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Sunghoon Kim

Publications and source records attributed to Sunghoon Kim.

At least 19 recordsLinked to original sources

Imaging flat band electron hydrodynamics in biased bilayer graphene

Hydrodynamic electron transport arises when carrier kinetics are dominated by interelectron collisions rather than the relaxation of momentum out of the electron system. In recent years, signatures of electron hydrodynamics have been reported in graphene devices owing to the low disorder and weak electron-phonon coupling. However, these experiments have been performed in regimes where the carrier mass is light, and the electron-electron collision length--though smaller than corresponding lengths for phonon or impurity scattering--remains large in absolute terms, typically several hundred nanometers. This restricts hydrodynamic transport phenomena to large length scales, limiting miniaturization of devices based on hydrodynamic flow. The advent of dual-gated rhombohedral graphene multilayers introduces a new route toward enhanced hydrodynamic behavior via their large--and tunable--effective mass. Here, we employ a scanning superconducting magnetic sensor to image local current flow in dual-gated bilayer graphene. Exploiting a sample geometry sensitive to both laminar and vortical flow, we identify three distinct transport regimes--ballistic, hydrodynamic, and diffusive--across the full phase space spanned by carrier density and displacement field. The strongest hydrodynamic transport is observed in the flat band regime, where fitting our results to a unified Boltzmann transport model reveals the electron-electron scattering length to be comparable to the Fermi wavelength of ~50 nm. High-current measurements, meanwhile, reveal striking nonlinearities in the flow pattern. Our results pave the way for miniaturized electronic devices based on linear and nonlinear electron hydrodynamics.

cond-mat.mes-hall

SU(4) Kondo Lattice in Semiconductor Moir\'e Materials

Motivated by recent advances in transition metal dichalcogenide (TMD) moir\'e materials, we propose TMD moir\'e multilayers as a platform for realizing an approximately SU(4)-symmetric triangular Kondo lattice, generalizing the concept of the double quantum dot model. Our model extends the conventional Kondo lattice by incorporating a three-site exchange of SU(4) local moments, which drives spontaneous time-reversal and lattice symmetry breaking. Using a parton mean-field approach, we map out the phase diagram as a function of three-site exchange and hole doping. In the Kondo-unscreened regime, we identify Mott insulating phases, including bond-ordered states and a chiral spin liquid. With increasing doping, Kondo hybridization gives rise to a heavy Fermi liquid that exhibits distinct patterns of lattice symmetry breaking, with or without topological responses. We conclude with directions for future study.

cond-mat.str-el

Scalable, nanoscale positioning of highly coherent color centers in prefabricated diamond nanostructures

Nanophotonic devices in color center-containing hosts provide efficient readout, control, and entanglement of the embedded emitters. Yet control over color center formation - in number, position, and coherence - in nanophotonic devices remains a challenge to scalability. Here, we report a controlled creation of highly coherent diamond nitrogen-vacancy (NV) centers with nanoscale three-dimensional localization in prefabricated nanostructures with high yield. Combining nitrogen $\delta$-doping during chemical vapor deposition diamond growth and localized electron irradiation, we form shallow NVs registered to the center of diamond nanopillars with wide tunability over NV number. We report positioning precision of ~ 4 nm in depth and 46(1) nm laterally in pillars (102(2) nm in bulk diamond). We reliably form single NV centers with long spin coherence times (average $T_2^{Hahn}$ = 98 $\mu s$) and 1.8x higher average photoluminescence compared to NV centers randomly positioned in pillars. We achieve a 3x improved yield of NV centers with single electron-spin sensitivity over conventional implantation-based methods. Our high-yield defect creation method will enable scalable production of solid-state defect sensors and processors.

quant-ph

Homogenization of an obstacle problem with highly oscillating coefficients and obstacles

We develop the viscosity method for the homogenization of an obstacle problem with highly oscillating obstacles. The associated operator, in non-divergence form, is linear and elliptic with variable coefficients. We first construct a highly oscillating corrector, which captures the singular behavior of solutions near periodically distributed holes of critical size. We then prove the uniqueness of a critical value that encodes the coupled effects of oscillations in both the coefficients and the obstacles.

math.AP

Correlated Topological Mixed-Valence Insulators in Moir\'e Hetero-Bilayers

Moir\'e transition metal dichalcogenide (TMD) materials provide an ideal playground for studying the combined interplay of strong interactions and band-topology over a range of electronic fillings. Here we investigate the panoply of interaction-induced electronic phases that arise at a total commensurate filling of $\nu_T=2$ in moir\'e TMD heterobilayers, focusing specifically on their renormalized band-topology. We carry out a comprehensive self-consistent parton mean-field analysis on an interacting mixed-valence Hamiltonian describing AB-stacked MoTe$_2$/WSe$_2$ to highlight different ingredients that arise due to "Mottness", band-flattening, an enhanced excitonic tendency, and band-inversion, leading to correlated topological semi-metals and insulators. We also propose a possible route towards realizing fractionalized insulators with emergent neutral fermionic excitations in this and other closely related platforms.

cond-mat.str-el

Theory of Correlated Insulators and Superconductor at $\nu=1$ in Twisted WSe$_2$

The observation of a superconducting phase, an intertwined insulating phase, and a continuous transition between the two at a commensurate filling of $\nu=1$ in bilayers of twisted WSe$_2$ at $\theta=3.65^0$ raises a number of intriguing questions about the origin of this phenomenology. Here we report the possibility of a displacement-field induced continuous transition between a superconductor and a quantum spin-liquid Mott insulator at $\nu=1$, starting with a simplified three-orbital model of twisted WSe$_2$, including on-site, nearest-neighbor density-density interactions, and a chiral-exchange interaction, respectively. By employing parton mean-field theory, we discuss the nature of these correlated insulators, their expected evolution with the displacement-field, and their phenomenological properties.

cond-mat.str-el

Quasicrystalline Spin Liquid

The interplay of electronic interactions and frustration in crystalline systems leads to a panoply of correlated phases, including exotic Mott insulators with non-trivial patterns of entanglement. Disorder introduces additional quantum interference effects that can drive localization phenomena. Quasicrystals, which are neither disordered nor perfectly crystalline, are interesting playgrounds for studying the effects of interaction, frustration, and quantum interference. Here we consider a solvable example of a quantum spin liquid on a tri-coordinated quasicrystal. We extend Kitaev's original construction for the spin model to our quasicrystalline setting and perform a large scale flux-sampling to find the ground-state configuration in terms of the emergent majorana fermions and flux excitations. This reveals a fully gapped and time-reversal symmetric quantum spin liquid, regardless of the exchange anisotropies, accompanied by a tendency towards non-trivial (de-)localization at the edge and the bulk. The advent of moir\'e materials and a variety of quantum simulators provide a new platform to bring phases of quasicrystalline quantum matter to life in a controlled fashion.

cond-mat.str-el

Emergence of ferromagnetism at the onset of moir\'e Kondo breakdown

The interaction of a lattice of localized magnetic moments with a sea of conduction electrons in Kondo lattice models induces rich quantum phases of matter, such as Fermi liquids with heavily renormalized electronic quasiparticles, quantum critical non-Fermi liquid metals and unconventional superconductors, among others. The recent demonstration of moir\'e Kondo lattices has opened the door to investigate the Kondo problem with continuously tunable parameters. Although a heavy Fermi liquid phase has been identified in moir\'e Kondo lattices, the magnetic phases and Kondo breakdown transitions remain unexplored. Here we report a density-tuned Kondo destruction in AB-stacked MoTe2/WSe2 moir\'e bilayers by combining magneto transport and optical studies. As the itinerant carrier density decreases, the Kondo temperature decreases. At a critical density, we observe a heavy Fermi liquid to insulator transition, and a nearly concomitant emergence of ferromagnetic order. The observation is consistent with the scenario of a ferromagnetic Anderson insulator and suppression of the Kondo screening effect. Our results pave the path for inducing other exotic quantum phase transitions in moir\'e Kondo lattices.

cond-mat.str-el

Unveiling the double-peak structure of quantum oscillations in the specific heat

Quantum oscillation phenomenon is an essential tool to understand the electronic structure of quantum matter. Here we report a systematic study of quantum oscillations in the electronic specific heat $C_{el}$ in natural graphite. We show that the crossing of a single spin Landau level and the Fermi energy give rise to a double-peak structure, in striking contrast to the single peak expected from Lifshitz-Kosevich theory. Intriguingly, the double-peak structure is predicted by the kernel term for $C_{el}/T$ in the free electron theory. The $C_{el}/T$ represents a spectroscopic tuning fork of width 4.8 $k_B T$ which can be tuned at will to resonance. Using a coincidence method, the double-peak structure can be used to accurately determine the Lande $g$-factor of quantum materials. More generally, the tuning fork can be used to reveal any peak in fermionic density of states tuned by magnetic field, such as Lifshitz transition in heavy-fermion compounds.

physics.app-ph

Fractionalization and topology in amorphous electronic solids

Band-topology is traditionally analyzed in terms of gauge-invariant observables associated with crystalline Bloch wavefunctions. Recent work has demonstrated that many of the free fermion topological characteristics survive even in an amorphous setting. In this work, we extend these studies to incorporate the effect of strong repulsive interactions on the fate of topology and other correlation induced phenomena. Using a parton-based approach, we obtain the interacting phase diagram for an electronic two-orbital model with tunable topology in a two dimensional amorphous network. In addition to the (non-)topological phases that are adiabatically connected to the free fermion limit, we find a number of strongly interacting amorphous analogs of crystalline Mott insulating phases with non-trivial chiral neutral edge modes, and a fractionalized Anderson insulating phase. The amorphous networks thus provide a new playground for studying a plethora of exotic states of matter, and their glassy dynamics, due to the combined effects of non-trivial topology, disorder, and strong interactions.

cond-mat.str-el

Continuous Mott transition in moir\'e semiconductors: role of long-wavelength inhomogeneities

Recent experiments in moir\'{e} transition metal dichalcogenide materials have reported the observation of a continuous bandwidth-tuned transition from a metal to a paramagnetic Mott insulator at a fixed filling of one electron per moir\'{e} unit cell. The electrical transport measurements reveal a number of puzzling features that are seemingly at odds with the theoretical expectations of an interaction induced, but disorder-free, bandwidth-tuned metal-insulator transition. In this work, we include the effects of long-wavelength inhomogeneities, building on the results for a continuous metal-insulator transition at fixed filling in the clean limit. We examine the effects of meso-scale inhomogeneities near the critical point on transport using the framework of random resistor networks, highlighting the salient differences from a simple percolation-based picture. We place our results in the context of recent and ongoing experiments.

cond-mat.str-el

Diffusive density response of electrons in anisotropic multiband systems

We explicitly calculate the density-density response function with conserving vertex corrections for anisotropic multiband systems in the presence of impurities including long-range disorder. The direction-dependence of the vertex corrections is correctly considered to obtain the diffusion constant which is given by the combination of the componentwise transport relaxation times and velocities on the Fermi surface. We also investigate the diffusive density response of various anisotropic systems, propose some empirical rules for the corresponding diffusion constant, and demonstrate that it is crucial to consider the component-dependence of the transport relaxation times to correctly interpret the transport properties of anisotropic systems, especially various topological materials with a different power-law dispersion in each direction.

cond-mat.mes-hall

Properties of Generalized Degenerate Parabolic Systems

In this paper, we consider the solution $\bold{u}=\left(u^1,\cdots,u^k\right)$ of the generalized parabolic system \begin{equation*} \left(u^i\right)_t=\nabla\cdot\left(mU^{m-1}\mathcal{A}\left(\nabla u^i,u^i,x,t\right)+\mathcal{B}\left(u^i,x,t\right)\right), \qquad \left(1\leq i\leq k\right) \end{equation*} in the range of exponents $m>\frac{n-2}{n}$ where the diffusion coefficient $U$ depends on the components of the solution $\bold{u}$. Under suitable structure conditions on the vector fields $\mathcal{A}$ and $\mathcal{B}$, we first show the uniform $L^{\infty}$ bound of the function $U$ for $t\geq τ>0$ and law of $L^1$ mass conservation of each component $u^i$, $(i=1,\cdots,k)$, with system version of Harnack type inequality. As the last result, we also deal with the local continuity of solution $\bold{u}=\left(u^1,\cdots,u^k\right)$ with the intrinsic scaling. If the ratio between $U$ and components $u^i$, $(i=1,\cdots,k)$, is uniformly bounded above and below, all components of the solution $\bold{u}$ have the same modulus of continuity.

math.AP

System of Degenerate Parabolic $p$-Laplacian

In this paper, we study the mathematical properties of the solution $\bold{u}=\left(u^1,\cdots,u^k\right)$ to the degenerate parabolic system \begin{equation*} \bold{u}_t=\nabla\cdot\left(\left|\nabla\bold{u}\right|^{p-2}\nabla \bold{u}\right), \qquad \qquad \left(p>2\right). \end{equation*} More precisely, we show the uniqueness and existence of solution $\bold{u}$ and investigate a priori $L^{\infty}$ boundedness of the gradient of the solution. Assuming that the solution decays quickly at infinity, we also prove that the component $u^l$, $\left(1\leq l\leq k\right)$, converges to the function $c^l\mathcal{B}$ in space as $t\to\infty$. Here, the function $\mathcal{B}$ is the fundamental or Barenblatt solution of $p$-Laplacian equation and the constant $c^l$ is determined by the $L^1$-mass of $u^l$. The proof is based on the existence of entropy functional.\\ \indent As an application of the asymptotic large time behaviour, we establish a Harnack type inequality which makes the size of spatial average being controlled by the value of solution at one point.

math.AP

Bayesian neural network with pretrained protein embedding enhances prediction accuracy of drug-protein interaction

The characterization of drug-protein interactions is crucial in the high-throughput screening for drug discovery. The deep learning-based approaches have attracted attention because they can predict drug-protein interactions without trial-and-error by humans. However, because data labeling requires significant resources, the available protein data size is relatively small, which consequently decreases model performance. Here we propose two methods to construct a deep learning framework that exhibits superior performance with a small labeled dataset. At first, we use transfer learning in encoding protein sequences with a pretrained model, which trains general sequence representations in an unsupervised manner. Second, we use a Bayesian neural network to make a robust model by estimating the data uncertainty. As a result, our model performs better than the previous baselines for predicting drug-protein interactions. We also show that the quantified uncertainty from the Bayesian inference is related to the confidence and can be used for screening DPI data points.

cs.LG

GCIceNet: A Graph Convolutional Network for Accurate Classification of Water Phases

Understanding phases of water molecules based on local structure is essential for understanding their anomalous properties. However, due to complicated structural motifs formed via hydrogen bonds, conventional order parameters represent the water molecules incompletely. In this paper, we develop a GCIceNet, which automatically generates machine-based order parameters for classifying the phases of the water molecules via supervised and unsupervised learning. Multiple graph convolutional layers in the GCIceNet can learn topological informations of the complex hydrogen bond networks. It shows a substantial improvement of accuracy for predicting the phase of water molecules in the bulk system and the ice/vapor interface system. A relative importance analysis shows that the GCIceNet can capture the structural features of the given system hidden in the input data. Augmented with the vast amount of data provided by molecular dynamics simulations, the GCIceNet is expected to serve as a powerful tool for the fields of glassy liquids and hydration layers around biomolecules.

cond-mat.soft

Tunable quantum interference effect on magnetoconductivity in few-layer black phosphorus

In this study, we develop a systematic weak localization/antilocalization theory fully considering the anisotropy and Berry phase of the system, and apply it to various phases of few-layer black phosphorus (BP), which has a highly anisotropic electronic structure with an electronic gap size tunable even to a negative value. The derivation of a Cooperon ansatz for the Bethe-Salpeter equation in a general anisotropic system is presented, revealing the existence of various quantum interference effects in different phases of few-layer BP, including a crossover from weak localization to antilocalization. We also predict that the magnetoconductivity at the semi-Dirac transition point will exhibit a nontrivial power-law dependence on the magnetic field, while following the conventional logarithmic field-dependence of 2D systems in the insulator and Dirac semimetal phases. Notably, the ratio between the magnetoconductivity and Boltzmann conductivity turns out to be independent of the direction, even in strongly anisotropic systems. Finally, we discuss the tunability of the quantum corrections of few-layer BP in terms of the symmetry class of the system.

cond-mat.mes-hall

System of Porous Medium Equations

We investigate the evolution of population density vector, $\bold{u}=\left(u^1,\cdots,u^k\right)$, of $k$-species whose diffusion is controlled by its absolute value $\left|\bold{u}\right|$. More precisely we study the properties and asymptotic large time behaviour of solution $\bold{u}=\left(u^1,\cdots,u^k\right)$ of degenerate parabolic system \begin{equation*} \left(u^i\right)_t=\nabla\cdot\left(\left|\bold{u}\right|^{m-1}\nabla u^i\right) \qquad \mbox{for $m>1$ and $i=1,\cdots,k$}. \end{equation*} Under some regularity assumption, we prove that the function $u^i$ which describes the population density of $i$-th species with population $M_i$ converges to $\frac{M_i}{\left|\bold{M}\right|}\mathcal{B}_{\left|\bold{M}\right|}$ in space with two different approaches where $\mathcal{B}_{\left|\bold{M}\right|}$ is the Barenblatt solution of the porous medium equation with $L^1$-mass $\left|\bold{M}\right|=\sqrt{M_1^2+\cdots+M_k^2}$. \indent As an application of the asymptotic behaviour, we establish a suitable harnack type inequality which makes the spatial average of $u^i$ under control by the value of $u^i$ at one point. We also find an 1-directional travelling wave type solutions and the properties of solutions which has travelling wave behaviour at infinity.

math.AP