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Subhro Bhattacharjee

Publications and source records attributed to Subhro Bhattacharjee.

At least 37 records · Page 2Linked to original sources

Many-body Chaos in Thermalised Fluids

Linking thermodynamic variables like temperature $T$ and the measure of chaos, the Lyapunov exponents $λ$, is a question of fundamental importance in many-body systems. By using nonlinear fluid equations in one and three dimensions, we prove that in thermalised flows $λ\propto \sqrt{T}$, in agreement with results from frustrated spin systems. This reveals an underlying universality and provides evidence for recent conjectures on the thermal scaling of $λ$. We also reconcile seemingly disparate effects -- equilibration on one hand and pushing systems out-of-equilibrium on the other -- of many-body chaos by relating $λ$ to $T$ through the dynamical structures of the flow.

cond-mat.stat-mech↗

Phases and Quantum Phase Transitions in Anisotropic Antiferromagnetic Kitaev-Heisenberg-$Γ$ magnet

We study the Kitaev-Heisenberg-$Γ$ model with antiferromagnetic Kitaev exchanges in the strong anisotropic (toric code) limit to understand the phases and the intervening phase transitions between the gapped $Z_2$ quantum spin liquid and the spin-ordered (in the Heisenberg limit) as well as paramagnetic phases (in the pseudo-dipolar, $Γ$, limit). We find that the paramagnetic phase obtained in the large $Γ$ limit has no topological entanglement entropy and is proximate to a gapless critical point of a system described by an equal superposition of differently oriented stacked one-dimensional $Z_2\times Z_2$ symmetry protected topological phases. Using a combination of exact diagonalization calculations and field-theoretic analysis we map out the phases and phase transitions to reveal the complete phase diagram as a function of the Heisenberg, the Kitaev, and the pseudo-dipolar interactions. Our work shows a rich plethora of unconventional phases and phase transitions and provides a comprehensive understanding of the physics of anisotropic Kitaev-Heisenberg-$Γ$ systems along with our recent paper [Phys. Rev. B 102, 235124 (2020)] where the ferromagnetic Kitaev exchange was studied.

cond-mat.str-el↗

Probing signatures of fractionalization in candidate quantum spin liquid Cu2IrO3 via anomalous Raman scattering

Long-range entanglement in quantum spin liquids (QSLs) lead to novel low energy excitations with fractionalised quantum numbers and (in 2D) statistics. Experimental detection and manipulation of these excitations present a challenge particularly in view of diverse candidate magnets. A promising probe of fractionalisation is their coupling to phonons. Here we present Raman scattering results for the S = 1/2 honeycomb iridate Cu2IrO3, a candidate Kitaev QSL with fractionalised Majorana fermions and Ising flux excitations. We observe anomalous low temperature frequency shift and linewidth broadening of the Raman intensities in addition to a broad magnetic continuum both of which, we derive, are naturally attributed to the phonon decaying into itinerant Majoranas. The dynamic Raman susceptibility marks a crossover from the QSL to a thermal paramagnet at ~120 K. The phonon anomalies below this temperature demonstrate a strong phonon-Majorana coupling. These results provide for evidence of spin fractionalisation in Cu2IrO3.

cond-mat.str-el↗

Classical many-body chaos with and without quasiparticles

We study correlations, transport and chaos in a Heisenberg magnet as a classical model many-body system. By varying temperature and dimensionality, we can tune between settings with and without symmetry breaking and accompanying collective modes or quasiparticles. We analyse both conventional and out-of-time-ordered spin correlators (`decorrelators') to track the spreading of a spatiotemporally localised perturbation -- the wingbeat of the butterfly -- as well as transport coefficients and Lyapunov exponents. We identify a number of qualitatively different regimes. Trivially, at $T=0$, there is no dynamics at all. In the limit of low temperature, $T=0^+$, integrability emerges, with infinitely long-lived magnons; here the wavepacket created by the perturbation propagates ballistically, yielding a lightcone at the spin wave velocity which thus subsumes the butterfly velocity; inside the lightcone, a pattern characteristic of the free spin wave spectrum is visible at short times. On top of this, residual interactionslead to spin wave lifetimes which, while divergent in this limit, remain finite at any nonzero $T$. At the longest times, this leads to a `standard' chaotic regime; for this regime, we show that the Lyapunov exponent is simply proportional to the inverse spin-wave lifetime. Visibly strikingly, between this and the `short-time' integrable regimes, a scarred regime emerges: here, the decorrelator is spatiotemporally highly non-uniform, being dominated by rare and random scattering events seeding secondary lightcones. As the spin correlation length decreases with increasing $T$, the distinction between these regimes disappears and at high temperature the previously studied chaotic paramagnetic regime emerges. For this, we elucidate how, somewhat counterintuitively, the ballistic butterfly velocity arises from a diffusive spin dynamics.

cond-mat.stat-mech↗

Statistics tuned entanglement of the boundary modes in coupled Su-Schrieffer-Heeger chains

We show that mutual statistics between quantum particles can be tuned to generate emergent novel few particle quantum mechanics for the boundary modes of symmetry-protected topological phases of matter. As a concrete setting, we study a system of pseudofermions, defined as quantum particles with tunable algebra, which lie on two distinct Su-Schrieffer-Heeger (SSH) chains. We find that as the mutual statistics of the particles are tuned -- the boundary modes present in the two chains gets non-trivially entangled showing a sudden jump in their mutual entanglement entropy. We further show that, such tuning of statistics engenders a first-order transition between two topologically non-trivial phases which differ in the behavior of inter-chain entanglement. Using a combination of analytical and numerical techniques and effective modeling, we uncover the rich physics that this system hosts. The results are of particular relevance in context of the study of the effective low energy quantum mechanics of topological edge modes in one hand and their recent realization in ultracold atoms on the other. This then provides for controlled manipulation of such low energy modes.

cond-mat.str-el↗

Emergent Elasticity in Amorphous Solids

The mechanical response of naturally abundant amorphous solids such as gels, jammed grains, and biological tissues are not described by the conventional paradigm of broken symmetry that defines crystalline elasticity. In contrast, the response of such athermal solids are governed by local conditions of mechanical equilibrium, i.e., force and torque balance of its constituents. Here we show that these constraints have the mathematical structure of a generalized electromagnetism, where the electrostatic limit successfully captures the anisotropic elasticity of amorphous solids. The emergence of elasticity from local mechanical constraints offers a new paradigm for systems with no broken symmetry, analogous to emergent gauge theories of quantum spin liquids. Specifically, our $U(1)$ rank-2 symmetric tensor gauge theory of elasticity translates to the electromagnetism of fractonic phases of matter with the stress mapped to electric displacement and forces to vector charges. We corroborate our theoretical results with numerical simulations of soft frictionless disks in both two and three dimensions, and experiments on frictional disks in two dimensions. We also present experimental evidence indicating that force chains in granular media are sub-dimensional excitations of amorphous elasticity similar to fractons.

cond-mat.dis-nn↗

Signatures of a spin-1/2 cooperative paramagnet in the diluted triangular lattice of Y$_2$CuTiO$_6$

We present a combination of thermodynamic and dynamic experimental signatures of a disorder driven dynamic cooperative paramagnet in a 50% site diluted triangular lattice spin-1/2 system, Y$_2$CuTiO$_6$. Magnetic ordering and spin freezing are absent down to 50 mK, far below the Curie Weiss scale of ~-134 K. We observe scaling collapses of the magnetic field- and temperature-dependent magnetic heat capacity and magnetisation data, respectively, in conformity with expectations from the random singlet physics. Our experiments establish the suppression of any freezing scale, if at all present, by more than three orders of magnitude, opening a plethora of interesting possibilities such as disorder-stabilized long range quantum entangled ground states.

cond-mat.mtrl-sci↗

Gapless state of interacting Majorana fermions in a strain-induced Landau level

Mechanical strain can generate a pseudo-magnetic field, and hence Landau levels (LL), for low energy excitations of quantum matter in two dimensions. We study the collective state of the fractionalised Majorana fermions arising from residual generic spin interactions in the central LL, where the projected Hamiltonian reflects the spin symmetries in intricate ways: emergent U(1) and particle-hole symmetries forbid any bilinear couplings, leading to an intrinsically strongly interacting system; also, they allow the definition of a filling fraction, which is fixed at 1/2. We argue that the resulting many-body state is gapless within our numerical accuracy, implying ultra-short-ranged spin correlations, while chirality correlators decay algebraically. This amounts to a Kitaev `non-Fermi' spin liquid, and shows that interacting Majorana Fermions can exhibit intricate behaviour akin to fractional quantum Hall physics in an insulating magnet.

cond-mat.str-el↗

Interplay of Magnetism and Topological Superconductivity in Bilayer Kagome Metals

The binary intermetallic materials, $M_3$Sn$_2$ ($M$ = 3d transition metal) present a new class of strongly correlated systems that naturally allows for the interplay of magnetism and metallicity. Using first principles calculations we confirm that bulk Fe$_3$Sn$_2$ is a ferromagnetic metal, and show that $M$ = Ni and Cu are paramagnetic metals with non-trivial band structures. Focusing on Fe$_3$Sn$_2$ to understand the effect of enhanced correlations in an experimentally relevant atomistically thin single kagome-bilayer, our ab-initio results show that dimensional confinement naturally exposes the flatness of band structure associated with the bilayer kagome geometry in a resultant ferromagnetic Chern metal. We use a multistage minimal modeling of the magnetic bands progressively closer to the Fermi energy. This effectively captures the physics of the Chern metal with a non-zero anomalous Hall response over a material relevant parameter regime along with a possible superconducting instability of the spin-polarised band resulting in a topological superconductor.

cond-mat.str-el↗

Phases and Quantum Phase Transitions in an Anisotropic Ferromagnetic Kitaev-Heisenberg-$\ Γ$ Magnet

We study the spin-$1/2$ ferromagnetic Heisenberg-Kitaev-$Γ$ model in the anisotropic (Toric code) limit to reveal the nature of the quantum phase transition between the gapped $Z_2$ quantum spin liquid and a spin ordered phase (driven by Heisenberg interactions) as well as a trivial paramagnet (driven by pseudo-dipolar interactions, $Γ$). The transitions are obtained by a simultaneous condensation of the Ising electric and magnetic charges-- the fractionalized excitations of the $Z_2$ quantum spin liquid. Both these transitions can be continuous and are examples of deconfined quantum critical points. Crucial to our calculations are the symmetry implementations on the soft electric and magnetic modes that become critical. In particular, we find strong constraints on the structure of the critical theory arising from time reversal and lattice translation symmetries with the latter acting as an anyon permutation symmetry that endows the critical theory with a manifestly self-dual structure. We find that the transition between the quantum spin liquid and the spin-ordered phase belongs to a self-dual modified Abelian Higgs field theory while that between the spin liquid and the trivial paramagnet belongs to a self-dual $Z_2$ gauge theory. We also study the effect of an external Zeeman field to show an interesting similarity between the polarised paramagnet obtained due to the Zeeman field and the trivial paramagnet driven the pseudo-dipolar interactions. Interestingly, both the spin liquid and the spin ordered phases have easily identifiable counterparts in the isotropic limit and the present calculations may shed insights into the corresponding transitions in the material relevant isotropic limit.

cond-mat.str-el↗

Topological and conventional phases of a three dimensional electron glass

We investigate a symmetry protected $Z_2$ topological electron glass -- a glassy equivalent of the $Z_2$ topological band insulator in crystalline systems -- and uncover associated quantum phase transitions in this three dimensional amorphous network of atoms. Through explicit numerical calculations of the Witten effect, we show that the $Z_2$ glass is characterized by an anomalous electromagnetic response -- dyons with 1/2 electronic charge. We further study, using a variety of numerical diagnostics including such electromagnetic responses, the phase transitions of the $Z_2$ glass into a metallic and/or a trivial insulating phase. We find that the phase transitions here are governed by subtle features of mobility edges and "spectral inversion" which are possibly unique to structurally amorphous systems. Our results provide a concrete setting to understand the general underpinnings of such phases -- where strong structural disorder interplays with symmetry-protected topological order.

cond-mat.dis-nn↗

Statistics-tuned phases of pseudofermions in one dimension

We show that a quadratic system of pseudofermions, with tunable fractionalised statistics, can host a rich phase diagram on a one dimensional chain with nearest and next nearest neighbor hopping. Using a combination of numerical and analytical techniques, we show that that by varying the statistical angle and the ratio of the hopping, the system stabilizes two Tomonaga-Luttinger liquids (TLL) with central charges c = 1 and 2 respectively along with the inversion symmetry broken bond ordered (BO) insulating phase. Interestingly, the two quantum phase transitions in the system - (1) between the two TLLs, and, (2) the c = 1 TLL and BO phase can be engendered by solely tuning the statistics of the pseudofermions. Our analysis shows that both these transition are continuous and novel with the former lacking a local order-parameter based description and the latter of Berezinskii-Kosterlitz-Thouless type. These phases and phase transitions can be of direct experimental relevance in context of recent studies of fermionic cold atoms.

cond-mat.str-el↗

Temperature dependence of butterfly effect in a classical many-body system

We study the chaotic dynamics in a classical many-body system of interacting spins on the kagome lattice. We characterise many-body chaos via the butterfly effect as captured by an appropriate out-of-time-ordered correlator. Due to the emergence of a spin liquid phase, the chaotic dynamics extends all the way to zero temperature. We thus determine the full temperature dependence of two complementary aspects of the butterfly effect: the Lyapunov exponent, $μ$, and the butterfly speed, $v_b$, and study their interrelations with usual measures of spin dynamics such as the spin-diffusion constant, $D$ and spin-autocorrelation time, $τ$. We find that they all exhibit power law behaviour at low temperature, consistent with scaling of the form $D\sim v_b^2/μ$ and $τ^{-1}\sim T$. The vanishing of $μ\sim T^{0.48}$ is parametrically slower than that of the corresponding quantum bound, $μ\sim T$, raising interesting questions regarding the semi-classical limit of such spin systems.

cond-mat.stat-mech↗

Interplay of uniform U(1) quantum spin liquid and magnetic phases in rare earth pyrochlore magnets : a fermionic parton approach

We study the uniform time reversal invariant $U(1)$ quantum spin liquid (QSL) with low energy fermionic quasi-particles for rare earth pyrochlore magnets and explore its magnetic instability employing an augmented fermionic parton mean field theory approach. Self consistent calculations stabilise an uniform $U(1)$ QSL with both gapped and gapless parton excitations as well as fractionalised magnetically ordered phases in an experimentally relevant part of the phase diagram near the classical phase boundaries of the magnetically ordered phases. The gapped QSL has a band-structure with a non-zero $Z_2$ topological invariant. The fractionalised magnetic ordered phases bears signature of both QSL through fermionic excitations as well as magnetic order. Thus this provides a possible way to understand the unconventional diffuse neutron scattering in rare-earth pyrochlores such as Yb$_2$Ti$_2$O$_7$, Er$_2$Sn$_2$O$_7$ and Er$_2$Pt$_2$O$_7$ at low/zero external magnetic fields. We calculate the dynamic spin structure factor to understand the nature of the diffuse two-particle continuum.

cond-mat.str-el↗

Light-cone spreading of perturbations and the butterfly effect in a classical spin chain

We find that localised perturbations in a chaotic classical many-body system-- the classical Heisenberg We find that the effects of a localised perturbation in a chaotic classical many-body system--the classical Heisenberg chain at infinite temperature--spread ballistically with a finite speed even when the local spin dynamics is diffusive. We study two complementary aspects of this butterfly effect: the rapid growth of the perturbation, and its simultaneous ballistic (light-cone) spread, as characterised by the Lyapunov exponents and the butterfly speed respectively. We connect this to recent studies of the out-of-time-ordered commutators (OTOC), which have been proposed as an indicator of chaos in a quantum system. We provide a straightforward identification of the OTOC with a natural correlator in our system and demonstrate that many of its interesting qualitative features are present in the classical system. Finally, by analysing the scaling forms, we relate the growth, spread and propagation of the perturbation with the growth of one-dimensional interfaces described by the Kardar-Parisi-Zhang (KPZ) equation.

cond-mat.stat-mech↗

Dynamics of a quantum spin liquid beyond integrability $-$ the Kitaev-Heisenberg-$Γ$ model in an augmented parton mean-field theory

We present an augmented parton mean-field theory which (i) reproduces the $exact$ ground state, spectrum, and dynamics of the quantum spin liquid phase of Kitaev's honeycomb model; and (ii) is amenable to the inclusion of integrability breaking terms, allowing a perturbation theory from a controlled starting point. Thus, we exemplarily study dynamical spin correlations of the honeycomb Kitaev quantum spin liquid within the $K-J-Γ$ model which includes Heisenberg and symmetric-anisotropic (pseudo-dipolar) interactions. This allows us to trace changes of the correlations in the regime of slowly moving fluxes, where the theory captures the dominant deviations when integrability is lost. These include an asymmetric shift together with a broadening of the dominant peak in the response as a function of frequency; the generation of further-neighbour correlations and their structure in real- and spin-space; and a resulting loss of an approximate rotational symmetry of the structure factor in reciprocal space. We discuss the limitations of this approach, and also view the neutron scattering experiments on the putative proximate quantum spin liquid material, $α$-RuCl$_3$, in the light of the results from this extended parton theory.

cond-mat.str-el↗

Electric field control of emergent electrodynamics in quantum spin ice

We study the coupling between conventional (Maxwell) and emergent electrodynamics in quantum spin ice, a 3+1-dimensional $U(1)$ quantum spin liquid. We find that a uniform electric field can be used to tune the properties of both the ground state and excitations of the spin liquid. In particular, it induces emergent birefringence, rendering the speed of the emergent light anisotropic and polarization-dependent. A sufficiently strong electric field triggers a quantum phase transition into new $U(1)$ quantum spin liquid phases which trap emergent electric $π$-fluxes. The flux patterns of these new phases depend on the direction of the electric field. Strikingly, some of the canonical pinch points in the spin structure factor, characteristic of classical spin ice, emerge near the phase transition, while they are absent in the quantum spin liquid phases. Estimating the electric field strength required, we find that this transition is potentially accessible experimentally. Finally, we propose a minimal mechanism by which an oscillating electric field can generate emergent radiation inside a quantum spin ice material with non-Kramers spin doublets.

cond-mat.str-el↗

Kagome spin liquid: a deconfined critical phase driven by $U(1)$ gauge fluctuation

We investigate the nature of quantum spin liquid (QSL) phase of the spin-$1/2$ nearest-neighbor XXZ antiferromagnet on the kagome lattice. Recent numerical calculations suggest that such a kagome spin liquid is insensitive to the XXZ anisotropy and is adjacent to a chiral spin liquid phase. Reformulating the problem in terms of a $U(1)$ lattice gauge theory with dynamical bosonic spinons, we propose that the kagome spin liquid can be understood as a deconfined critical phase extended by the $U(1)$ gauge fluctuation from a deconfined critical point between a symmetry-protected topological phase and a superfluid phase. Crucially, the stability of this QSL is ensured by the gauge fluctuation and hence our description necessarily falls beyond the conventional mean-field constructions of QSLs. Our work also makes an interesting connection between the critical spin liquid, deconfined criticality, symmetry protected topological phase and topological order.

cond-mat.str-el↗