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Sven Hoefling

Publications and source records attributed to Sven Hoefling.

At least 19 recordsLinked to original sources

Photonic Cluster State Generation from a Quantum Dot Emitting in the Telecom C-band

Photonic cluster states are a key resource for photonic quantum information processing. So far, deterministic generation of these states has been limited to the near-infrared wavelength range. To achieve quantum advantage in communication while maintaining compatibility with silicon photonics, operation in the telecom wavelength range is required. In this work, we demonstrate deterministic cluster state generation directly in the telecom C-band. This is achieved through repetitive excitation of a hole spin confined in an indium-arsenide quantum dot subjected to an external magnetic field. We characterize the quantum process that generates the cluster state by measuring its process map, obtaining a fidelity of $\mathrm{F} = 0.71 \pm 0.01$ to the ideal case. As part of this characterization, we observe spin--photon polarization entanglement with a negativity of $\mathrm{N} = 0.27 \pm 0.02$. The emitted photons exhibit indistinguishability of at least 83%, demonstrating the potential for future fusion gates necessary for photonic cluster state generation beyond linear connectivity.

quant-ph

Exciton diffusion in two-dimensional chiral perovskites

Two-dimensional (2D) organic-inorganic hybrid perovskites emerged as a versatile platform for light-emitting and photovol-taic applications due to their unique structural design and chemical flexibility. Their properties depend heavily on both the choice of the inorganic lead halide framework and the surrounding organic layers. Recently, the introduction of chiral cations into 2D perovskites has attracted major interest due to their potential for introducing chirality and tuning the chiro-optical response. Importantly, the optical properties in these materials are dominated by tightly bound excitons that also serve as primary carriers for the energy transport. The mobility of photoinjected excitons is thus important from the perspectives of fundamental material properties and optoelectronic applications, yet remains an open question. Here, we demonstrate exciton propagation in a 2D chiral perovskite methylbenzylammonium lead iodide (MBA2PbI4) using transient photoluminescence microscopy and reveal density-dependent transport over more than 100 nanometers at room temperature with diffusion coeffi-cients as high as 2 cm2/s. We observe two distinct regimes of initially rapid diffusive propagation and subsequent localiza-tion. Moreover, perovskites with enantiomer pure cations are found to exhibit faster exciton diffusion compared to the race-mic mixture, correlated with the impact of the material composition on disorder. Altogether, the observations of efficient exciton diffusion at room temperature highlight the potential of 2D chiral perovskites to merge chiro-optical properties with strong light-matter interaction and efficient energy transport.

cond-mat.mtrl-sci

Polarized and Un-Polarized Emission from a Single Emitter in a Bullseye Resonator

We present polarized |S|=0.99$\pm$0.01, and unpolarized |S|=0.03$\pm$0.01 emission from a single emitter embedded in a single, cylindrically symmetric device design. We show that the polarization stems from a position offset of the single emitter with respect to the cavity center, which breaks the cylindrical symmetry, and a position-dependent coupling to the frequency degenerate eigenmodes of the resonator structure. The experimental results are interpreted by using numerical simulations and by experimental mapping of the polarization-resolved far-field emission patterns. Our findings can be generalized to any nanophotonic structure where two orthogonal eigenmodes are not fully spatially overlapping.

physics.optics

Magneto-optics of a charge-tunable quantum dot: Observation of a negative diamagnetic shift

We present magneto-optical studies of a self-assembled semiconductor quantum dot in neutral and positively charged states. The diamagnetic shifts and Zeeman splitting of many well-identified optical transitions are precisely measured. Remarkably, a pronounced negative diamagnetic shift is observed for spectral lines resulting from a doubly positively charged excitonic complex. We use the Hartree - Fock approximation for describing the direct Coulomb and exchange interactions between the quantum dot confined carriers in various configurations. A simple harmonic potential model, which we extend to capture the influence of an externally applied magnetic field in Faraday configuration, is then used to quantitatively account for all the measured diamagnetic shifts. We show that the negative shift is due to the change in the hole-hole exchange interaction energy induced by the magnetic field. Using this model and the measured shifts we extract the dielectric constant of the quantum dot material and get a decent estimate of the quantum dot dimensions. Further, the measured Zeeman splitting of the various spectral lines are also explained by a simple model using algebraic sums and differences of the $g$-factors of the confined charge carriers in their respective first and second discrete energy levels. Finally, the obtained values of the electronic $g$-factor and that of the dielectric constant are independently used to determine the effective composition (x) of the ternary In$_{x}$Ga$_{1-x}$As quantum dot. Both agree to within the experimental uncertainties.

cond-mat.mes-hall

Experimental Multi-state Quantum Discrimination in the Frequency Domain with Quantum Dot Light

The quest for the realization of effective quantum state discrimination strategies is of great interest for quantum information technology, as well as for fundamental studies. Therefore, it is crucial to develop new and more efficient methods to implement discrimination protocols for quantum states. Among the others, single photon implementations are more advisable, because of their inherent security advantage in quantum communication scenarios. In this work, we present the experimental realization of a protocol employing a time-multiplexing strategy to optimally discriminate among eight non-orthogonal states, encoded in the four-dimensional Hilbert space spanning both the polarization degree of freedom and photon energy. The experiment, built on a custom-designed bulk optics analyser setup and single photons generated by a nearly deterministic solid-state source, represents a benchmarking example of minimum error discrimination with actual quantum states, requiring only linear optics and two photodetectors to be realized. Our work paves the way for more complex applications and delivers a novel approach towards high-dimensional quantum encoding and decoding operations.

quant-ph

Observation of intensity squeezing in resonance fluorescence from a solid-state device

Intensity squeezing, i.e., photon number fluctuations below the shot noise limit, is a fundamental aspect of quantum optics and has wide applications in quantum metrology. It was predicted in 1979 that the intensity squeezing could be observed in resonance fluorescence from a two-level quantum system. Yet, its experimental observation in solid states was hindered by inefficiencies in generating, collecting and detecting resonance fluorescence. Here, we report the intensity squeezing in a single-mode fibre-coupled resonance fluorescence single-photon source based on a quantum dot-micropillar system. We detect pulsed single-photon streams with 22.6% system efficiency, which show subshot-noise intensity fluctuation with an intensity squeezing of 0.59 dB. We estimate a corrected squeezing of 3.29 dB at the first lens. The observed intensity squeezing provides the last piece of the fundamental picture of resonance fluorescence; which can be used as a new standard for optical radiation and in scalable quantum metrology with indistinguishable single photons.

quant-ph

Boson sampling with 20 input photons in 60-mode interferometers at $10^{14}$ state spaces

Quantum computing experiments are moving into a new realm of increasing size and complexity, with the short-term goal of demonstrating an advantage over classical computers. Boson sampling is a promising platform for such a goal, however, the number of involved single photons was up to five so far, limiting these small-scale implementations to a proof-of-principle stage. Here, we develop solid-state sources of highly efficient, pure and indistinguishable single photons, and 3D integration of ultra-low-loss optical circuits. We perform an experiment with 20 single photons fed into a 60-mode interferometer, and, in its output, sample over Hilbert spaces with a size of $10^{14}$ $-$over ten orders of magnitude larger than all previous experiments. The results are validated against distinguishable samplers and uniform samplers with a confidence level of 99.9%.

quant-ph

Towards optimal single-photon sources from polarized microcavities

An optimal single-photon source should deterministically deliver one and only one photon at a time, with no trade-off between the source's efficiency and the photon indistinguishability. However, all reported solid-state sources of indistinguishable single photons had to rely on polarization filtering which reduced the efficiency by 50%, which fundamentally limited the scaling of photonic quantum technologies. Here, we overcome this final long-standing challenge by coherently driving quantum dots deterministically coupled to polarization-selective Purcell microcavities--two examples are narrowband, elliptical micropillars and broadband, elliptical Bragg gratings. A polarization-orthogonal excitation-collection scheme is designed to minimize the polarization-filtering loss under resonant excitation. We demonstrate a polarized single-photon efficiency of 0.60+/-0.02 (0.56+/-0.02), a single-photon purity of 0.975+/-0.005 (0.991+/-0.003), and an indistinguishability of 0.975+/-0.006 (0.951+/-0.005) for the micropillar (Bragg grating) device. Our work provides promising solutions for truly optimal single-photon sources combining near-unity indistinguishability and near-unity system efficiency simultaneously.

quant-ph

Coherently driving a single quantum two-level system with dichromatic laser pulses

Efficient excitation of a single two-level system usually requires that the driving field is at the same frequency as the atomic transition. However, the scattered laser light in solid-state implementations can dominate over the single photons, imposing an outstanding challenge to perfect single-photon sources. Here, we propose a background-free method using a phase-locked dichromatic electromagnetic field with no spectral overlap with the optical transition for a coherent control of a two-level system, and we demonstrate this method experimentally with a single quantum dot embedded in a micropillar. Single photons generated by pi excitation show a purity of 0.988(1) and indistinguishability of 0.962(6). Further, the phase-coherent nature of the two-color excitation is captured by the resonance-fluorescence intensity dependence on the relative phase between the two pulses. Our two-color excitation method adds a useful toolbox to the study of atom-photon interaction, and the generation of spectrally isolated indistinguishable single photons.

quant-ph

Resonance fluorescence from an atomic-quantum-memory compatible single photon source based on GaAs droplet quantum dots

Single photon sources, which are compatible with quantum memories are an important component of quantum networks. In this article, we show optical investigations on isolated GaAs/Al$_{0.25}$Ga$_{0.75}$As quantum dots grown via droplet epitaxy, which emit single photons on resonance with the Rb-87-D$_2$ line (780 nm). Under continuous wave resonant excitation conditions, we observe bright, clean and narrowband resonance fluorescence emission from such a droplet quantum dot. Furthermore, the second-order correlation measurement clearly demonstrates the single photon emission from this resonantly driven transition. Spectrally resolved resonance fluorescence of a similar quantum dot yields a linewidth as narrow as 660 MHz ($ 2.7~μeV $), which corresponds to a coherence time of 0.482 ns. The observed linewidth is the smallest reported so far for strain free GaAs quantum dots grown via the droplet method. We believe that this single photon source can be a prime candidate for applications in optical quantum networks.

cond-mat.mes-hall

Highly excited exciton-polariton condensates

Exciton-polaritons are a coherent electron-hole-photon (e-h-p) system where condensation has been observed in semiconductor microcavities. In contrast to equilibrium Bose-Einstein condensation (BEC) for long lifetime systems, polariton condensates have a dynamical nonequilibrium feature owing to the similar physical structure that they have to semiconductor lasers. One of the distinguishing features of a condensate to a laser is the presence of strong coupling between the matter and photon fields. Irrespective of its equilibrium or nonequilibrium nature, exciton-polariton have been observed to maintain strong coupling. We show that by investigating high density regime of exciton-polariton condensates, the negative branch directly observed in photoluminescence. This is evidence that the present e-h-p system is still in the strong coupling regime, contrary to past results where the system reduced to standard lasing at high density.

cond-mat.quant-gas

Quantum State Transfer from a Single Photon to a Distant Quantum-Dot Electron Spin

Quantum state transfer from flying photons to stationary matter qubits is an important element in the realization of quantum networks. Self-assembled semiconductor quantum dots provide a promising solid-state platform hosting both single photon and spin, with an inherent light-matter interface. Here, we develop a method to coherently and actively control the single-photon frequency bins in superposition using electro-optic modulators, and measure the spin-photon entanglement with a fidelity of $0.796\pm0.020$. Further, by Greenberger-Horne-Zeilinger-type state projection on the frequency, path and polarization degrees of freedom of a single photon, we demonstrate quantum state transfer from a single photon to a single electron spin confined in an InGaAs quantum dot, separated by 5 meters. The quantum state mapping from the photon's polarization to the electron's spin is demonstrated along three different axis on the Bloch sphere, with an average fidelity of $78.5\%$.

quant-ph

Multi-photon boson-sampling machines beating early classical computers

Boson sampling is considered as a strong candidate to demonstrate the quantum computational supremacy over classical computers. However, previous proof-of-principle experiments suffered from small photon number and low sampling rates owing to the inefficiencies of the single-photon sources and multi-port optical interferometers. Here, we develop two central components for high-performance boson sampling: robust multi-photon interferometers with 0.99 transmission rate, and actively demultiplexed single-photon sources from a quantum-dot-micropillar with simultaneously high efficiency, purity and indistinguishability. We implement and validate 3-, 4-, and 5-photon boson sampling, and achieve sampling rates of 4.96 kHz, 151 Hz, and 4 Hz, respectively, which are over 24,000 times faster than the previous experiments, and over 220 times faster than obtaining one sample through calculating the matrices permanent using the first electronic computer (ENIAC) and transistorized computer (TRADIC) in the human history. Our architecture is feasible to be scaled up to larger number of photons and with higher rate to race against classical computers, and might provide experimental evidence against the Extended Church-Turing Thesis.

quant-ph

Exciton-polariton condensates in zero-, one-, and two-dimensional lattices

Microcavity exciton-polaritons are quantum quasi-particles arising from the strong light-matter coupling. They have exhibited rich quantum dynamics rooted from bosonic nature and inherent non-equilibrium condition. Dynamical condensation in microcavity exciton-polaritons has been observed at much elevated temperatures in comparison to ultrocold atom condensates. Recently, we have investigated the behavior of exciton-polariton condensates in artificial trap and lattice geometries in zero-dimension, one-dimension (1D) and two-dimension (2D). Coherent $π$-state with p-wave order in a 1D condensate array and d-orbital state in a 2D square lattice are observed. We anticipate that the preparation of high-orbital condensates can be further extended to probe dynamical quantum phase transition in a controlled manner as quantum emulation applications.

cond-mat.quant-gas

Quantum dot micropillar cavities with quality factors exceeding 250,000

We report on the spectroscopic investigation of quantum dot - micropillar cavities with unprecedented quality factors. We observe a pronounced dependency of the quality factor on the measurement scheme, and find that significantly larger quality factors can be extracted in photoreflectance compared to photoluminescence measurements. While the photoluminescence spectra of the microcavity resonances feature a Lorentzian lineshape and Q-factors up to 184,000, the reflectance spectra have a Fano-shaped asymmetry and feature significantly higher Q-factors in excess of 250,000 resulting from a full saturation of the embedded emitters. The very high quality factors in our cavities promote strong light-matter coupling with visibilities exceeding 0.5 for a single QD coupled to the cavity mode.

quant-ph

Spatial correlation of two-dimensional Bosonic multi-mode condensates

We studied the spatial coherence of a Bosonic two-dimensional multi-mode condensate both through measurements and simulations. It is shown that condensates with a constant spatial density must be described as the superposition of several quantized modes which reduces the overall coherence. In this case, the spatial coherence can appear to decay faster than allowed by the Berezinskii-Kosterlitz-Thouless (BKT) theory. However, we find through spectroscopic measurements that the individual modes show a slower decay of the spatial coherence than the overall system.

cond-mat.quant-gas

Zero Dimensional Polariton Laser in a Sub-Wavelength Grating Based Vertical Microcavity

Semiconductor exciton-polaritons in planar microcavities form coherent two-dimensional condensates in non-equilibrium. However, coupling of multiple lower-dimensional polariton quantum systems, critically needed for polaritonic quantum device applications and novel cavity-lattice physics, has been limited due to the conventional cavity structures. Here we demonstrate full confinement of the polaritons non-destructively using a hybrid cavity made of a single-layer sub-wavelength grating mirror and a distributed Bragg reflector. Single-mode polariton lasing was observed at a chosen polarization. Incorporation of a designable slab mirror into the conventional vertical cavity, when operating in the strong-coupling regime, enables confinement, control and coupling of polariton gasses in a scalable fashion. It may open a door to experimental implementation of polariton-based quantum photonic devices and coupled cavity quantum electrodynamics systems.

cond-mat.quant-gas

Algebraic order and the Berezinskii-Kosterlitz-Thouless transition in an exciton-polariton gas

We observe quasi-long range coherence in a two-dimensional condensate of exciton-polaritons. Our measurements are the first to confirm that the spatial correlation algebraically decays with a slow power-law, whose exponent quantitatively behaves as predicted by the Berezinskii-Kosterlitz-Thouless theory. The exciton-polaritons are created by non-resonant optical pumping of a micro-cavity sample with embedded GaAs quantum-wells at liquid helium temperature. Michelson interference is used to measure the coherence of the photons emitted by decaying exciton-polaritons.

cond-mat.quant-gas