arXiv subjects

Stefano Barbieri

Publications and source records attributed to Stefano Barbieri.

8 recordsLinked to original sources

arXiv2026

Mid-IR single- and dual-electro-optic comb generation with an ultrafast modulator

Mid-infrared (mid-IR) frequency combs are powerful tools for molecular sensing, industrial monitoring, and precision spectroscopy, yet their development beyond 5 um remains limited. Electro-optic modulation offers a promising path toward compact, agile comb generation, but extending this approach into the mid-infrared has been hindered by the lack of practical, high-performance modulators. Here we present an approach that leads to efficient generation of mid infrared frequency combs around 9 um, by employing ultrafast, room temperature, free space electro optic intensity modulators. By driving a single modulator with short electrical pulse trains, we realize both single- and dual-comb operation from a continuous-wave quantum cascade laser, providing a compact and versatile platform for mid-IR spectroscopy. This scheme produces combs with tunable repetition rates down to the megahertz range with direct observation on an electrical spectrum analyzer without any interferometer. As a proof of concept, we perform single- and dual-comb spectroscopy of a germanium etalon and an ammonia cell, achieving resolution far beyond that of conventional Fourier-transform infrared (FTIR) spectrometers and highlighting the potential of this approach for precise measurements in the long-wavelength molecular-fingerprint region. These results establish high-performance mid-IR modulators as a promising route toward practical, energy-efficient frequency-comb systems for sensing and spectroscopy.

physics.optics↗

arXiv2024

Ultrafast (10 GHz) mid-IR modulator based on ultra-fast electrical switching of the light-matter coupling

We demonstrate a free-space amplitude modulator for mid-infrared radiation (lambda=9.6 um) that operates at room temperature up to at least 20 GHz (above the -3dB cutoff frequency measured at 8.2 GHz). The device relies on the ultra-fast transition between weak and strong-coupling regimes induced by the variation of the applied bias voltage. Such transition induces a modulation of the device reflectivity. It is made of a semiconductor heterostructure enclosed in a judiciously designed array of metal-metal optical resonators, that - all-together - behave as an electrically tunable surface. At negative bias, it operates in the weak light-matter coupling regime. Upon application of an appropriate positive bias, the quantum wells populate with electrons and the device transitions to the strong-coupling regime. The modulator transmission keeps linear with input RF power in the 0dBm - 9dBm range. The increase of optical powers up to 25 mW exhibit a weak beginning saturation a little bit below.

physics.app-ph↗

arXiv2024

Real-time, chirped-pulse heterodyne detection at room-temperature with 100GHz 3dB-bandwidth mid-infrared quantum-well photodetectors

Thanks to intrinsically short electronic relaxation on the ps time scale, III-V semiconductor unipolar devices are ideal candidates for ultrahigh-speed operation at mid-infrared frequencies. In this work, antenna-coupled, GaAs-based multi quantum-well photodetectors operating in the 10-11um range are demonstrated, with a responsivity of 0.3A/W and a 3dB-cutoff bandwidth of 100GHz at room-temperature. The frequency response is measured up to 220GHz: beyond 100GHz we find a roll-off dominated by the 2.5 ps-long recombination time of the photo-excited electrons. The potential of the detectors is illustrated by setting up an experiment where the time dependent emission frequency of a quantum cascade laser operated in pulsed mode is measured electronically and in real-time, over a frequency range >60GHz. By exploiting broadband electronics, and thanks to its high signal-to-noise ratio, this technique allows the acquisition, in a single-shot, of frequency-calibrated, mid-infrared molecular spectra spanning up to 100GHz and beyond, which is particularly attractive for fast, active remote sensing applications in fields such as environmental or combustion monitoring.

physics.ins-det↗

arXiv2021

Active Stabilization of Terahertz Semiconductor Dual-Comb Laser Sources Employing a Phase Locking Technique

Dual-comb sources with equally spaced and low phase noise frequency lines are of great importance for high resolution spectroscopy and metrology. In the terahertz frequency range, electrically pumped semiconductor quantum cascade lasers (QCLs) are suitable candidates for frequency comb and dual-comb operation. For a single laser frequency comb, the repetition rate can be locked using a microwave injection locking and the carrier frequency can be locked to a highly stable source. However, for the locking of two laser combs, four frequencies (two repetition rates and two carrier offset frequencies) should be simultaneously locked; If one only refers to the dual-comb signal, two relative frequencies, i.e., the offset frequency and repetition frequency of one laser against those of the other laser, should be locked. Although the locking techniques that have been successfully used for a single laser comb can be, in principle, applied to a dual-comb laser source, the complete locking considerably complicates the implementation of such a system. Here, we propose a method to stabilize a terahertz QCL dual-comb source by phase locking one of the dual-comb lines to a radio frequency (RF) synthesizer. This technique forces one of the lasers to follow the tone of the other one (keeping the sum of the carrier offset frequency difference and repetition frequency difference between the two laser combs as a constant) by exploiting a laser self-detection that avoids the use of an external detector. Through the demonstration of this locking technique, we demonstrate that the dual-comb can generate periodic pulses over a 2 us time scale, showing that the terahertz QCL comb without a control of the repetition rate can produce pulsed-type waveforms.

physics.app-ph↗

arXiv2020

Comment on "Widely tunable terahertz gas lasers"

Chevalier et al. (Science, 15 November 2019, p. 856-860) report mathematical formulas and a table predicting the threshold and the output power of terahertz molecular lasers based on various molecules. We show that these formulas are not coherent with the simple model used to describe this kind of laser, and that they largely overestimate the conversion efficiency. We suggest an alternative calculation.

physics.app-ph↗

arXiv2019

Quantum cascade laser-pumped terahertz molecular lasers: frequency noise and phase-locking using a 1560nm frequency comb

The recent demonstration of a terahertz (THz) molecular gas laser pumped by a mid-infrared quantum cascade laser (QCL) has opened up new perspectives for this family of sources, traditionally relying on CO2-laser pumping. A so far open question concerning QCL-pumped THz molecular lasers (MLs) is related to their spectral purity. Indeed, assessing their frequency/phase noise is crucial for a number of applications potentially exploiting these sources as local oscillators. Here this question is addressed by reporting the measurement of the frequency noise power spectral density (PSD) of a THz ML pumped by a 10.3μm-wavelength QCL, and emitting 1mW at 1.1THz in continuous wave. This is achieved by beating the ML frequency with the 1080th harmonic of the repetition rate of a 1560nm frequency comb. We find a frequency noise PSD < 10Hz2/Hz (-95dBc/Hz) at 100kHz from the carrier. To demonstrate the effect of the stability of the pump laser on the spectral purity of the THz emission we also measure the frequency noise PSD of a CO2-laser-pumped 2.5THz ML, reaching 0.1Hz2/Hz (-105dBc/Hz) at 40kHz from the carrier, limited by the frequency noise of the frequency comb harmonic. Finally, we show that it is possible to actively phase-lock the QCL-pumped molecular laser to the frequency comb repetition rate harmonic by controlling the QCL current, demonstrating a sub-Hz linewidth.

physics.optics↗

arXiv2017

Optomechanical THz detection with a sub-wavelength resonator

The terahertz (THz) spectral domain offers a myriad of applications spanning chemical spectroscopy, medicine, security and imaging[1]. It has also recently become a playground for fundamental studies of light-matter interactions [2-6]. THz science and technology could benefit from optomechanical approaches, which harness the interaction of light with miniature mechanical resonators [7,8]. So far, optomechanics has mostly focused on the optical and microwave domains, leading to new types of quantum experiments [9-11] and to the development of optical-microwave converters [12-14]. Here we demonstrate an integrated meta-atom [15] THz resonator with a flexible part acting as a mechanical oscillator. In this device free space THz photons are collected by the resonator and induce high frequency currents and charges that, in turn, couple to the mechanical degrees of freedom. The resulting mechanical motion is read-out optically, allowing our device to function as a compact and efficient terahertz detector at room temperature. Furthermore the device operates at high modulation frequencies (>10MHz), well beyond the cut-off frequencies of Golay cells, pyroelectric detectors and cryogenic semiconductor bolometers [16,17]. Notably, our experiments unambiguously reveal an instantaneous THz detection mechanism arising from a nano-scale Coulomb interaction, with a Noise Equivalent Power that is potentially frequency independent. Alongside this effect, our compact geometry allows for an uncooled bolometric detection [18] with extremely short heat diffusion times (few microseconds) and high detectivity.

physics.optics↗

arXiv2013

Continuous-wave coherent imaging with terahertz quantum cascade lasers using electro-optic harmonic sampling

We demonstrate a coherent imaging system based on a terahertz (THz) frequency quantum cascade laser (QCL) phase-locked to a near-infrared fs-laser comb. The phase locking enables coherent electro-optic sampling of the continuous-wave radiation emitted by the QCL through the generation of a heterodyne beat-note signal. We use this beat-note signal to demonstrate raster scan coherent imaging using a QCL emitting at 2.5 THz. At this frequency the detection noise floor of our system is of 3 pW/Hz and the long-term phase stability is <3 degrees/h, limited by the mechanical stability of the apparatus.

physics.optics↗