arXiv subjects

Stefan Schütz

Publications and source records attributed to Stefan Schütz.

15 recordsLinked to original sources

arXiv2020

Collective Dissipative Molecule Formation in a Cavity

We propose a mechanism to realize high-yield molecular formation from ultracold atoms. Atom pairs are continuously excited by a laser, and a collective decay into the molecular ground state is induced by a coupling to a lossy cavity mode. Using a combination of analytical and numerical techniques, we demonstrate that the molecular yield can be improved by simply increasing the number of atoms, and can overcome efficiencies of state-of-the-art association schemes. We discuss realistic experimental setups for diatomic polar and nonpolar molecules, opening up collective light matter interactions as a tool for quantum state engineering, enhanced molecule formation, collective dynamics, and cavity mediated chemistry.

cond-mat.quant-gas↗

arXiv2020

Dark state semilocalization of quantum emitters in a cavity

We study a disordered ensemble of quantum emitters collectively coupled to a lossless cavity mode. The latter is found to modify the localization properties of the "dark" eigenstates, which exhibit a character of being localized on multiple, noncontiguous sites. We denote such states as semi-localized and characterize them by means of standard localization measures. We show that those states can very efficiently contribute to coherent energy transport. Our paper underlines the important role of dark states in systems with strong light-matter coupling.

quant-ph↗

arXiv2020

Ensemble-induced strong light-matter coupling of a single quantum emitter

We discuss a technique to strongly couple a single target quantum emitter to a cavity mode, which is enabled by virtual excitations of a nearby mesoscopic ensemble of emitters. A collective coupling of the latter to both the cavity and the target emitter induces strong photon non-linearities in addition to polariton formation, in contrast to common schemes for ensemble strong coupling. We demonstrate that strong coupling at the level of a single emitter can be engineered via coherent and dissipative dipolar interactions with the ensemble, and provide realistic parameters for a possible implementation with SiV$^{-}$ defects in diamond. Our scheme can find applications, amongst others, in quantum information processing or in the field of cavity-assisted quantum chemistry.

quant-ph↗

arXiv2019

Adiabatic elimination for ensembles of emitters in cavities with dissipative couplings

We consider an ensemble of cavity-coupled two-level emitters interacting via full (coherent and dissipative) dipole-dipole interactions. Using an adiabatic elimination procedure we derive effective equations of motion for a subsystem consisting of the cavity and a single emitter. Those equations can be used for schemes to enhance the cavity-coupling of single emitters as shown in [S. Schütz, J. Schachenmayer, D. Hagenmüller, G. K. Brennen, T. Volz, V. Sandoghdar, T. W. Ebbesen, C. Genes, and G. Pupillo, e-print arXiv:1904.08888]. We analyze limitations of effective subsystem parameters, and study how joint dissipative decay processes in the subsystem affect cavity-coupling properties of the single emitter and cavity transmission spectra.

quant-ph↗

arXiv2019

Exploring Superconductivity under Strong Coupling with the Vacuum Electromagnetic Field

Light-matter interactions have generated considerable interest as a means to manipulate material properties. Light-induced superconductivity has been demonstrated using pulsed lasers. An attractive alternative possibility is to exploit strong light-matter interactions arising by coupling phonons to the vacuum electromagnetic field of a cavity mode as has been suggested and theoretically studied. Here we explore this possibility for two very different superconductors, namely YBCO (YBa$_2$Cu$_3$O$_{6+x}$) and Rb$_3$C$_{60}$, coupled to surface plasmon polaritons, using a novel cooperative effect based on the presence of a strongly coupled vibrational environment allowing efficient dressing of the otherwise weakly coupled phonon bands of these compounds. By placing the superconductor-surface plasmon system in a SQUID magnetometer, we find that the superconducting transition temperatures ($T_{c}$) for both compounds are modified in the absence of any external laser field. For YBCO, $T_{c}$ decreases from 92 K to 86 K while for Rb$_3$C$_{60}$, it increases from 30 K to 45 K at normal pressures. In the latter case, a simple theoretical framework is provided to understand these results based on an enhancement of the electron-phonon coupling. This proof-of-principle study opens a new tool box to not only modify superconducting materials but also to understand the mechanistic details of different superconductors.

cond-mat.supr-con↗

arXiv2018

Cavity-assisted mesoscopic transport of fermions: Coherent and dissipative dynamics

We study the interplay between charge transport and light-matter interactions in a confined geometry, by considering an open, mesoscopic chain of two-orbital systems resonantly coupled to a single bosonic mode close to its vacuum state. We introduce and benchmark different methods based on self-consistent solutions of non-equilibrium Green's functions and numerical simulations of the quantum master equation, and derive both analytical and numerical results. It is shown that in the dissipative regime where the cavity photon decay rate is the largest parameter, the light-matter coupling is responsible for a steady-state current enhancement scaling with the cooperativity parameter. We further identify different regimes of interest depending on the ratio between the cavity decay rate and the electronic bandwidth. Considering the situation where the lower band has a vanishing bandwidth, we show that for a high-finesse cavity, the properties of the resonant Bloch state in the upper band are transfered to the lower one, giving rise to a delocalized state along the chain. Conversely, in the dissipative regime with low cavity quality factors, we find that the current enhancement is due to a collective decay of populations from the upper to the lower band.

quant-ph↗

arXiv2017

Quenches across the self-organization transition in multimode cavities

A cold dilute atomic gas in an optical resonator can be radiatively cooled by coherent scattering processes when the driving laser frequency is tuned close but below the cavity resonance. When sufficiently illuminated, moreover, the atoms' steady state undergoes a phase transition from homogeneous density to crystalline order. We characterize the dynamics of this self-ordering process in the semi-classical regime when distinct cavity modes with commensurate wavelengths are quasi-resonantly driven by laser fields via scattering by the atoms. The lasers are simultaneously applied and uniformly illuminate the atoms, their frequencies are chosen so that the atoms are cooled by the radiative processes, their intensity is either suddenly switched or slowly ramped across the self-ordering transition. Numerical simulations for different ramp protocols predict that the system exhibits long-lived metastable states, whose occurrence strongly depends on initial temperature, ramp speed, and number of atoms.

quant-ph↗

arXiv2017

Cavity-enhanced transport of charge

We theoretically investigate charge transport through electronic bands of a mesoscopic one-dimensional system, where inter-band transitions are coupled to a confined cavity mode, initially prepared close to its vacuum. This coupling leads to light-matter hybridization where the dressed fermionic bands interact via absorption and emission of dressed cavity-photons. Using a self-consistent non-equilibrium Green's function method, we compute electronic transmissions and cavity photon spectra and demonstrate how light-matter coupling can lead to an enhancement of charge conductivity in the steady-state. We find that depending on cavity loss rate, electronic bandwidth, and coupling strength, the dynamics involves either an individual or a collective response of Bloch states, and explain how this affects the current enhancement. We show that the charge conductivity enhancement can reach orders of magnitudes under experimentally relevant conditions.

quant-ph↗

arXiv2017

Semiclassical theory of synchronization-assisted cooling

We analyse the dynamics leading to radiative cooling of an atomic ensemble confined inside an optical cavity when the atomic dipolar transitions are incoherently pumped and can synchronize. Our study is performed in the semiclassical regime and assumes that cavity decay is the largest rate in the system dynamics. We identify three regimes characterising the cooling. At first hot atoms are individually cooled by the cavity friction forces. After this stage, the atoms' center-of-mass motion is further cooled by the coupling to the internal degrees of freedom while the dipoles synchronize. In the latest stage dipole-dipole correlations are stationary and the center-of-mass motion is determined by the interplay between friction and dispersive forces due to the coupling with the collective dipole. We analyse this asymptotic regime by means of a mean-field model and show that the width of the momentum distribution can be of the order of the photon recoil. Furthermore, the internal excitations oscillate spatially with the cavity standing wave forming an antiferromagnetic-like order.

quant-ph↗

arXiv2016

Dissipation-assisted prethermalization in long-range interacting atomic ensembles

We theoretically characterize the semiclassical dynamics of an ensemble of atoms after a sudden quench across a driven-dissipative second-order phase transition. The atoms are driven by a laser and interact via conservative and dissipative long-range forces mediated by the photons of a single-mode cavity. These forces can cool the motion and, above a threshold value of the laser intensity, induce spatial ordering. We show that the relaxation dynamics following the quench exhibits a long prethermalizing behaviour which is first dominated by coherent long-range forces, and then by their interplay with dissipation. Remarkably, dissipation-assisted prethermalization is orders of magnitude longer than prethermalization due to the coherent dynamics. We show that it is associated with the creation of momentum-position correlations, which remain nonzero for even longer times than mean-field predicts. This implies that cavity cooling of an atomic ensemble into the selforganized phase can require longer time scales than the typical experimental duration. In general, these results demonstrate that noise and dissipation can substantially slow down the onset of thermalization in long-range interacting many-body systems.

quant-ph↗

arXiv2016

Mean-field theory of atomic self-organization in optical cavities

Photons mediate long-range optomechanical forces between atoms in high finesse resonators, which can induce the formation of ordered spatial patterns. When a transverse laser drives the atoms, the system undergoes a second order phase transition, that separates a uniform spatial density from a Bragg grating maximizing scattering into the cavity and is controlled by the laser intensity. Starting from a Fokker-Planck equation describing the semiclassical dynamics of the $N$-atom distribution function, we systematically develop a mean-field model and analyse its predictions for the equilibrium and out-of-equilibrium dynamics. The validity of the mean-field model is tested by comparison with the numerical simulations of the $N$-body Fokker-Planck equation and by means of a BBGKY hierarchy. The mean-field theory predictions well reproduce several results of the $N$-body Fokker-Planck equation for sufficiently short times, and are in good agreement with existing theoretical approaches based on field-theoretical models. Mean-field, on the other hand, predicts thermalization time scales which are at least one order of magnitude shorter than the ones predicted by the $N$-body dynamics. We attribute this discrepancy to the fact that the mean-field ansatz discards the effects of the long-range incoherent forces due to cavity losses.

quant-ph↗

arXiv2015

Thermodynamics and dynamics of atomic self-organization in an optical cavity

Pattern formation of atoms in high-finesse optical resonators results from the mechanical forces of light associated with superradiant scattering into the cavity mode. It occurs when the laser intensity exceeds a threshold value, such that the pumping processes counteract the losses. We consider atoms driven by a laser and coupling with a mode of a standing-wave cavity and describe their dynamics with a Fokker-Planck equation, in which the atomic motion is semiclassical but the cavity field is a full quantum variable. The asymptotic state of the atoms is a thermal state, whose temperature is solely controlled by the detuning between the laser and the cavity frequency and by the cavity loss rate. From this result we derive the free energy and show that in the thermodynamic limit selforganization is a second-order phase transition. The order parameter is the field inside the resonator, to which one can associate a magnetization in analogy to ferromagnetism, the control field is the laser intensity, however the steady state is intrinsically out-of-equilibrium. In the symmetry-broken phase quantum noise induces jumps of the spatial density between two ordered patterns: We characterize the statistical properties of this temporal behaviour at steady state and show that the thermodynamic properties of the system can be extracted by detecting the light at the cavity output. The results of our analysis are in full agreement with previous studies, extend them by deriving a self-consistent theory which is valid also when the cavity field is in the shot-noise limit, and elucidate the nature of the selforganization transition.

quant-ph↗

arXiv2014

Prethermalization of atoms due to photon-mediated long-range interactions

Atoms can spontaneously form spatially-ordered structures in optical resonators when they are transversally driven by lasers. This occurs when the laser intensity exceeds a threshold value and results from the mechanical forces on the atoms associated with superradiant scattering into the cavity mode. We treat the atomic motion semiclassically and show that, while the onset of spatial ordering depends on the intracavity-photon number, the stationary momentum distribution is a Maxwell-Boltzmann whose width is determined by the rate of photon losses. Above threshold, the dynamics is characterized by two time scales: after a violent relaxation, the system slowly reaches the stationary state over time scales exceeding the cavity lifetime by several orders of magnitude. In this transient regime the atomic momenta form non-Gaussian metastable distributions, which emerge from the interplay between the long-range dispersive and dissipative mechanical forces of light. We argue that the dynamics of selforganization of atoms in cavities offers a testbed for studying the statistical mechanics of long-range interacting systems.

quant-ph↗

arXiv2013

Cooling of atomic ensembles in optical cavities: Semiclassical limit

The semiclassical dynamics of atoms are theoretically studied, when the atoms are confined inside a standing-wave high-finesse resonator. The atoms are cooled by scattering processes in which the photons of a transverse laser are coherently scattered into the cavity mode. We derive a Fokker-Planck equation for the atomic center-of-mass variables which allows us to determine the equations of motion in the semiclassical limit for any value of the intensity of the laser field. We extract its prediction for the dynamics when the resonator is essentially in the vacuum state and the atoms are cooled by scattering photons into the cavity mode, which then decays. Its predictions for the stationary atomic distribution are compared with the ones of the Fokker-Planck equation in [P. Domokos, P. Horak, and H. Ritsch, J. Phys. B 34, 187 (2001)], which has been derived under different assumptions. We find full agreement in the considered parameter regime.

quant-ph↗

arXiv2013

Seeding patterns for self-organization of photons and atoms

When atoms scatter photons from a transverse laser into a high-finesse optical cavity, they form crystalline structures which maximize the intracavity light field and trap the atoms in the ordered array. Stable organization occurs when the laser field amplitude exceeds a certain threshold. For planar single-mode cavities there exist two equivalent possible atomic patterns, which determine the phase of the intracavity light field. Under these premises, we show that the effect of an additional laser pumping the cavity makes one pattern more favorable than the other and that it can dynamically force the system into a predetermined configuration. This is an instance of pattern formation and seeding in a nonlinear quantum-optical system.

quant-ph↗