arXiv subjects

T. Devolder

Publications and source records attributed to T. Devolder.

At least 19 recordsLinked to original sources

arXiv2026

Field-driven triggering of self-induced Floquet magnons in a magnetic vortex

We report the experimental control of Floquet magnons in a magnetic vortex. Using microwave spectroscopy of vortex state magnetic tunnel junctions (MTJs), we find that self-induced Floquet sidebands form frequency combs whose existence depend on the vortex core orbit. By shifting the vortex core with an applied magnetic field, we switch the system between regular and Floquet magnons at identical drive conditions, demonstrating hysteretic control of the Floquet spectrum. A nonlinear vortex-magnon model shows that this behavior originates from multiple stable vortex gyration radii created by Floquet-mediated feedback. These results establish magnetic state initialization as a means to switch between regular and Floquet magnons.

cond-mat.mtrl-sci↗

arXiv2025

Time-resolved observation of magnon splitting into vortex gyration and Floquet spin waves

Forced excitations at frequencies in the range of the first order azimuthal spin waves of a magnetic disk in the vortex state are known to scatter into the vortex gyration mode, thereby allowing the growth of Floquet spin waves forming a frequency comb. We study the temporal emergence of this dynamical state using time-resolved microwave electrical measurements. The most intense Floquet mode emerges synchronously with the gyration mode after a common incubation delay which diverges at the scattering threshold. This delay is minimal when the drive is resonant with one of the first order azimuthal spin waves. It can be as short as 3 ns for the maximum investigated power. We conclude that the first-to-occur scattering mechanism is the three-wave splitting of a regular azimuthal eigenmode into a coherent pair formed by a gyration magnon and a Floquet spin wave.

cond-mat.mtrl-sci↗

arXiv2024

Spectroscopy of the spin waves of a synthetic antiferromagnet grown on a piezoelectric substrate

Efficient coupling between magnons and phonons requires material platforms that contain magnetic multilayers with versatile high-frequency properties grown on piezoelectric substrates with large electromechanical coupling coefficients. One of these systems is the CoFeB/Ru/CoFeB Synthetic antiferromagnet grown on Lithium Niobate substrate. We investigate its microwave magnetic properties using a combination of ferromagnetic resonance and propagating spin wave spectroscopy, from which we extract the dispersion relation of the acoustic branch of spin waves. The frequency and the linewidth of this spin wave resonance, its field dependence and its dispersion relation indicate that the magnetic properties are as good as when grown on standard non-piezoelectric substrates, as well as being in line with theory. This new material platform opens opportunities to extend microwave acousto-magnonics beyond the use of single layer magnets.

cond-mat.mtrl-sci↗

arXiv2024

Experimental observation of vortex gyrotropic mode excited by surface acoustic waves

The traditional method for exciting spin-wave dynamics in magnetic materials involves microwave magnetic fields generated by current injection into inductive antennas. However, there is a growing interest in non-inductive excitation methods. Magneto-acoustic effects present a viable alternative, where strains produced by applying voltages to a piezoelectric substrate can couple to spin-waves in a magnetic film. Recently, it has been proposed that surface acoustic waves (SAWs) can excite the gyrotropic mode of the vortex state in a magnetic disk. Here we report on experiments utilizing a magnetic resonance force microscope to investigate magnetization dynamics in CoFeB sub-micrometer disks in the vortex state, grown on a Z-cut LiNbO$_3$ substrate. The device design enables excitation of the gyrotropic mode either inductively, using an antenna on top of the disks, or acoustically via SAWs launched from an interdigital transducer. Our modelling indicates that the lattice rotation {\omega}xz generates a localized magneto-acoustic field that displaces the vortex core from the disk center, initiating the gyration motion. Tuning of the magneto-acoustic torque acting on the vortex structure is achieved by a perpendicular magnetic field. These results demonstrate the clear excitation of the vortex gyrotropic mode by magneto-acoustic excitation.

cond-mat.mtrl-sci↗

arXiv2024

Unidirectional spin waves measured using propagating spin wave spectroscopy

The dispersion relation of spin waves can vary monotonically about the center of the Brillouin zone, allowing zero-momentum wavepackets to flow unidirectionally, which is of interest for applications. Techniques such as propagating spin wave spectroscopy are inoperative in such cases because of the difficulty to identify the spin wave wavevector at a particular frequency within a spectrum. Here we present a method to analyse this case and apply it to acoustic spin waves in a synthetic antiferromagnet in the scissors state, in which we confirm that propagation parallel to the applied fields is unidirectional. Interestingly, we find that in this unidirectional situation, the phase accumulated by the spin waves propagating between two antenna is not proportional to the antenna spacing. It is also a function of the two other lengths of the problem: the antenna width and the spin wave decay length. Accounting for them is required to avoid wavevector errors in the dispersion relations.

cond-mat.mtrl-sci↗

arXiv2024

Symmetry of the coupling between surface acoustic waves and spin waves in synthetic antiferromagnets

Synthetic antiferromagnets host spin waves that are highly tunable. It is of practical interest to analyze the symmetry of their coupling to surface acoustic waves with the design of hybrid devices in view. For this we calculate the layer-resolved susceptibility tensor of a synthetic antiferromagnet, the effective magneto-elastic and magneto-rotation fields associated to a travelling elastic wave, and the power irreversibly transferred by the elastic wave to the magnetic layers. We consider Rayleigh-type surface acoustic waves: (a) that travel in an elastically isotropic, non-piezoelectric substrate, or (b) that propagate along the X direction at the surface of a Z-cut LiNbO$_3$ substrate, or (c) that are guided in a thin Z-cut LiNbO$_3$ film grown on a sapphire substrate. In particular, we show that the complementary angular dependencies of the acoustic and optical spin wave modes in synthetic antiferromagnets makes it possible to excite spin waves for any relative orientation of magnetization and acoustic wavevector. In addition, we discuss the symmetries of the driving fields and of the energy transferred to the magnetic degree of freedom. We evidence new interaction channels coupling the magnetization eigenmodes when elastic anisotropy and piezoelectricity of the substrate are considered.

cond-mat.mtrl-sci↗

arXiv2023

Unidirectionality of spin waves in Synthetic Antiferromagnets

We study the frequency non-reciprocity of the spin waves in symmetric CoFeB/Ru/CoFeB synthetic antiferromagnets stacks set in the scissors state by in-plane applied fields. Using a combination of Brillouin Light Scattering and propagating spin wave spectroscopy experiments, we show that the acoustical spin waves in synthetic antiferromagnets possess a unique feature if their wavevector is parallel to the applied field: the frequency non-reciprocity due to layer-to-layer dipolar interactions can be so large that the acoustical spin waves transfer energy in a unidirectional manner for a wide and bipolar interval of wavevectors. Analytical modeling and full micromagnetic calculations are conducted to account for the dispersion relations of the optical and acoustical spin waves for arbitrary field orientations. Our formalism provides a simple and direct method to understand and design devices harnessing unidirectional propagation of spin waves in synthetic antiferromagnets.

cond-mat.mtrl-sci↗

arXiv2023

Inducing or suppressing the anisotropy in multilayers based on CoFeB

Controlling the uniaxial magnetic anisotropy is of practical interest to a wide variety of applications. We study Co$_{40}$Fe$_{40}$B$_{20}$ single films grown on various crystalline orientations of LiNbO$_3$ substrates and on oxidized silicon. We identify the annealing conditions that are appropriate to induce or suppress uniaxial anisotropy. Anisotropy fields can be increased by annealing up to 11 mT when using substrates with anisotropic surfaces. They can be decreased to below 1 mT when using isotropic surfaces. In the first case, the observed increase of the anisotropy originates from the biaxial strain in the film caused by the anisotropic thermal contraction of the substrate when back at room temperature after strain relaxation during annealing. In the second case, anisotropy is progressively removed by applying successive orthogonal fields that are assumed to progressively suppress any chemical ordering within the magnetic film. The method can be applied to CoFeB/Ru/CoFeB synthetic antiferromagnets but the tuning of the anisotropy comes with a decrease of the interlayer exchange coupling and a drastic change of the exchange stiffness.

cond-mat.mtrl-sci↗

arXiv2022

Exchange energies in CoFeB/Ru/CoFeB Synthetic Antiferromagnets

The interlayer exchange coupling confers specific properties to Synthetic Antiferromagnets that make them suitable for several applications of spintronics. The efficient use of this magnetic configuration requires an in-depth understanding of the magnetic properties and their correlation with the material structure. Here we establish a reliable procedure to quantify the interlayer exchange coupling and the intralayer exchange stiffness in synthetic antiferromagnets; we apply it to the ultrasmooth and amorphous Co$_{40}$Fe$_{40}$B$_{20}$ (5-40 nm)/Ru/ Co$_{40}$Fe$_{40}$B$_{20}$ material platform. The complex interplay between the two exchange interactions results in a gradient of the magnetization orientation across the thickness of the stack which alters the hysteresis and the spin wave eigenmodes of the stack in a non trivial way. We measured the field-dependence of the frequencies of the first four spin waves confined within the thickness of the stack. We modeled these frequencies and the corresponding thickness profiles of these spin waves using micromagnetic simulations. The comparison with the experimental results allows to deduce the magnetic parameters that best account for the sample behavior. The exchange stiffness is established to be 16 $\pm$ 2 pJ/m, independently of the Co$_{40}$Fe$_{40}$B$_{20}$ thickness. The interlayer exchange coupling starts from -1.7 mJ/m$^2$ for the thinnest layers and it can be maintained above -1.3 mJ/m$^2$ for CoFeB layers as thick as 40 nm. The comparison of our method with earlier characterizations using the sole saturation fields argues for a need to revisit the tabulated values of interlayer exchange coupling in thick synthetic antiferromagnets.

cond-mat.mtrl-sci↗

arXiv2022

Measuring a population of spin waves from the electrical noise of an inductively coupled antenna

We study how a population of spin waves can be characterized from the analysis of the electrical microwave noise delivered by an inductive antenna placed in its vicinity. The measurements are conducted on a synthetic antiferromagnetic thin stripe covered by a micron-sized antenna that feeds a spectrum analyser after amplification. The antenna noise contains two contributions. The population of incoherent spin waves generates a fluctuating field that is sensed by the antenna: this is the "magnon noise". The antenna noise also contains the contribution of the electronic fluctuations: the Johnson-Nyquist noise. The latter depends on all impedances within the measurement circuit, which includes the antenna self-inductance. As a result, the electronic noise contains information about the magnetic susceptibility of the stripe, though it does not inform on the absolute amplitude of the magnetic fluctuations. For micrometer-sized systems at thermal equilibrium, the electronic noise dominates and the pure magnon noise cannot be determined. If in contrast the spinwave bath is not at thermal equilibrium with the measurement circuit, and if the spin wave population can be changed then one could measure a mode-resolved effective magnon temperature provided specific precautions are implemented.

cond-mat.mtrl-sci↗

arXiv2021

Measuring the dispersion relations of spin wave bands using time-of-flight spectroscopy

We develop a generic all-inductive procedure to measure the band structure of spin waves in a magnetic thin stripe. In contrast to existing techniques, our method works even if several spin wave branches coexist in the investigated frequency interval, provided that the branches possess sufficiently different group velocities. We first measure the microwave scattering matrix of a network composed of distant antennas inductively coupled to the spin wave bath of the magnetic film. After a mathematical transformation to the time-domain to get the transmission impulse response, the different spin wave branches are viewed as wavepackets that reach successively the receiving antenna after different travel times. In analogy with time-of flight spectroscopy, the wavepackets are then separated by time-gating. The time-gated responses are used to recalculate the contribution of each spin wave branch to the frequency domain scattering matrix. The dispersion relation of each branch stems from the absolute phase of the time-gated transmission parameter. The spin wave wavevector can be determined unambiguously if the results for several propagation distances are combined, so as to get the dispersion relations.

cond-mat.mtrl-sci↗

arXiv2021

Real-time Hall-effect detection of current-induced magnetization dynamics in ferrimagnets

Measurements of the transverse Hall resistance are widely used to investigate electron transport, magnetization phenomena, and topological quantum states. Owing to the difficulty of probing transient changes of the transverse resistance, the vast majority of Hall effect experiments are carried out in stationary conditions using either dc or ac currents. Here we present an approach to perform time-resolved measurements of the transient Hall resistance during current-pulse injection with sub-nanosecond temporal resolution. We apply this technique to investigate in real-time the magnetization reversal caused by spin-orbit torques in ferrimagnetic GdFeCo dots. Single-shot Hall effect measurements show that the current-induced switching of GdFeCo is widely distributed in time and characterized by significant activation delays, which limit the total switching speed despite the high domain-wall velocity typical of ferrimagnets. Our method applies to a broad range of current-induced phenomena and can be combined with non-electrical excitations to perform pump-probe Hall effect measurements.

cond-mat.mes-hall↗

arXiv2021

Quantitative study of the response of a single NV defect in diamond to magnetic noise

The nitrogen-vacancy (NV) defect in diamond is an efficient quantum sensor of randomly fluctuating signals via relaxometry measurements. In particular, the longitudinal spin relaxation of the NV defect accelerates in the presence of magnetic noise with a spectral component at its electron spin resonance frequency. We look into this effect quantitatively by applying a calibrated and tunable magnetic noise on a single NV defect. We show that an increase of the longitudinal spin relaxation rate translates into a reduction of the photoluminescence (PL) signal emitted under continuous optical illumination, which can be explained using a simplified three-level model of the NV defect. This PL quenching mechanism offers a simple, all-optical method to detect magnetic noise sources at the nanoscale.

cond-mat.mes-hall↗

arXiv2020

Back-hopping in Spin-Transfer-Torque switching of perpendicularly magnetized tunnel junctions

We analyse the phenomenon of back-hopping in spin-torque induced switching of the magnetization in perpendicularly magnetized tunnel junctions. The analysis is based on single-shot time-resolved conductance measurements of the pulse-induced back-hopping. Studying several material variants reveals that the back-hopping is a feature of the nominally fixed system of the tunnel junction. The back-hopping is found to proceed by two sequential switching events that lead to a final state P' of conductance close to --but distinct from-- that of the conventional parallel state. The P' state does not exist at remanence. It generally relaxes to the conventional antiparallel state if the current is removed. The P' state involves a switching of the sole spin-polarizing part of the fixed layers. The analysis of literature indicates that back-hopping occurs only when the spin-polarizing layer is too weakly coupled to the rest of the fixed system, which justifies a posteriori the mitigation strategies of back-hopping that were implemented empirically in spin-transfer-torque magnetic random access memories.

cond-mat.mtrl-sci↗

arXiv2020

Electrical spectroscopy of forward volume spin waves in perpendicularly magnetized materials

We study the potential of all-electrical inductive techniques for the spectroscopy of propagating forward volume spin waves. We develop a one-dimensional model to account for the electrical signature of spin-wave reflection and transmission between inductive antennas and validate it with experiments on a perpendicularly magnetized Co/Ni multilayer. We describe the influence of the antenna geometry and antenna-to-antenna separation, as well as that of the material parameters on the lineshape of the inductive signals. For a finite damping, the broadband character of the antenna emission in the wave vector space imposes to take into account the growing decoherence of the magnetization waves upon their spatial propagation. The transmission signal can be viewed as resulting from two contributions: a first one from propagating spin-waves leading to an oscillatory phase of the broadband transmission coefficient, and another one originating from the distant induction of ferromagnetic resonance because of the long-range stray fields of realistic antennas. Depending on the relative importance of these two contributions, the decay of the transmitted signal with the propagation distance may not be exponential and the oscillatory character of the spin-wave phase upon propagation may be hidden. Our model and its experimental validation allow to define geometrical and material specifications to be met to enable the use of forward volume spin waves as efficient information carriers.

cond-mat.mes-hall↗

arXiv2020

Backward volume vs Damon-Eshbach: a travelling spin wave spectroscopy comparison

We compare the characteristics of electrically transduced Damon-Eshbach (DESWs) and backward volume (BVSWs) configurations within the same, 30 nm thick, ferromagnetic, CoFeB waveguide. Sub-micron U-shaped antennas are used to deliver the necessary in-plane and out-of-plane RF fields. We measure the spin-wave transmission with respect to in-plane field orientation, frequency and propagation distance. Unlike DESW, BVSWs are reciprocally transduced and collected for either direction of propagation, but their ability to transport energy is lower than DESWs for two reasons. This arises first because BVSW are inductively transduced less efficiently than DESWs. Also, in the range of wavevectors (~5 rad. um-1) typically excited by our antennas, the group velocity of BVSWs stays lower than that of DESW, which leads to reduced propagation ability that impact transmission signals in an exponential manner. In contrast, the group velocity of DESWs is maximum at low fields and decreases continuously with the applied field. The essential features of the measured SW characteristics are well reciprocated by a simple, 1-D analytical model which can be used to assess the potential of each configuration.

physics.app-ph↗

arXiv2019

BPZT HBARs for bias-tunable, stress generation at GHz frequencies

The high frequency performance of strong piezoelectric materials like PZT remains relatively less explored due to the assumption of large dielectric/ferroelectric losses at GHz frequencies. Recently, the advent of magnetoelectric technology as an on-chip route to excite magnetization dynamics has provided the impetus to evaluate the electromechanical performance of PZT at microwave frequencies. In this work, we demonstrate that HBARs fabricated using Barium-doped PZT (BPZT) films can efficiently generate acoustic waves up to 15 GHz. The ferroelectricity of BPZT endows added functionality to the resonator in the form of voltage tunability of the electromechanical performance. We extract the piezoelectric coefficient by numerically comparing the performance of BPZT with the Mason model. The extracted piezoelectric coefficient ~60 pm/V agrees well with reported values on thin film PZT measured at low frequencies (<100 MHz). Our results suggest that with further improvement in device design and material processing, BPZT resonators could operate as large amplitude, tunable stress transducers at GHz frequencies.

physics.app-ph↗

arXiv2019

Effect of Tantalum spacer thickness and deposition conditions on the properties of MgO/CoFeB/Ta/CoFeB/MgO free layers

To get stable perpendicularly magnetized tunnel junctions at small device dimensions, composite free layers that comprise two MgO/FeCoB interfaces as sources of interface anisotropy are generally used. Proper cristallisation and annealing robustness is typically ensured by the insertion of a spacer layer of the early transition metal series within the FeCoB layer. We study the influence of the spacer thickness and growth condition on the switching metrics of tunnel junctions thermally annealed at 400$^\circ$C for the case of 1-4 \r{A} Ta spacers. Thick Ta spacer results in a large anisotropies indicative of a better defined top FeCoB/MgO interface, but this is achieved at the systematic expense of a stronger damping. For the best anisotropy-damping compromise, junctions of diameter 22 nm can still be stable and spin-torque switched. Coercivity and inhomogeneous linewidth broadening, likely arising from roughness at the FeCoB/Ta interface, can be reduced if a sacrificial Mg layer is inserted before the Ta spacer deposition.

cond-mat.mtrl-sci↗