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T. Hogan

Publications and source records attributed to T. Hogan.

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Extraordinary physical properties of superconducting YBa$_{1.4}$Sr$_{0.6}$Cu$_3$O$_6$Se$_{0.51}$ in a multiphase ceramic material

We report on a novel material obtained by modifying pristine YBCO superconductor in solid phase synthesis via simultaneous partial substitution of Ba by Sr and O by Se. Simultaneous application of EDX and EBSD confirmed that Se atoms indeed enter the crystalline lattice cell. The detailed XRD analysis further confirmed this conclusion and revealed that the obtained polycrystalline material contains 5 phases, with the major phase ($>$30\%) being a cuprate YBa$_{1.4}$Sr$_{0.6}$Cu$_{3}$O$_{6}$Se$% _{0.51}$. The obtained superconductor demonstrates unique properties, including i) two superconducting transitions with $T_{c1}\approx$ 35 K (granular surface phase) and $T_{c2}\approx$ 13 K (bulk granular phase) - this granular phase arrangement naturally yields the Wohlleben effect; ii) reentrant diamagnetism and resistive state; iii) strong paramagnetism with Curie-Weiss behavior (% $\theta_{CW} \approx$ 4 K) and the ferromagnetic phase overruled by superconductivity; iv) Schottky anomaly visible in the heat capacity data and most likely delivered by small clusters of magnetic moments. Thorough analysis of the heat capacity data reveals a strong-coupling $d-$wave pairing in its bulk phase (with $2\Delta /T_{c}\approx 5$), and, most importantly, a very unusual anomaly in this cuprate. There are reasons to associate this anomaly with the quantum criticality observed in traditional cuprate superconductors at much higher fields (achievable only in certain laboratories). In our case, the fields leading to quantum criticality are much weaker ($\sim $7-9 T) thus opening avenues for exploration of the interplay between superconductivity and pair density waves by the wider research community.

cond-mat.supr-con

A charge density wave-like instability in a doped spin-orbit-assisted weak Mott insulator

Layered perovskite iridates realize a rare class of Mott insulators that are predicted to be strongly spin-orbit coupled analogues of the parent state of cuprate high-temperature superconductors. Recent discoveries of pseudogap, magnetic multipolar ordered and possible $d$-wave superconducting phases in doped Sr$_2$IrO$_4$ have reinforced this analogy among the single layer variants. However, unlike the bilayer cuprates, no electronic instabilities have been reported in the doped bilayer iridate Sr$_3$Ir$_2$O$_7$. Here we show that Sr$_3$Ir$_2$O$_7$ realizes a weak Mott state with no cuprate analogue by using ultrafast time-resolved optical reflectivity to uncover an intimate connection between its insulating gap and antiferromagnetism. However, we detect a subtle charge density wave-like Fermi surface instability in metallic electron doped Sr$_3$Ir$_2$O$_7$ at temperatures ($T_{DW}$) close to 200 K via the coherent oscillations of its collective modes, which is reminiscent of that observed in cuprates. The absence of any signatures of a new spatial periodicity below $T_{DW}$ from diffraction, scanning tunneling and photoemission based probes suggests an unconventional and possibly short-ranged nature of this density wave order.

cond-mat.str-el

Fermi Arcs vs. Fermi Pockets in Electron-doped Perovskite Iridates

We report on an angle resolved photoemission (ARPES) study of bulk electron-doped perovskite iridate, (Sr1-xLax)3Ir2O7. Fermi surface pockets are observed with a total electron count in keeping with that expected from La substitution. Depending on the energy and polarization of the incident photons, these pockets show up in the form of disconnected "Fermi arcs", reminiscent of those reported recently in surface electron-doped Sr2IrO4. Our observed spectral variation is consistent with the coexistence of an electronic supermodulation with structural distortion in the system.

cond-mat.str-el

Spectroscopic evidence for negative electronic compressibility in a quasi-three-dimensional spin-orbit correlated metal

Negative compressibility is a sign of thermodynamic instability of open or non-equilibrium systems. In quantum materials consisting of multiple mutually coupled subsystems, the compressibility of one subsystem can be negative if it is countered by positive compressibility of the others. Manifestations of this effect have so far been limited to low-dimensional dilute electron systems. Here we present evidence from angle-resolved photoemission spectroscopy (ARPES) for negative electronic compressibility (NEC) in the quasi-three-dimensional (3D) spin-orbit correlated metal (Sr1-xLax)3Ir2O7. Increased electron filling accompanies an anomalous decrease of the chemical potential, as indicated by the overall movement of the deep valence bands. Such anomaly, suggestive of NEC, is shown to be primarily driven by the lowering in energy of the conduction band as the correlated bandgap reduces. Our finding points to a distinct pathway towards an uncharted territory of NEC featuring bulk correlated metals with unique potential for applications in low-power nanoelectronics and novel metamaterials.

cond-mat.str-el

Effect of carrier concentration on magnetism and magnetic order in the pyrochlore iridates

We present resistivity, magnetization, and zero field muon spin relaxation ($μ$SR) data for the pyrochlore iridate materials Nd$_{2-x}$Ca$_{x}$Ir$_{2}$O$_{7}$ ($x = 0, 0.06$, and $0.10$) and Sm$_2$Ir$_2$O$_7$. While Nd$_{2}$Ir$_{2}$O$_{7}$ (Nd227) is weakly conducting, Sm$_{2}$Ir$_{2}$O$_{7}$ (Sm227) has slowly diverging resistivity at low temperature. Nd227 and Sm227 exhibit magnetic anomalies at $T_{M} = 105 K$ and $137 K$, respectively. However, zero-field $μ$SR measurements show that long-range magnetic order of the Ir$^{4+}$ sublattice sets in at much lower temperatures ($T_{LRO} \sim 8 K$ for Nd227 and $70 K$ for Sm227); both materials show heavily damped muon precession with a characteristic frequency near 9 MHz. The magnetic anomaly at $T_{M}$ in Nd227 is not significantly affected by the introduction of hole carriers by Ca-substitution in the conducting Nd$_{2-x}$Ca$_{x}$Ir$_{2}$O$_{7}$ samples, but the muon precession is fully suppressed for both.

cond-mat.str-el