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Sue Hyeon Hwang

Publications and source records attributed to Sue Hyeon Hwang.

2 recordsLinked to original sources

Plasmonic polaron in self-intercalated 1T-TiS2

Electron-boson coupling is central to a comprehensive understanding of the diverse physical phenomena emerging from many-body interactions. Yet less attention has been paid to how plasmons, collective bosonic modes of electron density oscillation, interact with conduction electrons and how external parameters can tune this interaction. Here, we present a clear display of composite quasiparticles stemming from electron-plasmon coupling, known as the plasmonic polaron, in self-intercalated 1T-TiS2, by using angle-resolved photoemission spectroscopy (ARPES), high-resolution electron energy loss spectroscopy (HR-EELS) and first-principles calculations. The single particle spectral function exhibits a distinctive plasmon-loss satellite with the same characteristic energy scale determined by HR-EELS measurements. The bosonic energy scale of plasmonic polaron is tunable by controlling charge carrier density and temperature, distinguishing itself from conventional polarons arising from electron-phonon interactions. Furthermore, we find that the dielectric screening strongly affects the formation of the plasmonic polaron states. Our findings provide direct spectroscopic evidence of plasmonic polarons and establish self-intercalated layered materials as a promising platform for studying, controlling, and harnessing plasmonic interactions in quantum materials.

cond-mat.mtrl-sci↗

Band-selective simulation of photoelectron intensity and converging Berry phase in trilayer graphene

Berry phase is one of the key elements to understand quantum-mechanical phenomena such as the Aharonov-Bohm effect and the unconventional Hall effect in graphene. The Berry phase in monolayer and bilayer graphene has been manifested by the anisotropic distribution of photoelectron intensity along a closed loop in the momentum space as well as its rotation by a characteristic angle upon rotating light polarization. Here we report the band-selective simulation of photoelectron intensity of trilayer graphene to understand its Berry phase within the tight-binding formalism. ABC- and ABA-stacked trilayer graphene show characteristic rotational angles of photoelectron intensity distribution, as predicted from their well-known Berry phases. Surprisingly, however, in ABA-stacked trilayer graphene, the rotational angle changes upon approaching toward the band touching point between the conduction and valence bands, which suggest that Berry phase changes as a function of binding energy. The binding energy-dependent Berry phase is attributed to the enhanced hybridization of the two electron bands of ABA-stacked trilayer graphene that converge at the band touching point, resulting in the converging Berry phase. These findings will provide an efficient way of tuning Berry phase and hence exotic phenomena stemming from the Berry phase.

cond-mat.mtrl-sci↗