arXiv subjects

Stefan Witte

Publications and source records attributed to Stefan Witte.

13 recordsLinked to original sources

arXiv2026

The 2D approximation quickly breaks down in reflection ptychography

Ptychographic reconstructions in reflection geometries are commonly interpreted with the same two-dimensional thin-sample model used in transmission, yet the validity of this approximation has not been established. We develop a three-dimensional weak-scattering description of reflection ptychography and derive explicit thickness criteria for when a two-dimensional model remains accurate. Because the sampled axial spatial frequency range is dominated by the rotation of the Ewald sphere rather than its curvature, reflection geometries impose far stricter thin-sample conditions than transmission geometries. The allowable thickness is reduced by one to two orders of magnitude for a representative extreme ultraviolet geometry, depending on the tolerance for appearance of artifacts. Simulations verify that conventional two-dimensional reconstructions may exhibit the thickness-dependent artifacts as predicted by the theory, with particularly strong distortions near specular Bragg minima. We further show that incorporating the correct depth-dependent propagation into the forward model resolves these distortions and enables recovery of sample thickness. These results establish practical validity limits for two-dimensional reflection ptychography and identify a path toward quantitative depth-sensitive reconstructions at all geometries.

physics.optics↗

arXiv2025

Improving signal-to-noise ratios in pump-probe spectroscopy on light-sensitive samples by adapting pulse repetition rates

Ultrafast optical pump-probe spectroscopy is a powerful tool to study dynamics in solid materials on femto- and picosecond timescales. In such experiments, a pump pulse induces dynamics inside a sample by impulsive light-matter interaction, resulting in dynamics that can be detected using a time-delayed probe pulse. In addition to the desired dynamics, the initial interaction may also lead to unwanted effects that may result in irreversible changes and even damage. Therefore, the achievable signal strength is often limited by the pumping conditions that a sample can sustain. Here we investigate the optimization of ultrafast photoacoustics in various solid thin films. We perform systematic experiments aimed at maximizing the achievable signal-to-noise (SNR) ratio in a given measurement time while limiting sample damage. By varying pump and probe pulse energies, average pump fluence, and repetition rate, we identify different paths towards optimal SNR depending on material properties. Our results provide a strategy for the design of pump-probe experiments, to optimize achievable SNR for samples in which different damage mechanisms may dominate.

physics.optics↗

arXiv2024

Breaking Abbe's diffraction limit with harmonic deactivation microscopy

Nonlinear optical microscopy provides elegant means for label-free imaging of biological samples and condensed matter systems. The widespread areas of application could even be increased if resolution was improved, which is currently limited by the famous Abbe diffraction limit. Super-resolution techniques can break the diffraction limit but rely on fluorescent labeling. This makes them incompatible with (sub-)femtosecond temporal resolution and applications that demand the absence of labeling. Here, we introduce harmonic deactivation microscopy (HADES) for breaking the diffraction limit in non-fluorescent samples. By controlling the harmonic generation process on the quantum level with a second donut-shaped pulse, we confine the third harmonic generation to three times below the original focus size and use this pulse for scanning microscopy. We demonstrate that resolution improvement by deactivation is more efficient for higher harmonic orders, and only limited by the maximum applicable deactivation-pulse fluence. This provides a route towards sub-100~nm resolution in a regular nonlinear microscope. The new capability of label-free super-resolution can find immediate applications in condensed matter physics, semiconductor metrology, and biomedical imaging.

physics.optics↗

arXiv2024

Fast spectroscopic imaging using extreme ultraviolet interferometry

Extreme ultraviolet pulses as generated by high harmonic generation (HHG) are a powerful tool for both time-resolved spectroscopy and coherent diffractive imaging. However, the integration of spectroscopy and microscopy to harness the unique broadband spectra provided by HHG is hardly explored due to the challenge to decouple spectroscopic and microscopic information. Here, we present an interferometric approach to this problem that combines Fourier transform spectroscopy (FTS) with Fourier transform holography (FTH). This is made possible by the generation of phase-locked pulses using a pair of HHG sources. Crucially, in our geometry the number of interferometric measurements required is at most equal to the number of high harmonics in the illumination, and can be further reduced by incorporating prior knowledge about the structure of the FTH sample. Compared to conventional FTS, this approach achieves over an order of magnitude increase in acquisition speed for full spectro-microscopic data, and furthermore allows diffraction-limited computational imaging.

physics.optics↗

arXiv2023

PtyLab.m/py/jl: a cross-platform, open-source inverse modeling toolbox for conventional and Fourier ptychography

Conventional (CP) and Fourier (FP) ptychography have emerged as versatile quantitative phase imaging techniques. While the main application cases for each technique are different, namely lens-less short wavelength imaging for CP and lens-based visible light imaging for FP, both methods share a common algorithmic ground. CP and FP have in part independently evolved to include experimentally robust forward models and inversion techniques. This separation has resulted in a plethora of algorithmic extensions, some of which have not crossed the boundary from one modality to the other. Here, we present an open source, cross-platform software, called PtyLab, enabling both CP and FP data analysis in a unified framework. With this framework, we aim to facilitate and accelerate cross-pollination between the two techniques. Moreover, the availability in Matlab, Python, and Julia will set a low barrier to enter each field.

physics.comp-ph↗

arXiv2021

Spatial coherence control and analysis via micromirror-based mixed-state ptychography

Flexible and fast control of the phase and amplitude of coherent light, enabled by digital micromirror devices (DMDs) and spatial light modulators (SLMs), has been a driving force for recent advances in optical tweezers, nonlinear microscopy, and wavefront shaping. In contrast, engineering spatially partially coherent light remains widely elusive due to the lack of tools enabling a joint analysis and control sequence. Here, we report an approach to coherence engineering that combines a quasi-monochromatic, thermal source and a DMD together with a ptychographic scanning microscope. The reported method opens up new routes to low-cost coherence control, with applications in micromanipulation, nanophotonics, and quantitative phase contrast imaging.

physics.optics↗

arXiv2019

Detection of hidden gratings through multilayer nanostructures using light and sound

We report on the detection of diffraction gratings buried below a stack of tens of 18 nm thick $\mathrm{SiO_2}$ and $\mathrm{Si_3N_4}$ layers and an optically opaque metal layer, using laser-induced, extremely-high frequency ultrasound. In our experiments, the shape and amplitude of a buried metal grating is encoded on the spatial phase of the reflected acoustic wave. This grating-shaped acoustic echo from the buried grating is detected by diffraction of a delayed probe pulse. The shape and strength of the time-dependent diffraction signal can be accurately predicted using a 2D numerical model. Surprisingly, our numerical calculations show that the diffracted signal strength is not strongly influenced by the number of dielectric layers through which the acoustic wave has to propagate. Replacing the $\mathrm{SiO_2}$/$\mathrm{Si_3N_4}$ layer stack with a single layer having an equivalent time-averaged sound velocity and average density, has only a small effect on the shape and amplitude of the diffracted signal as a function of time. Our results show that laser-induced ultrasound is a promising technique for sub-surface nano-metrology applications.

physics.app-ph↗

arXiv2018

Expansion Dynamics After Laser-Induced Cavitation in Liquid Tin Microdroplets

The cavitation-driven expansion dynamics of liquid tin microdroplets is investigated, set in motion by the ablative impact of a 15-ps laser pulse. We combine high-resolution stroboscopic shadowgraphy with an intuitive fluid dynamic model that includes the onset of fragmentation, and find good agreement between model and experimental data for two different droplet sizes over a wide range of laser pulse energies. The dependence of the initial expansion velocity on these experimental parameters is heuristically captured in a single power law. Further, the obtained late-time mass distributions are shown to be governed by a single parameter. These studies are performed under conditions relevant for plasma light sources for extreme-ultraviolet nanolithography.

physics.flu-dyn↗

arXiv2018

Controlling ion kinetic energy distributions in laser produced plasma sources by means of a picosecond pulse pair

The next generation of lithography machines uses extreme ultraviolet (EUV) light originating from laser-produced plasma (LPP) sources, where a small tin droplet is ionized by an intense laser pulse to emit the requested light at 13.5 nm. Numerous irradiation schemes have been explored to increase conversion efficiency (CE), out of which a double-pulse approach comprising a weak picosecond Nd:YAG pre-pulse followed by a powerful pulse is considered to be very promising [1]. Nevertheless, even for such CE-optimized schemes, ion debris ejected from the plasma with kinetic energies up to several keV remain a factor that hampers the maximum performance of LPP sources. In this letter we propose a novel pre-pulse scheme consisting of a picosecond pulse pair at 1064 nm, which decreases the amount of undesirable fast ions, avoids back-reflections to the lasers and enables one to tailor the target shape.

physics.plasm-ph↗

arXiv2018

Sn ion energy distributions of ns- and ps-laser produced plasmas

Ion energy distributions arising from laser-produced plasmas of Sn are measured over a wide laser parameter space. Planar-solid as well as liquid-droplet targets are exposed to infrared laser pulses with energy densities between 1J/cm$^2$ and 4kJ/cm$^2$ and durations spanning 0.5ps to 6ns. The measured ion energy distributions are compared to two self-similar solutions of a hydrodynamic approach assuming isothermal expansion of the plasma plume into vacuum. For planar and droplet targets exposed to ps-long pulses we find a good agreement between the experimental results and the self-similar solution of a semi-infinite simple planar plasma configuration with an exponential density profile. The ion energy distributions resulting from solid Sn exposed to ns-pulses agrees with solutions of a limited-mass model that assumes a Gaussian-shaped initial density profile.

physics.plasm-ph↗

arXiv2013

High-Precision Spectroscopy with Counter-Propagating Femtosecond Pulses

An experimental realization of high-precision direct frequency comb spectroscopy using counter-propagating femtosecond pulses on two-photon atomic transitions is presented. Doppler broadened background signal, hampering precision spectroscopy with ultrashort pulses, is effectively eliminated with a simple pulse shaping method. As a result, all four 5S-7S two-photon transitions in a rubidium vapor are determined with both statistical and systematic uncertainties below 10$^{-11}$, which is an order of magnitude better than previous experiments on these transitions.

physics.atom-ph↗

arXiv2013

Ultra-broadband extreme-ultraviolet lensless imaging of extended complex structures

Lensless imaging is an elegant approach to high-resolution microscopy, which is rapidly gaining popularity in applications where imaging optics are problematic. However, current lensless imaging methods require objects to be placed within a well-defined support structure, while the light source needs to have a narrow, stable, and accurately known spectrum. Here we introduce a general approach to lensless imaging without spectral bandwidth limitations or sample requirements. We use two time-delayed coherent light pulses, and show that scanning the pulse-to-pulse time delay allows the reconstruction of diffraction-limited images for all spectral components in the pulse. Moreover, an iterative phase retrieval algorithm is introduced, which uses these spectrally resolved Fresnel diffraction patterns to obtain high-resolution images of complex extended objects without any support requirements. We demonstrate this two-pulse imaging method with octave-spanning visible light sources (in both transmission and reflection geometries), and with broadband extreme-ultraviolet radiation from a high-harmonic source. This demonstrates that our approach enables effective use of low-flux ultra-broadband sources, such as table-top soft-X-ray systems, for high-resolution imaging.

physics.optics↗

arXiv2012

Spatial and Spectral Coherent Control with Frequency Combs

Quantum coherent control (1-3) is a powerful tool for steering the outcome of quantum processes towards a desired final state, by accurate manipulation of quantum interference between multiple pathways. Although coherent control techniques have found applications in many fields of science (4-9), the possibilities for spatial and high-resolution frequency control have remained limited. Here, we show that the use of counter-propagating broadband pulses enables the generation of fully controlled spatial excitation patterns. This spatial control approach also provides decoherence reduction, which allows the use of the high frequency resolution of an optical frequency comb (10,11). We exploit the counter-propagating geometry to perform spatially selective excitation of individual species in a multi-component gas mixture, as well as frequency determination of hyperfine constants of atomic rubidium with unprecedented accuracy. The combination of spectral and spatial coherent control adds a new dimension to coherent control with applications in e.g nonlinear spectroscopy, microscopy and high-precision frequency metrology.

physics.atom-ph↗