arXiv subjects

Szilard Szoke

Publications and source records attributed to Szilard Szoke.

6 recordsLinked to original sources

arXiv2022

Single Photon Scattering Can Account for the Discrepancies Between Entangled Two-Photon Measurement Techniques

Entangled photon pairs are predicted to linearize and increase the efficiency of two-photon absorption, allowing continuous wave laser diodes to drive ultrafast time-resolved spectroscopy and nonlinear processes. Despite a range of theoretical studies and experimental measurements, inconsistencies persist about the value of the entanglement enhanced interaction cross section. A spectrometer is constructed that can temporally and spectrally characterize the entangled photon state before, during, and after any potential two-photon excitation event. For the molecule Rhodamine 6G, which has a virtual state pathway, any entangled two-photon interaction is found to be equal to or lower than classical, single photon scattering events. This result can account for the discrepancies between the wide variety of entangled two-photon absorption cross sections reported from different measurement techniques. The reported instrumentation can unambiguously separate classical and entangled effects and therefore is of importance for the growing field of nonlinear and multiphoton entangled spectroscopy.

quant-ph↗

arXiv2021

Designing High-Power, Octave Spanning Entangled Photon Sources for Quantum Spectroscopy

Entangled photon spectroscopy is a nascent field that has important implications for measurement and imaging across chemical, biology, and materials fields. Entangled photon spectroscopy potentially offers improved spatial and temporal-frequency resolutions, increased cross sections for multiphoton and nonlinear measurements, and new abilities in inducing or measuring quantum correlations. A critical step in enabling entangled photon spectroscopies is the creation of high-flux entangled sources that can use conventional detectors, as well as provide redundancy for the losses in realistic samples. Here, we report a periodically poled, chirped, lithium tantalate platform that generates entangled photon pairs with a $10^{-7}$ efficiency. For a near watt level diode laser, this results in a near $μ$W-level flux. The single photon per mode limit that is necessary to maintain non-classical photon behavior is still satisfied by distributing this power over up to an octave-spanning bandwidth. The spectral-temporal photon correlations are observed via a Michelson-type interferometer that measures the broadband Hong-Ou-Mandel two-photon interference. A coherence time of 245 fs for a 10 nm bandwidth in the collinear case and a 62 fs for a 125 nm bandwidth in the non-collinear case is measured using a CW pump laser, and, essentially, collecting the full photon cone. We outline in detail the numerical methods used for designing and tailoring the entangled photons source, such as changing center wavelength or bandwidth, with the ultimate aim of increasing the availability of high-flux UV-Vis entangled photon sources in the optical spectroscopy community.

physics.optics↗

arXiv2020

Entangled light-matter interactions and spectroscopy

Entangled photons exhibit non-classical light-matter interactions that create new opportunities in materials and molecular science. For example, in entangled two-photon absorption, the intensity-dependence scales linearly as if only one photon was present. The entangled two-photon absorption cross section approaches but does not match the one-photon absorption cross section. The entangled two photon cross section also does not follow classical two photon molecular design motifs. Questions such as these seed the rich but nascent field of entangled light-matter interactions. In this perspective, we use the experimental developments in entangled photon spectroscopy to outline the current status of the field. Now that the fundamental tools are outlined, it is time to start the exploration of how materials, molecules, and devices can control or utilize interactions with entangled photons.

physics.optics↗

arXiv2019

Layer-Resolved Ultrafast XUV Measurement of Hole Transport in a Ni-TiO2-Si Photoanode

Metal-oxide-semiconductor junctions are central to most electronic and optoelectronic devices. Here, the element-specificity of broadband extreme ultraviolet (XUV) ultrafast pulses is used to measure the charge transport and recombination kinetics in each layer of a Ni-TiO2-Si junction. After photoexcitation of silicon, holes are inferred to transport from Si to Ni ballistically in ~100 fs, resulting in spectral shifts in the Ni M2,3 XUV edge that are characteristic of holes and the absence of holes initially in TiO2. Meanwhile, the electrons are observed to remain on Si. After picoseconds, the transient hole population on Ni is observed to back-diffuse through the TiO2, shifting the Ti spectrum to higher oxidation state, followed by electron-hole recombination at the Si-TiO2 interface and in the Si bulk. Electrical properties, such as the hole diffusion constant in TiO2 and the initial hole mobility in Si, are fit from these transient spectra and match well with values reported previously.

cond-mat.mtrl-sci↗

arXiv2018

Telecom-band quantum optics with ytterbium atoms and silicon nanophotonics

Wavelengths in the telecommunication window (~1.25-1.65 microns) are ideal for quantum communication due to low transmission loss in fiber networks. To realize quantum networks operating at these wavelengths, long-lived quantum memories that couple to telecom-band photons with high efficiency need to be developed. We propose coupling neutral ytterbium atoms, which have a strong telecom-wavelength transition, to a silicon photonic crystal cavity. Specifically, we consider the 3P0-3D1 transition in neutral 171Yb to interface its long-lived nuclear spin in the metastable 3P0 'clock' state with a telecom-band photon at 1.4 microns. We show that Yb atoms can be trapped using a short wavelength (~470 nm) tweezer at a distance of 350 nm from the silicon photonic crystal cavity. At this distance, due to the slowly decaying evanescent cavity field at a longer wavelength, we obtain a single-photon Rabi frequency of g/(2pi)~100 MHz and a cooperativity of C~47 while maintaining a high photon collection efficiency into a single mode fiber. The combination of high system efficiency, telecom-band operation, and long coherence times makes this platform well suited for quantum optics on a silicon chip and long-distance quantum communication.

physics.atom-ph↗

arXiv2016

Maximum-Entropy Inference with a Programmable Annealer

Optimisation problems in science and engineering typically involve finding the ground state (i.e. the minimum energy configuration) of a cost function with respect to many variables. If the variables are corrupted by noise then this approach maximises the likelihood that the solution found is correct. An alternative approach is to make use of prior statistical information about the noise in conjunction with Bayes's theorem. The maximum entropy solution to the problem then takes the form of a Boltzmann distribution over the ground and excited states of the cost function. Here we use a programmable Josephson junction array for the information decoding problem which we simulate as a random Ising model in a field. We show experimentally that maximum entropy decoding at finite temperature can in certain cases give competitive and even slightly better bit-error-rates than the maximum likelihood approach at zero temperature, confirming that useful information can be extracted from the excited states of the annealing device. Furthermore we introduce a microscopic bit-by-bit analytical method which is agnostic to the specific application and use it to show that the annealing device samples from a highly Boltzmann-like distribution. Machines of this kind are therefore candidates for use in a wide variety of machine learning applications which exploit maximum entropy inference, including natural language processing and image recognition. We further show that the limiting factor for performance in our experiments is likely to be control errors rather than failure to reach equilibrium. Our work also provides a method for determining if a system is in equilibrium which can be easily generalized. We discuss possible applications of this method to spin glasses and probing the performance of the quantum annealing algorithm.

quant-ph↗