $\mathbf{Z}_2$ spin inversion symmetry. At half filling for sufficiently strong pump strengths, the combined $U(1)\times \mathbf{Z}_2$ symmetry is spontaneously broken at the onset of a superradiant phase transition to a state with self-ordered density and spin structures. We predominately find an antiferromagnetic lattice order at the cavity wavelength. The self-ordered states exhibit unexpected positive momentum pair correlations between fermions with opposite spin. These strong cavity-mediated correlations vanish at higher pump strength.

cond-mat.quant-gas↗

arXiv2018

Cavity-induced emergent topological spin textures in a Bose Einstein condensate

The coupled nonlinear dynamics of ultracold quantum matter and electromagnetic field modes in an optical resonator exhibits a wealth of intriguing collective phenomena. Here we study a $Λ$-type, three-component Bose-Einstein condensate coupled to four dynamical running-wave modes of a ring cavity, where only two of the modes are externally pumped. However, the unpumped modes play a crucial role in the dynamics of the system due to coherent back-scattering of photons. On a mean- field level we identify three fundamentally different steady-state phases with distinct characteristics in the density and spatial spin textures: a combined density and spin wave, a continuous spin spiral with a homogeneous density, and a spin spiral with a modulated density. The spin-spiral states, which are topological, are intimately related to cavity-induced spin-orbit coupling emerging beyond a critical pump power. The topologically trivial density-wave--spin-wave state has the characteristics of a supersolid with two broken continuous symmetries. The transitions between different phases are either simultaneously topological and first order, or second order. The proposed setup allows the simulation of intriguing many-body quantum phenomena by solely tuning the pump amplitudes and frequencies, with the cavity output fields serving as a built-in nondestructive observation tool.

quant-ph↗

arXiv2018

Driven-Dissipative Supersolid in a Ring Cavity

Supersolids are characterized by the counter-intuitive coexistence of superfluid and crystalline order. Here we study a supersolid phase emerging in the steady state of a driven-dissipative system. We consider a transversely pumped Bose-Einstein condensate trapped along the axis of a ring cavity and coherently coupled to a pair of degenerate counter-propagating cavity modes. Above a threshold pump strength the interference of photons scattered into the two cavity modes results in an emergent superradiant lattice, which spontaneously breaks the continuous translational symmetry towards a periodic atomic pattern. The crystalline steady state inherits the superfluidity of the Bose-Einstein condensate, thus exhibiting genuine properties of a supersolid. A gapless collective Goldstone mode correspondingly appears in the superradiant phase, which can be non-destructively monitored via the relative phase of the two cavity modes on the cavity output. Despite cavity-photon losses the Goldstone mode remains undamped, indicating the robustness of the supersolid phase.

cond-mat.quant-gas↗

arXiv2017

Probing and characterizing the growth of a crystal of ultracold bosons and light

The non-linear coupled particle light dynamics of an ultracold gas in the field of two independent counter-propagating laser beams can lead to the dynamical formation of a self-ordered lattice structure as presented in Phys. Rev. X 6, 021026 (2016). Here we present new numerical studies on experimentally observable signatures to monitor the growth and properties of such a crystal in real time. While, at least theoretically, optimal non-destructive observation of the growth dynamics and the hallmarks of the crystalline phase can be performed by analyzing the scattered light, monitoring the evolution of the particle's momentum distribution via time-of-flight probing is an experimentally more accessible choice. In this work we show that both approaches allow to unambiguously distinguish the crystal from independent collective scattering as it occurs in matter wave super-radiance. As a clear crystallization signature we identify spatial locking between the two emerging standing laser waves together creating the crystal potential. For sufficiently large systems the system allows reversible adiabatic ramping into the crystalline phase as an alternative to a quench across the phase transition and growth from fluctuations.

quant-ph↗

arXiv2016

Generating a stationary infinite range tractor force via a multimode optical fiber

Optical fibers confine and guide light almost unattenuated and thus convey light forces to polarizable nano-particles over very long distances. Radiation pressure forces arise from scattering of guided photons into free space while gradient forces are based on coherent scattering between different fiber modes or propagation directions. Interestingly, even scattering between co-propagating modes induces longitudinal forces as the transverse confinement of the light modes creates mode dependent longitudinal wave-vectors and photon momenta. We generalize a proven scattering matrix based approach to calculate single as well as inter-particle forces to include several forward and backward propagating modes. We show that an injection of the higher order mode only in a two mode fiber will induce a stationary tractor force against the injection direction, when the mode coupling to the lower order mode dominates against backscattering and free space losses. Generically this arises for non-absorbing particles at the center of a waveguide. The model also gives improved predictions for inter-particle forces in evanescent nanofiber fields as experimentally observed recently. Surprisingly strong tractor forces can also act on whole optically bound arrays.

quant-ph↗

arXiv2016

Spontaneous crystallization of light and ultracold atoms

Coherent scattering of light from ultracold atoms involves an exchange of energy and momentum introducing a wealth of non-linear dynamical phenomena. As a prominent example particles can spontaneously form stationary periodic configurations which simultaneously maximize the light scattering and minimize the atomic potential energy in the emerging optical lattice. Such self-ordering effects resulting in periodic lattices via bimodal symmetry breaking have been experimentally observed with cold gases and Bose-Einstein condensates (BECs) inside an optical resonator. Here we study a new regime of periodic pattern formation for an atomic BEC in free space, driven by far off-resonant counterpropagating and non-interfering lasers of orthogonal polarization. In contrast to previous works, no spatial light modes are preselected by any boundary conditions and the transition from homogeneous to periodic order amounts to a crystallization of both light and ultracold atoms breaking a continuous translational symmetry. In the crystallized state the BEC acquires a phase similar to a supersolid with an emergent intrinsic length scale whereas the light-field forms an optical lattice allowing phononic excitations via collective back scattering, which are gapped due to the infinte-range interactions. The studied system constitutes a novel configuration allowing the simulation of synthetic solid state systems with ultracold atoms including long-range phonon dynamics.

quant-ph↗

arXiv2014

Scattering approach to two-colour light forces and self-ordering of polarizable particles

Collective coherent scattering of laser light by an ensemble of polarizable point particles creates long range interactions, whose properties can be tailored by choice of injected laser powers, frequencies and polarizations. We use a transfer matrix approach to study the forces induced by non-interfering fields of orthogonal polarization or different frequencies in a 1D geometry and find long range self-ordering of particles without a prescribed order. Adjusting laser frequencies and powers allows to tune inter-particle distances and provides a wide range of possible dynamical couplings not accessible in usual standing light wave geometries with prescribed order. In this work we restrict the examples to two frequencies and polarisations but the framework also allows to treat multicolour light beams with random phases. These dynamical effects should be observable in existing experimental setups with effective 1D geometries such as atoms or nanoparticles coupled to the field of an optical nanofibre or transversely trapped in counterpropagating Gaussian beams.

quant-ph↗