arXiv subjects

T. Asaba

Publications and source records attributed to T. Asaba.

28 records · Page 2Linked to original sources

arXiv2020

Evidence for a pressure-induced antiferromagnetic quantum critical point in intermediate valence UTe2

UTe$_2$ is a recently discovered unconventional superconductor that has attracted much interest due to its many intriguing properties - a large residual density-of-states in the superconducting state, re-entrant superconductivity in high magnetic fields, and potentially spin-triplet topological superconductivity. Our ac calorimetry, electrical resistivity, and x-ray absorption study of UTe$_2$ under applied pressure reveals key new insights on the superconducting and magnetic states surrounding pressure-induced quantum criticality at P$_{c1}$ = 1.3 GPa. First, our specific heat data at low pressures, combined with a phenomenological model, show that pressure alters the balance between two closely competing superconducting orders. Second, near 1.5 GPa we detect two bulk transitions that trigger changes in the resistivity which are consistent with antiferromagnetic order, rather than ferromagnetism. The presence of both bulk magnetism and superconductivity at pressures above P$_{c2}$ = 1.4 GPa results in a significant temperature difference between resistively and thermodynamically determined transitions into the superconducting state, which indicates a suppression of the superconducting volume fraction by magnetic order. Third, the emergence of magnetism is accompanied by an increase in valence towards a U$^{4+}$ (5f2) state, which indicates that UTe$_2$ exhibits intermediate valence at ambient pressure. Our results suggest that antiferromagnetic fluctuations may play a more significant role on the superconducting state of UTe$_2$ than previously thought.

cond-mat.str-el↗

arXiv2019

Quantum spin liquids by geometric lattice design

On a lattice composed of triangular plaquettes where antiferromagnetic exchange interactions between localized spins cannot be simultaneously satisfied, the system becomes geometrically frustrated with magnetically disordered phases remarkably different from a simple paramagnet. Spin liquid belongs to one of these exotic states, in which a macroscopic degeneracy of the ground state gives rise to the rich spectrum of collective phenomena. Here, we report on the discovery of a new magnetic state in the heterostructures derived from a single unit cell (111)-oriented spinel CoCr2O4 sandwiched between nonmagnetic Al2O3 spacers. The artificial quasi-two-dimensional material composed of three triangle and one kagome atomic planes shows a degree of magnetic frustration which is almost two orders of magnitude enlarged compared to the bulk crystals. Combined resonant X-ray absorption and torque magnetometry measurements confirm that the designer system exhibits no sign of spin ordering down to 30 mK, implying a possible realization of a quantum spin liquid state in the two dimensional limit.

cond-mat.str-el↗

arXiv2019

Unconventional thermal metallic state of charge-neutral fermions in an insulator

Quantum oscillations (QOs) in transport and thermodynamic parameters at high magnetic fields are an unambiguous signature of the Fermi surface, the defining characteristic of a metal. Therefore, recent observations of QOs in insulating SmB$_6$ and YbB$_{12}$, in particular the QOs of the resistivity $ρ_{xx}$ in YbB$_{12}$, have been a big surprise, pointing to the formation of a novel state of quantum matter. Despite the large charge gap inferred from the insulating behaviour of $ρ_{xx}$, these compounds seemingly host a Fermi surface at high magnetic fields. However, the nature of the ground state in zero field has been little explored. Here we report the use of low-temperature heat-transport measurements to discover gapless, itinerant, charge-neutral excitations in the ground state of YbB$_{12}$. At zero field, despite $ρ_{xx}$ being far larger than that of conventional metals, a sizable linear temperature dependent term in the thermal conductivity is clearly resolved in the zero-temperature limit ($κ_{xx}/T(T\rightarrow0)=κ_{xx}^0/T\neq0$). Such a residual $κ_{xx}^0/T$ term at zero field, which is absent in SmB$_6$, leads to a spectacular violation of the Wiedemann-Franz law: the Lorenz ratio $L=κ_{xx}ρ_{xx}/T$ is $10^{4}$-$10^{5}$ times larger than that expected in conventional metals. These data indicate that YbB$_{12}$ is a charge insulator but a thermal metal, suggesting the presence of itinerant neutral fermions. Remarkably, more insulating crystals with larger activation energies exhibit a larger amplitude of the resistive QOs as well as a larger $κ_{xx}^0/T$, in stark contrast to conventional metals. Moreover, we find that these fermions couple to magnetic field, despite their charge neutrality. Our findings expose novel gapless and highly itinerant, charge-neutral quasiparticles in this unconventional quantum state.

cond-mat.str-el↗

arXiv2019

Quantum Oscillations of Electrical Resistivity in an Insulator

In metals, orbital motions of conduction electrons on the Fermi surface are quantized in magnetic fields, which is manifested by quantum oscillations in electrical resistivity. This Landau quantization is generally absent in insulators. Here we report a notable exception in an insulator, ytterbium dodecaboride (YbB12). Despite much larger than that of metals, the resistivity of YbB12 exhibits profound quantum oscillations. This unconventional oscillation is shown to arise from the insulating bulk, yet the temperature dependence of their amplitude follows the conventional Fermi liquid theory of metals. The large effective masses indicate the presence of Fermi surface consisting of strongly correlated electrons. Our result reveals a mysterious bipartite ground state of YbB12: it is both a charge insulator and a strongly correlated metal.

cond-mat.str-el↗

arXiv2019

Ferromagnetism and conductivity in atomically thin SrRuO3

Atomically thin ferromagnetic and conducting electron systems are highly desired for spintronics, because they can be controlled with both magnetic and electric fields. We present (SrRuO3)1-(SrTiO3)5 superlattices and single-unit-cell-thick SrRuO3 samples that are capped with SrTiO3. We achieve samples of exceptional quality. In these samples, the electron systems comprise only a single RuO2 plane. We observe conductivity down to 50 mK, a ferromagnetic state with a Curie temperature of 25 K, and signals of magnetism persisting up to approximately 100 K.

cond-mat.mtrl-sci↗

arXiv2017

Bulk Rotational Symmetry Breaking in Kondo Insulator SmB6

Kondo insulator samarium hexaboride (SmB6) has been intensely studied in recent years as a potential candidate of a strongly correlated topological insulator. One of the most exciting phenomena observed in SmB6 is the clear quantum oscillations appearing in magnetic torque at a low temperature despite the insulating behavior in resistance. These quantum oscillations show multiple frequencies and varied effective masses. The origin of quantum oscillation is, however, still under debate with evidence of both two-dimensional Fermi surfaces and three-dimensional Fermi surfaces. Here, we carry out angle-resolved torque magnetometry measurements in a magnetic field up to 45 T and a temperature range down to 40 mK. With the magnetic field rotated in the (010) plane, the quantum oscillation frequency of the strongest oscillation branch shows a four-fold rotational symmetry. However, in the angular dependence of the amplitude of the same branch, this four-fold symmetry is broken and, instead, a twofold symmetry shows up, which is consistent with the prediction of a two-dimensional Lifshitz-Kosevich model. No deviation of Lifshitz-Kosevich behavior is observed down to 40 mK. Our results suggest the existence of multiple light-mass surface states in SmB6, with their mobility significantly depending on the surface disorder level.

cond-mat.str-el↗

arXiv2016

Consistency of Photoemission and Quantum Oscillations for Surface States of SmB6

The mixed valent compound SmB6 is of high current interest as the first candidate example of topologically protected surface states in a strongly correlated insulator and also as a possible host for an exotic bulk many-body state that would manifest properties of both an insulator and a metal. Two different de Haas van Alphen (dHvA) experiments have each supported one of these possibilities, while angle resolved photoemission spectroscopy (ARPES) for the (001) surface has supported the first, but without quantitative agreement to the dHvA results. We present new ARPES data for the (110) surface and a new analysis of all published dHvA data and thereby bring ARPES and dHvA into substantial consistency around the basic narrative of two dimensional surface states.

cond-mat.str-el↗

arXiv2014

Quantum Oscillations in Cu$_x$Bi$_2$Se$_3$ in High Magnetic Fields

Cu$_x$Bi$_2$Se$_3$ has drawn much attention as the leading candidate to be the first topological superconductor and the realization of coveted Majorana particles in a condensed matter system. However, there has been increasing controversy about the nature of its superconducting phase. This study sheds light on present ambiguity in the normal state electronic state, by providing a complete look at the quantum oscillations in magnetization in Cu$_x$Bi$_2$Se$_3$ at intense high fields up to 31T. Our study focuses on the angular dependence of the quantum oscillation pattern in a low carrier concentration. As magnetic field tilts from along the crystalline c-axis to ab-plane, the change of the oscillation period follows the prediction of the ellipsoidal Fermi surface. As the doping level changes, the 3D Fermi surface is found to transform into quasi-cylindrical at high carrier density. Such a transition is potentially a Lifshitz transition of the electronic state in Cu$_x$Bi$_2$Se$_3$.

cond-mat.str-el↗

arXiv2013

Quantum oscillations in Kondo Insulator SmB$_6$

In Kondo insulator samarium hexaboride SmB$_6$, strong correlation and band hybridization lead to an insulating gap and a diverging resistance at low temperature. The resistance divergence ends at about 5 Kelvin, a behavior recently demonstrated to arise from the surface conductance. However, questions remain whether and where a topological surface state exists. Quantum oscillations have not been observed to map the Fermi surface. We solve the problem by resolving the Landau Level quantization and Fermi surface topology using torque magnetometry. The observed Fermi surface suggests a two dimensional surface state on the (101) plane. Furthermore, the tracking of the Landau Levels in the infinite magnetic field limit points to -1/2, which indicates a 2D Dirac electronic state.

cond-mat.str-el↗

arXiv2010

Photon Frequency Bears More At Less

Construction of an optical quantum computer (OQC) is finished by implementing all necessary ingredients with light (photon). There is, however, one more hurdle to clear. It is scalability, which is easily lost when accommodating many qubits by densely nesting quantum circuits. Any of the reported OQC schemes is not neces-sarily best placed in this regard. Here we demonstrate the power of "frequency" de-gree of freedom of light, which outperforms others with its potentially infinite basis states: as multiple qubits share the same "one-photon" superposition state all along, a realistic OQC design in frequency basis adopts only one port each for input and out-put. As such quantum logic gates are configurable in a cascade of compact in-line modules, which ensures scalable computing. Finally, our implementation of Deutsch-Jozsa's algorithm using standard laboratory laser demonstrates that fre-quency-basis OQC is ideally suited for such tasks even without help of nonclassicality of light.

quant-ph↗