arXiv subjects

Sujoy Karan

Publications and source records attributed to Sujoy Karan.

5 recordsLinked to original sources

arXiv2026

Enhancing the Energy Resolution in Scanning Tunneling Microscopy: from dynamical Coulomb blockade to cavity quantum electrodynamics

Scanning tunneling microscopy and spectroscopy have become indispensable tools for probing condensed matter at atomic length scales, yet achieving ultimate energy resolution remains a persistent challenge. At mK temperatures, the dynamical Coulomb blockade regime fundamentally limits spectroscopic precision through energy exchange between tunneling electrons and the electromagnetic environment. Here, we demonstrate that combining local electromagnetic shielding with low-pass filtering directly at the cryogenic scan head improves the energy resolution by nearly an order of magnitude, reaching benchmark values as low as 3.7$\mu$eV at 10mK. We attribute this enhancement to efficient suppression of high-frequency radiation and capacitive shunting of the tunnel junction. Remarkably, this improved sensitivity reveals that the Josephson current couples to electromagnetic cavity modes of the centimeter-scale scan head, establishing a direct connection between atomic-scale tunneling processes and macroscopic cavity quantum electrodynamics. These advances open pathways for exploring ultra-low-energy phenomena with unprecedented precision.

cond-mat.supr-con↗

arXiv2023

Tracking a Spin-Polarized Superconducting Bound State across a Quantum Phase Transition

The magnetic exchange coupling between magnetic impurities and a superconductor induce so-called Yu-Shiba-Rusinov (YSR) states which undergo a quantum phase transition (QPT) upon increasing the exchange interaction beyond a critical value. While the evolution through the QPT is readily observable, in particular if the YSR state features an electron-hole asymmetry, the concomitant change in the ground state is more difficult to identify. We use ultralow temperature scanning tunneling microscopy to demonstrate how the change in the YSR ground state across the QPT can be directly observed for a spin-1/2 impurity in a magnetic field. We observe a change in the excitation spectrum from the doublet ground state in the free spin regime (two spectral features) to the singlet ground state in the screened spin regime (four spectral features). We also identify a transition regime, where the YSR excitation energy is smaller than the Zeeman energy. We thus provide a straightforward way for unambiguously identifying the ground state of a spin-1/2 YSR state.

cond-mat.supr-con↗

arXiv2022

Universal scaling of tunable Yu-Shiba-Rusinov states across the quantum phase transition

Quantum magnetic impurities give rise to a wealth of phenomena attracting tremendous research interest in recent years. On a normal metal, magnetic impurities generate the correlation-driven Kondo effect. On a superconductor, bound states emerge inside the superconducting gap called the Yu-Shiba-Rusinov (YSR) states. Theoretically, quantum impurity problems have been successfully tackled by numerical renormalization group (NRG) theory, where the Kondo and YSR physics are shown to be unified and the normalized YSR energy scales universally with the Kondo temperature divided by the superconducting gap. However, experimentally the Kondo temperature is usually extracted from phenomenological approaches, which gives rise to significant uncertainties and cannot account for magnetic fields properly. Using scanning tunneling microscopy at 10mK, we apply a magnetic field to several YSR impurities on a vanadium tip to reveal the Kondo effect and employ the microscopic single impurity Anderson model with NRG to fit the Kondo spectra in magnetic fields accurately and extract the corresponding Kondo temperature unambiguously. Some YSR states move across the quantum phase transition (QPT) due to the changes in atomic forces during tip approach, yielding a continuous universal scaling with quantitative precision for quantum spin-1/2 impurities.

cond-mat.supr-con↗

arXiv2015

Spin Manipulation by Creation of Single-Molecule Radical Cations

All-trans-retinoic acid (ReA), a closed-shell organic molecule comprising only C, H, and O atoms, is investigated on a Au(111) substrate using scanning tunneling microscopy and spectroscopy. In dense arrays single ReA molecules are switched to a number of states, three of which carry a localized spin as evidenced by conductance spectroscopy in high magnetic fields. The spin of a single molecule may be reversibly switched on and off without affecting its neighbors. We suggest that ReA on Au is readily converted to a radical by the abstraction of an electron.

cond-mat.mtrl-sci↗

arXiv2015

Shifting the Voltage Drop in Electron Transport through a Single Molecule

A Mn-porphyrin was contacted on Au(111) in a low-temperature scanning tunneling microscope (STM). Differential conductance spectra show a zero-bias resonance that is due to an underscreened Kondo effect according to many-body calculations. When the Mn center is contacted by the STM tip, the spectrum appears to invert along the voltage axis. A drastic change in the electrostatic potential of the molecule involving a small geometric relaxation is found to cause this observation.

cond-mat.mes-hall↗