arXiv subjects

Stefan Walter

Publications and source records attributed to Stefan Walter.

24 records · Page 2Linked to original sources

arXiv2012

Direct and charge transfer mediated photogeneration in polymer-fullerene bulk heterojunction solar cells

We investigated photogeneration yield and recombination dynamics in blends of poly(3-hexyl thiophene) (P3HT) and poly[2-methoxy-5-(30,70-dimethyloctyloxy)-1,4-phenylenevinylene] (MDMO-PPV) with [6,6]- phenyl-C61 butyric acid methyl ester (PC61BM) by means of temperature dependent time delayed collection field (TDCF) measurements. In MDMO-PPV:PC61BM we find a strongly field dependent polaron pair dissociation which can be attributed to geminate recombination in the device. Our findings are in good agreement with field dependent photoluminescence measurements published before, supporting a scenario of polaron pair dissociation via an intermediate charge transfer (CT) state. In contrast, polaron pair dissociation in P3HT:PC61BM shows only a very weak field dependence, indicating an almost field independent polaron pair dissociation or a direct photogeneration. Furthermore, we found Langevin recombination for MDMO-PPV:PC61BM and strongly reduced Langevin recombination for P3HT:PC61BM.

cond-mat.mtrl-sci↗

arXiv2012

Failure of protection of Majorana based qubits against decoherence

Qubit realizations based on Majorana bound states have been considered promising candidates for quantum information processing which is inherently inert to decoherence. We put the underlying general arguments leading to this conjecture to the test from an open quantum system perspective. It turns out that, from a fundamental point of view, the Majorana qubit is as susceptible to decoherence as any local paradigm of a qubit.

cond-mat.mes-hall↗

arXiv2011

Detecting Majorana Bound States by Nanomechanics

We propose a nanomechanical detection scheme for Majorana bound states, which have been predicted to exist at the edges of a one-dimensional topological superconductor, implemented, for instance, using a semiconducting wire placed on top of an s-wave superconductor. The detector makes use of an oscillating electrode, which can be realized using a doubly clamped metallic beam, tunnel coupled to one edge of the topological superconductor. We find that a measurement of the nonlinear differential conductance provides the necessary information to uniquely identify Majorana bound states.

cond-mat.mes-hall↗

arXiv2010

Momentum and position detection in nanoelectromechanical systems beyond Born and Markov approximations

We propose and analyze different schemes to probe the quantum nature of nanoelectromechanical systems (NEMS) by a tunnel junction detector. Using the Keldysh technique, we are able to investigate the dynamics of the combined system for an arbitrary ratio of $eV/\hbar Ω$, where V is the applied bias of the tunnel junction and $Ω$ the eigenfrequency of the oscillator. In this sense, we go beyond the Markov approximation of previous works where these parameters were restricted to the regime $eV/\hbar Ω\gg 1$. Furthermore, we also go beyond the Born approximation because we calculate the finite frequency current noise of the tunnel junction up to fourth order in the tunneling amplitudes. Interestingly, we discover different ways to probe both position and momentum properties of NEMS. On the one hand, for a non-stationary oscillator, we find a complex finite frequency noise of the tunnel junction. By analyzing the real and the imaginary part of this noise separately, we conclude that a simple tunnel junction detector can probe both position- and momentum-based observables of the non-stationary oscillator. On the other hand, for a stationary oscillator, a more complicated setup based on an Aharonov-Bohm-loop tunnel junction detector is needed. It still allows us to extract position and momentum information of the oscillator. For this type of detector, we analyze for the first time what happens if the energy scales $eV$, $\hbar Ω$, and $k_B T$ take arbitrary values with respect to each other where T is the temperature of an external heat bath. Under these circumstances, we show that it is possible to uniquely identify the quantum state of the oscillator by a finite frequency noise measurement.

cond-mat.mes-hall↗

arXiv2010

Positivity of the two-dimensional Brown-Ravenhall operator

We determine the critical coupling of the two-dimensional Brown-Ravenhall operator with Coulomb potential. Boundedness from below has essentially been proven by Bouzouina, whose work however contains a trivial error leading to a wrong constant exactly one half of the actual critical constant. Furthermore we show that the operator is in fact positive. Our proof of that is for the most part analogous to Tix's proof of the corresponding result for the three-dimensional operator.

math-ph↗

arXiv2010

Bloch oscillations in lattice potentials with controlled aperiodicity

We numerically investigate the damping of Bloch oscillations in a one-dimensional lattice potential whose translational symmetry is broken in a systematic manner, either by making the potential bichromatic or by introducing scatterers at distinct lattice sites. We find that the damping strongly depends on the ratio of lattice constants in the bichromatic potential, and that even a small concentration of scatterers can lead to strong damping. Moreover, mean-field interactions are able to counteract aperiodicity-induced damping of Bloch oscillations.

cond-mat.quant-gas↗