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Sujin Suwanna

Publications and source records attributed to Sujin Suwanna.

At least 19 recordsLinked to original sources

Topology-Dependent Enhancement of Entanglement Extraction in Repeater Graph States

Quantum repeaters are essential for establishing long-distance quantum communication to overcome the exponential decay of entanglement due to photon loss. Traditional repeater architectures rely on physical quantum memory, which introduces decoherence and poses significant practical implementation challenges. The repeater graph state (RGS) architecture offers a promising memory-less alternative that is inherently resilient to photon losses. A key challenge in implementing RGS lies in the requirement for highly efficient graph state generators and complex qubit measurement. In this work, we aim to investigate the strategies for extracting the maximum number of Bell pairs from the RGS structure via its qubit connection to resolve the well-known bottleneck problem of RGS in which only a single Bell pair can be extracted from a complete bipartite graph state. From simulations, we observe that the maximum number of extracted Bell pairs depends on its connection topology, where the Bell-pair yield tends to be maximal at low to moderate edge densities. As the number of network hops increases, the RGS must be equipped with higher inner-qubit connectivity to maintain a sufficient yield of extractable Bell pairs. Thus, the expected resource requirement shifts toward the use of RGSs with higher inner-qubit connectivity.

quant-ph

Quantum Emitters at Telecommunication Wavelengths based on Carbon Defects in Transition Metal Dichalcogenides

Low-dimensional materials have emerged as promising hosts for quantum emitters, whose emission typically arises from either strain-induced band bending or defect-induced two-level systems. Among these materials, transition metal dichalcogenide (TMD) monolayers have attracted particular attention; however, their performance is limited by strong photoluminescence (PL) quenching at room temperature. As TMDs transition from a direct to an indirect bandgap when moving from monolayers to multilayers, we herein propose a strategy to overcome this quenching limitation by exploiting the indirect bandgap of TMD bilayers in combination with a point defect doping. The indirect gap suppresses excitonic PL, while specific defects enable robust defect-mediated quantum emission. Using hybrid-functional density functional theory, we investigate substitutional carbon defects at chalcogen sites (S and Se) in WS2, WSe2, MoS2, and MoSe2 bilayers and comprehensively characterize their optical properties. Both neutral and singly negative charge states are found to be thermodynamically stable. Neutral defects exhibit singlet configurations with emission in the O- and C-band telecommunication windows, whereas negatively charged defects adopt doublet configurations featuring spin-selective transitions and near-infrared emission. The electron-phonon coupling strength, radiative lifetime, and dipole orientation are found to depend sensitively on both the host material and defect site, providing distinct fingerprints for experimental identification. Our findings, therefore, establish carbon-doped TMD bilayers as promising platforms for room-temperature defect-based quantum emitters operating at telecommunication wavelengths.

quant-ph

Advancing the hBN Defects Database through Photophysical Characterization of Bulk hBN

Quantum emitters in hexagonal boron nitride (hBN) have gained significant attention due to a wide range of defects that offer high quantum efficiency and single-photon purity at room temperature. Most theoretical studies on hBN defects simulate monolayers, as this is computationally cheaper than calculating bulk structures. However, most experimental studies are carried out on multilayer to bulk hBN, which creates additional possibilities for discrepancies between theory and experiment. In this work, we present an extended database of hBN defects that includes a comprehensive set of bulk hBN defects along with their excited-state photophysical properties. The database features over 120 neutral defects, systematically evaluated across charge states ranging from -2 to 2 (600 defects in total). For each defect, the most stable charge and spin configurations are identified and used to compute the zero-phonon line, photoluminescence spectrum, absorption spectrum, Huang-Rhys (HR) factor, interactive radiative lifetimes, transition dipole moments, and polarization characteristics. Our analysis reveals that the electron-phonon coupling strength is primarily influenced by the presence of vacancies, which tend to induce stronger lattice distortions and broaden phonon sidebands. Additionally, correlation analysis shows that while most properties are independent, the HR factor strongly correlates with the configuration coordinates. All data are publicly available at https://h-bn.info, along with a new application programming interface (API) to facilitate integration with machine learning workflows. This database is therefore designed to bridge the gap between theory and experiment, aid in the reliable identification of quantum emitters, and support the development of machine-learning-driven approaches in quantum materials research.

quant-ph

Raman Signatures of Single Point Defects in Hexagonal Boron Nitride Quantum Emitters

Point defects in solid-state quantum systems are vital for enabling single-photon emission at specific wavelengths, making their precise identification essential for advancing applications in quantum technologies. However, pinpointing the microscopic origins of these defects remains a challenge. In this work, we propose Raman spectroscopy as a robust strategy for defect identification. Using density functional theory, we systematically characterize the Raman signatures of 100 defects in hexagonal boron nitride (hBN) spanning periodic groups III to VI, encompassing around 30,000 phonon modes. Our findings reveal that the local atomic environment plays a pivotal role in shaping the Raman lineshape, enabling the narrowing of potential defect candidates. Furthermore, we demonstrate that Raman spectroscopy can differentiate defects based on their spin and charge states as well as strain-induced variations, implying the versatility of this approach. Therefore, this study not only provides a comprehensive theoretical database of Raman spectra for hBN defects but also establishes a novel experiment framework for using tip-enhanced Raman spectroscopy to identify point defects. More broadly, our approach offers a universal method for defect identification in any quantum materials.

cond-mat.mtrl-sci

Modeling the performance and bandwidth of single-atom adiabatic quantum memories

Quantum memories are essential for quantum repeaters that will form the backbone of the future quantum internet. Such memory can capture a signal state for a controllable amount of time after which this state can be retrieved. In this work, we theoretically investigated how atomic material and engineering parameters affect the performance and bandwidth of a quantum memory. We have applied a theoretical model for quantum memory operation based on the Lindblad master equation and adiabatic quantum state manipulation. The materials properties and their uncertainty are evaluated to determine the performance of Raman-type quantum memories by showcasing two defects in two-dimensional hexagonal boron nitride (hBN). We have derived a scheme to calculate the signal bandwidth based on the material parameters as well as the maximum efficiency that can be realized. The bandwidth depends on four factors: the signal photon frequency, the dipole transition moments in the electronic structure, cavity volume, and the strength of the external control electric field. As our scheme is general and independent of materials, it can be applied to many other quantum materials with a suitable three-level structure. We therefore provided a promising route for designing and selecting materials for quantum memories. Our work is therefore an important step toward the realization of a large-scale quantum network.

quant-ph

Boosting end-to-end entanglement fidelity in quantum repeater networks via hybridized strategies

Quantum networks are expected to enhance distributed quantum computing and quantum communication over long distances while providing security dependent upon physical effects rather than mathematical assumptions. Through simulation, we show that a quantum network utilizing only entanglement purification or only quantum error correction as error management strategies cannot create Bell pairs with fidelity that exceeds the requirement for a secured quantum key distribution protocol for a broad range of hardware parameters. We propose hybrid strategies utilizing quantum error correction on top of purification and show that they can produce Bell pairs of sufficiently high fidelity. We identify the error parameter regime for gate and measurement errors in which these hybrid strategies are applicable.

quant-ph

Comparative study of quantum emitter fabrication in wide bandgap materials using localized electron irradiation

Quantum light sources are crucial foundational components for various quantum technology applications. With the rapid development of quantum technology, there has been a growing demand for materials with the capability of hosting quantum emitters. One such material platform uses fluorescent defects in hexagonal boron nitride (hBN) that can host deep sublevels within the bandgap. The localized electron irradiation has shown its effectiveness in generating deep sublevels to induce single emitters in hBN. The question is whether localized (electron beam) irradiation is a reliable tool for creating emitters in other wide bandgap materials and its uniqueness to hBN. Here, we investigate and compare the fabrication of quantum emitters in hBN and exfoliated muscovite mica flakes along with other 3D crystals, such as silicon carbide and gallium nitride, which are known to host quantum emitters. We used our primary fabrication technique of localized electron irradiation using a standard scanning electron microscope. To complement our experimental work, we employed density functional theory simulations to study the atomic structures of defects in mica. While our fabrication technique allows one to create hBN quantum emitters with a high yield and high single photon purity, it is unable to fabricate single emitters in the other solid-state crystals under investigation. This allows us to draw conclusions on the emitter fabrication mechanism in hBN, which could rely on activating pre-existing defects by charge state manipulation. Therefore, we provide an essential step toward the identification of hBN emitters and their formation process.

physics.app-ph

Polarization dynamics of solid-state quantum emitters

Quantum emitters in solid-state crystals have recently attracted a lot of attention due to their simple applicability in optical quantum technologies. The polarization of single photons generated by quantum emitters is one of the key parameters that play a crucial role in the applications, such as quantum computation that uses the indistinguishability of photons. However, the degree of single photon polarization is typically quantified using time-averaged photoluminescence intensity of single emitters, which provides limited information about the dipole properties in solids. In this work, we use single defects in hexagonal boron nitride and nanodiamond as efficient room-temperature single photon sources to reveal the origin and the temporal evolution of dipole orientation in solid-state quantum emitters. The angle of excitation and emission dipoles relative to the crystal axes are determined experimentally and then calculated using density functional theory, which results in characteristic angles for every specific defect that can be used as an efficient tool for defect identification and understanding their atomic structure. Moreover, the temporal polarization dynamics reveal a strongly modified linear polarization visibility that depends on the excited state decay time of individual excitation. This effect can be traced back potentially to the excitation of excess charges in the local crystal environment. Understanding such hidden time-dependent mechanisms can further be used to improve the performance of polarization-sensitive experiments, in particular that of quantum communication with single photon emitters.

quant-ph

Identifying electronic transitions of defects in hexagonal boron nitride for quantum memories

A quantum memory is a crucial keystone for enabling large-scale quantum networks. Applicable to the practical implementation, specific properties, i.e., long storage time, selective efficient coupling with other systems, and a high memory efficiency are desirable. Though many quantum memory systems are developed thus far, none of them can perfectly meet all requirements. This work herein proposes a quantum memory based on color centers in hexagonal boron nitride (hBN), where its performance is evaluated based on a simple theoretical model of suitable defects in a cavity. Employing density functional theory calculations, 257 triplet and 211 singlet spin electronic transitions are investigated. Among these defects, it is found that some defects inherit the $Λ$ electronic structures desirable for a Raman-type quantum memory and optical transitions can couple with other quantum systems. Further, the required quality factor and bandwidth are examined for each defect to achieve a 95% writing efficiency. Both parameters are influenced by the radiative transition rate in the defect state. In addition, inheriting triplet-singlet spin multiplicity indicates the possibility of being a quantum sensing, in particular, optically detected magnetic resonance. This work therefore demonstrates the potential usage of hBN defects as a quantum memory in future quantum networks.

quant-ph

Comprehensive scheme for identifying defects in solid-state quantum systems

A solid-state quantum emitter is one of the indispensable components for optical quantum technologies. Ideally, an emitter should have a compatible wavelength for efficient coupling to other components in a quantum network. It is therefore essential to understand fluorescent defects that lead to specific emitters. In this work, we employ density functional theory (DFT) to demonstrate the calculation of the complete optical fingerprints of quantum emitters in the two-dimensional material hexagonal boron nitride. These emitters are of great interest, yet many of them are still to be identified. Our results suggest that instead of comparing a single optical property, such as the commonly used zero-phonon line energy, multiple properties should be used when comparing theoretical simulations to the experiment. This way, the entire electronic structure can be predicted and quantum emitters can be designed and tailored. Moreover, we apply this approach to predict the suitability for using the emitters in specific quantum applications, demonstrating through the examples of the Al$_{\text{N}}$ and P$_{\text{N}}$V$_{\text{B}}$ defects. We therefore combine and apply DFT calculations to identify quantum emitters in solid-state crystals with a lower risk of misassignments as well as a way to design and tailor optical quantum systems. This consequently serves as a recipe for classification and the generation of universal solid-state quantum emitter systems in future hybrid quantum networks.

quant-ph

Localized creation of yellow single photon emitting carbon complexes in hexagonal boron nitride

Single photon emitters in solid-state crystals have received a lot of attention as building blocks for numerous quantum technology applications. Fluorescent defects in hexagonal boron nitride (hBN) stand out due to their high luminosity and robust operation at room temperature. The identical emitter fabrication at pre-defined sites is still challenging, which hampers the integration of these defects in optical systems and electro-optical devices. Here, we demonstrate the localized fabrication of hBN emitter arrays by electron beam irradiation using a standard scanning electron microscope with deep sub-micron lateral precision. The emitters are created with a high yield and a reproducible spectrum peaking at 575 nm. Our measurements of optically detected magnetic resonance have not revealed any addressable spin states. Using density functional theory, we attribute the experimentally observed emission lines to carbon-related defects, which are activated by the electron beam. Our scalable approach provides a promising pathway for fabricating room temperature single photon emitters in integrated quantum devices.

quant-ph

Hybrid Error-Management Strategies in Quantum Repeater Networks

A quantum network is expected to enhance distributed quantum computing and quantum communication over a long distance while providing unconditional security. As quantum entanglement is essential for a quantum network, major issues from various types of noise and decoherence prevent it from being realized, and research has been intensively active to obtain optimal configurations for a quantum network. In this work, we address the performance of a quantum network capable of quantum error correction and entanglement purification. Our results show that one should distribute Bell pairs as fast as possible while balancing the deployment of fidelity enhancement. We also show suitable hybrid strategies in quantum cryptography tasks under some noise regimes that need to use purification and quantum error correction together. Our results suggest that using purification to distribute high fidelity Bell pairs and preserving them for application using quantum error correction is a promising way to achieve a near-term quantum network for secure communication.

quant-ph

Tailoring the Emission Wavelength of Color Centers in Hexagonal Boron Nitride for Quantum Applications

Optical quantum technologies promise to revolutionize today's information processing and sensors. Crucial to many quantum applications are efficient sources of pure single photons. For a quantum emitter to be used in such application, or for different quantum systems to be coupled to each other, the optical emission wavelength of the quantum emitter needs to be tailored. Here, we use density functional theory to calculate and manipulate the transition energy of fluorescent defects in the two-dimensional material hexagonal boron nitride. Our calculations feature the HSE06 functional which allows us to accurately predict the electronic band structures of 267 different defects. Moreover, using strain-tuning we can tailor the optical transition energy of suitable quantum emitters to match precisely that of quantum technology applications. We therefore not only provide a guide to make emitters for a specific application, but also have a promising pathway of tailoring quantum emitters that can couple to other solid-state qubit systems such as color centers in diamond.

quant-ph

Time-delayed quantum feedback and incomplete decoherence suppression with no-knowledge measurement

The no-knowledge quantum feedback was proposed by Szigeti et al., Phys. Rev. Lett. 113, 020407 (2014), as a measurement-based feedback protocol for decoherence suppression for an open quantum system. By continuously measuring environmental noises and feeding back controls on the system, the protocol can completely reverse the measurement backaction and therefore suppress the system's decoherence. However, the complete decoherence cancellation was shown only for the instantaneous feedback, which is impractical in real experiments. Therefore, in this work, we generalize the original work and investigate how the decoherence suppression can be degraded with unavoidable delay times, by analyzing non-Markovian average dynamics. We present analytical expressions for the average dynamics and numerically analyze the effects of the delayed feedback for a coherently driven two-level system, coupled to a bosonic bath via a Hermitian coupling operator. We also find that, when the qubit's unitary dynamics does not commute with the measurement and feedback controls, the decoherence rate can be either suppressed or amplified, depending on the delay time.

quant-ph

Modeling of Measurement-based Quantum Network Coding on IBM Q Experience Devices

Quantum network coding has been proposed to improve resource utilization to support distributed computation but has not yet been put in to practice. We investigate a particular implementation of quantum network coding using measurement-based quantum computation on IBM Q processors. We compare the performance of quantum network coding with entanglement swapping and entanglement distribution via linear cluster states. These protocols outperform quantum network coding in terms of the final Bell pair fidelities but are unsuitable for optimal resource utilization in complex networks with contention present. We demonstrate the suitability of noisy intermediate-scale quantum (NISQ) devices such as IBM Q for the study of quantum networks. We also identify the factors that limit the performance of quantum network coding on these processors and provide estimates or error rates required to boost the final Bell pair fidelities to a point where they can be used for generation of genuinely random cryptographic keys among other useful tasks. Surprisingly, the required error rates are only around a factor of 2 smaller than the current status and we expect they will be achieved in the near future.

quant-ph

Machine learning clustering technique applied to powder X-ray diffraction patterns to distinguish alloy substitutions

We applied the clustering technique using DTW (dynamic time wrapping) analysis to XRD (X-ray diffraction) spectrum patterns in order to identify the microscopic structures of substituents introduced in the main phase of magnetic alloys. The clustering is found to perform well to identify the concentrations of the substituents with successful rates (around 90%). The sufficient performance is attributed to the nature of DTW processing to filter out irrelevant informations such as the peak intensities (due to the incontrollability of diffraction conditions in polycrystalline samples) and the uniform shift of peak positions (due to the thermal expansions of lattices).

physics.comp-ph

Unitary-Scaling Decomposition and Dissipative Behaviour in Finite-Dimensional Linblad Dynamics

We investigate a decomposition of a unital Lindblad dynamical map of an open quantum system into two distinct types of mapping on the Hilbert-Schmidt space of quantum states. One component of the decomposed map corresponds to reversible behaviours, while the other to irreversible characteristics. For a finite dimensional system, we employ real vectors or Bloch representations and express a dynamical map on the state space as a real matrix acting on the representation. It is found that rotation and scaling transformations on the real vector space, obtained from the real-polar decomposition, form building blocks for the dynamical map. Consequently, the change of the linear entropy or purity, which indicates dissipative behaviours, depends only on the scaling part of the dynamical matrix. The rate of change of the entropy depends on the structure of the scaling part of the dynamical matrix, such as eigensubspace partitioning, and its relationship with the initial state. In particular, the linear entropy is expressed as a weighted sum of the exponential-decay functions in each scaling component, where the weight is equal to $\vert\vec{x}_k(ρ)\vert^2$ of the initial state $ρ$ in the subspace. The dissipative behaviours and the partition of eigensubspaces in the decomposition are discussed and illustrated for qubit systems.

quant-ph

Time Evolution of Gaussian Wave Packets under Dirac Equation with Fluctuating Mass and Potential

Localization of relativistic particles have been of great research interests over many decades. We investigate the time evolution of the Gaussian wave packets governed by the one dimensional Dirac equation. For the free Dirac equation, we obtain the evolution profiles analytically in many approximation regimes, and numerical simulations consistent with other numerical schemes. Interesting behaviors such as Zitterbewegung and Klein paradox are exhibited. In particular, the dispersion rate as a function of mass is calculated, and it yields an interesting result that super-massive and massless particles both exhibit no dispersion in free space. For the Dirac equation with random potential or mass, we employ the Chebyshev polynomials expansion of the propagator operator to numerically investigate the probability profiles of the displacement distribution when the potential or mass is uniformly distributed. We observe that the widths of the Gaussian wave packets decrease approximately with the power law of order $o(s^{-ν})$ with $\frac{1}{2}<ν<1$ as the randomness strength $s$ increases. This suggests an onset of localization, but it is weaker than Anderson localization.

quant-ph