arXiv subjects

T. Adachi

Publications and source records attributed to T. Adachi.

83 records · Page 5Linked to original sources

arXiv2007

$^1$H-NMR Study of the Random Bond Effect in the Quantum Spin System (CH$_3$)$_2$CHNH$_3$Cu(Cl$_x$Br$_{1-x}$)$_3$

Spin-lattice relaxation rate $T_1^{-1}$ of $^1$H-NMR has been measured in (CH$_3$)$_2$CHNH$_3$Cu(Cl$_x$Br$_{1-x}$)$_3$ with $x=0.88$, which has been reported to be gapped system with singlet ground state from the previous macroscopic magnetization and specific heat measurements, in order to investigate the bond randomness effect microscopically in the gapped composite Haldane system (CH$_3$)$_2$CHNH$_3$CuCl$_3$. It was found that the spin-lattice relaxation rate $T_1^{-1}$ in the present system includes both fast and slow relaxation parts indicative of the gapless magnetic ground state and the gapped singlet ground state, respectively. We discuss the obtained results with the previous macroscopic magnetization and specific heat measurements together with the microscopic $μ$SR experiments.

cond-mat.str-el↗

arXiv2006

Magnetic-field effects on the charge-spin stripe order in La-214 high-Tc cuprates

Magnetic-field effects on the charge-spin stripe order in La-214 high-Tc cuprates have been investigated from measurements of the in-plane electrical-resistivity, Rho_ab_. In La_2-x_Ba_x_CuO_4_ with x=0.10 and La_2-x_Sr_x_CuO_4_ with x=0.115 where the incommensurate charge peaks are weak and unobservable in zero field in elastic neutron-scattering measurements, respectively, the normal-state value of Rho_ab_ at low temperatures markedly increases with increasing field up to 27 T. For La_2-x_Ba_x_CuO_4_ with x=0.11 and Zn-substituted La_2-x_Sr_x_Cu_1-y_Zn_y_O_4_ with x=0.115 and y=0.02 where the charge stripe order is fairly stabilized in zero field, on the other hand, the increase in Rho_ab_ with increasing field is negligibly small. In conclusion, when the charge-spin stripe order is not fully stable in zero field, magnetic field operates to stabilize the charge-spin stripe order. The value of Rho_ab_ increases with increasing field depending on the stability of the charge stripe order.

cond-mat.supr-con↗

arXiv2005

muSR study of the Cu-spin dynamics in the electron-doped high-Tc cuprate of Pr0.86LaCe0.14Cu1-y(Zn,Ni)yO4

Effects of the Zn- and Ni-substitution on the Cu-spin dynamics in the electron-doped Pr0.86LaCe0.14Cu1-y(Zn,Ni)yO4+a-d with y = 0, 0.01, 0.02, 0.05 and different values of the reduced oxygen content d have been studied using zero-field muon-spin-relaxation (muSR) measurements at temperatures down to 2 K. For the as-grown sample (d = 0, y = 0) and the sample with a very small d value (d < 0.01, y = 0), a muon-spin precession due to long-range antiferromagnetic order has been observed. On the other hand, no precession has been observed for moderately oxygen-reduced samples (0.01 < d < 0.09). It has been found that for all the samples of 0.01 < d < 0.09 the asymmetry A(t) (muSR time spectrum) in the long-time region increases with decreasing temperature at low temperatures, suggesting possible slowing-down of the Cu-spin fluctuations. On the other hand, no significant difference between Zn- and Ni-substitution effects on the slowing down of the Cu-spin fluctuations has been observed.

cond-mat.supr-con↗

arXiv2005

Superconducting Volume Fraction in Overdoped Regime of La_2-x_Sr_x_CuO_4_: Implication for Phase Separation from Magnetic-Susceptibility Measurement

We have grown a single crystal of La_2-x_Sr_x_CuO_4_ in which the Sr concentration, x, continuously changes from 0.24 to 0.29 in the overdoped regime and obtained many pieces of single crystals with different x values by slicing the single crystal. From detailed measurements of the magnetic susceptibility, chi, of each piece, it has been found that the absolute value of chi at the measured lowest temperature 2 K, |chi_2K_|, on field cooling rapidly decreases with increasing x as well as the superconducting (SC) transition temperature. As the value of |chi_2K_| is regarded as corresponding to the SC volume fraction in a sample, it has been concluded that a phase separation into SC and normal-state regions occurs in a sample of La_2-x_Sr_x_CuO_4_ in the overdoped regime.

cond-mat.supr-con↗

arXiv2005

Absence of the impurity-induced magnetic order in the electron-doped high-T_c_ cuprates Pr_0.86_LaCe_0.14_Cu_1-y_(Zn, Ni)_y_O_4_

Zero-field muon-spin-relaxation measurements have been carried out in order to investigate the Zn- and Ni-substitution effects on the Cu-spin dynamics in the electron-doped Pr_0.86_LaCe_0.14_Cu_1-y_(Zn, Ni)_y_O_4+\alpa-δ_ with y = 0, 0.01, 0.02, 0.05 and different values of the reduced oxygen content δ(δ\le 0.09). For the samples with y = 0 and very small δvalues of δ< 0.01, a muon-spin precession due to the formation of a long-range antiferromagnetic order has been observed at low temperatures below \~ 5 K. For the moderately oxygen-reduced samples of 0.01 \le δ\le 0.09, on the contrary, no muon-spin precession has been observed and the temperature dependence of the spectra is similar to one another regardless of the y value. That is, no impurity-induced slowing down of the Cu-spin fluctuations has been detected, which is very different from the results of the hole-doped high-T_c_ cuprates. The reason is discussed.

cond-mat.supr-con↗

arXiv2005

Magnetic-field effects on the in-plane electrical resistivity in the single-crystal La$_{2-x}$Ba$_x$CuO$_4$ and La$_{1.6-x}$Nd$_{0.4}$Sr$_x$CuO$_4$ around $x=1/8$: Relating to the field-induced stripe order

Temperature dependence of the in-plane electrical resistivity, $ρ_{\rm ab}$, in various magnetic fields has been measured in the single-crystal La$_{2-x}$Ba$_x$CuO$_4$ with $x=0.08$, 0.10, 0.11 and La$_{1.6-x}$Nd$_{0.4}$Sr$_x$CuO$_4$ with $x=0.12$. It has been found that the superconducting transition curve shows a so-called fan-shape broadening in magnetic fields for $x=0.08$, while it shifts toward the low-temperature side in parallel with increasing field for $x=0.11$ and 0.12 where the charge-spin stripe order is formed at low temperatures. As for $x=0.10$, the broadening is observed in low fields and it changes to the parallel shift in high fields above 9 T. Moreover, the normal-state value of $ρ_{\rm ab}$ at low temperatures markedly increases with increasing field up to 15 T. It is possible that these pronounced features of $x=0.10$ are understood in terms of the magnetic-field-induced stabilization of the stripe order suggested from the neutron-scattering measurements in the La-214 system. The $ρ_{\rm ab}$ in the normal state at low temperatures has been found to be proportional to ln(1/$T$) for $x=0.10$, 0.11 and 0.12. The ln(1/$T$) dependence of $ρ_{\rm ab}$ is robust even in the stripe-ordered state.

cond-mat.supr-con↗

arXiv2004

Field-induced magnetic order in La$sub {2-x}$Sr$sub x$CuO$sub 4$ (x = 0.10, 0.115, 0.13) studied by in-plane thermal conductivity measurements

We have measured the thermal conductivity in the $ab$-plane of La$_{2-x}$Sr$_x$CuO$_4$ ($x =$ 0.10, 0.115, 0.13) in magnetic fields up to 14 T parallel to the c-axis and also parallel to the $ab$-plane. By the application of magnetic fields parallel to the c-axis, the thermal conductivity has been found to be suppressed at low temperatures below the temperature $T_κ$ which is located above the superconducting transition temperature and is almost independent of the magnitude of the magnetic field. The suppression is marked in $x =$ 0.10 and 0.13, while it is small in $x =$ 0.115. Furthermore, no suppression is observed in the 1 % Zn-substituted La$_{2-x}$Sr$_x$Cu$_{0.99}$Zn$_{0.01}$O$_4$ with $x =$ 0.115. Taking into account the experimental results that the temperature dependence of the relative reduction of the thermal conductivity is quite similar to the temperature dependence of the intensity of the incommensurate magnetic Bragg peak corresponding to the static stripe order and that the Zn substitution tends to stabilize the static order, it is concluded that the suppression of the thermal conductivity in magnetic fields is attributed to the development of the static stripe order. The present results suggest that the field-induced magnetic order in La$_{2-x}$Sr$_x$CuO$_4$ originates from the pinning of the dynamical stripes of spins and holes by vortex cores.

cond-mat.supr-con↗

arXiv2004

Muon-spin-relaxation and magnetic-susceptibility studies of effects of the magnetic impurity Ni on the Cu-spin dynamics and superconductivity in La_2-x_Sr_x_Cu_1-y_Ni_y_O_4_ with x = 0.13

Effects of the magnetic impurity Ni on the Cu-spin dynamics and superconductivity have been studied in La_2-x_Sr_x_Cu_1-y_Ni_y_O_4_ with x = 0.13 changing y finely up to 0.10. Compared with the case of the nonmagnetic impurity Zn, it has been found from the muon-spin-relaxation measurements that a large amount of Ni is required to stabilize a magnetic order of Cu spins. However, the evolution toward the stabilization of the magnetic order with increasing impurity concentration is qualitatively similar to each other. The area of the non-superconducting and slowly fluctuating or static region of Cu spins around Ni has been found to be smaller than that around Zn, suggesting that the pinning of rather long-ranged dynamical spin correlation such as the so-called dynamical stripe by Ni is weaker than that by Zn. This may be the reason why Zn destroys the superconductivity in the hole-doped high-T_c_ cuprates more markedly than Ni.

cond-mat.supr-con↗

arXiv2004

Muon-spin-relaxation and magnetic-susceptibility studies of the effects of nonmagnetic impurities on the Cu-spin dynamics and superconductivity in La_2-x_Sr_x_Cu_1-y_Zn_y_O_4_ around x = 0.115

Zero-field muon-spin-relaxation (muSR) and magnetic-susceptibility measurements have been carried out in La_2-x_Sr_x_Cu_1-y_Zn_y_O_4_ with x = 0.10, 0.115 and 0.13 changing the Zn-concentration y finely up to 0.10, with the aim to clarify effects of the nonmagnetic impurity Zn on the Cu-spin dynamics and superconductivity. The muSR measurements have revealed that, in each x, a magnetic order of Cu spins is observed at y ~ 0.0075, while it disappears and Cu spins turn into a fast fluctuating state for y > 0.03. From the magnetic-susceptibility measurements, on the other hand, it has been found that the volume fraction of the superconducting state rapidly decreases through the slight doping of Zn and that its y dependence corresponds to the y dependence of the volume fraction of the fast fluctuating region of Cu spins estimated from the muSR results. Both the rapid decrease of the volume fraction of the superconducting state and the formation of the magnetic order through the slight doping of Zn can be interpreted in terms of the development of the so-called "Swiss cheese" model. That is, it is concluded that Cu spins in a non-superconducting region around Zn exhibit slowing-down of the fluctuations or form an incoherent or coherent static magnetic order. Moreover, the formation of a non-superconducting region around Zn is considered to be due to the pinning of the dynamical spin correlation or dynamical stripe correlations.

cond-mat.supr-con↗

arXiv2003

1/8 anomaly in the excess-oxygen-doped La_1.8_Nd_0.2_Cu_1-y_Zn_y_O_4+δ_

We have found the 1/8 anomaly, namely, the anomalous suppression of superconductivity at p (the hole concentration per Cu) = 1/8 in the excess-oxygen-doped La_1.8_Nd_0.2_Cu_1-y_Zn_y_O_4+δ_, where the excess oxygen is doped by the electrochemical technique and the phase separation of the excess oxygen is suppressed. The 1/8 anomaly has become marked by the 1 % substitution of Zn for Cu. The muon-spin-relaxation measurements have revealed that the magnetic correlation develops at low temperatures below about 50 K in both Zn-free and 1 % Zn-substituted samples with p = 1/8. Clear precession of muon spins suggesting the formation of a long-range magnetic order has been observed below 1 K in the 1 % Zn-substituted sample with p = 1/8. These results are consistent with the stripe-pinning model.

cond-mat.supr-con↗

arXiv2001

Crystal Growth, Transport Properties and Crystal Structure of the Single-Crystal La_{2-x}Ba_xCuO_4 with x=0.11

We have attempted the crystal growth by the traveling-solvent floating-zone (TSFZ) method of La_{2-x}Ba_xCuO_4 with x~1/8, where the superconductivity is strongly suppressed. Under flowing O_2-gas of a high pressure (4 bars), we have succeeded in growing single crystals of x=0.11 with 5 mm in diameter and 20 mm in length. It has been found that both in-plane and out-of-plane electrical resistivities of the single-crystal La_{2-x}Ba_xCuO_4 with x=0.11 exhibit a clear jump at ~53 K. The temperature corresponds to the structural phase transition temperature between the orthorhombic mid-temperature (OMT) and tetragonal low-temperature (TLT) phases, T_{d2}. It has also been found that both in-plane thermoelectric power and Hall coefficient drop rapidly at T_{d2} and decrease below T_{d2} with decreasing temperature. These results are quite similar to those observed in the single-crystal La_{1.6-x}Nd_{0.4}Sr_xCuO_4 with x~1/8, suggesting that the so-called static stripe order of holes and spins in the CuO_2 plane is formed below T_{d2} in La_{2-x}Ba_xCuO_4 with x~1/8 as well as in La_{1.6-x}Nd_{0.4}Sr_xCuO_4 with x~1/8.

cond-mat.supr-con↗