arXiv subjects

T. G. Rappoport

Publications and source records attributed to T. G. Rappoport.

18 recordsLinked to original sources

arXiv2026

Phase-selective orbital-charge conversion in $\mathrm{MoTe_2}$

Two-dimensional transition metal dichalcogenides (TMDs) have emerged as promising materials for spin--orbitronics owing to their strong spin--orbit coupling and rich electronic phases. However, their orbital transport properties remain largely unexplored. Here, we demonstrate that the orbitronic response of $\mathrm{MoTe_2}$ is governed by a thickness-driven structural phase transition. RF-sputtered $\mathrm{MoTe_2}$ thin films exhibit a crossover at a critical thickness of approximately $4.5\,\mathrm{nm}$, stabilizing in the metallic $1T^\prime$ phase below this threshold and in the semiconducting $2H$ phase above it. Raman spectroscopy and scanning tunneling spectroscopy (STS) confirm the structural and electronic transition, revealing gapless behavior in ultrathin films and a finite band gap in thicker samples. Spin-pumping measurements detect an additional transverse charge-conversion signal exclusively in metallic $1T^\prime$-$\mathrm{MoTe_2}$, in agreement with first-principles calculations that identify a dominant orbital Rashba--Edelstein response as the underlying conversion mechanism.

cond-mat.mtrl-sci↗

arXiv2020

Topological Photonic Tamm-States and the Su-Schrieffer-Heeger Model

In this paper we study the formation of topological Tamm states at the interface between a semi-infinite one-dimensional photonic-crystal and a metal. We show that when the system is topologically non-trivial there is a single Tamm state in each of the band-gaps, whereas if it is topologically trivial the band-gaps host no Tamm states. We connect the disappearance of the Tamm states with a topological transition from a topologically non-trivial system to a topologically trivial one. This topological transition is driven by the modification of the dielectric functions in the unit cell. Our interpretation is further supported by an exact mapping between the solutions of Maxwell's equations and the existence of a tight-binding representation of those solutions. We show that the tight-binding representation of the 1D photonic crystal, based on Maxwell's equations, corresponds to a Su-Schrieffer-Heeger-type model (SSH-model) for each set of pairs of bands. Expanding this representation near the band edge we show that the system can be described by a Dirac-like Hamiltonian. It allows one to characterize the topology associated with the solution of Maxwell's equations via the winding number. In addition, for the infinite system, we provide an analytical expression for the photonic bands from which the band-gaps can be computed.

cond-mat.mes-hall↗

arXiv2016

Numerical calculation of the Casimir-Polder interaction between a graphene sheet with vacancies and an atom

In this work the Casimir{Polder interaction energy between a rubidium atom and a disordered graphene sheet is investigated beyond the Dirac cone approximation by means of accurate real-space calculations. As a model of defected graphene, we consider a tight-binding model of Π-electrons on a honeycomb lattice with a small concentration of point defects. The optical response of the graphene sheet is evaluated with full spectral resolution by means of exact Chebyshev polynomial expansions of the Kubo formula in large lattices with in excess of ten million atoms. At low temperatures, the optical response of defected graphene is found to display two qualitatively distinct behavior with a clear transition around non-zero Fermi energy, μ~μ*. In the vicinity of the Dirac point, the imaginary part of optical conductivity is negative for low frequencies while the real part is strongly suppressed. On the other hand, for high doping, it has the same features found in the Drude model within the Dirac cone approximation, namely, a Drude peak at small frequencies and a change of sign in the imaginary part above the interband threshold ω> 2μ. These characteristics translate into a non-monotonic behavior of the Casimir{Polder interaction energy with very small variation with doping in the vicinity of the neutrality point while having the same form of the interaction calculated with Drude's model at high electronic density.

cond-mat.mes-hall↗

arXiv2016

Magnetic effects in sulfur-decorated graphene

The interaction between two different materials can present novel phenomena that are quite different from the physical properties observed when each material stands alone. Strong electronic correlations, such as magnetism and superconductivity, can be produced as the result of enhanced Coulomb interactions between electrons. Two-dimensional materials are powerful candidates to search for the novel phenomena because of the easiness of arranging them and modifying their properties accordingly. In this work, we report magnetic effects of graphene, a prototypical non-magnetic two-dimensional semi-metal, in the proximity with sulfur, a diamagnetic insulator. In contrast to the well-defined metallic behaviour of clean graphene, an energy gap develops at the Fermi energy for the graphene/sulfur compound with decreasing temperature. This is accompanied by a steep increase of the resistance, a sign change of the slope in the magneto-resistance between high and low fields, and magnetic hysteresis. A possible origin of the observed electronic and magnetic responses is discussed in terms of the onset of low-temperature magnetic ordering. These results provide intriguing insights on the search for novel quantum phases in graphene-based compounds.

cond-mat.mtrl-sci↗

arXiv2014

Extrinsic spin Hall effect induced by resonant skew scattering in graphene

We show that the extrinsic spin Hall effect can be engineered in monolayer graphene by decoration with small doses of adatoms, molecules, or nanoparticles originating local spin-orbit perturbations. The analysis of the single impurity scattering problem shows that intrinsic and Rashba spin-orbit local couplings enhance the spin Hall effect via skew scattering of charge carriers in the resonant regime. The solution of the transport equations for a random ensemble of spin-orbit impurities reveals that giant spin Hall currents are within the reach of the current state of the art in device fabrication. The spin Hall effect is robust with respect to thermal fluctuations and disorder averaging.

cond-mat.mes-hall↗

arXiv2011

Magnetic exchange mechanism for electronic gap opening in graphene

We show within a local self-consistent mean-field treatment that a random distribution of magnetic adatoms can open a robust gap in the electronic spectrum of graphene. The electronic gap results from the interplay between the nature of the graphene sublattice structure and the exchange interaction between adatoms.The size of the gap depends on the strength of the exchange interaction between carriers and localized spins and can be controlled by both temperature and external magnetic field. Furthermore, we show that an external magnetic field creates an imbalance of spin-up and spin-down carriers at the Fermi level, making doped graphene suitable for spin injection and other spintronic applications.

cond-mat.str-el↗

arXiv2011

Kondo Quantum Criticality of Magnetic Adatoms in Graphene

We examine the exchange Hamiltonian for magnetic adatoms in graphene with localized inner shell states. On symmetry grounds, we predict the existence of a class of orbitals that lead to a distinct class of quantum critical points in graphene, where the Kondo temperature scales as $T_{K}\propto|J-J_{c}|^{1/3}$ near the critical coupling $J_{c}$, and the local spin is effectively screened by a \emph{super-ohmic} bath. For this class, the RKKY interaction decays spatially with a fast power law $\sim1/R^{7}$. Away from half filling, we show that the exchange coupling in graphene can be controlled across the quantum critical region by gating. We propose that the vicinity of the Kondo quantum critical point can be directly accessed with scanning tunneling probes and gating.

cond-mat.str-el↗

arXiv2010

Ion-beam modification of the magnetic properties of GaMnAs epilayers

We study the controlled introduction of defects in GaMnAs by irradiating the samples with energetic ion beams, which modify the magnetic properties of the DMS. Our study focuses on the low-carrier-density regime, starting with as-grown GaMnAs films and decreasing even further the number of carriers, through a sequence of irradiation doses. We did a systematic study of magnetization as a function of temperature and of the irradiation ion dose. We also performed in-situ room temperature resistivity measurements as a function of the ion dose. We observe that both magnetic and transport properties of the samples can be experimentally manipulated by controlling the ion-beam parameters. For highly irradiated samples, the magnetic measurements indicate the formation of magnetic clusters together with a transition to an insulating state. The experimental data are compared with mean-field calculations for magnetization. The independent control of disorder and carrier density in the calculations allows further insight on the individual role of this two factors in the ion-beam-induced modification of GaMnAs.

cond-mat.dis-nn↗

arXiv2009

Magnetism and magnetotransport in disordered graphene

We perform Monte Carlo simulations to study the interplay of structural and magnetic order in single layer graphene covered with magnetic adatoms. We propose that the presence of ripples in the graphene structure can lead to clustering of the adatoms and to a variety of magnetic states such as super-paramagnetism, antiferromagnetism, ferromagnetism and spin glass behavior. We derive the magnetization hysteresis and also the magnetoresistance curves in the variable range hopping regime, which can provide experimental signatures for ripple induced clustering and magnetism. We propose that the magnetic states in graphene can be controlled by gate voltage and coverage fraction.

cond-mat.str-el↗

arXiv2009

Superconducting transition in Pb/Co nanocomposites: effect of Co volume fraction and external magnetic field

Pb films embedded with homogeneously distributed cobalt (Co) nanoparticles (mean size 4.5 nm) have been prepared. Previous transport investigations have shown that Co particles induce spontaneous vortices below the superconducting transition temperature (T$_{c}$) in zero external magnetic field. In this paper we study in detail the influence of the Co volume franction and an external magnetic field on the superconducting transition in such composites. The large difference in T$_c$-reduction between the as-prepared and annealed samples can be attributed to the different superconducting coherence lengths and the resulting different diameters of the spontaneous vortices in these samples.

cond-mat.supr-con↗

arXiv2008

Controlled switching between paramagnetic and diamagnetic Meissner effect in Pb/Co nanocomposites

A hybrid system which consists of a superconducting (SC) Pb film (100 nm thickness) containing $\sim$1 vol% single domain ferromagnetic (FM) Co particles of mean-size $\sim$4.5 nm reveal unusual magnetic properties: (i) a controlled switching between the usual diamagnetic and the unusual paramagnetic Meissner effect in field cooling as well as in zero-field cooling experiments (ii) amplification of the positive magnetization when the sample enters the SC state below T$_c$. These experimental findings can be explained by the formation of spontaneous vortices and the possible alignment of these vortices due to the foregoing alignment of the Co particle FM moments by an external magnetic field.

cond-mat.supr-con↗

arXiv2008

Spontaneous vortex phases in ferromagnet-superconductor nanocomposites

The interplay between superconductivity and magnetism gives rise to many intriguing and exciting phenomena. In this Letter we report about a novel manifestation of this interplay: a temperature induced phase transition between different spontaneous vortex phases in lead superconducting films with embedded magnetic nanoparticles. Unlike common vortices in superconductors the vortex phase appears without any applied magnetic field. The vortices nucleate exclusively due to the stray field of the magnetic nanoparticles, which serve the dual role of providing the internal field and simultaneously acting as pinning centers. As in usual superconductors, one can move the spontaneous vortices with an applied electric current. Transport measurements reveal dynamical phase transitions that depend on temperature (T) and applied field (H) and support the obtained (H-T) phase diagram. In particular, we used a scaling analysis to characterize a transition from a liquid to a novel disordered solid resembling a vortex glass.

cond-mat.supr-con↗

arXiv2006

Experimental observation of quantum entanglement in low dimensional spin systems

We report macroscopic magnetic measurements carried out in order to detect and characterize field-induced quantum entanglement in low dimensional spin systems. We analyze the pyroborate MgMnB_2O_5 and the and the warwickite MgTiOBO_3, systems with spin 5/2 and 1/2 respectively. By using the magnetic susceptibility as an entanglement witness we are able to quantify entanglement as a function of temperature and magnetic field. In addition, we experimentally distinguish for the first time a random singlet phase from a Griffiths phase. This analysis opens the possibility of a more detailed characterization of low dimensional materials.

cond-mat.str-el↗

arXiv2005

Zero- and one-dimensional magnetic traps for quasi-particles

We investigate the possibility of trapping quasi-particles possessing spin degree of freedom in hybrid structures. The hybrid system we are considering here is composed of a semi-magnetic quantum well placed a few nanometers below a ferromagnetic micromagnet. We are interested in two different micromagnet shapes: cylindrical (micro-disk) and rectangular geometry. We show that in the case of a micro-disk, the spin object is localized in all three directions and therefore zero-dimensional states are created, and in the case of an elongated rectangular micromagnet, the quasi-particles can move freely in one direction, hence one-dimensional states are formed. After calculating profiles of the magnetic field produced by the micromagnets, we analyze in detail the possible light absorption spectrum for different micromagnet thicknesses, and different distances between the micromagnet and the semimagnetic quantum well. We find that the discrete spectrum of the localized states can be detected via spatially-resolved low temperature optical measurement.

cond-mat.mtrl-sci↗

arXiv2004

Ferromagnetic/DMS hybrid structures: one- and zero-dimensional magnetic traps for quasiparticles

We investigated possibility of using local magnetic field originating from ferromagnetic island deposited on the top of semiconductor quantum well to produce zero- and one-dimensional traps for quasi-particles with spin. In particular we considered two shapes of experimentally made magnets - cylindrical and rectangular. In the case of ferromagnetic micro-disk the trap can localize spin in three dimensions, contrary to the rectangular micro-magnet which creates a trap that allows free propagation in one direction. We present in detail prediction for absorption spectrum around the main absorption edge in both type of micro-magnets.

cond-mat.mtrl-sci↗

arXiv2004

Optical response of a ferromagnetic/DMS hybrid structure

We investigate the possibility of using local magnetic fields to produce one-dimensional traps in hybrid structures for any quasiparticle possessing spin degree of freedom. We consider a system composed of a diluted magnetic semiconductor quantum well buried below a micron-sized ferromagnetic island. Localized magnetic field is produced by a rectangular ferromagnet in close proximity of a single domain phase. We make quantitative predictions for the optical response of the system as a function of distance between the micromagnet and the quantum well, electronic g-factor, and thickness of the micromagnet.

cond-mat.stat-mech↗

arXiv2003

Anomalous behavior of spin wave resonances in Ga_{1-x}Mn_{x}As thin films

We report ferromagnetic and spin wave resonance absorption measurements on high quality epitaxially grown Ga_{1-x}Mn_{x}As thin films. We find that these films exhibit robust ferromagnetic long-range order, based on the fact that up to seven resonances are detected at low temperatures, and the resonance structure survives to temperatures close to the ferromagnetic transition. On the other hand, we observe a spin wave dispersion which is linear in mode number, in qualitative contrast with the quadratic dispersion expected for homogeneous samples. We perform a detailed numerical analysis of the experimental data and provide analytical calculations to demonstrate that such a linear dispersion is incompatible with uniform magnetic parameters. Our theoretical analysis of the ferromagnetic resonance data, combined with the knowledge that strain-induced anisotropy is definitely present in these films, suggests that a spatially dependent magnetic anisotropy is the most likely reason behind the anomalous behavior observed.

cond-mat↗

arXiv2001

Role of Disorder on the Quantum Critical Point of a Model for Heavy Fermions

A zero temperature real space renormalization group (RG) approach is used to investigate the role of disorder near the quantum critical point (QCP) of a Kondo necklace (XY-KN) model. In the pure case this approach yields $J_{c}=0$ implying that any coupling $J \not = 0 $ between the local moments and the conduction electrons leads to a non-magnetic phase. We also consider an anisotropic version of the model ($X-KN$), for which there is a quantum phase transition at a finite value of the ratio between the coupling and the bandwidth, $(J/W)$. Disorder is introduced either in the on-site interactions or in the hopping terms. We find that in both cases randomness is irrelevant in the $X-KN$ model, i.e., the disorder induced magnetic-non-magnetic quantum phase transition is controlled by the same exponents of the pure case. Finally, we show the fixed point distributions $P_{J}(J/W)$ at the atractors of the disordered, non-magnetic phases.

cond-mat.dis-nn↗