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Szymon Pustelny

Publications and source records attributed to Szymon Pustelny.

34 records · Page 2Linked to original sources

Quantum sensor networks as exotic field telescopes for multi-messenger astronomy

Multi-messenger astronomy, the coordinated observation of different classes of signals originating from the same astrophysical event, provides a wealth of information about astrophysical processes with far-reaching implications. So far, the focus of multi-messenger astronomy has been the search for conventional signals from known fundamental forces and standard model particles, like gravitational waves (GW). In addition to these known effects, quantum sensor networks could be used to search for astrophysical signals predicted by beyond-standard-model (BSM) theories. Exotic bosonic fields are ubiquitous features of BSM theories and appear while seeking to understand the nature of dark matter and dark energy and solve the hierarchy and strong CP problems. We consider the case where high-energy astrophysical events could produce intense bursts of exotic low-mass fields (ELFs). We propose to expand the toolbox of multi-messenger astronomy to include networks of precision quantum sensors that by design are shielded from or insensitive to conventional standard-model physics signals. We estimate ELF signal amplitudes, delays, rates, and distances of GW sources to which global networks of atomic magnetometers and atomic clocks could be sensitive. We find that, indeed, such precision quantum sensor networks can function as ELF telescopes to detect signals from sources generating ELF bursts of sufficient intensity. Thus ELFs, if they exist, could act as additional messengers for astrophysical events.

astro-ph.IM↗

Analysis method for detecting topological defect dark matter with a global magnetometer network

The Global Network of Optical Magnetometers for Exotic physics searches (GNOME) is a network of time-synchronized, geographically separated, optically pumped atomic magnetometers that is being used to search for correlated transient signals heralding exotic physics. GNOME is sensitive to exotic couplings of atomic spins to certain classes of dark matter candidates, such as axions. This work presents a data analysis procedure to search for axion dark matter in the form of topological defects: specifically, walls separating domains of discrete degenerate vacua in the axion field. An axion domain wall crossing the Earth creates a distinctive signal pattern in the network that can be distinguished from random noise. The reliability of the analysis procedure and the sensitivity of the GNOME to domain-wall crossings is studied using simulated data.

astro-ph.IM↗

Nonlinear magneto-optical rotation with parametric resonance

We report on investigations of nonlinear magneto-optical rotation (NMOR) in rubidium vapor subjected to a modulated magnetic field and continuous-wave (CW) laser-light illumination. By superimposing modulation and a static (DC) magnetic field, we demonstrate the appearance of resonances at both small and large (compared to the ground-state relaxation rate) values of the static field. Since in conventional NMOR, there is no rotation at high fields, this suggests an existence of a novel mechanism generating anisotropy in the considered case, which we identify as parametric resonance. The experiments are performed using light of small ellipticity and rotation signals are significantly enhanced by combining atom-induced polarization rotation with a passive rotation induced with a wave plate. All the observations are supported with theoretical simulations. The density-matrix formalism and angular-momentum probability surfaces are used to provide intuitive explanation of the observed signals.

physics.atom-ph↗

Transient dynamics of nonlinear magneto-optical rotation in the presence of transverse magnetic field

Nonlinear magneto-optical rotation is studied under non-equilibrium conditions. The polarization rotation of linearly polarized light traversing a rubidium vapor cell is observed versus the time-dependent (swept) longitudinal magnetic field in the presence of static transverse magnetic fields. Presence of the transverse fields modifies the character of the observed signals. In particular, for weaker transverse fields, field sweep leads two-harmonic oscillation of the polarization rotation while crossing zero. Unlike the steady-state, it was found that two-frequency oscillations observed in the transient signals, are independent of the transverse-field direction. For stronger transverse fields, the oscillations deteriorate eventually reaching a situation when no-oscillating dynamic signal, with distinct minimum close to zero field, is observed. Experimental results are supported with theoretical analysis based on the density-matrix formalism. The analysis confirms all the features of experimental results while providing an provide intuitive explanation of the observed behavior based on angular-momentum probability surfaces used for density-matrix visualization.

physics.atom-ph↗

Different sensitivities of two optical magnetometers realized in the same experimental arrangement

In this article, operation of optical magnetometers detecting static (DC) and oscillating (AC) magnetic fields is studied and comparison of the devices is performed. To facilitate the comparison, the analysis is carried out in the same experimental setup, exploiting nonlinear magneto-optical rotation. In such a system, a control over static-field magnitude or oscillating-field frequency provides detection of strength of the DC or AC fields. Polarization rotation is investigated for various light intensities and AC-field amplitudes, which allows to determine optimum sensitivity to both fields. With the results, we demonstrate that under optimal conditions the AC magnetometer is about ten times more sensitive than its DC counterpart, which originates from different response of the atoms to the fields. Bandwidth of the magnetometers is also analyzed, revealing its different dependence on the light power. Particularly, we demonstrate that bandwidth of the AC magnetometer can be significantly increased without strong deterioration of the magnetometer sensitivity. This behavior, combined with the ability to tune the resonance frequency of the AC magnetometer, provide means for ultra-sensitive measurements of the AC field in a broad but spectrally-limited range, where detrimental role of static-field instability is significantly reduced.

physics.atom-ph↗

Limitations of rotating-wave approximation in magnetic resonance: Characterization and elimination of the Bloch-Siegert shift in magneto-optics

We present investigations of radio-frequency resonances observed in a rubidium vapor. With measurements of a systematic shift of radio-frequency resonances, induced by an off-resonance component of an oscillating field (the Bloch-Siegert shift), we demonstrate limitations of the rotating-wave approximation. Experimental results are supported with numerical calculations, reproducing all features of the observed signals. Based on the studies, we develop experimental scheme free from the problem. By liberating the measurements from a systematic error (the resonance shift), the new approach will increase accuracy of spectroscopic measurements and magnetic-field detection.

physics.atom-ph↗

Instrumentation for nuclear magnetic resonance in zero and ultralow magnetic field

We review instrumentation for nuclear magnetic resonance (NMR) in zero and ultra-low magnetic field (ZULF, below 0.1 $μ$T) where detection is based on a low-cost, non-cryogenic, spin-exchange relaxation free (SERF) $^{87}$Rb atomic magnetometer. The typical sensitivity is 20-30 fT/Hz$^{1/2}$ for signal frequencies below 1 kHz and NMR linewidths range from Hz all the way down to tens of mHz. These features enable precision measurements of chemically informative nuclear spin-spin couplings as well as nuclear spin precession in ultra-low magnetic fields.

physics.ins-det↗

Constraints on exotic spin-dependent interactions between electrons from helium fine-structure spectroscopy

Agreement between theoretical calculations of atomic structure and spectroscopic measurements is used to constrain possible contribution of exotic spin-dependent interactions between electrons to the energy differences between states in helium-4. In particular, constraints on dipole-dipole interactions associated with the exchange of pseudoscalar bosons (such as axions or axion-like particles, ALPs) with masses $10^{-2}~{\rm eV} \lesssim m \lesssim 10^{4}~{\rm eV}$ are improved by a factor of $\sim 100$. The first atomic-scale constraints on several exotic velocity-dependent dipole-dipole interactions are established as well.

physics.atom-ph↗

Efficient polarization of high-angular-momentum systems

We propose methods of optical pumping that are applicable to open, high-angular-momentum transitions in atoms and molecules, for which conventional optical pumping would lead to significant population loss. Instead of applying circularly polarized cw light, as in conventional optical pumping, we propose to use techniques for coherent population transfer (e.g., adiabatic fast passage) to arrange the atoms so as to increase the entropy removed from the system with each spontaneous decay from the upper state. This minimizes the number of spontaneous-emission events required to produce a stretched state, thus reducing the population loss due to decay to other states. To produce a stretched state in a manifold with angular momentum J, conventional optical pumping requires about 2J spontaneous decays per atom, one of our proposed methods reduces this to about log_2(2J), while another of the methods reduces it to about one spontaneous decay, independent of J.

physics.atom-ph↗

Characterization of high-temperature performance of cesium vapor cells with anti-relaxation coating

Vapor cells with antirelaxation coating are widely used in modern atomic physics experiments due to the coating's ability to maintain the atoms' spin polarization during wall collisions. We characterize the performance of vapor cells with different coating materials by measuring longitudinal spin relaxation and vapor density at temperatures up to 95°C. We found that the spin-projection-noise-limited sensitivity for atomic magnetometers with such cells improves with temperature, which demonstrates the potential of antirelaxation coated cells in applications of future high-sensitivity magnetometers.

physics.atom-ph↗

Light shift averaging in paraffin-coated alkali vapor cells

Light shifts are an important source of noise and systematics in optically pumped magnetometers. We demonstrate that the long spin coherence time in paraffin-coated cells leads to spatial averaging of the light shifts over the entire cell volume. This renders the averaged light shift independent, under certain approximations, of the light-intensity distribution within the sensor cell. These results and the underlying mechanism can be extended to other spatially varying phenomena in anti-relaxation-coated cells with long coherence times.

physics.atom-ph↗

Multi-Channel Data Acquisition System with Absolute Time Synchronization

A low-cost, stand-alone Global-Positioning-System-time-synchronized data acquisition system is described. The constructed prototype allows recoding up to four analog signals with a 16-bit resolution in variable ranges and a maximum sampling rate of 1000 S/s. Additionally, two digital readouts of external sensors can be acquired. A complete data set is stored on a Secure Digital (SD) card or transmitted to a computer using Universal Serial Bus (USB). The estimated time accuracy of the data acquisition is better than 0.2 μs. The device is envisioned for the use in a global distributed sensor network (the Global Network of Optical Magnetometers for Exotic physics - GNOME), whose aim is to search for new particles and interactions.

physics.ins-det↗

Long-lived heteronuclear spin-singlet states

We report observation of long-lived spin-singlet states in a 13C-1H spin pair at zero magnetic field. In 13C-labeled formic acid, we observe spin-singlet lifetimes as long as 37 seconds, about a factor of three longer than the T1 lifetime of dipole polarization in the triplet state. We also observe that the lifetime of the singlet-triplet coherence, T2, is longer than T1. Moreover, we demonstrate that this singlet states formed by spins of a heteronucleus and a 1H nucleus, can exhibit longer lifetimes than the respective triplet states in systems consisting of more than two nuclear spins. Although long-lived homonuclear spin-singlet states have been extensively studied, this is the first experimental observation of analogous spin-singlets consisting of a heteronucleus and a proton.

physics.chem-ph↗

Modeling an optical magnetometer with electronic circuits - Analysis and optimization

Optical magnetometers are currently able to achieve magnetometric sensitivities below 1 fT/Hz^1/2. Although such sensitivities are typically obtained for ultra-low-field measurements, a group of optical magnetometers allows the detection of the fields in much broader dynamic range without a significant compromise in the sensitivity. A particular example of such a device is the magnetometer exploiting amplitude-modulated nonlinear magneto-optical rotation. It enables to measure a magnetic field via detection of a polarization state of light traversing a medium subjected to the field. In this paper, an electronic-circuit analogue of such the magnetometer is elaborated. Its operation is investigated with an electronic-circuit design software, which allows to study the "magnetometer" performance as a function of various parameters. The ability to automate operation of the magnetometer and automatically track "magnetic field" is demonstrated. The simulations are verified with experimental results obtained with the magnetometer operating in one of the investigated arrangements.

physics.atom-ph↗

Liquid-state nuclear spin comagnetometers

We discuss nuclear spin comagnetometers based on ultra-low-field nuclear magnetic resonance in mixtures of miscible solvents, each rich in a different nuclear spin. In one version thereof, Larmor precession of protons and ${\rm ^{19}F}$ nuclei in a mixture of thermally polarized pentane and hexafluorobenzene is monitored via a sensitive alkali-vapor magnetometer. We realize transverse relaxation times in excess of 20 s and suppression of magnetic field fluctuations by a factor of 3400. We estimate it should be possible to achieve single-shot sensitivity of about $5\times{\rm 10^{-9} Hz}$, or about $5\times 10^{-11} {\rm Hz}$ in $\approx 1$ day of integration. In a second version, spin precession of protons and ${\rm ^{129}Xe}$ nuclei in a mixture of pentane and hyperpolarized liquid xenon is monitored using superconducting quantum interference devices. Application to spin-gravity experiments, electric dipole moment experiments, and sensitive gyroscopes is discussed.

physics.atom-ph↗

Density effects in forward scattering of resonant light in rubidium vapor

Transmission of light through an atomic sample placed between crossed polarizers in a magnetic field is jointly determined by Faraday rotation and net absorption: transmission increases with rotation and decreases with absorption. Both rotation and absorption are proportional to the atomic density N0, hence, in a certain range of N0, the two effects may compete yielding a distinct density dependence of the transmitted light. We have studied such dependence in rubidium vapor for N0 = 7.5*10^9 to 7.5*10^11 at/cm^3 with resonant laser light. We present interpretation of the competition effect and discuss its possible application for atomic density determination.

physics.optics↗