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T. G. Walker

Publications and source records attributed to T. G. Walker.

At least 19 recordsLinked to original sources

Experimental observation of subabsorption

We predict and experimentally demonstrate a new type of collective (cooperative) coupling effect where a disordered atomic ensemble absorbs light with a rise-time longer (i. e., at a rate slower) than what is dictated by single-atom physics. This effect, which we name subabsorption, can be viewed as the absorptive analog of subradiance. The experiment is performed using a dilute ensemble of ultracold $^{87}$Rb atoms with a low optical depth, and time-resolving the absorption of a weak (tens of photons per pulse) resonant laser beam. In this dilute regime, the collective interaction relies on establishing dipole-dipole correlations over many atoms; i.e., the interaction is not dominated by the nearest neighbors. As a result, subabsorption is highly susceptible to motional dephasing: even a temperature increase of 60 $\mu$K is enough to completely extinguish the subabsorption signal. We also present a theoretical model whose results are in reasonable agreement with the experimental observations. The model uses density-dependent dephasing rate of the long-range dipole-dipole correlations as a single adjustable parameter. Experiment-theory comparison indicates a dephasing coefficient of $\beta/2 \pi = 4.9 \times 10^{-5}$ Hz~cm$^3$, which is more than two orders of magnitude larger than the known dipole-dipole line broadening coefficient in $^{87}$Rb.

quant-ph

Nanoscale addressing and manipulation of neutral atoms using electromagnetically induced transparency

We propose to integrate dark-state based localization techniques into a neutral atom quantum computing architecture and numerically investigate two specific schemes. The first scheme implements state-selective projective measurement by scattering photons from a specific qubit with very little cross talk on the other atoms in the ensemble. The second scheme performs a single-qubit phase gate on the target atom with an incoherent spontaneous emission probability as low as 0.01. Our numerical simulations in rubidium (Rb) atoms show that for both of these schemes a spatial resolution at the level of tens of nanometers using near-infrared light can be achieved with experimentally realistic parameters.

quant-ph

Spatial Coherence of Light in Collective Spontaneous Emission

When a quantum system is put into an excited state, it will decay back to the ground state through a process termed spontaneous emission. It is generally assumed that spontaneous emission between different individual emitters would not be coherent with each other; to produce coherent light one would need population inversion and stimulated emission. In this work, we show that an optically-thin ensemble of 11,000 radiating atoms spontaneously organize to produce spatially coherent light. The reason for this coherence is collective-coupling of the individual emitters via Dicke superradiance and subradiance (as opposed to amplification through stimulated emission).

quant-ph

An all-optical intrinsic atomic gradiometer with sub-20 fT/cm/$\sqrt{\rm Hz}$ sensitivity in a 22 $μ$T earth-scale magnetic field

In this work we demonstrate a high sensitivity atomic gradiometer capable of operation in earth-field level environments. We apply a light-pulse sequence at four times the Larmor frequency to achieve gradiometer sensitivity <20 fT/cm/$\sqrt{\rm Hz}$ at the finite field strength of 22 $μ$T. The experimental timing sequence can be tuned to the field magnitude of interest. Our one dimensional all-optical gradiometer performs a differential measurement between two regions of a single vapor cell on a 4 cm baseline. Our results pave the way for extensions to operation in higher dimensions, vector sensitivity, and more advanced gradiometers.

physics.atom-ph

Continuous Comagnetometry using Transversely Polarized Xe Isotopes

We demonstrate a transversely polarized spin-exchange pumped noble gas comagnetometer which suppresses systematic errors from longitudinal polarization. Rb atoms as well as $^{131}$Xe and $^{129}$Xe nuclei are simultaneously polarized perpendicular to a pulsed bias field. Both Xe isotopes' nuclear magnetic resonance conditions are simultaneously satisfied by frequency modulation of the pulse repetition rate. The Rb atoms detect the Xe precession. We highlight the importance of magnetometer phase shifts when performing comagnetometry. For detection of non-magnetic spin-dependent interactions the sensing bandwidth is 1 Hz, the white-noise level is 7 $μ$Hz /$\sqrt{\text{Hz}}$, and the bias stability is $\approx1$ $μ$Hz.

physics.atom-ph

Characterizing atomic magnetic gradiometers for fetal magnetocardiography

Atomic magnetometers (AMs) offer many advantages over superconducting quantum interference devices (SQUIDs) due to, among other things, having comparable sensitivity while not requiring cryogenics. One of the major limitations of AMs is the challenge of configuring them as gradiometers. We report the development of a spin-exchange relaxation free (SERF) vector atomic magnetic gradiometer with sensitivity of $3\, \rm{fT} \,{cm}^{-1}{Hz}^{-1/2}$ and common mode rejection ratio (CMRR) $> 150$ in the band from DC to 100 Hz. We introduce a background suppression figure of merit for characterizing the performance of gradiometers. It allows for optimally setting the measurement baseline, and for quickly assessing the advantage, if any, of performing a measurement in gradiometric mode. As an application, we consider the problem of fetal magnetocardiography (fMCG) detection in the presence of a large background maternal MCG signal.

physics.ins-det

Optically Polarized $^3$He

This article reviews the physics and technology of producing large quantities of highly spin-polarized, or hyperpolarized, $^3$He nuclei using spin-exchange (SEOP) and metastability-exchange (MEOP) optical pumping, and surveys applications of polarized $^3$He. Several recent developments are emphasized for each method. For SEOP, the use of spectrally narrowed lasers and Rb/K mixtures has substantially increased the achievable polarization and polarizing rate. MEOP in high magnetic fields has likewise significantly increased the pressure at which this method can be performed, and has led to the observation of a light-induced relaxation mechanism. In both methods the increased capabilities have led to more extensive study and modeling of the basic underlying physics. New unexplained dependences of relaxation on temperature and magnetic field have been discovered in SEOP cells. Applications of both methods are also reviewed, including targets for charged particle and photon beams, neutron spin filters, magnetic resonance imaging, and precision measurements.

physics.atom-ph

Coherence and Rydberg blockade of atomic ensemble qubits

We demonstrate $|W\rangle$ state encoding of multi-atom ensemble qubits. Using optically trapped Rb atoms the $T_2$ coherence time is 2.6(3) ms for $\bar N=7.6$ atoms and scales approximately inversely with the number of atoms. Strong Rydberg blockade between two ensemble qubits is demonstrated with a fidelity of $0.89(1)$ and a fidelity of $\sim \hspace{-.05cm}1.0$ when postselected on control ensemble excitation. These results are a significant step towards deterministic entanglement of atomic ensembles.

quant-ph

A Laboratory Search for a Long-Range T-odd, P-odd Interaction from Axion-Like Particles using Dual Species Nuclear Magnetic Resonance with Polarized Xe-129 and Xe-131 Gas

We place new limits on potential T- and P- violating monopole-dipole interactions between unpolarized nucleons and neutrons using dual species magnetic resonance in polarzed Xe gas. Free-induction decay transients with relaxation times ~20 s allow high precision measurements of the NMR frequencies, whose ratios cancel magnetic fluctuations. The new limits on the product gsgp improve on previous laboratory work by 2 orders of magnitude.

physics.atom-ph

Suppression of Spin-Exchange Relaxation Using Pulsed Parametric Resonance

We demonstrate that spin-exchange dephasing of Larmor precession at near-earth-scale fields is effectively eliminated by dressing the alkali-metal atom spins in a sequence of AC-coupled 2-pi pulses, repeated at the Larmor precession frequency. The contribution of spin-exchange collisions to the spectroscopic line width is reduced by a factor of the duty cycle of the pulses. We experimentally demonstrate resonant transverse pumping in magnetic fields as high as 0.1 Gauss, present experimental measurements of the suppressed spin-exchange relaxation, and show enhanced magnetometer response relative to a light-narrowed scalar magnetometer.

physics.atom-ph

Diffusive Suppression of AC-Stark Shifts in Atomic Magnetometers

In atomic magnetometers, the vector AC-Stark shift associated with circularly polarized light generates spatially varying effective magnetic fields which limit the magnetometer response and serve as sources of noise. We describe a scheme whereby optically pumping a small sub-volume of the magnetometer cell and relying on diffusion to transport polarized atoms allows a magnetometer to be operated with minimal sensitivity to the AC-Stark field.

physics.atom-ph

High efficiency preparation of single trapped atoms using blue detuned light assisted collisions

We report on a procedure by which we obtain a 91% loading efficiency of single 85Rb atoms in an optical microtrap. This can be achieved within a total preparation time of 542 ms. We employ blue detuned light assisted collisions to realize a process in which only one of the collision partners is lost. We explain the mechanism for efficiently loading a single atom and discuss the factors that limit the final efficiency.

physics.atom-ph

Excitation Suppression Due to Interactions Between Microwave-Dressed Rydberg Atoms

Atom-atom interactions within a small volume were investigated through the excitation of ultracold Rb atoms. The application of microwaves enhances these interactions, causing the suppression of Rydberg state excitation. The suppression of Rydberg atom excitation was both qualitatively observed and quantitatively analyzed using a universal scaling law, giving a measure of the atom-atom interaction strength in agreement with theoretical prediction.

physics.atom-ph

Fidelity of a Rydberg blockade quantum gate from simulated quantum process tomography

We present a detailed error analysis of a Rydberg blockade mediated controlled-NOT quantum gate between two neutral atoms as demonstrated recently in Phys. Rev. Lett. 104, 010503 (2010) and Phys. Rev. A 82, 030306 (2010). Numerical solutions of a master equation for the gate dynamics, including all known sources of technical error, are shown to be in good agreement with experiments. The primary sources of gate error are identified and suggestions given for future improvements. We also present numerical simulations of quantum process tomography to find the intrinsic fidelity, neglecting technical errors, of a Rydberg blockade controlled phase gate. The gate fidelity is characterized using trace overlap and trace distance measures. We show that the trace distance is linearly sensitive to errors arising from the finite Rydberg blockade shift and introduce a modified pulse sequence which corrects the linear errors. Our analysis shows that the intrinsic gate error extracted from simulated quantum process tomography can be under 0.002 for specific states of $^{87}$Rb or Cs atoms. The relation between the process fidelity and the gate error probability used in calculations of fault tolerance thresholds is discussed.

quant-ph

Formation of van der Waals molecules in buffer gas cooled magnetic traps

We show that a large class of helium-containing cold polar molecules form readily in a cryogenic buffer gas, achieving densities as high as 10^12 cm^-3. We explore the spin relaxation of these molecules in buffer gas loaded magnetic traps, and identify a loss mechanism based on Landau-Zener transitions arising from the anisotropic hyperfine interaction. Our results show that the recently observed strong T^6 thermal dependence of spin change in buffer gas trapped silver (Ag) is accounted for by the formation and spin change of AgHe, thus providing evidence for molecular formation in a buffer gas trap.

physics.atom-ph

Effects of Nitrogen Quenching Gas on Spin-Exchange Optical Pumping of He-3

We consider the degree of conservation of nuclear spin polarization in the process of optical pumping under typical spin-exchange optical pumping conditions. Previous analyses have assumed that negligible nuclear spin precession occurs in the brief periods of time the alkali-metal atoms are in the excited state after absorbing photons and before undergoing quenching collisions with nitrogen molecules. We include excited-state hyperfine interactions, electronic spin relaxation in collisions with He and N_2, spontaneous emission, quenching collisions, and a simplified treatment of radiation trapping.

physics.atom-ph

Circular Dichroism of RbHe and RbN$_2$ Molecules

We present measurements of the circular dichroism of optically pumped Rb vapor near the D1 resonance line. Collisions with the buffer gases $^3$He and N$_2$ reduce the transparency of the vapor, even when fully polarized. We use two methods to measure this effect, show that the He results can be understood from RbHe potential curves, and show how this effect conspires with the spectral profile of the optical pumping light to increase the laser power demands for optical pumping of very optically thick samples.

physics.atom-ph

Deterministic entanglement of two neutral atoms via Rydberg blockade

We demonstrate the first deterministic entanglement of two individually addressed neutral atoms using a Rydberg blockade mediated controlled-NOT gate. Parity oscillation measurements reveal an entanglement fidelity of $F=0.58\pm0.04$, which is above the entanglement threshold of $F=0.5$, without any correction for atom loss, and $F=0.71\pm0.05$ after correcting for background collisional losses. The fidelity results are shown to be in good agreement with a detailed error model.

quant-ph