arXiv subjects

T. Delord

Publications and source records attributed to T. Delord.

12 recordsLinked to original sources

arXiv2026

Measurement of a quantum system using spin-mechanical conversion

Levitated macroscopic particles exhibiting quantum mechanical effects are garnering increased attention as a means for precision sensing and testing quantum mechanics. Defects in diamond, such as the nitrogen-vacancy (NV) centre possess optically-addressable spins with long coherence times at room temperature and offer an intriguing system to examine quantum spin dynamics coupled to a macroscopic classical particle. In this work, we convert the outcome of a quantum measurement on an ensemble of spins into a macroscopic rotation of the host particle via spin-mechanical coupling. Following a sequence of green laser and microwave control pulses, spin-mechanical coupling between the final qubit spin state and the host particle -- an electrically-levitated diamond -- exerts a torque on the particle that deflects a weak near-infra-red laser beam. We measure spin readout contrast in excess of 70\%, and demonstrate pulsed mechanical detection of coherent Rabi oscillations, spin-echo interferometry and $T_1$-induced relaxation. We directly measure with temporal resolution the particle reorientation from a 60\,attonewton-metre spin torque induced by flipping the spins. Our results open up interesting new opportunities for levitated spin-mechanical systems using pulsed control, from improved sensing to the prospect of realising macroscopic quantum superposition states.

quant-ph↗

arXiv2024

3D-mapping and manipulation of photocurrent in an optoelectronic diamond device

Characterising charge transport in a material is central to the understanding of its electrical properties, and can usually only be inferred from bulk measurements of derived quantities such as current flow. Establishing connections between host material impurities and transport properties in emerging electronics materials, such as wide bandgap semiconductors, demands new diagnostic methods tailored to these unique systems, and the presence of optically-active defect centers in these materials offers a non-perturbative, in-situ characterisation system. Here, we combine charge-state sensitive optical microscopy and photoelectric detection of nitrogen-vacancy (NV) centres to directly image the flow of charge carriers inside a diamond optoelectronic device, in 3D and with temporal resolution. We optically control the charge state of background impurities inside the diamond on-demand, resulting in drastically different current flow such as filamentary channels nucleating from specific, defective regions of the device. We then optically engineered conducting channels that control carrier flow, key steps towards optically reconfigurable, wide bandgap designer optoelectronics. We anticipate our approach might be extended to probe other wide-bandgap semiconductors (SiC, GaN) relevant to present and emerging electronic technologies.

cond-mat.mtrl-sci↗

arXiv2020

Coherent Microwave Control of a Nuclear Spin Ensemble at Room Temperature

We use nominally forbidden electron-nuclear spin transitions in nitrogen-vacancy (NV) centers in diamond to demonstrate coherent manipulation of a nuclear spin ensemble using microwave fields at room temperature. We show that employing an off-axis magnetic field with a modest amplitude($\approx$ 0.01 T) at an angle with respect to the NV natural quantization axes is enough to tilt the direction of the electronic spins, and enable efficient spin exchange with the nitrogen nuclei of the NV center. We could then demonstrate fast Rabi oscillations on electron-nuclear spin exchanging transitions, coherent population trapping and polarization of nuclear spin ensembles in the microwave regime. Coupling many electronic spins of NV centers to their intrinsic nuclei offers full scalability with respect to the number of controllable spins and provides prospects for transduction. In particular, the technique could be applied to long-lived storage of microwave photons and to the coupling of nuclear spins to mechanical oscillators in the resolved sideband regime.

quant-ph↗

arXiv2020

Spin-mechanics with levitating ferromagnetic particles

We propose and demonstrate first steps towards schemes where the librational mode of levitating ferromagnets is strongly coupled to the electronic spin of Nitrogen-Vacancy (NV) centers in diamond. Experimentally, we levitate ferromagnets in a Paul trap and employ magnetic fields to attain oscillation frequencies in the hundreds of kHz range with Q factors close to $10^4$. These librational frequencies largely exceed the decoherence rate of NV centers in typical CVD grown diamonds offering prospects for sideband resolved operation. We also prepare and levitate composite diamond-ferromagnet particles and demonstrate both coherent spin control of the NV centers and read-out of the particle libration using the NV spin. Our results will find applications in ultra-sensitive gyroscopy and bring levitating objects a step closer to spin-mechanical experiments at the quantum level.

quant-ph↗

arXiv2019

Spin-Cooling of the Motion of a Trapped Diamond

Observing and controlling macroscopic quantum systems has long been a driving force in research on quantum physics. In this endeavor, strong coupling between individual quantum systems and mechanical oscillators is being actively pursued. While both read-out of mechanical motion using coherent control of spin systems and single spin read-out using pristine oscillators have been demonstrated, temperature control of the motion of a macroscopic object using long-lived electronic spins has not been reported. Here, we observe both a spin-dependent torque and spin-cooling of the motion of a trapped microdiamond. Using a combination of microwave and laser excitation enables the spin of nitrogen-vacancy centers to act on the diamond orientation and to cool the diamond libration via a dynamical back-action. Further, driving the system in the non-linear regime, we demonstrate bistability and self-sustained coherent oscillations stimulated by the spin-mechanical coupling, which offers prospects for spin-driven generation of non-classical states of motion. Such a levitating diamond operated as a compass with controlled dissipation has implications in high-precision torque sensing, emulation of the spin-boson problem and probing of quantum phase transitions. In the single spin limit and employing ultra-pure nano-diamonds, it will allow quantum non-demolition read-out of the spin of nitrogen-vacancy centers under ambient conditions, deterministic entanglement between distant individual spins and matter-wave interferometry.

quant-ph↗

arXiv2019

Sub-GHz linewidths ensembles of SiV centers in a diamond nano-pyramid revealed by charge state conversion

Producing nano-structures with embedded bright ensembles of lifetime-limited emitters is a challenge with potential high impact in a broad range of physical sciences. In this work, we demonstrate controlled charge transfer to and from dark states exhibiting very long lifetimes in high density ensembles of SiV centers hosted in a CVD-grown diamond nano-pyramid. Further, using a combination of resonant photoluminescence excitation and a frequency-selective persistent hole burning technique that exploits such charge state transfer, we could demonstrate close to lifetime-limited linewidths from the SiV centers. Such a nanostructure with thousands of bright narrow linewidth emitters in a volume much below $λ^3$ will be useful for coherent light-matter coupling, for biological sensing, and nanoscale thermometry.

quant-ph↗

arXiv2018

Ramsey interferences and spin echoes from electron spins inside a levitating macroscopic particle

We report observations of Ramsey interferences and spin echoes from electron spins inside a levitating macroscopic particle. The experiment is realized using nitrogen-vacancy (NV) centers hosted in a micron-sized diamond stored in a Paul trap both under atmospheric conditions and under vacuum. Spin echoes are used to show that the Paul trap preserves the coherence time of the embedded electron spins for more than microseconds. Conversely, the NV spin is employed to demonstrate high angular stability of the diamond even under vacuum. These results are significant steps towards strong coupling of NV spins to the rotational mode of levitating diamonds.

quant-ph↗

arXiv2018

Diamond nano-pyramids with narrow linewidth SiV centers for quantum technologies

Color centers in diamond are versatile solid state atomic-like systems suitable for quantum technological applications. In particular, the negatively charged silicon vacancy center (SiV) can exhibit a narrow photoluminescence (PL) line and lifetime-limited linewidth in bulk diamonds at cryogenic temperature. We present a low-temperature study of chemical vapour deposition (CVD)-grown diamond nano-pyramids containing SiV centers. The PL spectra feature a bulk-like zero-phonon line with ensembles of SiV centers, with a linewidth below 10 GHz which demonstrates very low crystal strain for such a nano-object.

quant-ph↗

arXiv2017

Coherent Population Trapping with a controlled dissipation: applications in optical metrology

We analyze the properties of a pulsed Coherent Population Trapping protocol that uses a controlled decay from the excited state in a $Λ$-level scheme. We study this problem analytically and numerically and find regimes where narrow transmission, absorption, or fluorescence spectral lines occur. We then look for optimal frequency measurements using these spectral features by computing the Allan deviation in the presence of ground state decoherence and show that the protocol is on a par with Ramsey-CPT. We discuss possible implementations with ensembles of alkali atoms and single ions and demonstrate that typical pulsed-CPT experiments that are realized on femto-second time-scales can be implemented on micro-seconds time-scales using this scheme.

quant-ph↗

arXiv2017

Strong Coupling between a Single NV Spin and the Rotational Mode of Diamonds Levitating in an Ion Trap

A scheme for strong coupling between a single atomic spin and the rotational mode of levitating nanoparticles is proposed. The idea is based on spin read-out of NV centers embedded in aspherical nanodiamonds levitating in an ion trap. We show that the asymmetry of the diamond induces a rotational confinement in the ion trap. Using a weak homogeneous magnetic field and a strong microwave driving we then demonstrate that the spin of the NV center can be strongly coupled to the rotational motion of the diamond.

quant-ph↗

arXiv2017

Diamonds levitating in a Paul trap under vacuum: measurements of laser-induced heating via NV center thermometry

We present measurements of the Electronic Spin Resonance (ESR) of Nitrogen Vacancy (NV) centers in diamonds that are levitating in a ring Paul trap under vacuum. We observe ESR spectra of NV centers embedded in micron-sized diamonds at vacuum pressures down to $2\times 10^{-1}$ mbar, limited by the green laser heating of the diamond. We also observe the NV photoluminescence at vacuum pressures down to $10^{-2}$ mbar and discuss the steps required to control the NV spin under ultra-high vacuum.

quant-ph↗

arXiv2014

Polarization entangled photon-pair source based on quantum nonlinear photonics and interferometry

We present a versatile, high-brightness, guided-wave source of polarization entangled photons, emitted at a telecom wavelength. Photon-pairs are generated using an integrated type-0 nonlinear waveguide, and subsequently prepared in a polarization entangled state via a stabilized fiber interferometer. We show that the single photon emission wavelength can be tuned over more than 50 nm, whereas the single photon spectral bandwidth can be chosen at will over more than five orders of magnitude (from 25 MHz to 4 THz). Moreover, by performing entanglement analysis, we demonstrate a high degree of control of the quantum state via the violation of the Bell inequalities by more than 40 standard deviations. This makes this scheme suitable for a wide range of quantum optics experiments, ranging from fundamental research to quantum information applications. We report on details of the setup, as well as on the characterization of all included components, previously outlined in F. Kaiser et al. (2013 Laser Phys. Lett. 10, 045202).

quant-ph↗