Sung-Il Kim | Searcharxiv

arXiv2024

Thermoelectric signature of quantum criticality in the heavy-fermion superconductor CeRhIn$_5$

The evolution of the Fermi surface across the quantum critical point (QCP), which is relevant for characterizing the quantum criticality and understanding its relation with unconventional superconductivity, is an intriguing subject in the study of strongly correlated electron systems. In this study, we report the thermopower measurements to investigate a change in Fermi surface across the QCP in pure and 4.4% Sn-doped CeRhIn$_5$. Results show that their thermopower behavior differs significantly in the vicinity of their respective pressure-induced QCP. In pure CeRhIn$_5$, a drastic collapse of the thermopower takes place at the Kondo breakdown QCP, where the Fermi surface reconstructs concurrently with the development of the magnetic order. By contrast, the thermopower exhibits a broadly symmetric behavior around the QCP in 4.4% Sn-doped CeRhIn$_5$, which is a characteristic of the spin-density-wave QCP. These observations are consistent with the theoretical expectations and suggest the effectiveness of thermopower measurement in discriminating the nature of quantum criticality in heavy-fermion systems.

cond-mat.supr-con↗

arXiv2019

Tunable quantum critical point and detached superconductivity in Al-doped CrAs

The origin of unconventional superconductivity and its relationship to a T=0 K continuous quantum phase transition (a quantum critical point, QCP), which is hidden inside the dome of a superconducting state, have long been an outstanding puzzle in correlated superconductors. The observation and tuning of the hidden QCP, which is critical in resolving the mystery, however, has been rarely reported due to lack of ideal systems. The helical antiferromagnet CrAs provides an example in which a dome of superconductivity appears at a pressure where its magnetic transition goes to zero temperature. Here we report the tuning of a projected critical point in CrAs via Al chemical doping (Al-CrAs) and separation of the magnetic critical point from the pressure-induced superconducting phase. When CrAs is doped with Al, its AFM ordering temperature TN increases from 260 K to 270 K. With applied pressure, TN decreases and extrapolates to zero Kelvin near 4.5 kbar, which is shifted from 8 kbar for undoped CrAs. A funnel of anomalously enhanced electron scattering and a non-Fermi liquid resistivity underscore an AFM QCP near 4.5 kbar in Al-CrAs. Pressure-induced superconductivity, in contrast, is almost independent of Al doping and forms a dome with essentially the identical maximum Tc and same optimal pressure as in pure CrAs. The clear separation between the tuned AFM QCP and Tc maximum in Al-CrAs suggests that superconductivity is independent of the AFM QCP, illustrating subtleties in the interplay between superconductivity and quantum criticality in correlated electron systems.

cond-mat.supr-con↗