arXiv subjects

T. Das

Publications and source records attributed to T. Das.

11 recordsLinked to original sources

arXiv2025

Temperature-Dependent Dielectric Function of Calcium Fluoride

The optical properties of calcium fluoride (fluorspar, CaF2) are mainly determined by a strongly temperature-dependent giant infrared (IR) peak, and a series of nearly temperature-independent ultraviolet (UV) peaks. We find that the temperature dependence of the IR peak can be modeled, to good accuracy, by a radiation-reaction improved coupled-oscillator model (RRCO model), with temperature-dependent parameters. For the UV peaks, we find a convenient functional form which covers both the real as well as the imaginary parts of the dielectric function and provide a comparison to first-principles calculations based on time-dependent density-functional theory (TDDFT). The result is a compact functional form for the dielectric function of undoped CaF2 applicable to wide frequency and temperature ranges (0 < hbar omega < 60 eV, 22C < T < 500C). With the help of the temperature-dependent dielectric function, we obtain temperature-dependent values of the short-range and long-range asymptotics of atom-surface interactions with CaF2, for hydrogen, as well as ground-state and metastable helium. The giant IR absorption peak of CaF2 is shown to lead to a delayed onset of the fully retarded Casimir--Polder limit in the long-range interaction regime. We present arguments supporting a more general applicability of the RRCO model to materials of general interest.

cond-mat.mtrl-sci↗

arXiv2025

Coupled Oscillators and Dielectric Function

A generalized Sellmeier model, also referred to as the Lorentz-Dirac model, has been used for the description of the dielectric function of a number of technologically important materials in the literature. This model represents the frequency-dependent dielectric function as a sum over Green functions of classical damped harmonic oscillators, much in analogy with the functional form used for the dynamic polarizability of an atom, but with one important addition, namely, a complex-valued oscillator strength in the numerator. Here, we show that this generalized functional form can be justified based on the response function of coupled damped oscillators. The encountered analogies suggest an explanation for the generally observed success of the Lorentz--Dirac model in describing the dielectric function of crystals of consummate technological significance.

cond-mat.mtrl-sci↗

arXiv2024

A Small Brown Dwarf in an Aligned Orbit around a Young, Fully-Convective M Star

A star's spin-orbit angle can give us insight into a system's formation and dynamical history. In this paper, we use MAROON-X observations of the Rossiter-McLaughlin (RM) effect to measure the projected obliquity of the LP 261-75 (also known as TOI-1779) system, focusing on the fully-convective M dwarf LP 261-75A and the transiting brown dwarf LP 261-75C. This is the first obliquity constraint of a brown dwarf orbiting an M dwarf and the seventh obliquity constraint of a brown dwarf overall. We measure a projected obliquity of $5^{+11}_{-10}$ degrees and a true obliquity of $14^{+8}_{-7}$ degrees for the system, meaning that the system is well-aligned and that the star is rotating very nearly edge-on, with an inclination of $90^o\,\pm\,11^o$. The system thus follows along with the trends observed in transiting brown dwarfs around hotter stars, which typically have low obliquities. The tendency for brown dwarfs to be aligned may point to some enhanced obliquity damping in brown dwarf systems, but there is also a possibility that the LP 261-75 system was simply formed aligned. In addition, we note that the brown dwarf's radius ($R_C\,=\,0.9$ R$_J$) is not consistent with the youth of the system or radius trends observed in other brown dwarfs, indicating that LP 261-75C may have an unusual formation history.

astro-ph.EP↗

arXiv2023

Retardation Effects in Atom-Wall Interactions

The onset of retardation effects in atom-wall interactions is studied. It is shown that the transition range from the 1/z^3 short-range (van der Waals) interaction to the 1/z^4 long-range (Casimir) retarded interaction critically depends on the atomic properties and on the dielectric function of the material. For simple non-alkali atoms (e.g., ground-state hydrogen and ground-state helium) interacting with typical dielectric materials such as intrinsic silicon, the transition to the retarded regime is shown to proceed at a distance of about 10 nm (200 Bohr radii). This is much shorter than typical characteristic absorption wavelengths of solids. Larger transition regimes are obtained for atoms with a large static polarizability such as metastable helium. We present a simple estimate for the critical distance, z_cr=137*(\alpha(0)/Z)^(1/2) atomic units, where alpha(0) is the static polarizability (expressed in atomic units) and Z is the number of electrons of the atom.

cond-mat.other↗

arXiv2022

Temperature-dependent dielectric function of intrinsic silicon: Analytic models and atom-surface potentials

The optical properties of monocrystalline, intrinsic silicon are of interest for technological applications as well as fundamental studies of atom-surface interactions. For an enhanced understanding, it is of great interest to explore analytic models which are able to fit the experimentally determined dielectric function $\epsilon(T_\Delta, \omega)$, over a wide range of frequencies and a wide range of the temperature parameter $T_\Delta = (T-T_0)/T_0$, where $T_0 = 293\,{\rm K}$ represents room temperature. Here, we find that a convenient functional form for the fitting of the dielectric function of silicon involves a Lorentz-Dirac curve with a complex, frequency-dependent amplitude parameter, which describes radiation reaction. We apply this functional form to the expression $[\epsilon(T_\Delta, \omega) -1]/[ \epsilon(T_\Delta, \omega)+2]$, inspired by the Clausius-Mossotti relation. With a very limited set of fitting parameters, we are able to represent, to excellent accuracy, experimental data in the (angular) frequency range $0 < \omega < 0.16 \, {\rm a.u.}$ and $0< T_\Delta < 2.83$, corresponding to the temperature range $ 293\,{\rm K} < T < 1123\, {\rm K}$. Using our approach, we evaluate the short-range $C_3$ and the long-range $C_4$ coefficients for the interaction of helium atoms with the silicon surface. In order to validate our results, we compare to a separate temperature-dependent direct fit of $\epsilon(T_\Delta, \omega)$ to the Lorentz-Dirac model.

cond-mat.mtrl-sci↗

arXiv2017

Coulomb-corrected quantum interference in above-threshold ionization: Working towards multi-trajectory electron holography

Using the recently developed Coulomb Quantum Orbit Strong-Field Approximation (CQSFA), we perform a systematic analysis of several features encountered in above-threshold ionization (ATI) photoelectron angle-resolved distributions (PADs), such as side lobes, and intra- and intercycle interference patterns. The latter include not only the well-known intra-cycle rings and the near-threshold fan-shaped structure, but also previously overlooked patterns. We provide a direct account of how the Coulomb potential distorts different types of interfering trajectories and changes the corresponding phase differences, and show that these patterns may be viewed as generalized holographic structures formed by up to three types of trajectories. We also derive analytical interference conditions and estimates valid in the presence or absence of the residual potential, and assess the range of validity of Coulomb-corrected interference conditions provided in the literature.

physics.atom-ph↗

arXiv2016

Evidence for trivial Berry phase and absence of chiral anomaly in semimetal NbP

We report a detailed magneto-transport study in single crystals of NbP. High quality crystals were grown by vapour transport method. An exceptionally large magnetoresistance is confirmed at low temperature which is non-saturating and is linear at high fields. Models explaining the linear magnetoresistance are discussed and it is argued that in NbP this is linked to charge carrier mobility fluctuations. Negative longitudinal magnetoresistance is not seen, unlike several other Weyl monopnictides, suggesting lack of well defined chiral anomaly in NbP. Unambiguous Shubnikov-de-Haas oscillations are observed at low temperatures that are correlated to Berry phases. The Landau fan diagram indicates trivial Berry phase in NbP crystals corresponding to Fermi surface extrema at 30.5 Tesla.

cond-mat.mtrl-sci↗

arXiv2016

Shifting nodal-plane suppressions in high-order harmonic spectra from diatomic molecules in orthogonally polarized driving fields

We analyze the imprint of nodal planes in high-order harmonic spectra from aligned diatomic molecules in intense laser fields whose components exhibit orthogonal polarizations. We show that the typical suppression in the spectra associated to nodal planes is distorted, and that this distortion can be employed to map the electron's angle of return to its parent ion. This investigation is performed semi-analytically at the single-molecule response and single-active orbital level, using the strong-field approximation and the steepest descent method. We show that the velocity form of the dipole operator is superior to the length form in providing information about this distortion. However, both forms introduce artifacts that are absent in the actual momentum-space wavefunction. Furthermore, elliptically polarized fields lead to larger distortions in comparison to two-color orthogonally polarized fields. These features are investigated in detail for $\mathrm{O}_2$, whose highest occupied molecular orbital provides two orthogonal nodal planes.

physics.atom-ph↗

arXiv2015

Extracting an electron's angle of return from shifted interference patterns in macroscopic high-harmonic spectra of diatomic molecules

We investigate high-order harmonic spectra from aligned diatomic molecules in intense driving fields whose components have orthogonal polarizations. We focus on how the driving-field ellipticity influences structural interference patterns in a macroscopic medium. In a previous publication [Phys. Rev. A 88, 023404 (2013)] we have shown that the non-vanishing ellipticity introduces an effective dynamic shift in the angle for which the two-center interference maxima and minima occur, with regard to the existing condition for linearly polarized fields. In this work we show through simulation that it is still possible to observe this shift in harmonic spectra that have undergone macroscopic propagation, and discuss the parameter range for doing so. These features are investigated for $H_2$ in a bichromatic field composed of two orthogonally polarized waves. The shift is visible both in the near- and in the far-field regime, so that, in principle, it can be observed in experiments.

physics.atom-ph↗

arXiv2013

High-order harmonic generation from diatomic molecules in elliptically polarized driving fields: a generalized interference condition

We investigate the influence of intense, elliptically polarized driving fields on high-order harmonic spectra from aligned diatomic molecules. We derive a generalized two-center interference condition for elliptically polarized fields, which accounts for s-p mixing and the orbital symmetry, within the strong-field and the single-active electron approximation. We show that the non-vanishing ellipticity introduces an effective dynamic shift in the angle for which the two-center interference maxima and minima occur, with regard to the existing condition for linearly polarized fields. This shift depends on the ratio between the field-dressed momentum components of the returning electron parallel and perpendicular to the major ellipticity axis along each possible orbit. Because of this dependence, we find that there will be a blurring in the two-center interference minima, and that increasing ellipticity leads to splitting in such patterns. These features are investigated in detail for H2 and Ar2.

physics.atom-ph↗

arXiv2007

Low angular momentum accretion flow model of Sgr A* activity

Sgr A* is a source of strongly variable emission in several energy bands. It is generally agreed that this emission comes from the material surrounding the black hole which is either falling in or flowing out. The activity must be driven by accretion but the character of accretion flow in this object is an open question. We suggest that the inflow is dominated by the relatively low angular momentum material originating in one of the nearby group of stars. Such material flows in directly towards the black hole up to the distance of order of ten Schwarzschild radii or less, where it hits the angular momentum barrier which leads naturally to a flow variability. We study both the analytical and the numerical solutions for the flow dynamics, and we analyze the radiation spectra in both cases using the Monte Carlo code to simulate the synchrotron, bremsstrahlung and the Compton scattering. Our model roughly reproduces the broad band spectrum of Sgr A* and its variability if we allow for a small fraction of energy to be converted to non-thermal population of electrons. It is also consistent (for a range of viewing angles) with the strong constraints on the amount of circumnuclear material imposed by the measurements of the Faraday rotation.

astro-ph↗