arXiv subjects

T. E. Mehlstäubler

Publications and source records attributed to T. E. Mehlstäubler.

At least 19 recordsLinked to original sources

arXiv2026

Extreme-ultraviolet spectroscopy using quantum logic: a feasibility study for the 1S-2S transition in singly-ionized helium

Extreme-ultraviolet (XUV) spectroscopy represents an important new direction in precision physics, with potential applications ranging from the metrology of fundamental constants to tests of physics beyond the Standard Model. However, the application of quantum control methods for precision spectroscopy remains an open challenge in the XUV range. Here we present a novel quantum logic (QL) spectroscopy method for precision spectroscopy of weak XUV transitions, and numerically validate its feasibility for the $1S-2S$ transition at 40.81\,eV in singly-ionized helium (He$^{+}$). We propose a scheme based on a single He$^{+}$ ion co-trapped with a Be$^{+}$ ion in a Paul trap, and He$^{+}$ excitation with pairs of frequency-comb (FC) laser pulses upconverted to the XUV via High-Harmonic Generation (HHG). We investigate a nondestructive QL scheme to detect $1S-2S$ excitation, and compare its performance with a destructive readout based on state-selective ionization. Phase coherence of the XUV light is modelled and an optical cavity is used to filter the FC pulses prior to HHG. We model the motional excitation dynamics of trapped ions outside the Lamb-Dicke regime, and numerically validate a scheme we proposed in \cite{Grundeman} to cancel the first-order Doppler broadening and the recoil shift by synchronizing the ion's secular period with the time delay between the two excitation pulses. We show that precision spectroscopy of the $1S-2S$ transition in He$^{+}$ at the 10 kHz level is feasible, for improved tests of quantum electrodynamics (QED), a measurement of the Rydberg constant $R_{\infty}$ independent of hydrogen measurements, or an improved determination of the alpha particle and helion charge radii. The proposed method may also be applied to XUV spectroscopy of other ions outside the Lamb-Dicke regime.

physics.atom-ph↗

arXiv2026

Shell formation and two-dimensional nanofriction in three-dimensional ion Coulomb crystals

Self-organized three-dimensional (3D) ion Coulomb crystals in linear Paul traps naturally form concentric shells that provide a curved, atomically resolved interface for studying two-dimensional (2D) nanofriction. Building on earlier studies of one-dimensional nanofriction and orientational melting in 2D ion crystals, we extend friction studies from linear chains and planar rings to 3D shell structures. Using molecular-dynamics simulations, we map shell formation as a function of ion number N and trap aspect ratio and obtain a simple scaling relation that can aid ion-number estimation in experiments. We compute a Peierls-Nabarro-type potential for rotating the outer shell against a static inner core, using the rotation angle as a collective coordinate. Changing N by one can alter the effective rotational barrier by up to a factor of ~7, while changes by only a few ions can lead to variations up to a factor of ~60. Combining geometric commensurability analysis with energy decomposition, we show that the barrier is governed by a system-dependent interplay between inter-shell interaction, outer-shell response and trap confinement. Dynamical simulations with applied torques reveal pinned, stick-slip and smooth-sliding regimes with depinning thresholds that depend on ion number, inner-shell geometry and trap aspect ratio. Some configurations show hysteresis due to torque-induced metastable states. We further find that spatially varying coupling to the inner-core corrugation can create coexisting fast and slow domains within the rotating outer shell, realizing multidimensional friction in which intra-shell shear and inter-shell nanofriction act simultaneously. Our results establish self-organized ion Coulomb crystals as model systems for 2D nanofriction and suggest routes toward ion-based nanorotors, torque sensors and ultra-low-friction nanomechanical systems.

physics.atom-ph↗

arXiv2025

Robust and scalable rf spectroscopy in first-order magnetic sensitive states at second-long coherence time

Trapped-ion quantum sensors have become highly sensitive tools for the search of physics beyond the Standard Model. Recently, stringent tests of local Lorentz-invariance (LLI) have been conducted with precision spectroscopy in trapped ions. We here elaborate on robust radio-frequency composite-pulse spectroscopy at second long coherence times in the magnetic sublevels of the long-lived $^{2}F_{7/2}$ state of a trapped $^{172}$Yb$^{+}$ ion which is scalable to spatially extended multi-ion systems. We compare two Ramsey-type composite rf pulse sequences, a GSE sequence and a UR10 that decouple the energy levels from magnetic field noise, enabling robust and accurate spectroscopy. Both sequences are characterized theoretically and experimentally in the spin-$1/2$\ $^{2}S_{1/2}$ electronic ground state of $^{172}$Yb$^+$ and results show that the UR10 sequence is 38 (13) times more robust against pulse duration (frequency detuning) errors than the GSE sequence. We extend our simulations to the eight-level manifold of the $^2F_{7/2}$ state, which is highly sensitive to a possible violation of LLI, and show that the UR10 sequence can be used for high-fidelity Ramsey spectroscopy in noisy environments. The UR10 sequence is implemented experimentally in the $^2F_{7/2}$ manifold and a coherent signal of up to 2.5\,s is reached. In reference we have implemented this sequence and used it to perform the most stringent test of LLI in the electron-photon sector to date with a single Yb$^{+}$ ion. Due to the high robustness of the UR10 sequence, it can be applied on larger ion crystals to improve tests of Lorentz symmetry further. We demonstrate that the sequence can also be used to extract the quadrupole moment of the meta-stable $^{2}F_{7/2}$ state, obtaining a value of $Θ\,=\,-0.0298(38)\,ea^{2}_{0}$ which is in agreement with the value deduced from clock measurements.

physics.atom-ph↗

arXiv2025

High-accuracy multi-ion spectroscopy with mixed-species Coulomb crystals

Multi-ion optical clocks offer the possibility of overcoming the low signal-to-noise ratio of single-ion clocks, while still providing low systematic uncertainties. We present simultaneous spectroscopy of up to four ${}^{115}$In${}^+$ clock ions in a linear Coulomb crystal, sympathetically cooled with ${}^{172}$Yb${}^+$ ions. In first clock comparisons, we see agreement below $1\times10^{-17}$ with results obtained using a single In${}^+$ ion, for which we have evaluated the systematic uncertainty to be $2.5\times10^{-18}$. Operation with four clock ions reduces the instability from $1.6\times10^{-15}/\sqrt{t/(1\;\mathrm{s})}$ to $9.2\times10^{-16}/\sqrt{t/(1\;\mathrm{s})}$. We derive a model for decay-related dead time during state preparation, which matches the observed scaling of instability with clock ion number $N$, and indicates that $1/\sqrt{N}$ scaling can be achieved with the addition of a repump laser.

physics.atom-ph↗

arXiv2025

$^{115}$In$^+$-$^{172}$Yb$^+$ Coulomb crystal clock with $2.5\times10^{-18}$ systematic uncertainty

We present a scalable mixed-species Coulomb crystal clock based on the $^1S_0$ $\leftrightarrow$ $^3P_0$ transition in $^{115}$In$^+$. $^{172}$Yb$^+$ ions are co-trapped and used for sympathetic cooling. Reproducible interrogation conditions for mixed-species Coulomb crystals are ensured by a conditional preparation sequence with permutation control. We demonstrate clock operation with a 1In$^+$-3Yb$^+$ crystal, achieving a relative systematic uncertainty of $2.5\times10^{-18}$ and a relative frequency instability of $1.6\times10^{-15}/\sqrt{τ/1\;\mathrm{s}}$. We report on absolute frequency measurements with an uncertainty of $1.3\times10^{-16}$ and optical frequency comparisons with clocks based on $^{171}$Yb$^+$ (E3) and $^{87}$Sr. With a fractional uncertainty of $4.4\times10^{-18}$, the former is - to our knowledge - the most accurate frequency ratio value reported to date. For the $^{115}$In$^+$/$^{87}$Sr ratio, we improve upon the best previous measurement by more than an order of magnitude. We also demonstrate operation with four $^{115}$In$^+$ clock ions, which reduces the instability to $9.2\times10^{-16}/\sqrt{τ/1\;\mathrm{s}}$.

physics.atom-ph↗

arXiv2024

Domain formation and structural stabilities in mixed-species Coulomb crystals induced by sympathetically cooled highly charged ions

There is a growing interest in high-precision spectroscopy and frequency metrology for fundamental studies using sympathetically cooled highly charged ions (HCIs) embedded in Coulomb crystals of laser-cooled ions. In order to understand how their strong repulsion affects the crystal structure and dynamics, we study the thermal motion and rearrangement of small mixed linear and homogeneous crystals by both measurements and simulations. Co-crystallized HCIs form superlattices and divide the crystal into domains, where different reordering rates, melting points and localized phase transitions are observed due to decoupling of motional modes across boundaries. These results improve our understanding of homogeneous and inhomogeneous ion strings over a wide range of charge-to-mass ratios. This allows us to test our own simulations of the dynamic behavior of ion strings and gives us confidence in their suitability for applications related to quantum simulation as well as computing and the search for new physics.

physics.atom-ph↗

arXiv2023

Bichromatic UV detection system for atomically-resolved imaging of ions

We present a compact and bichromatic imaging system, located outside of the vacuum chamber of a trapped ion apparatus, that collects the fluorescence of 230.6 nm and 369.5 nm photons simultaneously on a shared EMCCD camera. The system contains two lens doublets, consisting of a sphere and an asphere. It provides a numerical aperture of 0.45 and 0.40 at 230.6 nm and 369.5 nm, respectively, and enables spatially resolved state detection with a large field of view of 300 $μ$m for long $^{115}$In$^+$/$^{172}$Yb$^+$ Coulomb crystals. Instead of diffraction limited imaging for one wavelength, the focus in this system is on simultaneous single-ion resolved imaging of both species over a large field with special attention to the deep UV wavelength (230.6 nm) and the low scattering rate of In$^+$ ions. The introduced concept is applicable to other dual-species applications.

physics.atom-ph↗

arXiv2023

Heat transport in a Coulomb ion crystal with a topological defect

The thermodynamics of low-dimensional systems departs significantly from phenomenologically deducted macroscopic laws. Particular examples, not yet fully understood, are provided by the breakdown of Fourier's law and the ballistic transport of heat. Low-dimensional trapped ion systems provide an experimentally accessible and well-controlled platform for the study of these problems. In our work, we study the transport of thermal energy in low-dimensional trapped ion crystals, focusing in particular on the influence of the Aubry-like transition that occurs when a topological defect is present in the crystal. We show that the transition significantly hinders efficient heat transport, being responsible for the rise of a marked temperature gradient in the non-equilibrium steady state. Further analysis reveals the importance of the motional eigenfrequencies of the crystal.

physics.atom-ph↗

arXiv2023

Sub-kelvin temperature management in ion traps for optical clocks

The uncertainty of the ac Stark shift due to thermal radiation represents a major contribution to the systematic uncertainty budget of state-of-the-art optical atomic clocks. In the case of optical clocks based on trapped ions, the thermal behavior of the rf-driven ion trap must be precisely known. This determination is even more difficult when scalable linear ion traps are used. Such traps enable a more advanced control of multiple ions and have become a platform for new applications in quantum metrology, simulation and computation. Nevertheless, their complex structure makes it more difficult to precisely determine its temperature in operation and thus the related systematic uncertainty. We present here scalable linear ion traps for optical clocks, which exhibit very low temperature rise under operation. We use a finite-element model refined with experimental measurements to determine the thermal distribution in the ion trap and the temperature at the position of the ions. The trap temperature is investigated at different rf-drive frequencies and amplitudes with an infrared camera and integrated temperature sensors. We show that for typical trapping parameters for $\mathrm{In}^{+}$, $\mathrm{Al}^{+}$, $\mathrm{Lu}^{+}$, $\mathrm{Ca}^{+}$, $\mathrm{Sr}^{+}$ or $\mathrm{Yb}^{+}$ ions, the temperature rise at the position of the ions resulting from rf heating of the trap stays below 700 mK and can be controlled with an uncertainty on the order of a few 100 mK maximum.

physics.atom-ph↗

arXiv2023

Systematic study of tunable laser cooling for trapped-ion experiments

We report on a comparative analysis of quenched sideband cooling in trapped ions. We introduce a theoretical approach for time-efficient simulation of the temporal cooling characteristics and derive the optimal conditions providing fast laser cooling into the ion's motional ground state. The simulations were experimentally benchmarked with a single $^{172}$Yb$^+$ ion confined in a linear Paul trap. Sideband cooling was carried out on a narrow quadrupole transition, enhanced with an additional clear-out laser for controlling the effective linewidth of the cooling transition. Quench cooling was thus for the first time studied in the resolved sideband, intermediate and semi-classical regime. We discuss the non-thermal distribution of Fock states during laser cooling and reveal its impact on time dilation shifts in optical atomic clocks.

physics.atom-ph↗

arXiv2022

Evaluation of a $^{88}$Sr$^+$ optical clock with a direct measurement of the blackbody radiation shift and determination of the clock frequency

We report on an evaluation of an optical clock that uses the $\phantom{}^2S_{1/2} \rightarrow \phantom{}^2D_{5/2}$ transition of a single $^{88}$Sr$^+$ ion as the reference. In contrast to previous work, we estimate the effective temperature of the blackbody radiation that shifts the reference transition directly during operation from the corresponding frequency shift and the well-characterized sensitivity to thermal radiation. We measure the clock output frequency against an independent $^{171}$Yb$^+$ ion clock, based on the $\phantom{}^2S_{1/2} (F=0) \rightarrow \phantom{}^2F_{7/2} (F=3)$ electric octupole (E3) transition, and determine the frequency ratio with a total fractional uncertainty of $2.3\times 10^{-17}$. Relying on a previous measurement of the $^{171}$Yb$^+$ (E3) clock frequency, we find the absolute frequency of the $^{88}$Sr$^+$ clock transition to be $444779044095485.271(59)\,\text{Hz}$. Our result reduces the uncertainty by a factor of $3$ compared to the previously most accurate measurement and may help to resolve so far inconsistent determinations of this value. We also show that for three simultaneously interrogated $^{88}$Sr$^+$ ions, the increased number causes the expected improvement of the short-term frequency instability of the optical clock without degrading its systematic uncertainty.

physics.atom-ph↗

arXiv2022

Ab initio quantum theory of mass defect and time dilation in trapped-ion optical clocks

We derive a Hamiltonian for the external and internal dynamics of an electromagnetically bound, charged two-particle system in external electromagnetic and gravitational fields, including leading-order relativistic corrections. We apply this Hamiltonian to describe the relativistic coupling of the external and internal dynamics of cold ions in Paul traps, including the effects of micromotion, excess micromotion, and trap imperfections. This provides a systematic and fully quantum-mechanical treatment of relativistic frequency shifts in atomic clocks based on single trapped ions. Our approach reproduces well-known formulas for the second-order Doppler shift for thermal states, which were previously derived on the basis of semiclassical arguments. We complement and clarify recent discussions in the literature on the role of time dilation and mass defect in ion clocks.

physics.atom-ph↗

arXiv2022

Probe field ellipticity-induced shift in an atomic clock

We investigate the probe field induced shift for atomic lattice-based and ion-trap clocks, which can be considered as a near resonant ac-Stark shift, connected to the Zeeman structure of atomic levels and their splitting in a dc magnetic field. This shift arises from possible residual ellipticity in the polarization of the probe field and uncertainty in the magnetic field orientation. Such a shift can have an arbitrary sign and, for some experimental conditions, can reach the fractional value of the order of 10$^{-18}$-10$^{-19}$, i.e., it is not negligible. Thus, it should be taken into account in the uncertainty budgets for the modern ultra-precise atomic clocks. In addition, it is shown that when using hyper-Ramsey spectroscopy, this shift can be reduced to a level much lower than $10^{-19}$.

physics.atom-ph↗

arXiv2021

Quantum nanofriction in trapped ion chains with a topological defect

Trapped ion systems constitute a well controllable scenario for the study and emulation of nanofriction, and in particular of Frenkel-Kontorova-like models. This is in particular the case when a topological defect is created in a zigzag ion Coulomb crystal, which results in an Aubry transition from free sliding to pinned phase as a function of the trap aspect ratio. We explore the quantum effects of the Aubry transition by means of an effective simplified model, in which the defect is treated like a single quantum particle that experiences an effective Peierls-Nabarro potential and a position-dependent mass. We demonstrate the relevance of quantum tunneling in a finite range of aspect ratios close the critical point, showing that the quantum effects may be observed in the kink dynamics for sufficiently low temperatures. Finally, we discuss the requirements to reveal quantum effects at the Aubry transition in future experiments on trapped ions.

cond-mat.quant-gas↗

arXiv2021

Motional heating of spatially extended ion crystals

We study heating of motional modes of a single ion and of extended ion crystals trapped in a linear radio frequency (rf) Paul trap with a precision of $Δ\dot{\bar{n}} \approx 0.2 $ phonons s$^{-1}$. Single-ion axial and radial heating rates are consistent and electric field noise has been stable over the course of four years. At a secular frequency of $ω_\mathrm{sec}=2π\times620$ kHz, we measure $\dot{\bar{n}} = 0.56(6)$ phonons s$^{-1}$ per ion for the center-of-mass (com) mode of linear chains of up to eleven ions and observe no significant heating of the out-of-phase (oop) modes. By displacing the ions away from the nodal line, inducing excess micromotion, rf noise heats the com mode quadratically as a function of radial displacement $r$ by $\dot{\bar{n}}(r)/ r^2 = 0.89(4)$ phonons s$^{-1}$ $μ$m$^{-2}$ per ion, while the oop modes are protected from rf-noise induced heating in linear chains. By changing the quality factor of the resonant rf circuit from $Q=542$ to $Q=204$, we observe an increase of rf noise by a factor of up to 3. We show that the rf-noise induced heating of motional modes of extended crystals also depends on the symmetry of the crystal and of the mode itself. As an example, we consider several 2D and 3D crystal configurations. Heating rates of up to 500 phonons s$^{-1}$ are observed for individual modes, giving rise to a total kinetic energy increase and thus a fractional time dilation shift of up to $-0.3\times 10^{-18}$ s$^{-1}$ of the total system. In addition, we detail on how the excitation probability of the individual ions is reduced and decoherence is increased due to the Debye-Waller effect.

physics.atom-ph↗

arXiv2021

Creation of double-well potentials in a surface-electrode trap towards a nanofriction model emulator

We demonstrate a microfabricated surface-electrode ion trap that is applicable as a nanofriction emulator and studies of many-body dynamics of interacting systems. The trap enables both single-well and double-well trapping potentials in the radial direction, where the distance between the two potential wells can be adjusted by the applied RF voltage. In the double-well configuration, parallel ion strings can be formed, which is a suitable system for the emulation of the Frenkel-Kontorova (FK) model. We derive the condition under which the trap functions as a FK model emulator. The trap is designed so that the Coulomb interaction between two ion strings becomes significant. We report on the microfabrication process for such downsized trap electrodes and experimental results of single-well and double-well operation with calcium ions. With the trap demonstrated in this work we can create atomically accessible, self-assembled Coulomb systems with a wide tuning range of the corrugation parameter in the FK model. This makes it a promising system for quantum simulations, but also for the study of nanofriction in one and higher dimensional systems.

quant-ph↗

arXiv2019

Energy localization in interacting atomic chains with topological solitons

Topological defects in low-dimensional non-linear systems feature a sliding-to-pinning transition of relevance for a variety of research fields, ranging from biophysics to nano- and solid-state physics. We find that the dynamics after a local excitation results in a highly-non-trivial energy transport in the presence of a topological soliton, characterized by a strongly enhanced energy localization in the pinning regime. Moreover, we show that the energy flux in ion crystals with a topological defect can be sensitively regulated by experimentally accessible environmental parameters. Whereas, third-order non-linear resonances can cause an enhanced long-time energy delocalization, robust energy localization persists for distinct parameter ranges even for long evolution times and large local excitations.

quant-ph↗

arXiv2019

Towards a Transportable Aluminium Ion Quantum Logic Optical Clock

With the advent of optical clocks featuring fractional frequency uncertainties on the order of $10^{-17}$ and below, new applications such as chronometric levelling with few-cm height resolution emerge. We are developing a transportable optical clock based on a single trapped aluminium ion, which is interrogated via quantum logic spectroscopy. We employ singly-charged calcium as the logic ion for sympathetic cooling, state preparation and readout. Here we present a simple and compact physics and laser package for manipulation of $^{40}\mathrm{Ca}^+$. Important features are a segmented multi-layer trap with separate loading and probing zones, a compact titanium vacuum chamber, a near-diffraction-limited imaging system with high numerical aperture based on a single biaspheric lens, and an all-in-fiber $^{40}\mathrm{Ca}^+$ repump laser system. We present preliminary estimates of the trap-induced frequency shifts on $^{27}\mathrm{Al}^+$, derived from measurements with a single calcium ion. The micromotion-induced second-order Doppler shift for $^{27}\mathrm{Al}^+$ has been determined to be \sods and the black-body radiation shift is $δν_\mathrm{BBR}/ν=(-4.0\pm0.4)\times10^{-18}$. Moreover, heating rates of 30 (7) quanta per second at trap frequencies of $ω_\mathrm{rad,Ca+} \approx2π\times2.5\,\mathrm{MHz}$ ($ω_\mathrm{ax,Ca+} \approx2π\times1.5\,\mathrm{MHz}$) in radial (axial) direction have been measured, enabling interrogation times of a few hundreds of milliseconds.

physics.atom-ph↗