arXiv subjects

Stefan Skupin

Publications and source records attributed to Stefan Skupin.

15 recordsLinked to original sources

arXiv2026

High order harmonic Optical Reconstruction by delayed time-depeNdent Ellipticity perturbaTion: HORNET

We present and demonstrate an all-optical \textit{in situ} method for temporal characterisation of high-order harmonics generated in gas with a linearly polarised intense infrared (IR) laser. By using a delayed cross-polarised replica of the IR pulse with a lower amplitude, we introduce a weak and time-dependent ellipticity in the IR driving field. Since the XUV emission is very sensitive to the ellipticity of the driving field, it is perturbed precisely at the times when ellipticity is significant. The detected emission is then reduced only if the unperturbed XUV emission is substantial at these times. Perturbed XUV spectra are recorded for several delays and exhibit changes both in amplitude and in their spectral content. An iterative ptychographic algorithm is used to retrieve the electric field of individual harmonics in a very robust way. Experimental measurements are in good agreement with simulations. The reconstructed temporal profiles show a steady evolution of the XUV pulse duration and chirp with the harmonic order. The highest harmonics exhibit a positive chirp and are emitted in the rising front of the IR driving pulse, while the lowest ones exhibit a negative chirp and are emitted throughout the entire pulse.

physics.optics↗

arXiv2026

Modular multiscale approach to modelling high-harmonic generation in gases

We present a modular user-oriented simulation toolbox for studying highharmonic generation in gases. The first release consists of the computational pipeline to 1) compute the unidirectional IR-pulse propagation incylindrical symmetry, 2) solve the microscopic responses in the whole macroscopic volume using a 1D-TDSE solver, 3) obtain the far-field harmonic field using a diffraction-integral approach. The code comes with interfaces and tutorials, based on practical laboratory conditions, to facilitate the usage and deployment of the code both locally and in HPC-clusters. Additionally, the modules are designed to work as stand-alone applications as well, e.g., 1D-TDSE is available through Pythonic interface.

physics.optics↗

arXiv2024

Waveshape of THz radiation produced by two-color laser-induced air plasmas

The spatial and spectral distributions of terahertz (THz) pulses emitted by two-color air plasmas are theoretically investigated for focused laser pulses and in the filamentation regime. We derive a so-called ''augmented'' conical emission model, which, similarly to the one originally proposed by You et al.\ [Phys.\ Rev.\ Lett.\ {\bf 109}, 183902 (2012)], involves phase matching between laser harmonics along the plasma channel, the plasma density and length, and the emitted frequency as key parameters. Our augmented model, however, treats envelope effects and accounts for transverse variations of both plasma- and Kerr-driven potential THz emitters. We highlight the importance of the characteristic spatio-spectral distributions of these two conversion mechanisms in the expression of the angular radiated power. The results of our model are successfully compared with data provided by a comprehensive, fully space and time-resolved unidirectional solver. Importantly, these numerical simulations clear up the effective plasma length along which THz emission develops, compared with the dephasing length along which the laser fundamental and second harmonic become out-of-phase. The impact of common optical aberrations, such as sphericity, astigmatism, and coma, on the THz generation is also investigated. Aberrations are shown to generally decrease the laser-to-THz conversion efficiency and potentially induce spatial asymmetries and narrowing in the THz spectra.

physics.plasm-ph↗

arXiv2024

THz to far-infrared spectra of the known crystal polymorphs of Phenylalanine

There is renewed interest in the structure of the essential amino acid Phenylalanine in the solid state. Three new polymorphs were found in the years 2012 to 2014. Here, we investigate the structure, stability, and energetical ordering of these phases using first-principles simulations at the level of Density Functional Theory incorporating van-der-Waals interactions. Two of the distinct crystal forms are found to be structurally similar and energetically very close after vibrational free energy corrections have been taken into account. Infrared absorption spectra are likewise calculated and compared to experimental measurements. By combining measurements obtained with a commercial Fourier Transform Infra-Red spectrometer and a homemade air-photonics-based THz Time Domain spectrometer, we could carry out this comparison in the vibrational frequency region from 1 to 40~THz. The excellent agreement of the line positions and the established energy ranking allow us to identify the most stable polymorph of Phenylalanine.

physics.chem-ph↗

arXiv2023

Optical Probing of Ultrafast Laser-Induced Solid-to-Overdense-Plasma Transitions

Understanding the target dynamics during its interaction with a relativistic ultrashort laser pulse is a challenging fundamental multi-physics problem involving at least atomic and solid-state physics, plasma physics, and laser physics. Already, the properties of the so-called pre-plasma formed as the laser pulse's rising edge ionizes the target are complicated to access in experiments and modeling, and many aspects of this laser-induced transition from solid to overdense plasma over picosecond time scales are still open questions. At the same time, applications like laser-driven ion acceleration require precise knowledge and control of the pre-plasma because the efficiency of the acceleration process itself crucially depends on the target properties at the arrival of the relativistic intensity peak of the pulse. By capturing the dynamics of the initial stage of the interaction, we report on a detailed visualization of the pre-plasma formation and evolution. Nanometer-thin diamond-like carbon foils are shown to transition from solid to plasma during the laser rising edge with intensities < 10^16 W/cm^2. Single-shot near-infrared probe transmission measurements evidence sub-picosecond dynamics of an expanding plasma with densities above 10^23 cm^-3 (about 100 times the critical plasma density). The complementarity of a solid-state interaction model and a kinetic plasma description provides deep insight into the interplay of ionization, collisions, and expansion.

physics.plasm-ph↗

arXiv2021

Shaping convex edges in borosilicate glass by single pass perforation with an Airy beam

We demonstrate curved modifications with lengths of up to 2 mm within borosilicate glass produced by single 1030 nm picosecond laser shots with an Airy beam profile. Plasma ignition in the side lobes of the beam as well as surface damage prove to be the crucial limitations for confined bulk energy deposition on a curved trajectory. A combined experimental and numerical analysis reveals optimum laser parameters for confined bulk energy deposition. This way we achieved single pass cutting of a 525 $μ$m thick glass sheet with a well defined convex edge down to a bending radius of 774 $μ$m.

physics.optics↗

arXiv2019

Terahertz vortex wave generation in air plasma by two-color femtosecond laser pulses

We investigate the generation of broadband terahertz (THz) pulses with phase singularity from air plasmas created by fundamental and second harmonic laser pulses. We show that when the second harmonic beam carries a vortex charge, the THz beam acquires a vortex structure as well. A generic feature of such THz vortex is that the intensity is modulated along the azimuthal angle, which can be attributed to the spatially varying relative phase difference between the two pump harmonics. Fully space and time resolved numerical simulations reveal that transverse instabilities of the pump further affect the emitted THz field along nonlinear propagation, which produces additional singularities resulting in a rich vortex structure. The predicted intensity modulation is experimentally demonstrated with a thermal camera, in excellent agreement with simulation results. The presence of phase singularities in the experiment is revealed by astigmatic transformation of the beam using a cylindrical mirror.

physics.plasm-ph↗

arXiv2017

Broadband terahertz emission from two-color fs-laser-induced microplasmas

We investigate terahertz emission from two-color fs-laser-induced microplasmas. Under strongest focusing conditions, microplasmas are shown to act as point-sources for broadband terahertz-to-far-infrared radiation, where the emission bandwidth is determined by the plasma density. Semi-analytical modeling allows us to identify scaling laws with respect to important laser parameters. In particular, we find that the optical-to-THz conversion efficiency crucially depends on the focusing conditions. We use this insight to demonstrate by means of Maxwell-consistent 3D simulations, that for only 10-$μ$J laser energy a conversion efficiency well above $10^{-4}$ can be achieved.

physics.optics↗

arXiv2015

Modelling arbitrarily shaped and tightly focused laser pulses in electromagnetic codes

Investigation of laser matter interaction with electromagnetic codes requires to implement sources for the electromagnetic fields. A way to do so is to prescribe the fields at the numerical box boundaries in order to achieve the desired fields inside the numerical box. Here we show that the often used paraxial approximation can lead to unexpected field profiles with strong impact on the laser matter interaction results. We propose an efficient numerical algorithm to compute the required laser boundary conditions consistent with the Maxwell's equations for arbitrarily shaped, tightly focused laser pulses.

physics.plasm-ph↗

arXiv2014

Spectral self-action of THz emission from ionizing two-color laser pulses in gases

The spectrum of terahertz (THz) emission in gases via ionizing two-color femtosecond pulses is analyzed by means of a semi-analytic model and finite-difference-time-domain simulations in 1D and 2D geometries. We show that produced THz signals interact with free electron trajectories and thus influence significantly further THz generation upon propagation, i.e., make the process inherently nonlocal. This self-action plays a key role in the observed strong spectral broadening of the generated THz field. Diffraction limits the achievable THz bandwidth by efficiently depleting the low frequency amplitudes in the propagating field.

physics.plasm-ph↗

arXiv2014

Filamentation of ultrashort laser pulses in silica glass and KDP crystal: A comparative study

Ionizing 800-nm femtosecond laser pulses propagating in silica glass and in potassium dihydrogen phosphate (KDP) crystal are investigated by means of a unidirectional pulse propagation code. Filamentation in fused silica is compared with the self-channeling of light in KDP accounting for the presence of defect states and electron-hole dynamics. In KDP, laser pulses produce intense filaments with higher clamping intensities up to 200 TW/cm$^2$ and longer plasma channels with electron densities above $10^{16}$ cm$^{-3}$. Despite these differences, the propagation dynamics in silica and KDP are almost identical at equivalent ratios of input power over the critical power for self-focusing.

physics.optics↗

arXiv2013

On the Saturation of the Nonlinear Refractive Index in Atomic Gases

Motivated by the ongoing controversy on the origin of the nonlinear index saturation and subsequent intensity clamping in femtosecond filaments, we study the atomic nonlinear polarization induced by a high-intensity and ultrashort laser pulse in hydrogen by numerically solving the time dependent Schrödinger equation. Special emphasis is given to the efficient modeling of the nonlinear polarization at central laser frequency corresponding to 800 nm wavelength. Here, the recently proposed model of the Higher-Order Kerr Effect (HOKE) and two versions of the Standard model for femtosecond filamentation, including either a multi-photon or tunnel ionization rate, are compared. We find that around the clamping intensity the instantaneous HOKE model does not reproduce the temporal structure of the nonlinear response obtained from the quantum mechanical results. In contrast, the non-instantaneous charge contributions included in the Standard models ensure a reasonable quantitative agreement. Therefore, the physical origin for the observed saturation of the overall electron response is confirmed to mainly result from contributions of free or nearly free electrons.

physics.optics↗

arXiv2011

Directionality of THz emission from photoinduced gas plasmas

Forward and backward THz emission by ionizing two-color laser pulses in gas is investigated by means of a simple semi-analytical model based on Jefimenko's equation and rigorous Maxwell simulations in one and two dimensions. We find the emission in backward direction having a much smaller spectral bandwidth than in forward direction and explain this by interference effects. Forward THz radiation is generated predominantly at the ionization front and thus almost not affected by the opacity of the plasma, in excellent agreement with results obtained from a unidirectional pulse propagation model.

physics.optics↗

arXiv2010

Azimuthons in weakly nonlinear waveguides of different symmetries

We show that weakly guiding nonlinear waveguides support stable propagation of rotating spatial solitons (azimuthons). We investigate the role of waveguide symmetry on the soliton rotation. We find that azimuthons in circular waveguides always rotate rigidly during propagation and the analytically predicted rotation frequency is in excellent agreement with numerical simulations. On the other hand, azimuthons in square waveguides may experience spatial deformation during propagation. Moreover, we show that there is a critical value for the modulation depth of azimuthons above which solitons just wobble back and forth, and below which they rotate continuously. We explain these dynamics using the concept of energy difference between different orientations of the azimuthon.

nlin.PS↗

arXiv2005

Stable rotating dipole solitons in nonlocal optical media

We reveal that nonlocality can provide a simple physical mechanism for stabilization of multi-hump optical solitons, and present the first example of stable rotating dipole solitons and soliton spiraling, known to be unstable in all types of realistic nonlinear media with local response.

nlin.PS↗