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Subhasish Chaki

Publications and source records attributed to Subhasish Chaki.

15 recordsLinked to original sources

Translational and Rotational Temperature Difference in Coexisting Phases of Inertial Active Dumbbells

We investigate the effect of translational and rotational inertia on motility-induced phase separation in underdamped active dumbbells and identify the emergence of four distinct kinetic temperatures across the coexisting phases-unlike in overdamped systems. We find that the dilute, gas-like phase consistently exhibits a higher translational kinetic temperature than the dense, liquid-like phase, with this difference amplified by increasing the rotational inertia. Rotational kinetic temperatures display a similar trend, with the dense phase remaining colder than the dilute phase; however, in this case the temperature difference grows with translational inertia and activity, while becoming practically independent of rotational inertia. This counterintuitive behavior arises from the interplay of activity-driven collisions with both translational and rotational inertia in the coexisting phases. Our results highlight the critical role of translational and rotational inertia in shaping the kinetic temperature landscape of motility-induced phase separation and offer new insights into the nonequilibrium thermodynamics of active matter.

cond-mat.soft

Anisotropic active Brownian particle in two dimensions under stochastic resetting

We analytically investigate the dynamic behavior of an an-isotropic active Brownian particle under various stochastic resetting protocols in two dimensions. The motion of shape-asymmetric active Brownian particles in two dimensions leads to an-isotropic diffusion at short times, whereas rotational diffusion causes the transport to become isotropic at longer times. We have considered three different resetting protocols: (a) complete resetting, when both position and orientation are reset to their initial states, (b) only position is reset to its initial state, (c) only orientation is reset to its initial state. We reveal that orientation resetting sustains asymmetry even at late times. When both the spatial position and orientation are subject to resetting, a complex position probability distribution forms in the steady state. All the analytical findings are thoroughly validated by corresponding simulation results.

cond-mat.stat-mech

Anisotropic Brownian particles under resetting

We study analytically the dynamics of an anisotropic particle subjected to different stochastic resetting schemes in two dimensions. The Brownian motion of shape-asymmetric particles in two dimensions results in anisotropic diffusion at short times, while the late-time transport is isotropic due to rotational diffusion. We show that the presence of orientational resetting promotes the anisotropy to late times. When the spatial and orientational degrees of freedom are reset, we find that a non-trivial spatial probability distribution emerges in the steady state that is determined by the initial orientation, particle asymmetry and the resetting rate. When only spatial degrees of freedom are reset while the orientational degree of freedom is allowed to evolve freely, the steady state is independent of the particle asymmetry. When only particle orientation is reset, the late-time probability density is given by a Gaussian with an effective diffusion tensor, including off-diagonal terms, determined by the resetting rate. Generally, the coupling between the translational and rotational degrees of freedom, when combined with stochastic resetting, gives rise to unique behaviour at late times not present in the case of symmetric particles. Considering recent developments in experimental implementations of resetting, our results can be useful for the control of asymmetric colloids, for example in self-assembly processes.

cond-mat.stat-mech

Dynamic Clustering of Active Rings

A collection of rings made of active Brownian particles (ABPs) for different packing fractions and activities is investigated using computer simulations. We show that active rings display an emergent dynamic clustering instead of the conventional motility-induced phase separation (MIPS) as in the case of collection of ABPs. Surprisingly, increasing packing fraction of rings exhibits a non-monotonicity in the dynamics due to the formation of a large number of small clusters. The conformational fluctuations of the polymers suppress the usual MIPS exhibited by ABPs. Our findings demonstrate how the motion of a collection of rings is influenced by the interplay of activity, topology, and connectivity.

cond-mat.soft

Active Dynamics of Linear Chains and Rings in Porous Media

To understand the dynamical and conformational properties of deformable active agents in porous media, we computationally investigate the dynamics of linear chains and rings made of active Brownian monomers. In porous media, flexible linear chains and rings always migrate smoothly and undergo activity-induced swelling. However, semiflexible linear chains though navigate smoothly, shrink at lower activities, followed by swelling at higher activities, while semiflexible rings exhibit a contrasting behavior. Semiflexible rings shrink, get trapped at lower activities, and escape at higher activities. This demonstrates how activity and topology interplay and control the structure and dynamics of linear chains and rings in porous media. We envision that our study will shed light on understanding the mode of transport of shape-changing active agents in porous media.

cond-mat.soft

Reconfiguration, swelling and tagged monomer dynamics of a single polymer chain in Gaussian and non-Gaussian active baths

In this topical review, we give an overview of the structure and dynamics of a single polymer chain in active baths, Gaussian or non-Gaussian. The review begins with the discussion of single flexible or semiflexible linear polymer chains subjected to two noises, thermal and active. The active noise has either Gaussian or non-Gaussian distribution but has a memory, accounting for the persistent motion of the active bath particles. This finite persistence makes the reconfiguration dynamics of the chain slow as compared to the purely thermal case and the chain swells. The active noise also results superdiffusive or ballistic motion of the tagged monomer. We present all the calculations in details but mainly focus on the analytically exact or almost exact results on the topic, as obtained from our group in recent years. In addition, we briefly mention important works of other groups and include some of our new results. The review concludes with pointing out the implications of polymer chains in active bath in biologically relevant context and its future directions.

cond-mat.soft

A Polymer Chain with Dipolar Active Forces in Connection to Spatial Organization of Chromatin

A living cell is an active environment where the organization and dynamics of chromatin are affected by different forms of activity. Optical experiments report that loci show subdiffusive dynamics and the chromatin fiber is seen to be coherent over micrometer-scale regions. Using a bead-spring polymer chain with dipolar active forces, we study how the subdiffusive motion of the loci generate large-scale coherent motion of the chromatin. We show that in the presence of extensile (contractile) activity, the dynamics of loci grows faster (slower) and the spatial correlation length increases (decreases) compared to the case with no dipolar forces. Hence, both the dipolar active forces modify the elasticity of the chain. Interestingly in our model, the dynamics and organization of such dipolar active chains largely differ from the passive chain with renormalized elasticity.

cond-mat.soft

Migration of Active Rings in Porous Media

Inspired by how the shape deformations in active organisms help them to migrate through disordered porous environments, we simulate active ring polymers in two-dimensional random porous media. Flexible and inextensible active ring polymers navigate smoothly through the disordered media. In contrast, semiflexible rings undergo transient trapping inside the pore space; the degree of trapping is inversely correlated with the increase in activity. We discover that flexible rings swell while inextensible and semiflexible rings monotonically shrink upon increasing the activity. Together, our findings identify the optimal migration of active ring polymers through porous media.

cond-mat.soft

Role of Dissipation on the Stability of a Parametrically Driven Quantum Harmonic Oscillator

We study the dissipative dynamics of a single quantum harmonic oscillator subjected to a parametric driving with in an effective Hamiltonian approach. Using Liouville von Neumann approach, we show that the time evolution of a parametrically driven dissipative quantum oscillator has a strong connection with the classical damped Mathieu equation. Based on the numerical analysis of the Monodromy matrix, we demonstrate that the dynamical instability generated by the parametric driving are reduced by the effect of dissipation. Further, we obtain a closed relationship between the localization of the Wigner function and the stability of the damped Mathieu equation.

quant-ph

Translational and rotational dynamics of a self-propelled Janus probe in crowded environments

We computationally investigate the dynamics of a self-propelled Janus probe in crowded environments. The crowding is caused by the presence of viscoelastic polymers or non-viscoelastic disconnected monomers. Our simulations show that the translational, as well as rotational mean square displacements, have a distinctive three-step growth for fixed values of self-propulsion force, and steadily increase with self-propulsion, irrespective of the nature of the crowder. On the other hand, in the absence of crowders, the rotational dynamics of the Janus probe is independent of self-propulsion force. On replacing the repulsive polymers with sticky ones, translational and rotational mean square displacements of the Janus probe show a sharp drop. Since different faces of a Janus particle interact differently with the environment, we show that the direction of self-propulsion also affects its dynamics. The ratio of long-time translational and rotational diffusivities of the self-propelled probe with a fixed self-propulsion, when plotted against the area fraction of the crowders, passes through a minima and at higher area fraction merges to its value in the absence of the crowder. This points towards the decoupling of translational and rotational dynamics of the self-propelled probe at intermediate area fraction of the crowders. However, such translational-rotational decoupling is absent for passive probes.

cond-mat.soft

Escape of a passive particle from activity-induced energy landscape: Emergence of slow and fast effective diffusion

Spontaneous persistent motions driven by active processes play a central role to maintain the living cells far from equilibrium. In the majority of the research works, the steady state dynamics of an active system has been described in terms of an effective temperature. In the majority of the research works, the steady state dynamics of an active system has been described in terms of an effective temperature. By contrast, we have examined a prototype model for diffusion in an activity-induced rugged energy landscape to describe the slow dynamics of a tagged particle in a dense active environment. The expression for the mean escape time from the active rugged energy landscape holds only in the limit of low activity and the mean escape time from the rugged energy landscape increases with activity. The precise form of the active correlation will determine whether the mean escape time will depend on the persistence time or not. The active rugged energy landscape approach also allows an estimate of non-equilibrium effective diffusivity characterizing the slow diffusive motion of the tagged particle due to activity. On the other hand, in a dilute environment, high activity augments the diffusion of the tagged particle. The enhanced diffusion can be attributed to an effective temperature, higher than the ambient temperature and is used to calculate the Kramers' mean escape time, which decreases with activity. Our results have direct relevance to recent experiments on tagged particle diffusion in condensed phases.

cond-mat.stat-mech

Transport of probe particles in polymer network: effects of probe size, network rigidity and probe-polymer interaction

Fundamental understanding of the effect of microscopic parameters on the dynamics of probe particles in different complex environments has wide implications. Examples include diffusion of proteins in the biological hydrogels, porous media, polymer matrix, etc. Here, we use extensive molecular dynamics simulations to investigate the dynamics of the probe particle in a polymer network on a diamond lattice which provides substantial crowding to mimic the cellular environment. Our simulations show that the dynamics of the probe increasingly becomes restricted, non-Gaussian and subdiffusive on increasing the network rigidity, binding affinity and the probe size. In addition, the velocity autocorrelation functions show negative dips owing to the viscoelasticity and caging due to surrounding network. These observations go with general experimental findings. Surprisingly for a probe particle of size comparable to the mesh size, unrestricted motion engulfing large length scales has been observed. This happens with the more flexible polymer network, which is easily pushed by the bigger probe. Our study gives a general qualitative picture of transport of probes in gel like medium, as encountered in different contexts.

cond-mat.soft

Effects of active fluctuations on energetics of a colloidal particle: superdiffusion, dissipation and entropy production

We consider a colloidal particle immersed in an active bath and derive a Smoluchowski equation that governs the dynamics of colloidal particle. We address this as active Smoluchowski equation. Our analysis based on this active Smoluchowski equation shows a short time superdiffusive behavior that strongly depends on the activity. Our model also predicts a non-monotonic dependence of mean energy dissipation against time, a signature of activity-induced dynamics. By introducing a frequency-dependent effective temperature, we show that the mean rate of entropy production is time dependent unlike a thermal system. The prime reason for these anomalies is the absence of any fluctuation-dissipation theorem for the active noise. We also comment on how microscopic details of activity can reverse the trends for mean energy dissipation and mean rate of entropy production.

cond-mat.stat-mech

Enhanced diffusion, swelling and slow reconfiguration of a single chain in non-Gaussian active bath

A prime example of non-equilibrium or active environment is a biological cell. In order to understand in-vivo functioning of biomolecules such as proteins, chromatins, a description beyond equilibrium is absolutely necessary. In this context, biomolecules have been modeled as Rouse chains in Gaussian active bath. However, these non-equilibrium fluctuations in biological cells are non-Gaussian. This motivates us to take a Rouse chain subjected to a series of pulses of force with finite duration, mimicking run and tumble motion of a class of micro-organisms. Thus by construction, this active force is non-Gaussian. Our analytical calculations show that the mean square displacement (MSD) of center of mass (COM) grows faster and even shows superdiffusive behavior at higher activity, supporting recent experimental observation on active enzymes (A.-Y. Jee, Y.-K. Cho, S. Granick, and T. Tlusty, Proc. Natl. Acad. Sci. 115, 10812 (2018)), but chain reconfiguration is slower. The reconfiguration time of a chain with N monomers scales as N^sigma, where the exponent sigma=2. In addition, the chain swells. We compare this activity-induced swelling with that of a Rouse chain in a Gaussian active bath. In principle, our predictions can be verified by future single molecule experiments.

cond-mat.soft

Entropy production and work fluctuation relations for a single particle in active bath

A colloidal particle immersed in a bath of bacteria is a typical example of a passive particle in an active bath. To model this, we take an overdamped harmonically trapped particle subjected to a thermal and a non-equilibrium noise arising from the active bath. The harmonic well can be attributed to a laser trap or to the small amplitude motion of the sedimented colloid at the bottom of the capillary. In the long time, the system reaches a non-equilibrium steady state that can be described by an effective temperature. By adopting this notion of effective temperature, we investigate whether fluctuation relations for entropy hold. In addition, when subjected to a deterministic time dependent drag, we find that transient fluctuation theorem for work cannot be applied in conventional form. However, a steady state fluctuation relation for work emerges out with a renormalized temperature.

cond-mat.stat-mech