arXiv subjects

Stuart J. Masson

Publications and source records attributed to Stuart J. Masson.

At least 19 recordsLinked to original sources

arXiv2026

Stabilization of dark states in emitter arrays coupled to a half-waveguide

The radiative properties of quantum emitters are profoundly influenced by their electromagnetic environment. When coupled to a waveguide terminated at one end by a mirror, distant emitters interact strongly via virtual photon exchange, leading to collective superradiant and subradiant states with enhanced or suppressed decay rates. We demonstrate that applying optimal frequency shifts to each emitter enables the formation of perfect single-excitation dark states (i.e. states with zero decay rate) and near-perfect multi-excitation dark states in small ensembles. These collective states can be deterministically prepared with high fidelity using classical driving fields or few-photon pulses propagating along the waveguide. These results, readily implementable in superconducting qubit platforms, open new avenues for quantum information storage, networking and control of light.

quant-ph↗

arXiv2026

Emergent non-Markovianity in time-delayed waveguide QED

Quantum systems are invariably coupled to a surrounding environment. A common theoretical method to simplify the problem is to trace over the environment under a Markov approximation, which assumes that the environment holds no memory over the timescales that the system evolves under. In interacting many-body systems, it is often not trivial to extract which of the multiple collective timescales are relevant. We consider a time-delayed waveguide QED setup with a single excitation. By fixing the maximum propagation time and increasing the number of emitters, we show that, even for small delay times, collective effects are sufficient to cause non-Markovianity. The impact of memory is intrinsically state-dependent. For superradiant states, the relevant system timescale is the superradiant lifetime while the relevant bath timescale is the end-to-end delay time. For subradiant states, both timescales depend on the structure of the specific state. Our results demonstrate the importance of prudently making Markov approximations in quantum many-body systems, and highlight potential pitfalls to avoid in scaling up quantum devices to large system sizes.

quant-ph↗

arXiv2025

Exact Many-body Quantum Dynamics in One-Dimensional Baths via Collective Spins

Computing the exact dynamics of many-body quantum systems becomes intractable as system size grows. Here, we present a symmetry-based method that provides an exponential reduction in the complexity of a broad class of such problems $\unicode{x2014}$ qubits coupled to one-dimensional electromagnetic baths. We identify conditions under which partial permutational symmetry emerges and exploit it to group qubits into collective multi-level degrees of freedom, which we term ''superspins.'' These superspins obey a generalized angular momentum algebra, reducing the relevant Hilbert space dimension from exponential to polynomial. Using this framework, we efficiently compute many-body superradiant dynamics in large arrays of qubits coupled to waveguides and ring resonators, showing that $\unicode{x2014}$ unlike in conventional Dicke superradiance $\unicode{x2014}$ the total spin length is not conserved. At long times, dark states become populated. We identify configurations where these states exhibit metrologically useful entanglement. Our approach enables exact treatment of complex dissipative dynamics beyond the fully symmetric limit and provides a rigorous benchmark for approximate numerical methods.

quant-ph↗

arXiv2024

Optomechanical self-organization in a mesoscopic atom array

Increasing the number of particles in a system often leads to qualitative changes in its properties, such as breaking of symmetries and the appearance of phase transitions. This renders a macroscopic system fundamentally different from its individual microscopic constituents. Lying between these extremes, mesoscopic systems exhibit microscopic fluctuations that influence behavior on longer length scales, leading to critical phenomena and dynamics. Therefore, tracing the properties of well-controlled mesoscopic systems can help bridge the gap between an exact description of few-body microscopic systems and the emergent description of many-body systems. Here, we explore mesoscopic signatures of an optomechanical self-organization phase transition using arrays of cold atoms inside an optical cavity. By precisely engineering atom-cavity interactions, we reveal how critical behavior depends on atom number, identify characteristic dynamical behaviors in the self-organized regime, and observe a finite optomechanical susceptibility at the critical point. These findings advance our understanding of particle-number- and time-resolved properties of phase transitions in mesoscopic systems.

quant-ph↗

arXiv2024

Deterministic generation of photonic entangled states using decoherence-free subspaces

We propose the use of collective states of matter as a resource for the deterministic generation of quantum states of light, which are fundamental for quantum information technologies. Our minimal model consists of three emitters coupled to a half-waveguide, i.e., a one-dimensional waveguide terminated by a mirror. Photon-mediated interactions between the emitters result in the emergence of bright and dark states. The dark states form a decoherence-free subspace, protected from dissipation. Local driving of the emitters and control of their resonance frequencies allows to perform arbitrary quantum gates within the decoherence-free subspace. Coupling to bright states facilitates photon emission, thereby enabling the realization of quantum gates between light and matter. We demonstrate that sequential application of these gates leads to the generation of photonic entangled states, such as Greenberger-Horne-Zeilinger and one- and two-dimensional cluster states.

quant-ph↗

arXiv2024

Dicke superradiance in ordered lattices: dimensionality matters

Dicke superradiance in ordered atomic arrays is a phenomenon where atomic synchronization gives rise to a burst in photon emission. This superradiant burst only occurs if there is one -- or just a few -- dominant decay channels. For a fixed atom number, this happens only below a critical interatomic distance. Here we show that array dimensionality is the determinant factor that drives superradiance. In 2D and 3D arrays, superradiance occurs due to constructive interference, which grows stronger with atom number. This leads to a critical distance that scales sublogarithmically with atom number in 2D, and as a power law in 3D. In 1D arrays, superradiance occurs due to destructive interference that effectively switches off certain decay channels, yielding a critical distance that saturates with atom number. Our results provide a guide to explore many-body decay in state-of-the art experimental setups.

quant-ph↗

arXiv2024

Ground-state selection via many-body superradiant decay

For a single particle, relaxation into different ground states is governed by fixed branching ratios determined by the transition matrix element and the environment. Here, we show that in many-body open quantum systems the occupation probability of one ground state can be boosted well beyond what is dictated by single-particle branching ratios. Despite the competition, interactions suppress all but the dominant decay transition, leading to a 'winner takes all' dynamic where the system primarily settles into the dominant ground state. We prove that, in the presence of permutation symmetry, this problem is exactly solvable for any number of competing channels. Additionally, we develop an approximate model for the dynamics by mapping the evolution onto a fluid continuity equation, and analytically demonstrate that the dominant transition ratio converges to unity as a power law with increasing system size, for any branching ratios. This near-deterministic preparation of the dominant ground state has broad applicability. As an example, we discuss a protocol for molecular photoassociation where collective dynamics effectively acts as a catalyst, amplifying the yield in a specific final state. Our results open new avenues for many-body strategies in the preparation and control of quantum systems.

quant-ph↗

arXiv2024

State-insensitive wavelengths for light shifts and photon scattering from Zeeman states

Atoms are not two-level systems, and their rich internal structure often leads to complex phenomena in the presence of light. Here, we analyze off-resonant light scattering including the full hyperfine and magnetic structure. We find a set of frequency detunings where the induced atomic dipole is the same irrespective of the Zeeman state, and where two-photon transitions that alter the atomic state turn off. For alkali atoms and alkaline-earth ions, if the hyperfine splitting is dominated by the magnetic dipole moment contribution, these detunings approximately coincide. Therefore, at a given ``magical'' detuning, all Zeeman states in a hyperfine manifold behave almost identically, and can be traced out to good approximation. This feature prevents state decoherence due to light scattering, which impacts quantum optics experiments and quantum information applications.

quant-ph↗

arXiv2024

Dicke superradiance in ordered arrays of multilevel atoms

In inverted atomic ensembles, photon-mediated interactions give rise to Dicke superradiance, a form of many-body decay that results in a rapid release of energy as a photon burst. While originally studied in pointlike ensembles, this phenomenon persists in extended ordered systems if the inter-particle distance is below a certain bound. Here, we investigate Dicke superradiance in a realistic experimental setting using ordered arrays of alkaline-earth(-like) atoms, such as strontium and ytterbium. Such atoms offer exciting new opportunities for light-matter interactions as their internal structure allows for trapping at short interatomic distances compared to their long-wavelength transitions, providing the potential for collectively enhanced dissipative interactions. Despite their intricate electronic structure, we show that two-dimensional arrays of these atomic species should exhibit many-body superradiance for achievable lattice constants. Moreover, superradiance effectively ``closes'' transitions, such that multilevel atoms become more two-level like. This occurs because the avalanchelike decay funnels the emission of most photons into the dominant transition, overcoming the single-atom decay ratios dictated by their fine structure and Zeeman branching. Our work represents an important step in harnessing alkaline-earth atoms as quantum optical sources and as platforms to explore many-body dissipative dynamics.

quant-ph↗

arXiv2023

Super-radiant and Sub-radiant Cavity Scattering by Atom Arrays

We realize collective enhancement and suppression of light scattered by an array of tweezer-trapped $^{87}$Rb atoms positioned within a strongly coupled Fabry-Pérot optical cavity. We illuminate the array with light directed transverse to the cavity axis, in the low saturation regime, and detect photons scattered into the cavity. For an array with integer-optical-wavelength spacing each atom scatters light into the cavity with nearly identical scattering amplitude, leading to an observed $N^2$ scaling of cavity photon number as the atom number increases stepwise from $N=1$ to $N=8$. By contrast, for an array with half-integer-wavelength spacing, destructive interference of scattering amplitudes yields a non-monotonic, sub-radiant cavity intensity versus $N$. By analyzing the polarization of light emitted from the cavity, we find that Rayleigh scattering can be collectively enhanced or suppressed with respect to Raman scattering. We observe also that atom-induced shifts and broadenings of the cavity resonance are precisely tuned by varying the atom number and positions. Altogether, tweezer arrays provide exquisite control of atomic cavity QED spanning from the single- to the many-body regime.

quant-ph↗

arXiv2023

Many-body superradiance and dynamical mirror symmetry breaking in waveguide QED

The many-body decay of extended collections of two-level systems remains an open problem. Here, we investigate whether an array of emitters coupled to a one-dimensional bath undergoes Dicke superradiance. This is a process whereby a completely inverted system becomes correlated via dissipation, leading to the release of all the energy in the form of a rapid photon burst. We derive the minimal conditions for the burst to happen as a function of the number of emitters, the chirality of the waveguide, and the single-emitter optical depth, both for ordered and disordered ensembles. Many-body superradiance occurs because the initial fluctuation that triggers the emission is amplified throughout the decay process. In one-dimensional baths, this avalanchelike behavior leads to a spontaneous mirror symmetry breaking, with large shot-to-shot fluctuations in the number of photons emitted to the left and right. Superradiant bursts may thus be a smoking gun for the generation of correlated photon states of exotic quantum statistics.

quant-ph↗

arXiv2022

Metasurface Holographic Optical Traps for Ultracold Atoms

We propose metasurface holograms as a novel platform to generate optical trap arrays for cold atoms with high fidelity, efficiency, and thermal stability. We developed design and fabrication methodologies to create dielectric, phase-only metasurface holograms based on titanium dioxide. We experimentally demonstrated optical trap arrays of various geometries, including periodic and aperiodic configurations with dimensions ranging from 1D to 3D and the number of trap sites up to a few hundred. We characterized the performance of the holographic metasurfaces in terms of the positioning accuracy, size and intensity uniformity of the generated traps, and power handling capability of the dielectric metasurfaces. Our proposed platform has great potential for enabling fundamental studies of quantum many-body physics, and quantum simulation and computation tasks. The compact form factor, passive nature, good power handling capability, and scalability of generating high-quality, large-scale arrays also make the metasurface platform uniquely suitable for realizing field-deployable devices and systems based on cold atoms.

physics.optics↗

arXiv2021

Semiclassical bifurcations and quantum trajectories: a case study of the open Bose-Hubbard dimer

We consider the open two-site Bose-Hubbard dimer, a well-known quantum mechanical model that has been realised recently for photons in two coupled photonic crystal nanocavities. The system is described by a Lindblad master equation which, for large numbers of photons, gives rise to a limiting semiclassical model in the form of a four-dimensional vector field. From the situation where both sites trap the same amount of photons under symmetric pumping, one encounters a transition that involves symmetry breaking, the creation of periodic oscillations and multistability as the pump strength is increased. We show that the associated one-parameter bifurcation diagram of the semiclassical model captures the essence of statistical properties of computed quantum trajectories as the pump strength is increased. Even for small numbers of photons, the fingerprint of the semiclassical bifurcations can be recognised reliably in observables of quantum trajectories.

quant-ph↗

arXiv2021

Generation of Spin Cat States in an Engineered Dicke Model

We study trajectories of collective spin states of an ensemble of spinors. The spinors considered here are either trapped ions in free space or atoms confined in a cavity, both systems of which are engineered through their interactions with light fields to obey an effective Dicke model. In an appropriate limit of the Dicke model, one obtains one-axis twisting dynamics of the collective spin and evolution after a finite time to a spin cat state, or, in the long-time limit, the Dicke state $|S,0\rangle_x$, conditioned upon there being no photon emissions from the system (i.e., no quantum jumps). If there is a jump, however, the system evolves probabilistically into one of a finite number of entangled-state cycles, where the system then undergoes a persistent sequence of jumps between two Dicke state superpositions in a rotated basis. The different cycles can be distinguished by the frequency at which jumps occur.

quant-ph↗

arXiv2020

Many-body Signatures of Collective Decay in Atomic Chains

Fully inverted atoms placed at exactly the same location synchronize as they deexcite, and light is emitted in a burst (known as "Dicke's superradiance"). We investigate the role of finite interatomic separation on correlated decay in mesoscopic chains, and provide an understanding in terms of collective jump operators. We show that the superradiant burst survives at small distances, despite Hamiltonian dipole-dipole interactions. However, for larger separations, competition between different jump operators leads to dephasing, suppressing superradiance. Collective effects are still significant for arrays with lattice constants of the order of a wavelength, and lead to a photon emission rate that decays nonexponentially in time. We calculate the two-photon correlation function and demonstrate that emission is correlated and directional, as well as sensitive to small changes in the interatomic distance. These features can be measured in current experimental setups, and are robust to realistic imperfections.

quant-ph↗

arXiv2020

Deterministic single-atom source of quasi-superradiant $N$-photon pulses

We propose a single-atom, cavity quantum electrodynamics system, compatible with recently demonstrated, fiber-integrated micro- and nano-cavity setups, for the on-demand production of optical number-state, $0N$-state, and binomial-code-state pulses. The scheme makes use of Raman transitions within an entire atomic ground-state hyperfine level and operates with laser and cavity fields detuned from the atomic transition by much more than the excited-state hyperfine splitting. This enables reduction of the dynamics to that of a simple, cavity-damped Tavis-Cummings model with the collective spin determined by the total angular momentum of the ground hyperfine level.

quant-ph↗

arXiv2018

Dicke model simulation via cavity-assisted Raman transitions

The Dicke model is of fundamental importance in quantum mechanics for understanding the collective behaviour of atoms coupled to a single electromagnetic mode. In this paper, we demonstrate a Dicke-model simulation using cavity-assisted Raman transitions in a configuration using counter-propagating laser beams. The observations indicate that motional effects should be included to fully account for the results and these results are contrasted with the experiments using single-beam and co-propagating configurations. A theoretical description is given that accounts for the beam geometries used in the experiments and indicates the potential role of motional effects. In particular a model is given that highlights the influence of Doppler broadening on the observed thresholds.

quant-ph↗

arXiv2017

Cavity QED engineering of spin dynamics and squeezing in a spinor gas

We propose a method for engineering spin dynamics in ensembles of integer-spin atoms confined within a high-finesse optical cavity. Our proposal uses cavity-assisted Raman transitions to engineer a Dicke model for integer-spin atoms, which, in a dispersive limit, reduces to effective atom-atom interactions within the ensemble. This scheme offers a promising and flexible new avenue for the exploration of a wide range of spinor many-body physics. As an example of this, we present results showing that this method can be used to generate spin-nematic squeezing in an ensemble of spin-1 atoms. With realistic parameters the scheme should enable substantial squeezing on time scales much shorter than current experiments with spin-1 Bose-Einstein condensates.

quant-ph↗