arXiv subjects

T. Chaneliere

Publications and source records attributed to T. Chaneliere.

15 recordsLinked to original sources

arXiv2026

Precision hyperfine spectroscopy of an individual nuclear-spin-9/2

Single-spin magnetic resonance spectroscopy promises to yield structural and chemical information at the level of individual atoms or molecules, in a non-invasive way. Here, we use an Er3+ paramagnetic center in a CaWO4 crystal, detected by microwave photon counting at 10 mK, as a nanoscale magnetic sensor to measure the NMR spectrum of a proximal individual nuclear-spin-9/2 93Nb impurity with Hertz spectral resolution. From these measurements, we determine the 93Nb insertion site, its position relative to the Er3+ , and its complete quadrupolar tensor. We moreover harness the high spectral resolution of our measurements to establish the presence of two previously unobserved terms in the spin Hamiltonian. The first describes a coupling between the Er3+ spin and the 93Nb nuclear quadrupole; it possibly originates from a spin-dependent electrostatic interaction between the two systems. The second is a nuclear hexadecapolar term, and may be caused by the coupling of the electric field third derivative to the 93Nb nuclear hexadecapolar moment.

quant-ph↗

arXiv2025

Spin dependent fluorescence mediated by anti-symmetric exchange in triplet exciton pairs

Singlet fission and triplet-triplet annihilation (TTA) are spin-dependent phenomena critical to optoelectronics. The dynamics of spin populations during geminate triplet pair separation are crucial for controlling fission and TTA rates. We show that the Dzyaloshinskii-Moriya interaction (DMI) induces level crossings between spin manifolds, affecting spin populations and TTA rates in crystalline fission semiconductors. By investigating spin-dependent fluorescence in a triplet exciton pair with the magnetic field aligned along the fine structure tensor, we isolate the effect of DMI, as the triplet wavefunctions remain unaffected by the field. Our results reveal that DMI introduces additional TTA pathways that are forbidden by spin conservation, explaining the observed evolution of optically detected magnetic resonance signals with varying magnetic field. This study highlights the significant impact of DMI on the optical properties of triplet excitons, advancing our understanding of spin dynamics in these systems.

physics.chem-ph↗

arXiv2024

All-microwave spectroscopy and polarization of individual nuclear spins in a solid

We report magnetic resonance spectroscopy measurements of individual nuclear spins in a crystal coupled to a neighbouring paramagnetic center, detected using microwave fluorescence at millikelvin temperatures. We observe real-time quantum jumps of the nuclear spin state, a proof of their individual nature. By driving the forbidden transitions of the coupled electron-nuclear spin system, we also achieve single-spin solid-effect dynamical nuclear polarization. Relying exclusively on microwave driving and microwave photon counting, the methods reported here are in principle applicable to a large number of electron-nuclear spin systems, in a wide variety of samples.

quant-ph↗

arXiv2010

Adiabatic refocusing of nuclear spins in Tm3+:YAG

We show that the optical absorbance detection of nuclear spin echo gives direct access to the spin concentration, unlike most coherent signal detection techniques where the signal intensity/amplitude is difficult to connect experimentally with the spin concentration. This way we measure the spin refocusing efficiency in a crystal of Tm$^{3+}$:YAG. Given the large inhomogeneous broadening of the spin transition in this material, rephasing the spins with the usual hard pulse procedure would require excessively high radiofrequency power. Instead we resort to an adiabatic pulse sequence that perfectly returns the spins to their initial common orientation, at low power cost.

quant-ph↗

arXiv2009

Spectral hole burning for stopping light

We propose a novel protocol for storage and retrieval of photon wave packets in a $Λ$-type atomic medium. This protocol derives from spectral hole burning and takes advantages of the specific properties of solid state systems at low temperature, such as rare earth ion doped crystals. The signal pulse is tuned to the center of the hole that has been burnt previously within the inhomogeneously broadened absorption band. The group velocity is strongly reduced, being proportional to the hole width. This way the optically carried information and energy is carried over to the off-resonance optical dipoles. Storage and retrieval are performed by conversion to and from ground state Raman coherence by using brief $π$-pulses. The protocol exhibits some resemblance with the well known electromagnetically induced transparency process. It also presents distinctive features such as the absence of coupling beam. In this paper we detail the various steps of the protocol, summarize the critical parameters and theoretically examine the recovery efficiency.

quant-ph↗

arXiv2006

Dual species matter qubit entangled with light

We propose and demonstrate an atomic qubit based on a cold $^{85}$Rb-$^{87}$Rb isotopic mixture, entangled with a frequency-encoded optical qubit. The interface of an atomic qubit with a single spatial light mode, and the ability to independently address the two atomic qubit states, should provide the basic element of an interferometrically robust quantum network.

quant-ph↗

arXiv2006

Quantum interference of electromagnetic fields from remote quantum memories

We observe quantum, Hong-Ou-Mandel, interference of fields produced by two remote atomic memories. High-visibility interference is obtained by utilizing the finite atomic memory time in four-photon delayed coincidence measurements. Interference of fields from remote atomic memories is a crucial element in protocols for scalable generation of multi-node remote qubit entanglement.

quant-ph↗

arXiv2006

Deterministic single photons via conditional quantum evolution

A source of deterministic single photons is proposed and demonstrated by the application of a measurement-based feedback protocol to a heralded single photon source consisting of an ensemble of cold rubidium atoms. Our source is stationary and produces a photoelectric detection record with sub-Poissonian statistics.

quant-ph↗

arXiv2006

Quantum telecommunication based on atomic cascade transitions

A quantum repeater at telecommunications wavelengths with long-lived atomic memory is proposed, and its critical elements are experimentally demonstrated using a cold atomic ensemble. Via atomic cascade emission, an entangled pair of 1530 nm and 780 nm photons is generated. The former is ideal for long-distance quantum communication, and the latter is naturally suited for mapping to a long-lived atomic memory. Together with our previous demonstration of photonic-to-atomic qubit conversion, both of the essential elements for the proposed telecommunications quantum repeater have now been realized.

quant-ph↗

arXiv2005

Storage and retrieval of single photons transmitted between remote quantum memories

An elementary quantum network operation involves storing a qubit state in an atomic quantum memory node, and then retrieving and transporting the information through a single photon excitation to a remote quantum memory node for further storage or analysis. Implementations of quantum network operations are thus conditioned on the ability to realize such matter-to-light and/or light-to-matter quantum state mappings. Here, we report generation, transmission, storage and retrieval of single quanta using two remote atomic ensembles. A single photon is generated from a cold atomic ensemble at Site A via the protocol of Duan, Lukin, Cirac, and Zoller (DLCZ) [Nature v.414, 413 (2001)] and is directed to Site B through a 100 meter long optical fiber. The photon is converted into a single collective excitation via the dark-state polariton approach of Fleischhauer and Lukin [Phys. Rev. Lett. v.84, 5094 (2000)]. After a programmable storage time the atomic excitation is converted back into a single photon. This is demonstrated experimentally, for a storage time of 500 nanoseconds, by measurement of an anticorrelation parameter a. Storage times exceeding ten microseconds are observed by intensity cross-correlation measurements. The length of the storage period is two orders of magnitude longer than the time to achieve conversion between photonic and atomic quanta. The controlled transfer of single quanta between remote quantum memories constitutes an important step towards distributed quantum networks.

quant-ph↗

arXiv2005

Theory of dark-state polariton collapses and revivals

We investigate the dynamics of dark-state polaritons in an atomic ensemble with ground-state degeneracy. A signal light pulse may be stored and retrieved from the atomic sample by adiabatic variation of the amplitude of a control field. During the storage process, a magnetic field causes rotation of the atomic hyperfine coherences, leading to collapses and revivals of the dark-state polariton number. These collapses and revivals should be observable in measurements of the retrieved signal field, as a function of storage time and magnetic field orientation.

quant-ph↗

arXiv2005

Entanglement of remote atomic qubits

We report observations of entanglement of two remote atomic qubits, achieved by generating an entangled state of an atomic qubit and a single photon at Site A, transmitting the photon to Site B in an adjacent laboratory through an optical fiber, and converting the photon into an atomic qubit. Entanglement of the two remote atomic qubits is inferred by performing, locally, quantum state transfer of each of the atomic qubits onto a photonic qubit and subsequent measurement of polarization correlations in violation of the Bell inequality |S| <2. We experimentally determine S =2.16 +/- 0.03. Entanglement of two remote atomic qubits, each qubit consisting of two independent spin wave excitations, and reversible, coherent transfer of entanglement between matter and light, represent important advances in quantum information science.

quant-ph↗

arXiv2005

Observation of dark state polariton collapses and revivals

By time-dependent variation of a control field, both coherent and single photon states of light are stored in, and retrieved from, a cold atomic gas. The efficiency of retrieval is studied as a function of the storage time in an applied magnetic field. A series of collapses and revivals is observed, in very good agreement with theoretical predictions. The observations are interpreted in terms of the time evolution of the collective excitation of atomic spin wave and light wave, known as the dark-state polariton.

quant-ph↗

arXiv2005

Entanglement of a photon and a collective atomic excitation

We describe a new experimental approach to probabilistic atom-photon (signal) entanglement. Two qubit states are encoded as orthogonal collective spin excitations of an unpolarized atomic ensemble. After a programmable delay, the atomic excitation is converted into a photon (idler). Polarization states of both the signal and the idler are recorded and are found to be in violation of the Bell inequality. Atomic coherence times exceeding several microseconds are achieved by switching off all the trapping fields - including the quadrupole magnetic field of the magneto-optical trap - and zeroing out the residual ambient magnetic field.

quant-ph↗

arXiv2003

Light transport in cold atoms: the fate of coherent backscattering in the weak localization regime

The recent observation of coherent backscattering (CBS) of light by atoms has emphasized the key role of the velocity spread and of the quantum internal structure of the atoms. Firstly, using highly resonant scatterers imposes very low temperatures of the disordered medium in order to keep the full contrast of the CBS interference. This criterion is usually achieved with standard laser cooling techniques. Secondly, a non trivial internal atomic structure leads to a dramatic decrease of the CBS contrast. Experiments with Rubidium atoms (with a non trivial internal structure) and with Strontium (with the simplest possible internal structure) show this behaviour and confirm theoretical calculations.

physics.atom-ph↗