arXiv subjects

Stephen M. Morris

Publications and source records attributed to Stephen M. Morris.

15 recordsLinked to original sources

arXiv2026

Field-Programmable Topological Torons in Chiral Nematic Liquid Crystals

Torons are three-dimensional double-twist solitons in chiral nematic liquid crystals that form localised director configurations protected by topology and bounded by closed defect loops. They behave as particle-like entities while retaining a fully reconfigurable optical response. Here it is shown experimentally that individual torons can be created, steered and parked on demand using tailored alternating-current electric fields in planar cells, enabling deterministic control of both position and trajectory. By tuning the ratio of cell thickness to cholesteric pitch and systematically adjusting waveform parameters, including amplitude, modulation frequency, duty-cycle asymmetry and small DC offsets, robust toron nucleation is achieved and programmable translation is realised along arbitrary in-plane directions with submicrometre placement accuracy. Directional transport is controlled within a defined frequency and temperature window and can be reversed by changing modulation conditions even at zero offset. A dedicated graphical interface enables real-time switching between waveform presets so that torons follow scripted paths and draw user-defined shapes. Quantitative Landau-de Gennes Q-tensor simulations reproduce toron nucleation and the ensuing translational dynamics, supporting an interpretation in which waveform-controlled director reorientation, reorientation-driven flow and rectified polarity-sensitive coupling jointly bias the drift. Finally, three proof-of-concept functions are demonstrated: a software-defined liquid-crystal racetrack memory analogue with optical readout, deterministic path writing for reconfigurable patterning, and toron-mediated pick-and-place transport of microparticles for micromanipulation.

cond-mat.mtrl-sci↗

arXiv2026

Tunable Dynamic Speckle Generation for Random Illumination Microscopy

Speckled illumination enhances widefield fluorescence microscopy by enabling optical sectioning and super resolution. In random illumination microscopy, sequences of speckled illumination patterns are used to excite fluorescent samples and images are reconstructed based on a statistical analysis of the intensity fluctuations. Although random illumination microscopy has been shown to give excellent performance, its widespread implementation is hindered by the high cost and complexity of the generation of suitable speckled illumination patterns, which is achieved using digital micro-mirror devices or spatial light modulators. Here, we present a zwitterion-doped liquid crystal (LC) device capable of generating independent, high-contrast speckle patterns with a tunable decorrelation time in the 0.1 s to 0.1 ms range under visible laser illumination. This LC-based dynamic speckle generator is applied to widefield random illumination fluorescence microscopy of tissue and cell samples, where it enables optical sectioning with a 2 micron axial resolution, and a 1.5-fold improvement in lateral spatial resolution. Owing to its low cost and simplicity, this LC speckle generator offers an attractive alternative to digital micro-mirror and spatial light modulator devices for implementing widefield random illumination microscopy.

physics.optics↗

arXiv2026

Topologically robust programmable logic arrays using light and matter skyrmions

Photonic computing offers a low-power, high-bandwidth paradigm for information processing; however, the analogue nature of conventional architectures means that intrinsic noise and fabrication imperfections greatly impact performance, thereby severely limiting scalability. Recent work on optical skyrmions offers a route to overcoming these limitations by exploiting perturbation-resilient topological invariants assigned to the optical field for computation. Crucially, owing to its relative novelty, an architectural perspective on integrating individual components that manipulate topological charge into a functional system remains an important open goal. In this paper, we take concrete steps toward system-level design by introducing a platform-independent architecture for skyrmion-based logic, built around a modular library of topologically robust optical primitives, including generators, converters, registers, and adders. This framework enables the synthesis and arithmetic manipulation of topological numbers within a unified programmable architecture. We then experimentally validate this approach using multichannel arrays, demonstrating accurate charge readout and high robustness against alignment errors and environmental noise. These results provide a scalable foundation for topologically robust programmable logic arrays, paving the way for compact and integrated photonic processing circuits.

physics.optics↗

arXiv2025

Full vectorial field sensing using liquid crystal droplet arrays

Determining the amplitude, phase, and polarization profile of light is essential for both fundamental scientific discovery and applications spanning optical metrology, microscopy, astronomy, and optical communication/computing technologies. However, most modern measurement approaches are unable to retrieve such parameters readily, often relying on bulky and expensive hardware, or lacking the capability for single-shot sensing. Here, we introduce a low cost, compact, full vectorial field sensor based on an inkjet-printed nematic liquid crystal droplet array that enables simultaneous measurement of these important characteristics of light. Polarization and intensity are measured via division-of-wavefront polarimetry, exploiting the droplets' spatially varying birefringence, while the phase is reconstructed by treating each droplet as a separate microlens in a Shack-Hartmann-like wavefront sensor configuration. To demonstrate the system's performance, we characterize aberrated dual-wavelength beams carrying distinct intensity, phase, and polarization information, confirming accurate retrieval of the optical field profiles for both spectral components.

physics.optics↗

arXiv2025

Speckle suppression in digital in-line holographic microscopy through liquid crystal dynamic scattering

We demonstrate speckle noise reduction in an in-line holographic imaging system using a Zwitterion-doped liquid crystal dynamic scatterer (LCDS) cell diffuser. Integrated into a minimally modified bright-field microscope, the LCDS actively modulates system's spatial coherence. The proposed solution suppresses coherent artifacts without introducing bulky moving parts, while enhancing image resolution and preserving overall system simplicity. Quantitative performance tested on a phase and amplitude test targets, as well as phase-amplitude biological sample, shows significant noise reduction and methods versatility. Though validated in a holographic in-line setup, the approach is applicable to other imaging techniques requiring compact, vibration-free speckle suppression.

physics.optics↗

arXiv2025

Inkjet Printed Liquid Crystal Droplet for Complex Beam Manipulation

The inkjet-fabricated liquid crystal (LC) droplet device not only capitalizes on the intrinsic birefringence properties of liquid crystals but also leverages the hemispherical shape of droplet devices on substrates. This configuration facilitates self-alignment of the LC director under the influence of surface tension. The LC droplet devices we fabricated are capable of intricate beam manipulation, encompassing both generation and analysis of light beams. Such devices possess substantial prospective applications in the fields of optical communications and light beam characterization, highlighting their significant potential for advancement in optical technologies.

physics.optics↗

arXiv2025

Complex structured light generation using printed liquid crystal droplets

Inkjet-printed liquid crystal (LC) droplets exhibit an intricate spatially-varying birefringence due to their complex internal director configuration. While such anisotropy is often viewed as a drawback when LC droplets are used as microlenses, here we leverage this remarkable birefringence property to generate complex structured light. Through a selection of the alignment layer, and by varying the chiral pitch, we create three distinct droplet types with tailored intrinsic director configurations, each exhibiting a unique birefringence distribution for structured light beam generation. We show that these printed LC droplets can generate beams that exhibit skyrmionic structures carrying two units of orbital angular momentum, beams that contain azimuthal/radial polarized fields, and beams with polarization singularities. Our method enables new possibilities for using LC droplet technology to engineer sophisticated optical beam patterns.

physics.optics↗

arXiv2025

Physically Plausible Vectorial Metrics for Polarization Information Analysis

The Mueller Matrix Polar Decomposition method decomposes a Mueller matrix into a diattenuator, a retarder, and a depolarizer. Among these elements, the retarder, which plays a key role in medical and material characterization, is modelled as a circular retarder followed by a linear retarder when using this approach. However, this model may not accurately reflect the actual structure of the retarder in certain cases, as many practical retarders do not have a layered structure or consist of multiple (unknown) layers. Misinterpretation, therefore, may occur when the actual structure differs from the model. Here we circumvent this limitation by proposing to use a physically plausible parameter set that includes the axis orientation angle $ϕ$, the degree of ellipticity $χ$, and the elliptical retardance $ρ$. By working with this set of parameters, an overall characterization of a retarder is provided, encompassing its full optical response without making any assumptions about the structure of the material. In this study, experiments were carried out on liquid crystalline samples to validate the feasibility of our approach, demonstrating that the physically plausible parameter set adopted provides a useful tool for a broader range of applications in both biomedical imaging and optical material analysis.

physics.optics↗

arXiv2025

Intensity adaptive optics

Adaptive optics (AO) is a powerful tool employed across various research fields, from aerospace to microscopy. Traditionally, AO has focused on correcting optical phase aberrations, with recent advances extending to polarisation compensation. However, intensity errors are also prevalent in optical systems, yet effective correction methods are still in their infancy. Here, we introduce a novel AO approach, termed intensity adaptive optics (I-AO), which employs a dual-feedback loop mechanism to first address non-uniform intensity distribution and subsequently compensate for energy loss at the pupil plane. We demonstrate that I-AO can operate in both sensor-based and sensorless formats and validate its feasibility by quantitatively analysing the focus quality of an aberrated system. This technique expands the AO toolkit, paving the way for next-generation AO technology.

physics.optics↗

arXiv2024

Fine-tuning the Microstructure and Photophysical Characteristics of Fluorescent Conjugated Copolymers Using Photoalignment and Liquid-crystalline Ordering

Replicating the microstructure and near-unity excitation energy transfer efficiency in natural light-harvesting complexes (LHCs) remains a major challenge for synthetic energy-harvesting devices. Biological photosynthesis can spontaneously regulate the active ensembles of involved energy absorbing and funnelling chlorophyll-containing proteins in response to fluctuating sunlight. Here we utilize liquid crystalline (LC) ordering to fine-tune the polymer packing and photophysical properties in liquid crystalline conjugated polymer (LCCP) films for LHC biomimicry and optimizing photoluminescence quantum efficiency (PLQE). We show that the long-range orientational ordering present in a LC phase of poly(9,9-dioctylfluorene-co-benzothiadiazole) (F8BT) stabilizes a small fraction of randomly-oriented F8BT nanocrystals dispersed in an amorphous matrix of disordered F8BT chains, hence resembling a self-doped host-guest system whereby excitation energy funnelling and PLQE are reinforced significantly by three-dimensional donor-to-acceptor Forster resonance energy transfer (FRET) and dominant intrachain emission in the nano-crystalline acceptor. Furthermore, the photoalignment of nematic F8BT layers is combined to fabricate long-sought large-area-extended monodomains which exhibit >60% crystallinity and ~20 nm-long interchain packing order, whilst also promoting linearly polarized emission, a new band-edge absorption species, and an extra emissive interchain excited state. Our micro-PL spectral results support the feasibility of making use of self-doped F8BT nematic films for bio-mimicry of certain structural basis and light-harvesting properties of naturally occurring LHCs.

cond-mat.soft↗

arXiv2023

High-precision optical fiber sensing beyond 1000°C

Sapphire fiber can withstand around 2000°C, but it is multimoded, giving poor precision sensors. We demonstrate a single-mode sapphire fiber Bragg grating temperature sensor operating up to 1200°C. The repeatability above 1000°C is within {\pm}0.08%.

physics.optics↗

arXiv2023

Topologically controlled multiskyrmions in photonic gradient-index lenses

Skyrmions are topologically protected quasiparticles, originally studied in condensed-matter systems and recently in photonics, with great potential in ultra-high-capacity information storage. Despite the recent attention, most optical solutions require complex and expensive systems yet produce limited topologies. Here we demonstrate an extended family of quasiparticles beyond normal skyrmions, which are controlled in confined photonic gradient-index media, extending to higher-order members such as multiskyrmions and multimerons, with increasingly complex topologies. We introduce new topological numbers to describe these complex photonic quasiparticles and propose how this new zoology of particles could be used in future high-capacity information transfer. Our compact creation system lends integrated and programmable solutions of complex particle textures, with potential impacts on both photonic and condensed-matter systems for revolutionizing topological informatics and logic devices.

physics.optics↗

arXiv2022

Surface modulation of metal-organic frameworks for on-demand photochromism in the solid state

Organic photoswitchable molecules have struggled in solid state form to fulfill their remarkable potential, in terms of photoswitching performance and long-term stability when compared to their inorganic counterparts. We report the concept of non-electron deficient host's surface with optimal porosity and hydrophobicity, as a priori strategy to design photoefficient organic solid-state photochromic materials with outstanding mechanical robustness. When exposed to a light stimulus including natural sunlight, the photoswitchable nanocomposite changes color promptly and reversibly, in a matter of seconds along with excellent photo-fatigue resistance, which are on a par with inorganic photochromes. Exemplars of commercially viable prototypes that are optically clear, comprising smart windows, complex photochromic sculptures, and self-erasing rewritable devices, were engineered by direct blending with resilient polymers; particularly, the use of high-stiffness polymer (> 2 GPa) is no longer an insurmountable challenge. Finally, photochromic films with anticounterfeiting features could be manufactured through precision inkjet printing of nanocrystals.

physics.app-ph↗

arXiv2022

Nano-Trap Engineering in MOF Microenvironment for Ultratrace Iodine Sensors

Ultra-sensitive and highly selective iodine gas sensors play a crucial role during the nuclear radiation leak for a timely detection and mitigation of pollution, ensuring the safety of a vast number of operators and subsequent integrity of the facility. Herein, we rationally designed a metal-organic framework (MOF) that exhibits an outstanding performance with an almost billion-fold enhancement in the electrical response due to its optimized hydrophobicity, which allows the easy migration of iodine molecules though the channels and the presence of suitable interaction sites, temporarily anchoring the target molecule for ultra-trace sensing. The prototype sensor tested in demanding environments demonstrates its high selectivity, ultra-trace parts per billion (ppb)-level sensitivity, good reversibility, and a very fast response time even at high frequencies compared to existing adsorbents, including commercially available materials. Further, the iodine sensing at the atomic level was studied in detail by measuring the electrical response of a single crystal and, the optimal thickness of the MOF layer was identified for an industrially-viable prototype sensor by using inkjet printing. In a wider perspective, we propose a general strategy towards electrically efficient sensing materials with hybrid functionalities for engineering high-sensitivity iodine sensors for a safe and sustainable future.

physics.ins-det↗

arXiv2021

Single-mode sapphire fiber Bragg grating

We present here the inscription of single-mode waveguides with Bragg gratings in sapphire. The waveguide Bragg gratings have a novel multi-layer depressed cladding design in the 1550 nm telecommunications waveband. The Bragg gratings have a narrow bandwidth (<0.5 nm) and have survived annealing at 1000°C. The structures are inscribed with femtosecond laser direct writing, using adaptive beam shaping with a non-immersion objective. A single-mode sapphire fiber Bragg grating is created by writing a waveguide with a Bragg grating within a 425 μm diameter sapphire optical fiber, providing significant potential for accurate remote sensing in ultra-extreme environments.

physics.optics↗