arXiv subjects

Sven Ramelow

Publications and source records attributed to Sven Ramelow.

At least 19 recordsLinked to original sources

arXiv2026

Polymer identification via undetected photons using a low footprint nonlinear interferometer

Plastic pollution has become a critical global challenge, with microplastics pervading ecosystems and entering human food chains. Effectively monitoring this widespread contamination demands rapid, reliable, and portable material identification techniques that often elude conventional Raman and FTIR spectroscopy. Undetected photon spectroscopy within a nonlinear interferometer (NLI) offers a solution, allowing the retrieval of mid-infrared absorption spectra by detecting only near-infrared signal photons using standard silicon-based technology. Here, we demonstrate a highly compact, micro-integrated, thermally-stabilised NLI with a Michelson-like geometry designed for the rapid spectroscopy of plastics. We benchmarked its room-temperature performance, demonstrating a signal-to-noise ratio of 34 with a measurement rate of 100 Hz and a spectral resolution of 6 cm$^{-1}$. We show that we can accurately and rapidly retrieve the characteristic vibrational absorption spectra of common polymers such as polypropylene, polyethene, and polystyrene, without using mid-infrared technology. These results establish our compact module as a promising field-deployable platform for robust, real-time environmental monitoring systems and other mid-infrared spectroscopy applications.

quant-ph↗

arXiv2026

Infrared photonics for healthcare: A roadmap for proactive and predictive health management

The field of infrared (IR) photonics is currently undergoing remarkable progress, moving rapidly towards practical sensing applications demanded by medical therapy and diagnostics (theranostics). The Developments can be divided into three main categories: (i) novel devices and measurement concepts including advanced updates of classical approaches that push medical sensing into the spotlight; (ii) new demonstrations of photonic integrated circuit (PIC-)based IR devices enabling highly miniaturized sensors for point-of-care application as well as medical and wellness wearables; and (iii) technologically-mature IR demonstrators that enable first medical sensing and treatment applications. This roadmap paper provides a consolidated overview of this highly dynamic and interdisciplinary research field with a focus on the major roadblocks that limit the widespread adoption of IR photonics in large-scale medical diagnostics. Special attention is given to the ambivalence between the molecular-level spectroscopic interpretation and a broader health-state assessment, highlighting the need for a common framework. Additionally, the paper discusses the critical importance of unified measurement standards, calibration protocols, and medical certification processes to ensure the validity of experimental results, reproducibility, and clinical trust, particularly when novel experimental techniques and AI algorithms are involved. Perspectives from major past and current contributors to application-oriented IR photonics will be provided.

physics.app-ph↗

arXiv2025

Mid-IR hyperspectral imaging with undetected photons

Sensing with undetected photons has become a vibrant, application-driven research domain with a special focus on the mid-infrared (mid-IR) wavelength region. Since the mid-IR contains spectral bands with highly specific and strong molecular absorbance signatures, often referred to as fingerprints, a multitude of different samples and their compositions can be detected and quantified spectroscopically. Enhancing this inherently sample alteration-free spectroscopic method with imaging capabilities leads to a powerful technique for environmental monitoring and biomedical applications that enables automated diagnostics while omitting time-consuming and non-reversible labeling steps. To evade the shortcomings of state-of-the-art instruments for mid-IR hyperspectral microscopy related to cost, complexity, power-consumption, and performance, which are associated with technological challenges for mid-IR cameras and low-noise and broadband mid-IR sources, here, we construct a proof-of-concept nonlinear interferometer in a wide-field imaging arrangement combined with high-resolution spectral acquisition by pixelwise quantum Fourier transform infrared spectroscopy. For the broadband range of 2300-3100 cm$^{-1}$, covering the important CH-stretch band, we perform hyperspectral imaging that simultaneously resolves 3500 spatial modes, each with a spectral resolution of 10 cm$^{-1}$ leveraging in total around 10$^5$ spatio-spectrally entangled photon modes. Our image acquisition uses a commercial, megapixel sCMOS camera, while a medium-power and compact c.w. pump laser is the only necessary light source.

physics.optics↗

arXiv2025

Hong-Ou-Mandel effect with two frequency-entangled photons of vastly different color

In the original formulation of the Hong-Ou-Mandel (HOM) experiment, when two otherwise indistinguishable photons are incident upon the two input ports of a balanced beam splitter, they coalesce, always leaving via the same output port. It is often interpreted that this interference arises due to the indistinguishability of the single photons at the beam splitter; the situation, however, is often more nuanced. Here, we demonstrate an analog of HOM interference between two photons of completely different color. To do so, we utilize a quantum frequency converter based on sum- and difference-frequency generation as an `active' beam splitter -- coupling frequency-entangled red and telecom single photons with an octave-spanning energy difference of 282 THz. We achieve an uncorrected two-photon interference visibility beyond 90%. This work presents the first demonstration of HOM interference between two single photons of distinctly different color, deepening our understanding of what underlies quantum interference. It also suggests a novel approach to interfacing photonic qubits in heterogeneous quantum systems where frequency conversion and quantum interference are unified.

quant-ph↗

arXiv2025

Quantum Fourier Transform Infrared Spectroscopy: Evaluation, Benchmarking and Prospects

Sensing with undetected photons has enabled new, unconventional approaches to Fourier transform infrared (FTIR) spectroscopy. Leveraging properties of non-degenerated entangled photon pairs, mid-IR information can be accessed in the near-IR spectral domain to perform mid-IR spectroscopy with silicon-based detection schemes. Here, we address practical aspects of vibrational spectroscopy with undetected photons using a quantum-FTIR (QFTIR) implementation. The system operates in the spectral range from around $3000~\mathrm{cm}^{-1}$ to $2380~\mathrm{cm}^{-1}$ (detection at around $12500~\mathrm{cm}^{-1}$) and possesses only $68~\mathrm{pW}$ of mid-IR probing power for spectroscopic measurements with a power-dependence of the signal-to-noise ratio of $1.5\cdot 10^{5}~\mathrm{mW}^{-1/2}$. We evaluate the system's short- and long-term stability and experimentally compare it to a commercial FTIR instrument using Allan-Werle plots to benchmark our QFTIR implementation's overall performance and stability. In addition, comparative qualitative spectroscopic measurements of polymer thin films are performed using the QFTIR spectrometer and a commercial FTIR with identical resolution and integration times. Our results show under which conditions QFTIR can practically be competitive or potentially outperform conventional FTIR technology.

physics.optics↗

arXiv2024

Advances in quantum imaging

Modern imaging technologies are widely based on classical principles of light or electromagnetic wave propagation. They can be remarkably sophisticated, with recent successes ranging from single molecule microscopy to imaging far-distant galaxies. However, new imaging technologies based on quantum principles are gradually emerging. They can either surpass classical approaches or provide novel imaging capabilities that would not otherwise be possible. {Here }we provide an overview {of the most recently developed quantum imaging systems, highlighting the non-classical properties of sources such as bright squeezed light, entangled photons, and single-photon emitters that enable their functionality.} We outline potential upcoming trends and the associated challenges, all driven by a central inquiry, which is to understand whether quantum light can make visible the invisible.

quant-ph↗

arXiv2024

Noise analysis of a quasi-phase-matched quantum frequency converter and higher-order counter-propagating SPDC

Quantum frequency conversion (QFC) will be an indispensable ingredient in future quantum technologies. For example, large-scale fibre-based quantum networks will require QFC to interconnect heterogeneous building blocks like emitters, channels, memories and detectors. The performance of existing QFC devices - typically realised in periodically-poled nonlinear crystals - is often severely limited by parasitic noise that arises when the pump wavelength lies between the inter-converted wavelengths. Here we comprehensively investigate the noise spectrum of a QFC device pumped by a CW 1064 nm laser. The converter was realised as a bulk periodically-poled potassium titanyl phosphate (ppKTP) crystal quasi-phase-matched for conversion between 637 nm and 1587 nm, which was also polished and coated to resonantly enhance the pump field by a factor of 50. While Raman scattering dominates the noise background from 1140 nm to 1330 nm, at larger energy shifts (beyond 60 THz), parasitic spontaneous parametric down-conversion (SPDC) is the strongest noise source. Further, the noise spectrum was contaminated by a regular succession of narrow-band peaks, which we attribute to a heretofore unidentified higher-order counter-propagating SPDC processes - with quasi-phase-matching orders up to 44 evident in our measurements. This work provides a comprehensive overview of the limiting noise sources in QFC devices that use quasi-phase-matched crystals and will prove an invaluable resource in guiding their future development.

quant-ph↗

arXiv2023

Telecom-Band SPDC in AlGaAs-on-Insulator Waveguides

Widespread commercial adoption of telecom-band quantum-key-distribution (QKD) will require fully integrated, room-temperature transmitters. Implementing highly efficient spontaneous parametric down-conversion (SPDC) on a platform that offers co-integration of the pump laser has been an outstanding challenge. Here, using such a platform based on AlGaAs-on-insulator waveguides, we report telecom-band SPDC (and second harmonic generation) with exceedingly large efficiencies of 26 GHz generated pairs/mW over a 7 THz bandwidth, which would saturate the usable photon-flux for a 70-channel wavelength-multiplexed QKD-system at merely 1.6 mW of pump laser power.

quant-ph↗

arXiv2023

Quantum light microscopy

Much of our progress in understanding microscale biology has been powered by advances in microscopy. For instance, super-resolution microscopes allow the observation of biological structures at near-atomic-scale resolution, while multi-photon microscopes allow imaging deep into tissue. However, biological structures and dynamics still often remain out of reach of existing microscopes, with further advances in signal-to-noise, resolution and speed needed to access them. In many cases, the performance of microscopes is now limited by quantum effects -- such as noise due to the quantisation of light into photons or, for multi-photon microscopes, the low cross-section of multi-photon scattering. These limitations can be overcome by exploiting features of quantum mechanics such as entanglement. Quantum effects can also provide new ways to enhance the performance of microscopes, such as new super-resolution techniques and new techniques to image at difficult to reach wavelengths. This review provides an overview of these various ways in which quantum techniques can improve microscopy, including recent experimental progress. It seeks to provide a realistic picture of what is possible, and what the constraints and opportunities are.

quant-ph↗

arXiv2023

Low-noise quantum frequency conversion in a monolithic cavity with bulk periodically poled potassium titanyl phosphate

Interfacing the different building blocks of a future large scale quantum network will demand efficient and noiseless frequency conversion of quantum light. Nitrogen-vacancy (NV) centers in diamond are a leading candidate to form the nodes of such a network. However, the performance of a suitable converter remains a bottleneck, with existing demonstrations severely limited by parasitic noise arising at the target telecom wavelength. Here, we demonstrate a new platform for efficient low-noise quantum frequency conversion based on a monolithic bulk ppKTP cavity and show its suitability for the conversion of 637 nm single photons from NV centers in diamond to telecommunication wavelengths. By resonantly enhancing the power of an off-the-shelf pump laser, we achieve an internal conversion efficiency of $(72.3\pm 0.4)\%$ while generating only $(110\pm 4) \mbox{ kHz/nm}$ noise at the target wavelength without the need for any active stabilization. This constitutes a 5-fold improvement in noise over existing state-of-the-art single-step converters at this wavelengths. We verify the almost ideal preservation of non-classical correlations by converting photons from a spontaneous parametric down-conversion source and moreover show the preservation of time-energy entanglement via Franson interferometry.

quant-ph↗

arXiv2022

Quantum imaging and metrology with undetected photons: a tutorial

We present a tutorial on the phenomenon of induced coherence without induced emission, and specifically its application to imaging and metrology. It is based on a striking effect where two nonlinear crystals, by sharing a coherent pump and one of two output beams each, can induce correlations between the other two individual, non-interacting beams. This can be thought of as a type of quantum-erasure effect, where the ``welcher-weg'' (which-way), or in this case ``which-source'' information is erased when the shared beams are aligned. With the correct geometry this effect can allow an object to be imaged using only photons which have never interacted with the object -- in other words the image is formed using undetected photons. Interest in this and related setups has been accelerating in recent years due to a number of desirable properties, mostly centered around the fact that the fields for detection and imaging (since separate) may have different optical properties, entailing significant advantages to various applications. The purpose of this tutorial is to introduce researchers to this area of research, to provide practical tools for setting up experiments as well as understanding the underlying theory, and to also provide a comprehensive overview of the sub-field as a whole.

quant-ph↗

arXiv2021

Mid-IR spectroscopy with NIR grating spectrometers

Mid-infrared (mid-IR) spectroscopy is a crucial workhorse for a plethora of analytical applications and is suitable for diverse materials, including gases, polymers or biological tissue. However, this technologically significant wavelength regime between 2.5-10$μ$m suffers from technical limitations primarily related to the large noise in mid-IR detectors and the complexity and cost of bright, broadband mid-IR light sources. Here, using highly non-degenerate, broadband photon pairs from bright spontaneous parametric down-conversion (SPDC) in a nonlinear interferometer, we circumvent these limitations and realise spectroscopy in the mid-IR using only a visible (VIS) solid-state laser and an off-the-shelf, commercial near-infrared (NIR) grating spectrometer. With this proof-of-concept implementation, covering a broad range from 3.2$μ$m to 4.4$μ$m, we access short integration times down to 1s and signal-to-noise ratios above 200 at a spectral resolution from 12cm$^{-1}$ down to 1.5cm$^{-1}$ for longer integration times. Through the analysis of polymer samples and the ambient CO$_2$ in our laboratory, we highlight the potential of this measurement technique for real-world applications.

physics.optics↗

arXiv2021

Talbot self-imaging and two-photon interference in ring-core fibers

Wave propagation on the surface of cylinders exhibits interferometric self imaging, much like the Talbot effect in the near-field diffraction at periodic gratings. We report the experimental observation of the cylindrical Talbot carpet in weakly-guiding ring-core fibers for classical light fields. We further show that the ring-core fiber acts as a high-order optical beamsplitter for single photons, whose output can be controlled by the relative phase between the input light fields. By also demonstrating high-quality two-photon interference between indistinguishable photons sent into the ring-core fiber, our findings open the door to applications in optical telecommunications as a compact beam multiplexer as well as in quantum information processing tasks as a scalable realization of a linear optical network.

physics.optics↗

arXiv2021

Mid-Infrared Microscopy via Position Correlations of Undetected Photons

Quantum imaging with undetected photons (QIUP) has recently emerged as a new powerful imaging tool. Exploiting the spatial entanglement of photon pairs, it allows decoupling of the sensing and detection wavelengths, facilitating imaging in otherwise challenging spectral regions with mature silicon-based detection technology. All existing implementations of QIUP have so far utilised the momentum correlations within the biphoton state. Here, for the first time, we implement and examine theoretically and numerically the complementary scenario - utilising the tight position correlations formed within photon pair at birth. This image plane arrangement facilitates high resolution imaging with comparative experimental ease, and we experimentally show resolutions below 10 $μ$m at a sensing wavelength of 3.7 $μ$m. Moreover, imaging a slice of mouse heart tissue at the mid-IR to reveal morphological features on the cellular level, we further demonstrate the viability of the technique for the life sciences. These results offer new perspectives on the capabilities of QIUP for label-free wide-field microscopy, enabling new real-world applications in biomedical as well as industrial imaging at inaccessible wavelengths.

quant-ph↗

arXiv2021

Low random duty-cycle errors in periodically-poled KTP revealed by sum-frequency generation

Low-noise quantum frequency conversion in periodically-poled nonlinear crystals has proved challenging when the pump wavelength is shorter than the target wavelength. This is - at least in large part - a consequence of the parasitic spontaneous parametric down-conversion of pump photons, whose efficiency is increased by fabrication errors in the periodic poling. Here we characterise the poling quality of commercial periodically-poled bulk potassium titanyl phosphate (ppKTP) by measuring the sum-frequency generation (SFG) efficiency over a large phase mismatch range from 0 to more than 400$π$. Over the probed range the SFG efficiency behaves nearly ideally and drops to a normalised efficiency of $10^{-6}$. Our results demonstrate that any background pedestal which would be formed by random duty cycle errors in ppKTP is substantially reduced when compared to periodically poled lithium niobate. The standard deviation of the random duty cycle errors can be estimated to be smaller than 2% of the domain length. From this, we expect a noise spectral density which is at least one order of magnitude smaller than that of current state-of-the-art single-step frequency converters.

quant-ph↗

arXiv2021

Versatile Super-Sensitive Metrology Using Induced Coherence

We theoretically analyze the phase sensitivity of the Induced-Coherence (Mandel-Type) Interferometer, including the case where the sensitivity is "boosted" into the bright input regime with coherent-light seeding. We find scaling which reaches below the shot noise limit, even when seeding the spatial mode which does not interact with the sample - or when seeding the undetected mode. It is a hybrid of a linear and a non-linear (Yurke-Type) interferometer, and aside from the supersensitivity, is distinguished from other systems by "preferring" an imbalance in the gains of the two non-linearities (with the second gain being optimal at low values), and non-monotonic behavior of the sensitivity as a function of the gain of the second non-linearity. Furthermore, the setup allows use of subtracted intensity measurements, instead of direct (additive) or homodyne measurements - a significant practical advantage. Bright, super-sensitive phase estimation of an object with different light fields for interaction and detection is possible, with various potential applications, especially in cases where the sample may be sensitive to light, or is most interesting in frequency domains outside what is easily detected, or when desiring bright-light phase estimation with sensitive/delicate detectors. We use an analysis in terms of general squeezing and discover that super-sensitivity occurs only in this case - that is, the effect is not present with the spontaneous-parametric-down-conversion approximation, which many previous analyses and experiments have focused on.

quant-ph↗

arXiv2020

Engineering AlGaAs-on-insulator towards quantum optical applications

Aluminum gallium arsenide has highly desirable properties for integrated parametric optical interactions: large material nonlinearities, maturely established nanoscopic structuring through epitaxial growth and lithography, and a large band gap for broadband low-loss operation. However, its full potential for record-strength nonlinear interactions is only released when the semiconductor is embedded within a dielectric cladding to produce highly confining waveguides. From simulations of such, we present second and third order pair generation that could improve upon state-of-the-art quantum optical sources and make novel regimes of strong parametric photon-photon nonlinearities accessible.

physics.optics↗

arXiv2020

Frequency-domain optical coherence tomography with undetected mid-infrared photons

Mid-infrared light scatters much less than shorter wavelengths, allowing greatly enhanced penetration depths for optical imaging techniques such as optical coherence tomography (OCT). However, both detection and broadband sources in the mid-IR are technologically challenging. Interfering entangled photons in a nonlinear interferometer enables sensing with undetected photons making mid-IR sources and detectors obsolete. Here we implement mid-infrared frequency-domain OCT based on ultra-broadband entangled photon pairs. We demonstrate 10 $μ$m axial and 20 $μ$m lateral resolution 2D and 3D imaging of strongly scattering ceramic and paint samples. Together with $10^6$ times less noise scaled for the same amount of probe light and also vastly reduced footprint and technical complexity this technique can outperform conventional approaches with classical mid-IR light.

physics.optics↗