arXiv subjects

Suman Chakraborty

Publications and source records attributed to Suman Chakraborty.

At least 55 records · Page 3Linked to original sources

arXiv2020

Simulations of a weakly conducting droplet under the influence of an alternating electric field

We investigate the electrohydrodynamics of an initially spherical droplet under the influence of an external alternating electric field by conducting axisymmetric numerical simulations using a charge-conservative volume-of-fluid based finite volume flow solver. The mean amplitude of shape oscillations of a droplet subjected to an alternating electric field for leaky dielectric fluids is the same as the steady-state deformation under an equivalent root mean squared direct electric field for all possible electrical conductivity ratio $(K_r)$ and permittivity ratio $(S)$ of the droplet to the surrounding fluid. In contrast, our simulations for weakly conducting media show that this equivalence between alternating and direct electric fields does not hold for $K_r \ne S$. Moreover, for a range of parameters, the deformation obtained using the alternating and direct electric fields is qualitatively different, i.e. for low $K_r$ and high $S$, the droplet becomes prolate under alternating electric field but deforms to an oblate shape in the case of the equivalent direct electric field. A parametric study is conducted by varying the time period of the applied alternating electric field, the permittivity and the electrical conductivity ratios. It is observed that while increasing $K_r$ has a negligible effect on the deformation dynamics of the droplet for $K_r S$ for both alternating and direct electric fields. We believe that our results may be of immense consequence in explaining the morphological evolution of droplets in a plethora of scenarios ranging from nature to biology.

physics.flu-dyn↗

arXiv2020

Induced flow inside a droplet by static electrical charge

Introducing controlled fluid motion inside a droplet turns out to be of outstanding scientific importance. In this work, we suggest a new method of flow manipulation inside a sessile droplet by simply deploying a static charge produced by triboelectric effect. This is physically actuated by charge transfer between the two lateral electrodes within which the droplet is entrained, triggering a strong ionized air current. The flow inside the droplet is generated due to the shear exerted at the liquid-air interface by the charged induced ionized air flow around the droplet, a paradigm that has hitherto remained unexplored. The strength of the fluid flow can be controlled by adjusting the supplied charge. Such unique controllability without sacrificing the physical simplicity opens up new possibilities of flow manipulation in a multitude of applications in droplet based microfluidics.

physics.flu-dyn↗

arXiv2020

Elastohydrodynamics of a soft coating under fluid-mediated loading by a spherical probe

Motion of an object near a soft wall with intervening fluid is a canonical problem in elastohydrodynamics, finding presence in subjects spanning biology to tribology. Particularly, motion of a sphere towards a soft substrate with intervening fluid is often encountered in the context of scanning probe microscopy. While there have been fundamental theoretical studies on this setup, they have focussed on specific applications and thus enforced suitable simplifications. Here we present a versatile semi-analytical framework for studying the elastohydrodynamics of axisymmetric loading of a rigid sphere near a soft elastic substrate coated on a rigid platform mediated by an aqueous electrolytic solution. Three loading modes are considered - approach, recession and oscillatory. The framework incorporates - large oscillation frequency and amplitude, two-way coupling between pressure and substrate deformation, and presence of DLVO forces. From computations using the framework, we gain insights on the effects of DLVO forces, substrate thickness, substrate material compressibility (quantified by Poisson's ratio) and high oscillation frequency for different physical setups encountered in SPM and the likes. We list some key observations. A substrate that is thicker and more compressible allows for larger deformation, i.e. is effectively softer. Presence of DLVO forces lead to magnification in force of upto two orders of magnitude and in substrate deformation of upto an order of magnitude for oscillatory loading at low frequencies and approach/recession loading at low speed. For oscillatory loading at high frequencies, DLVO forces do not appreciably affect the force and deflection behaviour of the system. Having demonstrated the versatility and utility of our framework, we expect it to evolve into a diverse and useful tool for solving problems of soft-lubrication.

cond-mat.soft↗

arXiv2020

Coriolis force-based instability of a shear-thinning microchannel flow

Instability mechanism based on Coriolis force, on a rapidly rotating portable device handling shear thinning fluids such as blood, is of utmost importance for eventual detection of diseases by mixing with the suitable reagents. Motivated by this proposition, the present study renders a modal stability analysis of shear thinning fluids in a rotating microchannel modelled by the Carreau rheological law. When a microchannel is engraved a rotating compact disc (CD) based device, the centrifugal force acts as the driving force that actuates the flow and the Coriolis force enhances the mixing process in significantly short span by destabilizing the flow. An OrrSommerfeld-Squire analysis is performed to explore the role of these forces on the linear stability of rotating shear-thinning flow. Reported results on shear thinning flow with streamwise disturbances indicate that the critical Reynolds number for the flow transition with viscosity perturbation is nearly half of that of the critical value for the same without viscosity perturbation. In sharp contrast, the present analysis considering spanwise disturbances reveals that the critical Reynolds numbers with and without viscosity perturbation remain virtually unaltered under rotational effects. However, the viscosity variation has no significant influence on the Coriolis force-based instability. Numerical results confirm that a momentous destabilization is possible by aid of the Coriolis force via generating secondary flow inside the channel. Interestingly, the roll cells corresponding to the instabilities at lower time constants exhibit the existence of two distinct vortices, and the centre of the stronger one is essentially settled towards the unstable stratified region. Moreover, for a higher value of the time constant, only one vortex occupies the entire channel.

physics.flu-dyn↗

arXiv2019

Universality in coalescence of polymeric fluid drops

Coalescence of liquid droplets involves an interplay between capillary forces, viscous forces and inertial forces. Here, we unveil a universal temporal evolution of the neck radius during the coalescence of two polymeric drops. Through high speed imaging we demonstrate that drops of polyacrylamide (PAM), poly-vinyl alcohol (PVA), polyethylene oxide (PEO), polyethylene glycol (PEG) and xanthan gum (XG) depict a universal behavior $R/\sqrt(ν_0λ) \sim (t/λ)^{0.36}(C/C^{*})^{-0.83}$ over a dilute, semi-dilute and non-dilute range of concentrations. A linear Phan-Thein-Tanner viscoelastic model captures the temporal aspect of universality.

physics.flu-dyn↗

arXiv2019

Temperature-gradient induced massive augmentation of solute dispersion in viscoelastic micro-flows

Enhancing solute dispersion in electrically actuated flows has always been a challenging proposition, as attributed to the inherent uniformity of the flow field in absence of surface patterns. Over the years, researchers have focused their attention towards circumventing this limitation, by employing several fluidic and geometric modulations. However, the corresponding improvements in solute dispersion often turn out to be inconsequential. Here we unveil that by exploiting the interplay between an externally imposed temperature gradient, subsequent electrical charge redistribution and ionic motion, coupled with the rheological complexities of the fluid, one can achieve up to one order of magnitude enhancement of solute dispersion in a pressure-driven flow of an electrolyte solution. Our results demonstrate that the complex coupling between thermal, electrical, hydro-dynamic and rheological parameters over small scales, responsible for such exclusive phenomenon, can be utilitarian in designing novel thermally-actuated micro and bio-microfluidic devices with favorable solute separation and dispersion characteristics.

physics.flu-dyn↗

arXiv2019

Near-wall hydrodynamic slip triggers swimming state transition of microorganisms

Interaction of motile microrganisms with a nearby solid substrate is a well studied phenomenon. However, the effects of hydrodynamic slippage on the substrate have received a little attention. In the present study, within the framework of the squirmer model, we impose a tangential velocity at the swimmer surface as a representation of the ciliatory propulsion and subsequently obtain exact solution of the Stokes equation based on a combined analytical-numerical approach. We illustrate how the near-wall swimming velocities are non-trivially altered by the interaction of wall slip and hydrodynamic forces. We report a characteristic transition of swimming trajectories for both puller and pusher type microswimmers by hydrodynamic slippage if the wall-slip length crosses a critical value. In case of puller microswimmers that are propelled by a breast-stroke like action of their swimming apparatus ahead of their cell body, the wall slip can cause wall-bound trapping swimming states, either as periodic or damped periodic oscillations which would otherwise escape from a no slip wall. The associated critical slip length has a non-monotonic dependence on the initial orientation of the swimmer which is represented by novel phase diagrams. Pushers, which get their propulsive thrust from posterior flagellar action, also show similar swimming state transitions but in this case the wall slip mediated reorientation dynamics and the swimming modes compete in a different fashion to that of the pullers. The present results pave the way for understanding the motion characteristic of biological microswimmers near confinements with hydrophobic walls or strategize the design of microfluidic devices used for sorting and motion rectification of artificial swimmers by tailoring their surface wettability.

cond-mat.soft↗

arXiv2019

Influence of non-hydrodynamic forces on the elastic response of an ultra-thin soft coating under fluid-mediated dynamic loading

The force between two approaching solids in a liquid medium becomes increasingly large with decreasing separation, a phenomenon that prevents contact between the two solids. This growth in force occurs because of the intervening liquid, and, studies of such physical systems constitute the classical discipline of lubrication. Furthermore, when the solid(s) are soft, there are quantitative as well as qualitative alterations in the force interaction due to the solids' deformation. The underlying physics as well as resultant system behaviour are even more complex when forces of non-hydrodynamic origin come into play, two major classes of such forces being the DLVO (Derjaguin-Landau-Verwey-Overbeek) forces and the non-DLVO molecular forces. Studies assessing the coupling of these physical phenomenon are avenues of contemporary research. With this view, we perform an analytical study of fluid-mediated oscillatory motion of a rigid sphere over an ultra-thin soft coating, delineating the distinctive effects of solvation force as well as substrate compliance. Our key finding is the major augmentation in the force and substrate-deformation characteristics of the system due to solvation force when the confinement reduces to a few nanometers. Consideration of solvation force leads to upto four orders of magnitude and upto three orders of magnitude increment in force and substrate-deformation respectively. While higher softness leads to higher deformation (as expected), its effect on force and substrate-deformation characteristics exhibits a tendency towards amelioration of the increment due to solvation force.

cond-mat.soft↗

arXiv2019

Generalizing Co-operative Evaporation in Two-Dimensional Droplet Arrays

Sessile droplets exposed to an incipient condition lead to an inevitable loss of mass, which is critical in many practical applications. By considering an arbitrarily configured two-dimensional array of droplets, here we provide a simple generalized theoretical limit to their lifetime in an evaporating state. Notwithstanding the geometrical and physical complexity of the effective confinement generated due to their cooperative interactions, we show that the consequent evaporation characteristics may be remarkably insensitive to the topographical details of the overall droplet organization, for a wide range of droplet-substrate combinations. With subsequent deployment of particle-laden droplets, however, our results lead to the discovery of a unique pathway towards tailoring the internal flows within the collective system by harnessing an exclusive topologically-driven symmetry breaking phenomenon, yielding a new strategy of patterning particulate matters around the droplet array.

physics.flu-dyn↗

arXiv2019

Streaming Potential in Bio-mimetic Microvessels Mediated by Capillary Glycocalyx

Implantable medical devices and biosensors are pivotal in revolutionizing the field of medical technology by opening new dimensions in the field of disease detection and cure. These devices need to harness a biocompatible and physiologically sustainable safe power source instead of relying on external stimuli, overcoming the constraints on their applicability in-vivo. Here, by appealing to the interplay of electromechanics and hydrodynamics in physiologically relevant microvessels, we bring out the role of charged Endothelial Glycocalyx layer (EGL) towards establishing a streaming potential across physiological fluidic conduits. We account for the complex rheology of blood-mimicking fluid by appealing to Newtonian fluid model representing the blood plasma and a viscoelastic fluid model representing the whole blood. We model the EGL as a poroelastic layer with volumetric charge distribution. Our results reveal that for physiologically relevant microflows, the streaming potential induced is typically of the order of 0.1 V/mm, which may turn out to be substantial towards energizing biosensors and implantable medical devices whose power requirements are typically in the range of micro to milli Watt. We also bring out the specific implications of the relevant physiological parameters towards establishment of the streaming potential, with a vision of augmenting the same within plausible functional limits. We further unveil that the dependence of streaming potential on EGL thickness might be one of the key aspects in unlocking the mystery behind the angiogenesis pattern. Our results may open up novel bio-sensing and actuating possibilities in medical diagnostics as well as may provide a possible alternative regarding the development of physiologically safe and biocompatible power sources within the human body.

physics.flu-dyn↗

arXiv2019

On-Chip Concentration and Patterning of Biological Cells Using Interplay of Electrical and Thermal Fields

We demonstrate a method of concentrating and patterning of biological cells on a chip, exploiting the confluence of electric and thermal fields, without necessitating the use of any external heating or illuminating source. The technique simply employs two parallel plate electrodes and an insulating layer over the bottom electrode, with a drilled insulating layer for inducing localized variations in the thermal field. A strong induced electric field, in the process, penetrates through the narrow hole and generates highly non-uniform heating, which in turn, results in gradients in electrical properties and induces mobile charges to impose directional fluid flow. The toroidal vortices, induced by secondary electrokinetic forces originating out of temperature-dependent electrical property variations, transport the suspended cells towards a hot-spot site of the chip, for rapid concentrating and patterning into different shaped clusters based on pre-designed conditions, without exceeding safe temperature limits that do not result in damage of thermally labile biological samples. We characterize the efficacy of the cell trapping process for two different biological entities, namely, Escherichia coli bacteria and yeast cell. These results may be of profound importance towards developing novel biomedical microdevices for drug discovery, antibiotic resistance assessment and medical diagnostics.

physics.bio-ph↗

arXiv2019

Electrokinetic Power Harvesting from Wet Textile

Developing low-weight, frugal and sustainable power sources for resource-limited settings appears to be a challenging proposition for the advancement of next-generation sensing devices and beyond. Here, we report the use of centimeter-sized simple wet fabric pieces for electrical power generation, by deploying the interplay of a spontaneously induced ionic motion across fabric channels due to capillary action and simultaneous water evaporation by drawing thermal energy from the ambient. Unlike other reported devices with similar functionalities, our arrangement does not necessitate any input mechanical energy or complex topographical structures to be embedded in the substrate. A single device is capable of generating a sustainable open circuit potential up to 700 mV. This suffices establishing an inherent capability of functionalizing self-power electronic devices, and also to be potentially harnessed for enhanced power generation with feasible up-scaling.

physics.app-ph↗

arXiv2019

Anomalous diffusion in an electrolyte saturated paper matrix

Diffusion of colored dye on water saturated paper substrates has been traditionally exploited with great skill by renowned water color artists. The same physics finds more recent practical applications in paper based diagnostic devices deploying chemicals that react with a bodily fluid yielding colorimetric signals for disease detection. During spontaneous imbibition through the tortuous pathways of a porous electrolyte saturated paper matrix, a dye molecule undergoes diffusion in a complex network of pores. The advancing front forms a strongly correlated interface that propagates diffusively but with an enhanced effective diffusivity. We measure this effective diffusivity and show that it is several orders of magnitude greater than the free solution diffusivity and has a significant dependence on the solution pH and salt concentration in the background electrolyte. We attribute this to electrically mediated interfacial interactions between the ionic species in the liquid dye and spontaneous surface charges developed at porous interfaces, and introduce a simple theory to explain this phenomenon.

cond-mat.soft↗

arXiv2019

Joule Heating-Induced Particle Manipulation on a Microfluidic Chip

We develop an electrokinetic technique that continuously manipulates colloidal particles to concentrate into patterned particulate groups in an energy efficient way, by exclusive harnessing of the intrinsic Joule heating effects. Our technique exploits the alternating current electrothermal flow phenomenon which is generated due to the interaction between non-uniform electric and thermal fields. Highly non-uniform electric field generates sharp temperature gradients by generating spatially-varying Joule heat that varies along radial direction from a concentrated point hotspot. Sharp temperature gradients induce local variation in electric properties which, in turn, generate strong electrothermal vortex. The imposed fluid flow brings the colloidal particles at the centre of the hotspot and enables particle aggregation. Further, manoeuvering structures of the Joule heating spots, different patterns of particle clustering may be formed in a low power budget, thus, opening up a new realm of on-chip particle manipulation process without necessitating highly focused laser beam which is much complicated and demands higher power budget. This technique can find its use in Lab-on-a-chip devices to manipulate particle groups, including biological cells.

physics.app-ph↗

arXiv2019

Energy-Efficient Micromixing in Paper Based Devices Mediated by the Interplay of Electrical and Thermal Fields

Biomedical and biochemical processes in paper-based microfluidic devices often deal with mixing of two analytes to perform important functions. Uniform mixing of analytes in paper matrix is a challenging proposition, often necessitating complicated channel design or high energy external fields for realizing the desired functionality. In sharp contrast, here we demonstrate an energy-efficient technique compatible with handing biofluids, to achieve a high level of mixing of two fluids in paper-based microfluidic devices without deploying complex channel shapes. Our method employs a simple, cost-effective printing-based method to fabricate paper channel with interdigitated electrodes laid out using pencil sketch. An alternating current electric field of sufficiently low voltage is used to generate perturbations on the interface of the two fluids streams undertaking spontaneous capillary imbibition. The consequent variations in electric field generate local thermal gradients, leading to localized volumetric forces triggering efficient fluid mixing. Our results find a wide variety of applications ranging from biochemical analysis to medical diagnostics.

physics.app-ph↗

arXiv2019

Electrorheology of a dilute emulsion of surfactant-covered drops

The effects of surfactant coating on a deformable viscous drop under the combined action of a shear flow and a uniform electric field, are investigated by solving the coupled equations of electrostatics, fluid flow and surfactant transport. Employing a comprehensive three-dimensional solution technique, the non-Newtonian shearing response of the bulk emulsion is analyzed in the dilute suspension regime. The present results reveal that the surfactant non-uniformity creates significant alterations in the flow disturbance around the drop, thereby influencing the viscous dissipation from the flowing emulsion. This, in effect, triggers changes in the bulk shear viscosity. It is striking to observe that the balance between electrical and hydrodynamic stresses is affected in such a way that surface tension gradient on the drop surface vanishes for some specific shear rates and the corresponding effective change in the bulk viscosity becomes negligible too. This critical condition hugely depends on the electrical permittivity and conductivity ratios of the two fluids and orientation of the applied electric field. Also the physical mechanisms of charge convection of surface deformation play their role in determining this critical shear rate. The charge convection instigated shear thinning or shear thickening behavior of the emulsion gets reversed due to a coupled interaction of the charge convection and Marangoni stress. In addition, the electrically created anisotropic normal stresses in the bulk rheology, get reduced due to the presence of surfactants, especially when the drop viscosity is much lesser than the continuous fluid. A thorough description of the drop-level flow physics and its connection to the bulk rheology of a dilute emulsion, may provide a fundamental understanding of a more complex emulsion system.

physics.flu-dyn↗

arXiv2019

Nanoparticles modulate contact angle hysteresis in electrowetting

The pinning of the contact line adversely influences the electrowetting performance of sessile liquid droplets. In this paper, we report the electrowetting hysteresis characteristics of 100 mM aq. KCl sessile liquid droplet placed on a hydrophobic PDMS surface. The effect of nanoparticles on the contact angle hysteresis under the imposed electric potential is further investigated. This study reveals that the contact angle hysteresis decreases beyond a certain threshold value of nanoparticles concentration. Therefore, nanoparticle suspension in the liquid droplet can be used to enhance or suppress the electrowetting hysteresis and consequentially rate of heat transfer during hot spot cooling.

cond-mat.soft↗

arXiv2018

Stable Oleoplaned Slippery Surfaces on Biomimetically Patterned Templates

With the advent of the technology of the oleoplaned slippery surfaces as the better solution to self-cleaning, anti fouling and self-healing smart surfaces, the stability of the oil layer on the surfaces has caught a great deal of attention from the research community. Rose petals irrespective of its superhydrophobic nature exhibits a very high adhesion owing to the hierarchical structures and can thus serve as an excellent surface to obtain a stable oil film. Also, with gradual covering of the rose petal structures by the oil the change in the adhesion force is observed to decrease and an increase in the film thickness beyond a certain height causes cloaking of the droplet and thus presents us with an optimum thickness which can give us a stable oil film and also exhibit high degree of slipperiness. The findings can be applied for further applications in droplet based microfluidics, as a low energy actuation surface, or as a self-healing and self-cleaning surface.

physics.flu-dyn↗