Searcharxiv⌕ Search

arXiv subjects

Stefan-Ludwig Drechsler

Publications and source records attributed to Stefan-Ludwig Drechsler.

At least 19 recordsLinked to original sources

Stabilization of Interband Phase Solitons in Two-Band Noncentrosymmetric Superconducting Rings

Two-band superconductors maintain a relative interband phase which can carry winding soliton excitations in a superconducting ring, supported by independent winding numbers in the two bands. In rings of superconductors obeying the inversion symmetry the interband phase solitons are metastable states, separated from the uniform ground state by the energy of screening currents. In this work we find that, breaking the inversion symmetry strongly enough, one can make the soliton a true ground state. In that case, a magneto-electric coupling, absent in centrosymmetric materials, contributes critically above a certain threshold, a relevant, free-energy term, odd with respect to the winding number, which biases the energy balance in favor of a particular winding sign. Once the bias outweighs the energy cost that originally made the soliton metastable, a phase soliton with a finite winding number becomes the ground state, with chirality set by the applied field. In current--flux measurements performed in equilibrium states, the effect is demonstrated by field-odd soliton branches, that replace the metastable ones existing in mesoscopic rings, built by two-component superconductors, realizing a magneto-electric analog of the Little--Parks fluxoid-branch physics in the interband relative-phase sector.

cond-mat.supr-con↗

A Kapitza Pendulum Route to Supercurrent Tunnel Diodes

Superconducting diodes that support nonreciprocal supercurrent flow in principle constitute attractive, non-dissipative, circuit elements for superconducting electronics. But their realization faces fundamental challenges, as conventional Josephson tunnel junctions are inherently reciprocal. Existing approaches to break reciprocity typically involve magnetism or spin-orbit coupling, which often increase device complexity and limit reproducibility. Here, we demonstrate an alternative dynamical route to supercurrent nonreciprocity based on parametric driving. By applying a frequency-modulated supercurrent amplitude we show that effective higher-order, nonharmonic terms are generated in the current-phase relation. Leveraging mathematical equivalences with the Kapitza pendulum, we show that these terms dynamically break reciprocity. This establishes the concept of a Kapitza supercurrent diode and demonstrates that nonreciprocal superconducting transport can be engineered by nonequilibrium driving conventional Josephson tunnel junctions. We propose two implementations of the Kapitza supercurrent diode - via gate-controlled superconducting interferometers or flux-driven double-loop SQUIDs - to achieve nonreciprocal supercurrent transport within experimentally accessible frequencies $ω/2π\sim 1$-$10\,\mathrm{GHz}$.

cond-mat.supr-con↗

Self-organised magnon condensation in quasi-1D edge-shared cuprates without external fields

Multimagnon bound states were predicted nearly a century ago and have since been a key topic in condensed matter physics due to their intriguing quantum properties. However, their realization in natural materials remains elusive, especially in low-dimensional quantum magnets, where stabilizing them is particularly challenging due to the traditionally required extreme external magnetic fields. Therefore, we introduce a novel mechanism that enables the stabilization of multimagnon bound states in quasi-one-dimensional edge-shared cuprates. Our theoretical framework, supported by numerical simulations and experimental data, demonstrates that small antiferromagnetic interchain couplings act as effective internal magnetic fields, promoting a collinear antiferromagnetic order and enabling magnon condensation even at zero external field. This intrinsic stabilisation mechanism eliminates the need for high external fields, offering a platform that is more accessible for experimental realization. We validate this concept by applying it to representative materials such as Li$_2$CuO$_2$, Ca$_2$Y$_2$Cu$5$O$_{10}$, LiCuSbO$_4$, and PbCuSO$_4$(OH)$_2$. Beyond its experimental feasibility, this mechanism could drive advancements in magnon-based quantum computing, low-power spintronic devices, and high-speed magnonic circuits. Moreover, our findings reveal that small interchain and/or interlayer couplings can generally unlock previously overlooked magnetic phenomena, redefining the nature of magnetically ordered states and expanding the frontiers of quantum magnetism.

cond-mat.str-el↗

Supercurrent Diode Effect in Josephson Interferometers with Multiband Superconductors

We investigate nonreciprocal supercurrent phenomena in superconducting quantum interference devices (SQUIDs) that integrate Josephson junctions with single and multiband order parameters, which may exhibit time-reversal symmetry breaking. Our results show that the magnetic field can independently control both the amplitude and direction of supercurrent rectification, depending on the multiband characteristics of the superconductors involved. We analyze the effects of zero and antiphase (π) pairing among different bands on the development of nonreciprocal effects and find that the rectification is not influenced by π-pairing. Furthermore, we demonstrate that incorporating multiband superconductors that break time-reversal symmetry produces significant signatures in rectification. The rectification exhibits an even parity dependence on the magnetic field and the average rectification amplitude across quantum flux multiples does not equal zero. These findings indicate that magnetic flux pumping can be accomplished with time-reversal symmetry broken multiband superconductors by adjusting the magnetic field. Overall, our findings provide valuable insights for identifying and utilizing phases with broken time-reversal symmetry in multiband superconductors.

cond-mat.supr-con↗

Supercurrent rectification with time-reversal symmetry broken multiband superconductors

We consider nonreciprocal supercurrent effects in Josephson junctions based on multiband superconductors with a pairing structure that can break time-reversal symmetry. We demonstrate that a nonreciprocal supercurrent can be generally achieved by the cooperation of interband superconducting phase mismatch and interband scattering as well as by multiband phase frustration. The effect of interband impurity scattering indicates that the amplitude and sign of the nonreciprocal supercurrent are sensitive to the interband phase relation. For the case of a three-band superconductor, due to phase frustration, we show that the profile of the supercurrent rectification is marked by a hexagonal pattern of nodal lines with vanishing amplitude. Remarkably, around the nodal lines, the supercurrent rectification amplitude exhibits three-fold structures with an alternating sign. We show that the hexagonal pattern and the three-fold structure in the interband phase space turn out to be dependent on the tunneling amplitude of each band. These findings provide hallmarks of the supercurrent rectification which can be potentially employed to unveil the occurrence of spin-singlet multiband superconductivity with time-reversal symmetry breaking.

cond-mat.supr-con↗

Unusual Low-Energy Collective Charge Excitations in High-$T_c$ Cuprate Superconductors

Despite decades of intensive experimental and theoretical efforts, the physics of cuprate high-temperature superconductors in general, and, in particular, their normal state, is still under debate. Here, we report our investigation of low-energy charge excitations in the normal state. We find that the peculiarities of the electronic band structure at low energies have a profound impact on the nature of the intraband collective modes. It gives rise to a new kind of mode with huge intensity and non-Lorentzian spectral function in addition to well-known collective excitations like conventional plasmons and spin fluctuation. We predict two such modes with maximal spectral weight in the nodal and antinodal directions. Additionally, we found a long-living quasi-one-dimensional plasmon becoming an intense soft mode over an extended momentum range along the antinodal direction. These modes might explain some of the resonant inelastic X-ray scattering spectroscopy data.

cond-mat.supr-con↗

Multiple-q current states in a multicomponent superconducting channel

It is well-established that multicomponent superconductors can host different nonstandard phenomena such as broken-time reversal symmetry (BTRS) states, exotic Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) phases, the fractional Josephson effect as well as plenty of topological defects like phase solitons, domain walls and unusual vortex structures. We show that in the case of a two-component superconducting quasi-one-dimensional channel this catalogue can be extended by a novel inhomogeneous current state, which we have termed as a multiple-momenta state or, in short, a multiple-q state, characterized by the coexistence of two different interpenetrating Cooper pair condensates with different total momenta. Within the Ginzburg-Landau formalism for a dirty two-band superconductor with sizable impurity scattering treated in the Born-approximation we reveal that under certain conditions, the occurrence of multiple-q states can induce a cascade of transitions involving switching between them and the homogeneous BTRS (non-BTRS) states and vice versa leading this way to a complex interplay of homogeneous and inhomogeneous current states. We find that hallmarks of such a multiple-q state within a thin wire or channel can be a saw-like dependence of the depairing current and the existence of two distinct stable branches on it (a bistable current state).

cond-mat.supr-con↗

Magneto-topological transitions in multicomponent superconductors

Multi-component spin-singlet superconductors with competing 0- and $π$-pairing couplings, as in $s_{++}$ and $s_{\pm}$ phases, are close to instabilities with a spontaneous breaking of time-reversal symmetry. We demonstrate that the modification of the kinetic energy of superconducting electrons in a doubly connected superconducting cylinder, determined by the applied flux, generally drives transitions from chiral superconducting states to configurations that are time-reversal symmetric. This magneto-topological-induced changeover is investigated by means of a Ginzburg-Landau approach for a two-band superconductor with interband interactions and impurity scattering investigated for the case of a sample in the form of a mesoscopically thin-walled cylinder. We find that the application of a magnetic flux can convert a chiral $s_{\pm}+is_{++}$ state into a $s_{\pm}$ configuration and vice versa or tune the energy splitting of chiral states having inequivalent pairing amplitudes. We discuss signatures for the detection of these phases and of the corresponding transitions in mesoscopic superconducting loops.

cond-mat.supr-con↗

Phase solitons in a weakly coupled three-component superconductor

Based on the phenomenological Ginzburg-Landau approach, we investigate phase solitonic states in a class of three-component superconductors for mesoscopic doubly-connected geometry (thin-walled cylinder) in external magnetic fields. Analysis of the Gibbs free energy of the system shows that solitonic states in a three-component superconductor are thermodynamically metastable and separated from the ground state by a sizable energy. Our results demonstrate that despite of the presence of the zoo of phase solitons states earlier proposed method [Phys. Rev. B 96, 144513 (2017)] for the detection of BTRS in multiband superconductors remains valid and useful.

cond-mat.supr-con↗

Variety of order-by-disorder phases in the asymmetric $J_1-J_2$ zigzag ladder: From the delta chain to the $J_1-J_2$ chain

We study an asymmetric $J_1$-$J_2$ zigzag ladder consisting of two different spin-$\frac{1}{2}$ antiferromagnetic (AFM; $J_2$, $γJ_2>0$) Heisenberg legs coupled by zigzag-shaped ferromagnetic (FM; $J_1<0$) inter-leg interaction. On the basis of density-matrix renormalization group based calculations the ground-state phase diagram is obtained as functions of $γ$ and $J_2/|J_1|$. It contains four kinds of frustration-induced ordered phases except a trivial FM phase. Two of the ordered phases are valence bond solid (VBS) with spin-singlet dimerization, which is a rather conventional order by disorder. Still, it is interesting to note that the VBS states possess an Affleck-Kennedy-Lieb-Tasaki-type topological hidden order. The remaining two phases are ferrimagnetic orders, each of which is distinguished by commensurate or incommensurate spin-spin correlation. It is striking that the ferrimagnetic orders are not associated with geometrical symmetry breaking; instead, the global spin-rotation symmetry is broken. In other words, the system lowers its energy via the FM inter-leg interaction by polarizing both of the AFM Heisenberg legs. This is a rare type of order by disorder. Besides, the incommensurate ferrimagnetic state appears as a consequence of the competition between a polarization and a critical Tomonaga-Luttinger-liquid behavior in the AFM Heisenberg legs.

cond-mat.str-el↗

Coexistence of valence-bond formation and topological order in the Frustrated Ferromagnetic $J_1$-$J_2$ Chain

Frustrated one-dimensional (1D) magnets are known as ideal playgrounds for new exotic quantum phenomena to emerge. We consider an elementary frustrated 1D system: the spin-$\frac{1}{2}$ ferromagnetic ($J_1$) Heisenberg chain with next-nearest-neighbor antiferromagnetic ($J_2$) interactions. On the basis of density-matrix renormalization group calculations we show the existence of a finite spin gap at $J_2/|J_1|>1/4$ and we find the ground state in this region to be a valence bond solid (VBS) with spin-singlet dimerization between third-neighbor sites. The VBS is the consequence of spontaneous symmetry breaking through order by disorder. Quite interestingly, this VBS state has a Affleck-Kennedy-Lieb-Tasaki-type topological order. This is the first example of a frustrated spin chain in which quantum fluctuations induce gapped topological order.

cond-mat.str-el↗

Cross-over from an incommensurate singlet spiral state with a vanishingly small spin-gap to a valence bond solid state in dimerized frustrated ferromagnetic spin-chains

Motivated by the magnetic properties of the spin-chain compounds LiCuSbO$_4$$\equiv$LiSbCuO$_4$ and Rb$_2$Cu$_2$Mo$_3$O$_{12}$, we study the ground state of the Heisenberg chain with dimerized nearest-neighbor ferromagnetic (FM)($J_1, J_1^\prime<0$) and next-nearest-neighbor antiferromagnetic ($J_2>0$) couplings. Using the density-matrix renormalization group technique and spin-wave theory we find a first-order transition between a fully-polarized FM and an incommensurate spiral state at $2α=β/(1+β)$, where $α$ is the frustration ratio $J_2/|J_1|$ and $β$ the degree of dimerization $J_1^\prime/J_1$.In the singlet spiral state the spin-gap is vanishingly small in the vicinity of the FM transition, corresponding to a situation of LiCuSbO$_4$. For larger $α$, corresponding to Rb$_2$Cu$_2$Mo$_3$O$_{12}$, and smaller $β$ there is a crossover from this frustration induced incommensurate state to an Affleck-Lieb-Kennedy-Tasaki-type valence bond solid state with substantial spin-gaps.

cond-mat.str-el↗

Probing inter- and intrachain Zhang-Rice excitons in Li$_2$CuO$_2$ and determining their binding energy

Cuprate materials, like those hosting high temperature superconductivity, represent a famous class of materials where the correlations between the strongly entangled charges and spins produce complex phase diagrams. Several years ago the Zhang-Rice singlet was proposed as a natural quasiparticle in hole-doped cuprates. The occurance and binding energy of this quasiparticle, consisting of a pair of bound holes with antiparallel spins on the same CuO$_4$ plaquette, depends on the local electronic interactions, which are fundamental quantities for understanding the physics of the cuprates. Here, we employ state-of-the-art Resonant Inelastic X-ray Scattering (RIXS) to probe the correlated physics of the CuO$_4$ plaquettes in the quasi-one dimensional chain cuprate Li$_2$CuO$_2$. By tuning the incoming photon energy to the O $K$-edge, we populate bound states related to the Zhang-Rice quasiparticles in the RIXS process. Both intra- and interchain Zhang-Rice singlets are observed and their occurrence is shown to depend on the nearest-neighbor spin-spin correlations, which are readily probed in this experiment. We also extract the binding energy of the Zhang-Rice singlet and identify the Zhang-Rice triplet excitation in the RIXS spectra.

cond-mat.str-el↗

Hall-plot of the phase diagram for Ba(Fe1-xCox)2As2

The Hall effect is a powerful tool for investigating carrier type and density. For single-band materials, the Hall coefficient is traditionally expressed simply by $R_H^{-1} = -en$, where $e$ is the charge of the carrier, and $n$ is the concentration. However, it is well known that in the critical region near a quantum phase transition, as it was demonstrated for cuprates and heavy fermions, the Hall coefficient exhibits strong temperature and doping dependencies, which can not be described by such a simple expression, and the interpretation of the Hall coefficient for Fe-based superconductors is also problematic. Here, we investigate thin films of Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ with compressive and tensile in-plane strain in a wide range of Co doping. Such in-plane strain changes the band structure of the compounds, resulting in various shifts of the whole phase diagram as a function of Co doping. We show that the resultant phase diagrams for different strain states can be mapped onto a single phase diagram with the Hall number. This universal plot is attributed to the critical fluctuations in multiband systems near the antiferromagnetic transition, which may suggest a direct link between magnetic and superconducting properties in the BaFe$_2$As$_2$ system.

cond-mat.supr-con↗

Electron-lattice interactions strongly renormalize the charge transfer energy in the spin-chain cuprate Li$_2$CuO$_2$

Strongly correlated insulators are broadly divided into two classes: Mott-Hubbard insulators, where the insulating gap is driven by the Coulomb repulsion $U$ on the transition-metal cation, and charge-transfer insulators, where the gap is driven by the charge transfer energy $Δ$ between the cation and the ligand anions. The relative magnitudes of $U$ and $Δ$ determine which class a material belongs to, and subsequently the nature of its low-energy excitations. These energy scales are typically understood through the local chemistry of the active ions. Here we show that the situation is more complex in the low-dimensional charge transfer insulator Li$_\mathrm{2}$CuO$_\mathrm{2}$, where $Δ$ has a large non-electronic component. Combining resonant inelastic x-ray scattering with detailed modeling, we determine how the elementary lattice, charge, spin, and orbital excitations are entangled in this material. This results in a large lattice-driven renormalization of $Δ$, which significantly reshapes the fundamental electronic properties of Li$_\mathrm{2}$CuO$_\mathrm{2}$.

cond-mat.str-el↗

Determining the Short-Range Spin Correlations in Cuprate Chain Materials with Resonant Inelastic X-ray Scattering

We report a high-resolution resonant inelastic soft x-ray scattering study of the quantum magnetic spin-chain materials Li2CuO2 and CuGeO3. By tuning the incoming photon energy to the oxygen K-edge, a strong excitation around 3.5 eV energy loss is clearly resolved for both materials. Comparing the experimental data to many-body calculations, we identify this excitation as a Zhang-Rice singlet exciton on neighboring CuO4-plaquettes. We demonstrate that the strong temperature dependence of the inelastic scattering related to this high-energy exciton enables to probe short-range spin correlations on the 1 meV scale with outstanding sensitivity.

cond-mat.str-el↗

The dual nature of As-vacancies in LaFeAsO-derived superconductors: magnetic moment formation while preserving superconductivity

As-vacancies (V_As) in La-1111-systems, which are nominally non-magnetic defects, are shown to create in their vicinity by symmetry ferromagnetically oriented local magnetic moments due to the strong, covalent bonds with neighboring Fe atoms that they break. From microscopic theory in terms of an appropriately modified Anderson-Wolff model, we find that the moment formation results in a substantially enhanced paramagnetic susceptibility in both the normal and superconducting (SC) state. Despite the V_As act as magnetic scatterers, they do not deteriorate SC properties which can even be improved by V_As by suppressing a competing or coexisting commensurate spin density wave or its remnant fluctuations. Due to the induced local magnetic moments an s_++-scenario in related systems is unlikely.

cond-mat.supr-con↗

Full Relativistic Electronic Structure and Fermi Surface Sheets of the First Honeycomb-Lattice Pnictide Superconductor SrPtAs

We report full-potential density functional theory (DFT)-based {\it ab initio} band structure calculations to investigate electronic structure properties of the first pnictide superconductor with a honeycomb-lattice structure: SrPtAs. As a result, electronic bands, density of states, Fermi velocities and the topology of the Fermi surface for SrPtAs are obtained. These quantities are discussed in comparison to the first available experimental data. Predictions for future measurements are provided.

cond-mat.supr-con↗