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T. A. Assefa

Publications and source records attributed to T. A. Assefa.

4 recordsLinked to original sources

Nematicity of a Magnetic Helix

A system that possesses translational symmetry but breaks orientational symmetry is known as a nematic phase. While there are many examples of nematic phases in a wide range of contexts, such as in liquid crystals, complex oxides, and superconductors, of particular interest is the magnetic analogue, where the spin, charge, and orbital degrees of freedom of the electron are intertwined. The difficulty of spin nematics is the unambiguous realization and characterization of the phase. Here we present an entirely new type of magnetic nematic phase, which replaces the basis of individual spins with magnetic helices. The helical basis allows for the direct measurement of the order parameters with soft X-ray scattering and a thorough characterization of the nematic phase and its thermodynamic transitions. We discover two distinct nematic phases with unique spatio-temporal correlation signatures. Using coherent X-ray methods, we find that near the phase boundary between the two nematic phases, fluctuations coexist on the timescale of both seconds and sub-nanoseconds. Additionally, we have determined that the fluctuations occur simultaneously with a reorientation of the magnetic helices, indicating that there is spontaneous symmetry breaking and new degrees of freedom become available. Our results provide a novel framework for characterizing exotic phases and the phenomena presented can be mapped onto a broad class of physical systems.

cond-mat.mtrl-sci

Laser-Induced Transient Magnons in Sr3Ir2O7 Throughout the Brillouin Zone

Although ultrafast manipulation of magnetism holds great promise for new physical phenomena and applications, targeting specific states is held back by our limited understanding of how magnetic correlations evolve on ultrafast timescales. Using ultrafast resonant inelastic x-ray scattering we demonstrate that femtosecond laser pulses can excite transient magnons at large wavevectors in gapped antiferromagnets, and that they persist for several picoseconds which is opposite to what is observed in nearly gapless magnets. Our work suggests that materials with isotropic magnetic interactions are preferred to achieve rapid manipulation of magnetism.

cond-mat.str-el

Charge density waves in cuprate superconductors beyond the critical doping

The unconventional normal-state properties of the cuprates are often discussed in terms of emergent electronic order that onsets below a putative critical doping of xc = 0.19. Charge-density wave (CDW) correlations represent one such order; however, experimental evidence for such order generally spans a limited range of doping that falls short of the critical value xc, leading to questions regarding its essential relevance. Here, we use x-ray diffraction to demonstrate that CDW correlations in La2-xSrxCuO4 persist up to a doping of at least x = 0.21. The correlations show strong changes through the superconducting transition, but no obvious discontinuity through xc = 0.19, despite changes in Fermi surface topology and electronic transport at this doping. These results demonstrate the interaction between CDWs and superconductivity even in overdoped cuprates and prompt a reconsideration of the role of CDW correlations in the high-temperature cuprate phase diagram.

cond-mat.supr-con

Scaling Behaviour of Low-Temperature Orthorhombic Domains in Prototypical High-Temperature Superconductor La$_{1.875}$Ba$_{0.125}$CuO$_{4}$

Translational/rotational symmetry breaking and recovery in condensed matter systems are closely related to exotic physical properties such as superconductivity (SC), magnetism, spin density waves (SDW) and charge density waves (CDW). The interplay between different order parameters is intricate and often subject to intense debate, as in the case of CDW order and superconductivity. In La1:875Ba0:125CuO4 (LBCO), the locations of CDW domains are found to be pinned on the nanometer size scale. Coherent X-ray diffraction techniques open routes to directly visualize the domain structures associated with these symmetry changes. We have pushed Bragg Coherent Diffractive Imaging (BCDI) into the cryogenic regime where most phase transitions in quantum materials reside. Utilizing BCDI, we image the structural evolution of LBCO microcrystal samples during the high-temperature-tetragonal (HTT) to low-temperature-orthorhombic (LTO) phase transition. Our results show the formation of LTO domains close to the transition temperature and how the domain size varies with temperature. The LTO domain size is shown to decrease with temperature and to be inversely proportional to the magnitude of the orthorhombic distortion. The number of domains follows the secondary order parameter (or orthorhombic strain) measurement with a critical exponent that is consistent with the 3D universality class.

cond-mat.mes-hall