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T. Asano

Publications and source records attributed to T. Asano.

13 recordsLinked to original sources
arXiv2026

Quantum spin liquid on a 3D bipartite lattice of spin trimers stabilized by enhanced effective anisotropy

Quantum spin liquids (QSLs) represent highly entangled states of matter in which frustration-induced quantum fluctuations suppress any symmetry-breaking phase transition down to absolute zero, giving rise to fractionalized excitations and emergent gauge fields. Theoretically, bond anisotropy can stabilize QSLs even on bipartite lattices, as exemplified by the Kitaev honeycomb model; however, no material has so far been established to realize such a state as its true ground state. Here we identify the three-dimensional spin-trimer magnet KBa$_3$Ca$_4$Cu$_3$V$_7$O$_{28}$ as a promising candidate for a bipartite quantum spin liquid persisting to the lowest temperatures. Strongly coupled Cu$^{2+}$ trimers form effective pseudospin-1/2 degrees of freedom upon cooling, which in turn constitute a three-dimensional bipartite network. Bulk thermodynamic measurements, neutron scattering, $\mu$SR, and NMR detect no spin freezing or symmetry-breaking phase transition down to 20 mK, but instead reveal a gapless dynamical ground state with algebraic spin autocorrelations. Complementary Monte Carlo and exact-diagonalization calculations show that this state is stabilized by a strong enhancement of effective anisotropy: a weak microscopic Cu-Cu exchange anisotropy of approximately 15 percent is generically amplified at the trimer level, producing effective pseudospin-pseudospin interaction anisotropies of 60 to 100 percent. Our results establish trimer-based networks as a promising platform for realizing anisotropy-stabilized quantum entangled states, even in three-dimensional bipartite systems with only weak microscopic anisotropy.

cond-mat.str-el↗
arXiv2026

The exponential growth of infinitesimal perturbations in the long-term evolution of simulated galaxies

Self-gravitating systems of $N$ particles are chaotic. We study how chaotic the Galaxy is, and what the consequences are. We therefore simulated the dynamical evolution of a galaxy-scale distribution of point masses in order to measure the degree of chaos in such a system. These calculations were performed using the softened gravitational $N$-body tree-code Bonsai, with up to 40 million equal-mass particles. Smaller simulations were performed to establish the scaling of the Lyapunov time $t_L$ with $N$. We established the relations between the degree of chaos, the number of particles, and the softening length in the gravitational force calculation of large-scale $N$-body simulations. The moment in which the bar forms appears to be insensitive to infinitesimal perturbations to the initial realisation. In contrast, the bar strength and its further evolution sensitively depend on these perturbations. Interestingly enough, the maximum in the run-to-run variation in the bar strength is at about the maximum bar strength, and it drops until the bar buckles. The galaxies we simulated are highly chaotic, but the softening in the simulations suppresses chaos. Still, our models show considerable variations in the macroscopic behaviour caused by infinitesimal perturbations to the initial conditions. Real galaxies, however, are expected to be orders of magnitude more chaotic than our simulations, and we are unable to quantify the consequences of this. Smooth galactic potentials for studying individual stellar orbits should be handled with caution on timescales longer than the Lyapunov time. When we extrapolate our results to the number of stars in the Galaxy without planets and other minor bodies, we conclude that Milky Way-size galaxies are chaotic on a timescale of less than a million years.

astro-ph.GA↗
arXiv2025

Delayed phase mixing in the self-gravitating Galactic disc

The Gaia phase spiral is considered to work as a dynamical clock for dating past perturbations, but some of the previous studies neglected the disc's self-gravity, potentially biasing estimates of the phase spiral's excitation time. We revisit the impact of self-gravitating effects on the evolution of vertical phase spirals and quantify the bias introduced in estimating their excitation time when such effects are ignored. We analysed a high-resolution, self-consistent $N$-body simulation of the MW-Sagittarius dwarf galaxy (Sgr) system, alongside four test particle simulations in potentials constructed from the $N$-body snapshots. In each case, we estimated the winding time of phase spirals by measuring the slope of the density contrast in the vertical angle-frequency space. In the test particle models, the phase spiral begins winding immediately after Sgr's pericentric passage, and the winding time closely tracks the true elapsed time since the Sgr impact. Adding the DM wake yields only a modest (< 100 Myr) reduction of the winding time relative to Sgr alone. By contrast, the self-consistent $N$-body simulation exhibits an initial, coherent vertical oscillation lasting $\gtrsim$ 300 Myr before a clear spiral forms, leading to systematic underestimation of excitation times. An analytical shearing-box model with self-gravity, developed by Widrow (2023), qualitatively reproduces this delay, supporting its origin in the disc's self-gravitating response. Assuming that self-gravity affects phase mixing in the MW to the same degree as the $N$-body model, the lag induced by self-gravity is estimated to be $\sim$ 0.3 Gyr in the solar neighbourhood. Accounting for this delay revises the inferred age of the MW's observed phase spiral to $\sim$0.6-1.2 Gyr, in better agreement with the Sgr's pericentric passage. (shortened for arXiv)

astro-ph.GA↗
arXiv2023

Dynamics of orbital degrees of freedom probed via isotope $^{121,123}$ Sb nuclear quadrupole moments in Sb-substituted iron-pnictide superconductors

Isotope $^{121,123}$Sb nuclei with large electric quadrupole moments are applied to investigate the dynamics of orbital degrees of freedom in Sb-substituted iron(Fe)-based compounds. In the parent compound LaFe(As$_{0.6}$Sb$_{0.4}$)O, the nuclear spin relaxation rate $^{121,123}(T_{1}^{-1})$ at $^{121,123}$Sb sites was enhanced at structural transition temperature ($T_{s}\sim$ 135 K), which is higher than N\'eel temperature ($T_{\rm N}\sim$125 K). The isotope ratio $^{123}(T_{1}^{-1})/^{121}(T_{1}^{-1})$ indicates that the electric quadrupole relaxation due to the dynamical electric field gradient at Sb site increases significantly toward $T_{s}$. It is attributed to the critically enhanced nematic fluctuations of stripe-type arrangement of Fe-$3d_{xz}$ (or $3d_{yz}$) orbitals. In the lightly electron-doped superconducting (SC) compound LaFe(As$_{0.7}$Sb$_{0.3}$)(O$_{0.9}$F$_{0.1}$), the nematic fluctuations are largely suppressed in comparison with the case of the parent compound, however, it remains a small enhancement below 80 K down to the $T_c$($\sim$ 20 K). The results indicate that the fluctuations from both the spin and orbital degrees of freedom on the $3d_{xz}$(or $3d_{yz}$) orbitals can be seen in lightly electron-doped SC state of LaFeAsO-based compounds. We emphasize that isotope $^{121,123}$Sb quadrupole moments are sensitive local probe to identify the dynamics of orbital degrees of freedom in Fe-pnictides, which provides with a new opportunity to discuss the microscopic correlation between the superconductivity and both nematic and spin fluctuations simultaneously even in the polycrystalline samples.

cond-mat.supr-con↗
arXiv2016

Localized and mixed valence state of Ce $4f$ in superconducting and ferromagnetic CeO$_{1-x}$F$_{x}$BiS$_{2}$ revealed by x-ray absorption and photoemission spectroscopy

We have performed Ce $L_3$-edge x-ray absorption spectroscopy (XAS) and Ce $4d$-$4f$ resonant photoemission spectroscopy (PES) on single crystals of CeO$_{1-x}$F$_x$BiS$_2$ for $x=0.0$ and 0.5 in order to investigate the Ce $4f$ electronic states. In the Ce $L_3$-edge XAS, mixed valence of Ce was found in the $x=0.0$ sample and the F-doping suppresses it, which is consistent with the results on polycrystalline samples. As for the resonant PES, we found that the Ce $4f$ electrons in both $x=0.0$ and $0.5$ systems respectively form a flat band at 1.0 eV and 1.4 eV below the Fermi level and there is no contribution to the Fermi surfaces. Interestingly, Ce valence in CeOBiS$_2$ deviates from Ce$^{3+}$ even though Ce $4f$ electrons are localized, indicating the Ce valence is not in a typical valence fluctuation regime. We assume that localized Ce $4f$ in CeOBiS$_2$ is mixed with the unoccupied Bi $6p_z$, which is consistent with the previous local structural study. Based on the analysis of the Ce $L_3$-edge XAS spectra using Anderson's impurity model calculation, we found that the transfer integral becomes smaller increasing the number of Ce $4f$ electrons upon the F substitution for O.

cond-mat.supr-con↗
arXiv2015

Fermi surfaces and orbital polarization in superconducting CeO$_{0.5}$F$_{0.5}$BiS$_{2}$ revealed by angle-resolved photoemission spectroscopy

We have investigated the electronic structure of BiS$_2$-based CeO$_{0.5}$F$_{0.5}$BiS$_2$ superconductor using polarization-dependent angle-resolved photoemission spectroscopy (ARPES), and succeeded in elucidating the orbital characters on the Fermi surfaces. In the rectangular Fermi pockets around X point, the straight portion parallel to the $k_y$ direction is dominated by Bi $6p_x$ character. The orbital polarization indicates the underlying quasi-one-dimensional electronic structure of the BiS$_2$ system. Moreover, distortions on tetragonally aligned Bi could give rise to the band Jahn-Teller effect.

cond-mat.supr-con↗
arXiv2014

Two-photon interference and coherent control of single InAs quantum dot emissions in an Ag-embedded structure

We have recently reported the successful fabrication of bright single-photon sources based on Ag-embedded nanocone structures that incorporate InAs quantum dots. The source had a photon collection efficiency as high as 24.6%. Here we show the results of various types of photonic characterizations of the Ag-embedded nanocone structures that confirm their versatility as regards a broad range of quantum optical applications. We measure the first-order autocorrelation function to evaluate the coherence time of emitted photons, and the second-order correlation function, which reveals the strong suppression of multiple photon generation. The high indistinguishability of emitted photons is shown by the Hong-Ou-Mandel-type two-photon interference. With quasi-resonant excitation, coherent population flopping is demonstrated through Rabi oscillations. Extremely high single-photon purity with a $g^{(2)}$(0) value of 0.008 is achieved with $π$-pulse quasi-resonant excitation.

cond-mat.mes-hall↗
arXiv2011

Co-existing Singlet and Ordered S=1/2 Moments in the Ground State of the Triclinic Quantum Magnet CuMoO4

CuMoO4 is a triclinic quantum magnet based on S = 1/2 moments at the Cu2+ site. It has recently attracted interest due to the remarkable changes in its chromic and volumetric properties at high temperatures, and in its magnetic properties at low temperatures. This material exhibits a first order structural phase transition at T_C ~ 190 K as well as a magnetic phase transition at T_N ~ 1.75 K. We report low temperature heat capacity measurements as well as extensive elastic and inelastic neutron scattering measurements on powder samples taken above and below T_N. We observe neutron diffraction consistent with a simple (1/2, 0, 0) antiferromagnetic structure indicating a doubling of the a-axis periodicity below T_N. In addition, inelastic neutron scattering above a spin gap of ~ 2.3 meV is consistent with triplet excitations out of paired S = 1/2 moments which form singlet dimers. Low lying spin wave excitations are also observed and these originate from ordered S = 1/2 moments below T_N. Taken together these measurements show the ground state of CuMoO4 to display both non-magnetic singlets, and ferromagnetically-coupled spins coexisting within an antiferromagnetic structure below T_N ~ 1.75 K.

cond-mat.str-el↗
arXiv2004

Ordering and Excitations in the Field-Induced Magnetic Phase of Cs_3Cr_2Br_9

Field-induced magnetic order has been investigated in detail in the interacting spin 3/2 dimer system Cs_3Cr_2Br_9. Elastic and inelastic neutron scattering measurements were performed up to H = 6 T, well above the critical field H_c1 = 1.5 T. The ordering displays incommensurabilities and a large hysteresis before a commensurate structure is reached. This structure is fully determined. Surprisingly, the lowest excitation branch never closes. Above H_c1, the gap increases slowly with field. An analysis in terms of projected pseudo-spin is given.

cond-mat.str-el↗
arXiv2003

Diffusive energy transport in the S=1 Haldane chain compound AgVP2S6

We present the results of measurements of the thermal conductivity $κ$ of the spin S=1 chain compound AgVP_2S_6 in the temperature range between 2 and 300 K and with the heat flow directed either along or perpendicular to the chain direction. The analysis of the anisotropy of the heat transport allowed for the identification of a small but non-negligible magnon contribution $κ_m$ along the chains, superimposed on the dominant phonon contribution $κ_ph$. At temperatures above about 100 K the energy diffusion constant D_E(T), calculated from the $κ_m(T)$ data, exhibits similar features as the spin diffusion constant D_S(T), previously measured by NMR. In this regime, the behaviour of both transport parameters is consistent with a diffusion process that is caused by interactions inherent to one-dimensional S=1 spin systems.

cond-mat.str-el↗
arXiv2000

Magnetic dilution in the geometrically frustrated SrCr$_{9p}$Ga$_{12-9p}$O$_{19}$ and the role of local dynamics: a $μ$SR study

We investigate the spin dynamics of SrCr$_{9p}$Ga$_{12-9p}$O$_{19}$ for p below and above the percolation threshold p_c using muon spin relaxation. Our major findings are: (I) At T->0 the relaxation rate is T independent and proportional to p^3, (II) the slowing down of spin fluctuation is activated with an energy U which is also a linear function of p^3 and lim_{p-> 0}U = 8 K; this energy scale could stem only from a single ion anisotropy, and (III) the p dependence of the dynamical properties is identical below and above p_c, indicating that they are controlled by local excitation.

cond-mat.str-el↗
arXiv1999

ESR investigation on the Breather mode and the Spinon-Breather dynamical crossover in Cu Benzoate

A new elementary-excitation, the so called "breather excitation", is observed directly by millimeter-submillimeter wave electron spin resonance (ESR) in the Heisenberg quantum spin-chain Cu benzoate, in which a field-induced gap is found recently by specific heat and neutron scattering measurements. Distinct anomalies were found in line width and in resonance field around the "dynamical crossover" regime between the gap-less spinon-regime and the gapped breather-regime. When the temperature becomes sufficiently lower than the energy gap, a new ESR-line with very narrow line-width is found, which is the manifestation of the breather excitation. The non-linear field dependence of the resonance field agrees well with the theoretical formula of the first breather-excitation proposed by Oshikawa and Affleck. The present work establishes experimentally for the first time that a sine-Gordon model is applicable to explain spin dynamics in a S=1/2 Heisenberg spin chain subjected to staggered field even in high fields.

cond-mat.str-el↗