arXiv subjects

Steven L. Rolston

Publications and source records attributed to Steven L. Rolston.

16 recordsLinked to original sources

arXiv2026

BIFROST: A First-Principles Model of Polarization Mode Dispersion in Optical Fiber

We present BIFROST, a first-principles model of polarization mode dispersion (PMD) in optical fibers. Unlike conventional models, BIFROST employs physically motivated representations of the PMD properties of fibers, allowing users to computationally investigate real-world fibers in ways that are connected to physical parameters such as environmental temperature and external stresses. Our model, implemented in an open-source Python module, incorporates birefringence from core geometry, material properties, environmental stress, and fiber spinning. We validate our model by examining commercial fiber specifications, fiber-paddle measurements, and published PMD statistics for deployed fiber links, and we showcase BIFROST's predictive power by considering wavelength-division-multiplexed PMD compensation schemes for polarization-encoded quantum networks. BIFROST's physical grounding enables investigations into such questions as the sensitivity of fiber sensors, the evaluation of PMD mitigation strategies in quantum networks, and many more applications across fiber technologies.

physics.optics↗

arXiv2022

Quantum Non-Demolition Photon Counting in a 2d Rydberg Atom Array

Rydberg arrays merge the collective behavior of ordered atomic arrays with the controllability and optical nonlinearities of Rydberg systems, resulting in a powerful platform for realizing photonic many-body physics. As an application of this platform, we propose a protocol for quantum non-demolition (QND) photon counting. Our protocol involves photon storage in the Rydberg array, an observation phase consisting of a series of Rabi flops to a Rydberg state and measurements, and retrieval of the stored photons. The Rabi frequency experiences a $\sqrt{n}$ collective enhancement, where $n$ is the number of photons stored in the array. Projectively measuring the presence or absence of a Rydberg excitation after oscillating for some time is thus a weak measurement of photon number. We demonstrate that the photon counting protocol can be used to distill Fock states from arbitrary pure or mixed initial states and to perform photonic state discrimination. We confirm that the protocol still works in the presence of experimentally realistic noise.

quant-ph↗

arXiv2021

Observation of vacuum-induced collective quantum beats

We demonstrate collectively enhanced vacuum-induced quantum beat dynamics from a three-level V-type atomic system. Exciting a dilute atomic gas of magneto-optically trapped $^{85}$Rb atoms with a weak drive resonant on one of the transitions, we observe the forward-scattered field after a sudden shut-off of the laser. The subsequent radiative dynamics, measured for various optical depths of the atomic cloud, exhibits superradiant decay rates, as well as collectively enhanced quantum beats. Our work is also the first experimental illustration of quantum beats arising from atoms initially prepared in a single excited level as a result of the vacuum-induced coupling between excited levels.

quant-ph↗

arXiv2020

Resonant enhancement of three-body loss between strongly interacting photons

Rydberg polaritons provide an example of a rare type of system where three-body interactions can be as strong or even stronger than two-body interactions. The three-body interactions can be either dispersive or dissipative, with both types possibly giving rise to exotic, strongly-interacting, and topological phases of matter. Despite past theoretical and experimental studies of the regime with dispersive interaction, the dissipative regime is still mostly unexplored. Using a renormalization group technique to solve the three-body Schrödinger equation, we show how the shape and strength of dissipative three-body forces can be universally enhanced for Rydberg polaritons. We demonstrate how these interactions relate to the transmission through a single-mode cavity, which can be used as a probe of the three-body physics in current experiments.

cond-mat.quant-gas↗

arXiv2020

Tunable three-body loss in a nonlinear Rydberg medium

Long-range Rydberg interactions, in combination with electromagnetically induced transparency (EIT), give rise to strongly interacting photons where the strength, sign, and form of the interactions are widely tunable and controllable. Such control can be applied to both coherent and dissipative interactions, which provides the potential to generate novel few-photon states. Recently it has been shown that Rydberg-EIT is a rare system in which three-body interactions can be as strong or stronger than two-body interactions. In this work, we study a three-body scattering loss for Rydberg-EIT in a wide regime of single and two-photon detunings. Our numerical simulations of the full three-body wavefunction and analytical estimates based on Fermi's Golden Rule strongly suggest that the observed features in the outgoing photonic correlations are caused by the resonant enhancement of the three-body losses.

quant-ph↗

arXiv2020

Exotic photonic molecules via Lennard-Jones-like potentials

Ultracold systems offer an unprecedented level of control of interactions between atoms. An important challenge is to achieve a similar level of control of the interactions between photons. Towards this goal, we propose a realization of a novel Lennard-Jones-like potential between photons coupled to the Rydberg states via electromagnetically induced transparency (EIT). This potential is achieved by tuning Rydberg states to a F{ö}rster resonance with other Rydberg states. We consider few-body problems in 1D and 2D geometries and show the existence of self-bound clusters ("molecules") of photons. We demonstrate that for a few-body problem, the multi-body interactions have a significant impact on the geometry of the molecular ground state. This leads to phenomena without counterparts in conventional systems: For example, three photons in 2D preferentially arrange themselves in a line-configuration rather than in an equilateral-triangle configuration. Our result opens a new avenue for studies of many-body phenomena with strongly interacting photons.

cond-mat.quant-gas↗

arXiv2020

Non-Markovian collective emission from macroscopically separated emitters

We study the collective radiative decay of a system of two two-level emitters coupled to a one-dimensional waveguide in a regime where their separation is comparable to the coherence length of a spontaneously emitted photon. The electromagnetic field propagating in the cavity-like geometry formed by the emitters exerts a retarded backaction on the system leading to strongly non-Markovian dynamics. The collective spontaneous emission rate of the emitters exhibits an enhancement or inhibition beyond the usual Dicke super- and sub-radiance due to a self-consistent coherent time-delayed feedback.

quant-ph↗

arXiv2018

A Wavefunction Microscope for Ultracold Atoms

Quantum simulations with ultracold atoms typically create atomic wavefunctions with structures at optical length scales, where direct imaging suffers from the diffraction limit. In analogy to advances in optical microscopy for biological applications, we use a non-linear atomic response to surpass the diffraction limit. Exploiting quantum interference, we demonstrate imaging with super-resolution of $λ/100$ and excellent temporal resolution of 500 ns. We characterize our microscope's performance by measuring the ensemble averaged wavefunction of atoms within the unit cells of an optical lattice, and observe the dynamics of atoms excited into periodic motion. This approach can be readily applied to image any atomic or molecular system, as long as it hosts a three-level system.

cond-mat.quant-gas↗

arXiv2018

Optimal and Secure Measurement Protocols for Quantum Sensor Networks

Studies of quantum metrology have shown that the use of many-body entangled states can lead to an enhancement in sensitivity when compared to product states. In this paper, we quantify the metrological advantage of entanglement in a setting where the quantity to be measured is a linear function of parameters coupled to each qubit individually. We first generalize the Heisenberg limit to the measurement of non-local observables in a quantum network, deriving a bound based on the multi-parameter quantum Fisher information. We then propose a protocol that can make use of GHZ states or spin-squeezed states, and show that in the case of GHZ states the procedure is optimal, i.e., it saturates our bound.

quant-ph↗

arXiv2017

Dark state optical lattice with sub-wavelength spatial structure

We report on the experimental realization of a conservative optical lattice for cold atoms with sub-wavelength spatial structure. The potential is based on the nonlinear optical response of three-level atoms in laser-dressed dark states, which is not constrained by the diffraction limit of the light generating the potential. The lattice consists of a 1D array of ultra-narrow barriers with widths less than 10~nm, well below the wavelength of the lattice light, physically realizing a Kronig-Penney potential. We study the band structure and dissipation of this lattice, and find good agreement with theoretical predictions. The observed lifetimes of atoms trapped in the lattice are as long as 60 ms, nearly $10^5$ times the excited state lifetime, and could be further improved with more laser intensity. The potential is readily generalizable to higher dimension and different geometries, allowing, for example, nearly perfect box traps, narrow tunnel junctions for atomtronics applications, and dynamically generated lattices with sub-wavelength spacings.

cond-mat.quant-gas↗

arXiv2017

Dissipation induced dipole blockade and anti-blockade in driven Rydberg systems

We study theoretically and experimentally the competing blockade and anti-blockade effects induced by spontaneously generated contaminant Rydberg atoms in driven Rydberg systems. These contaminant atoms provide a source of strong dipole-dipole interactions and play a crucial role in the system's behavior. We study this problem theoretically using two different approaches. The first is a cumulant expansion approximation, in which we ignore third-order and higher connected correlations. Using this approach for the case of resonant drive, a many-body blockade radius picture arises, and we find qualitative agreement with previous experimental results. We further predict that as the atomic density is increased, the Rydberg population's dependence on Rabi frequency will transition from quadratic to linear dependence at lower Rabi frequencies. We study this behavior experimentally by observing this crossover at two different atomic densities. We confirm that the larger density system has a smaller crossover Rabi frequency than the smaller density system. The second theoretical approach is a set of phenomenological inhomogeneous rate equations. We compare the results of our rate equation model to the experimental observations in [E. A. Goldschmidt, et al., PRL 116, 113001 (2016)] and find that these rate equations provide quantitatively good scaling behavior of the steady-state Rydberg population for both resonant and off-resonant drive.

quant-ph↗

arXiv2017

Super-radiance reveals infinite-range dipole interactions through a nanofiber

Atoms interact with each other through the electromagnetic field, creating collective states that can radiate faster or slower than a single atom, i.e. super- and sub-radiance. The generation and control of such states by engineering the dipolar interactions between atoms can enable new tools for atomic-based technologies. Atom-atom interactions in free space are limited in range, since the amplitude of the radiated field decreases inversely with distance. When the field is confined to one dimension it enables infinite-range interactions. This has been observed for atoms in an optical cavity, but remains to be proven in one-dimensional waveguides, where the extent of the interactions is not limited by the cavity size. Here we present the first report of infinite-range interactions between macroscopically separated atomic dipoles mediated by an optical waveguide. This is evidenced by the collective radiative decay of a single photon distributed between distant atoms. We use cold $^{87}$Rb atoms in the vicinity of a single-mode optical nanofiber (ONF) that coherently exchange evanescently coupled photons through the ONF mode. In particular, we observe super-radiance of a few atoms separated by hundreds of resonant wavelengths. This effect is not possible for atoms separated by more than a wavelength interacting through free space. The same platform allows us to measure sub-radiance, a rarely observed effect, presenting a novel tool for quantum optics. This result constitutes a proof-of-principle for collective behavior of macroscopically delocalized atomic states, a crucial element for new proposals in quantum information and many-body physics. Given the application of one-dimensional waveguides in photonic-based quantum technologies, we envision infinite-range interactions as the natural next step towards interconnecting quantum systems on scales suitable for practical applications.

quant-ph↗

arXiv2017

Alignment-dependent decay rate of an atomic dipole near an optical nanofiber

We study the modification of the atomic spontaneous emission rate, i.e. Purcell effect, of $^{87}$Rb in the vicinity of an optical nanofiber ($\sim$500 nm diameter). We observe enhancement and inhibition of the atomic decay rate depending on the alignment of the induced atomic dipole relative to the nanofiber. Finite-difference time-domain simulations are in quantitative agreement with the measurements when considering the atoms as simple oscillating linear dipoles. This is surprising since the multi-level nature of the atoms should produce a different radiation pattern, predicting smaller modification of the lifetime than the measured ones. This work is a step towards characterizing and controlling atomic properties near optical waveguides, fundamental tools for the development of quantum photonics.

quant-ph↗

arXiv2017

Optical Nanofibers: a new platform for quantum optics

The development of optical nanofibers (ONF) and the study and control of their optical properties when coupling atoms to their electromagnetic modes has opened new possibilities for their use in quantum optics and quantum information science. These ONFs offer tight optical mode confinement (less than the wavelength of light) and diffraction-free propagation. The small cross section of the transverse field allows probing of linear and non-linear spectroscopic features of atoms with exquisitely low power. The cooperativity -- the figure of merit in many quantum optics and quantum information systems -- tends to be large even for a single atom in the mode of an ONF, as it is proportional to the ratio of the atomic cross section to the electromagnetic mode cross section. ONFs offer a natural bus for information and for inter-atomic coupling through the tightly-confined modes, which opens the possibility of one-dimensional many-body physics and interesting quantum interconnection applications. The presence of the ONF modifies the vacuum field, affecting the spontaneous emission rates of atoms in its vicinity. The high gradients in the radial intensity naturally provide the potential for trapping atoms around the ONF, allowing the creation of one-dimensional arrays of atoms. The same radial gradient in the transverse direction of the field is responsible for the existence of a large longitudinal component that introduces the possibility of spin-orbit coupling of the light and the atom, enabling the exploration of chiral quantum optics.

quant-ph↗

arXiv2016

Near-field measurement of modal interference in optical nanofibers for sub-Angstrom radius sensitivity

Optical nanofibers (ONF) of subwavelength dimensions confine light in modes with a strong evanescent field that can trap, probe, and manipulate nearby quantum systems. To measure the evanescent field and propagating modes, and to optimize ONF performance, a surface probe is desirable during fabrication. We demonstrate a nondestructive measurement of light propagation in ONFs by sampling the local evanescent field with a microfiber. This approach reveals the behavior of all propagating modes, and because the modal beat lengths in cylindrical waveguides depend strongly on radius, simultaneously provides exquisite sensitivity to the ONF radius. We show that our measured spatial frequencies provide a map of the average ONF radius (over a 600 micrometer window) along the 10 mm ONF waist with 40 picometer resolution and high signal-to-noise ratio. The measurements agree with scanning electron microscopy (SEM) to within SEM instrument resolution. This fast method is immune to polarization, intrinsic birefringence, mechanical vibrations, scattered light, and provides a set of constraints to protect from systematic errors in the measurements

physics.optics↗

arXiv2015

Rayleigh scattering in an optical nanofiber as a probe of higher-order mode propagation

Optical nanofibers provide a rich platform for exploring atomic and optical phenomena even when they support only a single spatial mode. Nanofibers supporting higher-order modes provide additional degrees of freedom to enable complex evanescent field profiles for interaction with the surrounding medium, but local control of these profiles requires nondestructive evaluation of the propagating fields. Here, we use Rayleigh scattering for rapid measurement of the propagation of light in few-mode optical nanofibers. Imaging the Rayleigh scattered light provides direct visualization of the spatial evolution of propagating fields throughout the entire fiber, including the transition from core-cladding guidance to cladding-air guidance. We resolve the interference between higher-order modes to determine local beat lengths and modal content along the fiber, and show that the modal superposition in the waist can be systematically controlled by adjusting the input superposition. With this diagnostic we can measure variations in the radius of the fiber waist to below 3 nm in situ using purely optical means. This nondestructive technique also provides useful insight into light propagation in optical nanofibers.

quant-ph↗