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Sudesh

Publications and source records attributed to Sudesh.

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Crystal Growth & Physical Property Characterization of Mixed Topological Insulator BiSbTe$_3$

This article reports the synthesis of a single crystalline mixed topological insulator (TI) BiSbTe$_3$ and its detailed structural and magneto-transport properties. The single crystalline samples of BiSbTe$_3$ are grown by the melt-growth process and characterized by X-ray diffraction (XRD), Energy dispersive X-ray analysis (EDAX) and Raman spectroscopy. The single crystal XRD peaks dictated the growth direction along the c-axis. The Raman spectrum elucidated the characteristic peaks of the mixed topological insulator. The broadening of Raman peaks exhibited the formation of Te-Bi-Te and Te-Sb-Te bonds and associated vibrational modes. The single crystals are characterized by magneto-transport measurements down to 2 K and up to 14 Tesla transverse magnetic field. The residual resistance ratio (R200 K/R0 K) is found to be 3.64, which endorses the metallic nature of the synthesized crystal. The relative resistance turns out to be higher for the mixed TI than the pure TIs i.e., Bi$_2$Te$_3$ or Sb$_2$Te$_3$. The lower Debye temperature (82.64 K) of BiSbTe$_3$ connotes the presence of effective electron-phonon interaction at quite low temperatures in comparison to pure TI, which explains the observed suppression in magnetoresistance (MR) for the mixed TI. At 2 K, an MR of 150 percent is observed for BiSbTe$_3$, which is suppressed in contrast to the pure TIs i.e., Bi$_2$Te$_3$ or Sb$_2$Te$_3$. Though the MR% is suppressed significantly, its non-saturating linear behavior indicates the topological nature of the studied mixed TI. The modified Hikami-Larkin-Nagaoka (HLN) equation analysis of magneto-conductivity of mixed TI revealed that the conductivity has not only a surface states driven 2D component but also contributions from the bulk charge carriers and quantum scattering.

cond-mat.mtrl-sci

Evidence of Ferromagnetic Clusters and Griffiths Singularity in Magnetic Weyl Semimetal Co$ _{3} $Sn$ _{2} $S$ _{2} $

Cobalt based sulphides of compositional formula Co$ _{3} $A$ _{2} $S$ _{2} $ (A = Sn and In) are endowed with frustrated kagome lattice structure and a plethora of novel phenomena determined from the topological band structure. Here-in, we report on the detailed exploration of anisotropic magnetic properties of single crystals of ferromagnetic compound Co$ _{3} $Sn$ _{2} $S$ _{2} $ under magnetic field $H$ applied along the c-axis $(H\parallel c)$ and the ab-plane $(H\parallel ab)$. A low temperature clustered-glassy magnetic behaviour is revealed in field-cooled and zero field-cooled magnetization and memory effect measurement protocols. The sharp downturn and non-linearity observed in the inverse susceptibility above the critical temperature $T _{\text{C}} $ in the paramagnetic region corroborates to the presence of short-range ferromagnetic clusters above $ T _{\text{C}} $ in Co$ _{3} $Sn$ _{2} $S$ _{2} $. The deviation from linear Curie-Weiss behaviour in the paramagnetic state signifies the strong Griffiths singularity in the material. The slow spin dynamics behaviour and zero spontaneous magnetization above $ T _{\text{C}} $ give an evidence of Griffiths phase owing to the ferromagnetic clusters. The Arrott plots derived from magnetization reveal convex type curvature at low fields and linear positive behavior in the high field region, confirming the second order magnetic phase transition in Co$ _{3} $Sn$ _{2} $S$ _{2} $. The Takahashi spin fluctuation theory analysis provides sufficient evidence for itinerant ferromagnetism in Co$ _{3} $Sn$ _{2} $S$ _{2} $. A large magneto-crystalline anisotropy concomitant with a high anisotropy field suggests the dominance of strong spin orbit coupling phenomenon. Our experimental results emphasize an intuitive understanding of the complex nature of magnetism present in Co-based shandite systems.

cond-mat.str-el

Magnetic field-induced resistivity upturn and exceptional magneto-resistance in Weyl semimetal TaSb2

We study magneto-transport properties in single crystals of TaSb_2, which is a recently discovered topological semimetal. In the presence of magnetic field, the electrical resistivity shows onset of insulating behaviour followed by plateau at low temperature. Such resistivity plateau is generally assigned to topological surface states. TaSb2 exhibits extremely high magneto-resistance with non-saturating field dependence. We find that aspects of extremely large magneto resistance and resistivity plateau are well accounted by classical Kohler scaling. Unambiguous evidence for anomalous Chiral transport is provided with observation of negative longitudinal magneto-resistance. Shubnikov-de Haas oscillations reveal two dominating frequencies, 201 T and 455 T. These aspects categorize TaSb2 as a Type-II Weyl semimetal. At low temperature, the field dependence of Hall resistivity shows non-linear behaviour that indicates the presence of two types of charge carriers in consonance with reported electronic band structure. Analysis of Hall resistivity imply very high electron mobilities.

cond-mat.str-el

Evidence for trivial Berry phase and absence of chiral anomaly in semimetal NbP

We report a detailed magneto-transport study in single crystals of NbP. High quality crystals were grown by vapour transport method. An exceptionally large magnetoresistance is confirmed at low temperature which is non-saturating and is linear at high fields. Models explaining the linear magnetoresistance are discussed and it is argued that in NbP this is linked to charge carrier mobility fluctuations. Negative longitudinal magnetoresistance is not seen, unlike several other Weyl monopnictides, suggesting lack of well defined chiral anomaly in NbP. Unambiguous Shubnikov-de-Haas oscillations are observed at low temperatures that are correlated to Berry phases. The Landau fan diagram indicates trivial Berry phase in NbP crystals corresponding to Fermi surface extrema at 30.5 Tesla.

cond-mat.mtrl-sci