arXiv subjects

T. Fukushima

Publications and source records attributed to T. Fukushima.

6 recordsLinked to original sources

arXiv2018

Anomalous Hall conductivity and electronic structures of Si-substituted Mn$_{2}$CoAl epitaxial films

We study anomalous Hall conductivity ($σ$$_{\rm AHC}$) and electronic band structures of Si-substituted Mn$_{2}$CoAl (Mn$_{2}$CoAl$_{1-x}$Si$_{x}$). First-principles calculations reveal that the electronic band structure is like a spin-gapless system even after substituting a quaternary element of Si for Al up to $x = $0.2 in Mn$_{2}$CoAl$_{1-x}$Si$_{x}$. This means that the Si substitution enables the Fermi level shift without largely changing the electronic structures in Mn$_{2}$CoAl. By using molecular beam epitaxy (MBE) techniques, Mn$_{2}$CoAl$_{1-x}$Si$_{x}$ epitaxial films can be grown, leading to the systematic control of $x$ (0 $\le$ $x$ $\le$ 0.3). In addition to the electrical conductivity, the values of $σ$$_{\rm AHC}$ for the Mn$_{2}$CoAl$_{1-x}$Si$_{x}$ films are similar to those in Mn$_{2}$CoAl films shown in previous reports. We note that a very small $σ$$_{\rm AHC}$ of $\sim$ 1.1 S/cm is obtained for $x =$ 0.225 and the sign of $σ$$_{\rm AHC}$ is changed from positive to negative at around $x =$ 0.25. We discuss the origin of the sign reversal of $σ$$_{\rm AHC}$ as a consequence of the Fermi level shift in MCA. Considering the presence of the structural disorder in the Mn$_{2}$CoAl$_{1-x}$Si$_{x}$ films, we can conclude that the small value and sign reversal of $σ$$_{\rm AHC}$ are not related to the characteristics of spin-gapless semiconductors.

cond-mat.mtrl-sci↗

arXiv2015

Spinodal nanodecomposition in magnetically doped semiconductors

This review presents the recent progress in computational materials design, experimental realization, and control methods of spinodal nanodecomposition under three- and two-dimensional crystal-growth conditions in spintronic materials, such as magnetically doped semiconductors. The computational description of nanodecomposition, performed by combining first-principles calculations with kinetic Monte Carlo simulations, is discussed together with extensive electron microscopy, synchrotron radiation, scanning probe, and ion beam methods that have been employed to visualize binodal and spinodal nanodecomposition (chemical phase separation) as well as nanoprecipitation (crystallographic phase separation) in a range of semiconductor compounds with a concentration of transition metal (TM) impurities beyond the solubility limit. The role of growth conditions, co-doping by shallow impurities, kinetic barriers, and surface reactions in controlling the aggregation of magnetic cations is highlighted. According to theoretical simulations and experimental results the TM-rich regions appear either in the form of nanodots (the {\em dairiseki} phase) or nanocolumns (the {\em konbu} phase) buried in the host semiconductor. Particular attention is paid to Mn-doped group III arsenides and antimonides, TM-doped group III nitrides, Mn- and Fe-doped Ge, and Cr-doped group II chalcogenides, in which ferromagnetic features persisting up to above room temperature correlate with the presence of nanodecomposition and account for the application-relevant magneto-optical and magnetotransport properties of these compounds. Finally, it is pointed out that spinodal nanodecomposition can be viewed as a new class of bottom-up approach to nanofabrication.

cond-mat.mtrl-sci↗

arXiv2015

Computational materials design of attractive Fermion system with large negative effective $U$ in the hole-doped Delafossite of CuAlO$_2$, AgAlO$_2$ and AuAlO$_2$

In order to realize super-high-critical temperature $(T_c)$ superconductors ($T_c$>1,000 K) based on general design rules for negative effective $U$ $(U_{eff})$ systems by controlling purely-electronic and attractive Fermion mechanisms, we perform computational materials design for the negative $U_{eff}$ system in hole-doped two-dimensional (2D) Delafossite CuAlO$_2$, AgAlO$_2$ and AuAlO$_2$ from ${\it ab\ initio}$ calculations. It is found that the large negative $U_{eff}$ in the hole-doped attractive Fermion systems for CuAlO$_2$ ($U_{eff}$ = -4.53 eV), AgAlO$_2$ ($U_{eff}$ = -4.88 eV), AuAlO$_2$ ($U_{eff}$ = -4.14 eV). These values are 10 times larger than that in hole-doped three-dimensional (3D) CuFeS$_2$ ($U_{eff}$ = -0.44 eV). For future calculations of the $T_c$ and phase diagram by quantum Monte Carlo simulations, we propose the negative $U_{eff}$ Hubbard model with the anti-bonding single $π$-band model for CuAlO$_2$, AgAlO$_2$ and AuAlO$_2$ by using the parameters obtained from ${\it ab\ initio}$ electronic structure calculations. The behavior of $T_c$ in the 2D Delafossite of CuAlO$_2$, AgAlO$_2$ and AuAlO$_2$ and 3D Chalcopyrite of CuFeS$_2$ shows the interesting chemical trend, ${\it i.e.,}$ $T_c$ increases exponentially in the weak coupling regime $|U_{eff}| < W$ ($\sim$ 2 eV) (where $W$ is the band width of Hubbard model) for the hole-doped CuFeS$_2$, and then $T_c$ goes through a maximum when $|U_{eff}| \sim W$ (2.8 eV, 3.5 eV) for the hole-doped AgAlO$_2$ and AuAlO$_2$, and finally $T_c$ decreases with increasing $|U_{eff}|$ in the strong coupling regime, where $|U_{eff}| > W$ (1.7 eV), for the hole-doped CuAlO$_2$. In this strong coupling regime, one can expect that $T_c$ = 1,000 $\sim$ 2,000 K by assuming the relation of the very strong coupling as $2Δ/ k_{\rm B}T_c$ = 50 $\sim$100 and the superconducting gap $Δ\sim |U_{eff}|$ = 4.53 eV $\sim$ 50,000 K.

cond-mat.supr-con↗

arXiv2011

Large ferroelectric polarization in the new double perovskite NaLaMnWO$_{6}$ induced by non-polar instabilities

Based on density functional theory calculations and group theoretical analysis, we have studied NaLaMnWO$_{6}$ compound which has been recently synthesized [Phys. Rev. B 79, 224428 (2009)] and belongs to the $AA'BB'{\rm O}_{6}$ family of double perovskites. At low temperature, the structure has monoclinic $P2_{1}$ symmetry, with layered ordering of the Na and La ions and rocksalt ordering of Mn and W ions. The Mn atoms show an antiferromagnetic (AFM) collinear spin ordering, and the compound has been reported as a potential multiferroic. By comparing the low symmetry structure with a parent phase of $P4/nmm$ symmetry, two distortion modes are found dominant. They correspond to MnO$_{6}$ and WO$_{6}$ octahedron \textit{tilt} modes, often found in many simple perovskites. While in the latter these common tilting instabilities yield non-polar phases, in NaLaMnWO$_{6}$ the additional presence of the $A$-$A^{'}$ cation ordering is sufficient to make these rigid unit modes as a source of the ferroelectricity. Through a trilinear coupling with the two unstable tilting modes, a significant polar distortion is induced, although the system has no intrinsic polar instability. The calculated electric polarization resulting from this polar distortion is as large as $\sim$ 16 $μ{\rm C/cm^{2}}$. Despite its secondary character, this polarization is coupled with the dominant tilting modes and its switching is bound to produce the switching of one of two tilts, enhancing in this way a possible interaction with the magnetic ordering. The transformation of common non-polar purely steric instabilities into sources of ferroelectricity through a controlled modification of the parent structure, as done here by the cation ordering, is a phenomenon to be further explored.

cond-mat.mtrl-sci↗

arXiv2005

A novel type of proximity focusing RICH counter with multiple refractive index aerogel radiator

A proximity focusing ring imaging Cherenkov detector, with the radiator consisting of two or more aerogel layers of different refractive indices, has been tested in 1-4 GeV/c pion beams at KEK. Essentially, a multiple refractive index aerogel radiator allows for an increase in Cherenkov photon yield on account of the increase in overall radiator thickness, while avoiding the simultaneous degradation in single photon angular resolution associated with the increased uncertainty of the emission point. With the refractive index of consecutive layers suitably increasing in the downstream direction, one may achieve overlapping of the Cherenkov rings from a single charged particle. In the opposite case of decreasing refractive index, one may obtain well separated rings. In the former combination an approximately 40% increase in photon yield is accompanied with just a minor degradation in single photon angular resolution. The impact of this improvement on the pion/kaon separation at the upgraded Belle detector is discussed.

physics.ins-det↗

arXiv2003

The IAU 2000 resolutions for astrometry, celestial mechanics and metrology in the relativistic framework: explanatory supplement

This paper discusses the IAU Resolutions B1.3, B1.4, B1.5 and B1.9 (2000) that were adopted during the 24th General Assembly in Manchester, 2000 and provides details and explanations for these Resolutions. It is explained why they present significant progress over the corresponding IAU 1991 Resolutions and why they are necessary in the light of present accuracies in astrometry, celestial mechanics and metrology. In fact most of these Resolutions are consistent with astronomical models and software already in use. The metric tensors and gravitational potentials of both the Barycentric Celestial Reference System and Geocentric Celestial Reference System are defined and discussed. The necessity and relevance of the two celestial reference systems are explained. The transformations of coordinates and gravitational potentials are discussed. Potential coefficients parameterizing the post-Newtonian gravitational potentials are expounded. Simplified versions of the time transformations suitable for modern clock accuracies are elucidated. Various approximations used in the Resolutions are explicated and justified. Some models (e.g. for higher spin moments) that serve the purpose for estimating orders of magnitude have actually never been published before.

astro-ph↗