arXiv subjects

T. Katabuchi

Publications and source records attributed to T. Katabuchi.

7 recordsLinked to original sources

arXiv2024

Radiative neutron capture cross section of $^{242}$Pu measured at n_TOF-EAR1 in the unresolved resonance region up to 600 keV

Accurate neutron capture cross sections are essential for the design and operation of fast reactors using MOX fuels. For $^{242}$Pu, the Nuclear Energy Agency (NEA) recommends 8--12% accuracy in the fast energy region (2--500 keV), compared to the current uncertainty of 35%. Moreover, integral experiments and previous measurements suggest the evaluated $^{242}$Pu(n,$\gamma$) cross section is overestimated, particularly in the JEFF-3.3 library, which shows a 14% overestimation between 1 keV and 1 MeV. Recent measurements from LANSCE reported a 20--30% reduction in the 1--40 keV range relative to evaluations. To solve these discrepancies, the $^{242}$Pu(n,$\gamma$) cross section was measured from 1 to 600 keV at CERN n_TOF-EAR1 facility using a 95(4) mg $^{242}$Pu target, enriched to 99.959%. Gamma rays from neutron capture were detected with an array of C$_6$D$_6$ scintillators and a novel application of the Pulse Height Weighting Technique was employed. The resulting cross section presents a systematic uncertainty between 8 and 12%, reducing the current uncertainties of 35\% and achieving the accuracy requested by the NEA. Analysis using FITACS produced average resonance parameters, consistent with the analysis of the resolved resonance region. Our data align well with Wisshak and Kaeppeler, and are 10--14\% lower than JEFF-3.3 in the 1--250 keV range, helping to achieve consistency with integral benchmarks. At higher energies, our results are in reasonable agreement with ENDF/B-VIII.1 and JEFF-3.3. In contrast, DANCE results appear to underestimate the cross section by a factor of 2--3 above a few keV.

nucl-ex↗

arXiv2022

Muonic X-Ray Measurement for the Nuclear Charge Distribution: the Case of Stable Palladium Isotopes

Background: The nuclear charge radius and distribution are the most fundamental quantities of the atomic nucleus. From the muonic transition energies, the absolute charge radius has been experimentally obtained, while there have been no established methods to discuss the distribution. Purpose: The muonic transition energies for five palladium isotopes with the mass number $A = 104$, $105$, $106$, $108$ and $110$ were measured. The procedure to deduce the charge radii and the method to discuss the charge distribution from the muonic transition energies are proposed. Method: The experiment was performed at the MuSIC-M1 beamline at Research Center for Nuclear Physics, Osaka University. A continuous muon beam impinged on the enriched palladium targets. Muonic X rays were measured by high-purity germanium detectors. Results: The muonic transition energies up to $4f$-$3d$ transitions were determined for five palladium isotopes. Discussion and conclusion: The root-mean-square charge radii are deduced assuming the two-parameter Fermi distribution. The charge distribution of the nucleus is discussed employing the Barrett model. The muonic transition energies of the $3d$-$2p$ transitions are crucial to discuss both the charge radius and the charge distribution.

nucl-ex↗

arXiv2019

Quenching of gamma0 transition results from p-wave neutron inducing doorway mechanism

Gamma-strength function essentially distinguishes the reaction mechanisms of charged particle inelastic and neutron capture reactions, reflecting from the ratios of transition of neutron capture to low-lying states. The extraordinary quenching of gamma_0 transition of p-wave neutron resonance reaction in 3s-region nucleus 57Fe is observed, for the first time, due to the non-forming 2p-1h doorway state activation which raises the strong intensities of gamma_1 and gamma_2. The enhancement of low energy gamma-strength function doesn't emerge in the neutron capture reaction resulting from the population of cascade transitions of low-lying states rather than primary transitions. The astrophysical reaction rates that are extracted from total and partial neutron capture cross sections of 57Fe might be adopted to constrain the abundance of the successive heavier isotopes in s-process.

nucl-ex↗

arXiv2018

The $^{7}$Be($\boldsymbol{n,p}$)$^{7}$Li reaction and the Cosmological Lithium Problem: measurement of the cross section in a wide energy range at n_TOF (CERN)

We report on the measurement of the $^{7}$Be($n, p$)$^{7}$Li cross section from thermal to approximately 325 keV neutron energy, performed in the high-flux experimental area (EAR2) of the n\_TOF facility at CERN. This reaction plays a key role in the lithium yield of the Big Bang Nucleosynthesis (BBN) for standard cosmology. The only two previous time-of-flight measurements performed on this reaction did not cover the energy window of interest for BBN, and showed a large discrepancy between each other. The measurement was performed with a Si-telescope, and a high-purity sample produced by implantation of a $^{7}$Be ion beam at the ISOLDE facility at CERN. While a significantly higher cross section is found at low-energy, relative to current evaluations, in the region of BBN interest the present results are consistent with the values inferred from the time-reversal $^{7}$Li($p, n$)$^{7}$Be reaction, thus yielding only a relatively minor improvement on the so-called Cosmological Lithium Problem (CLiP). The relevance of these results on the near-threshold neutron production in the p+$^{7}$Li reaction is also discussed.

nucl-ex↗

arXiv2018

The $^{7}$Be(n,p)$^{7}$Li reaction and the Cosmological Lithium Problem: measurement of the cross section in a wide energy range at n_TOF (CERN)

We report on the measurement of the $^{7}$Be($n, p$)$^{7}$Li cross section from thermal to approximately 325 keV neutron energy, performed in the high-flux experimental area (EAR2) of the n_TOF facility at CERN. This reaction plays a key role in the lithium yield of the Big Bang Nucleosynthesis (BBN) for standard cosmology. The only two previous time-of-flight measurements performed on this reaction did not cover the energy window of interest for BBN, and showed a large discrepancy between each other. The measurement was performed with a Si-telescope, and a high-purity sample produced by implantation of a $^{7}$Be ion beam at the ISOLDE facility at CERN. While a significantly higher cross section is found at low-energy, relative to current evaluations, in the region of BBN interest the present results are consistent with the values inferred from the time-reversal $^{7}$Li($p, n$)$^{7}$Be reaction, thus yielding only a relatively minor improvement on the so-called Cosmological Lithium Problem (CLiP). The relevance of these results on the near-threshold neutron production in the p+$^{7}$Li reaction is also discussed.

nucl-ex↗

arXiv2016

Experimental setup and procedure for the measurement of the 7Be(n,α)α reaction at n_TOF

The newly built second experimental area EAR2 of the n_TOF spallation neutron source at CERN allows to perform (n, charged particles) experiments on short-lived highly radioactive targets. This paper describes a detection apparatus and the experimental procedure for the determination of the cross-section of the 7Be(n,α) reaction, which represents one of the focal points toward the solution of the cosmological Lithium abundance problem, and whose only measurement, at thermal energy, dates back to 1963. The apparently unsurmountable experimental difficulties stemming from the huge 7Be γ-activity, along with the lack of a suitable neutron beam facility, had so far prevented further measurements. The detection system is subject to considerable radiation damage, but is capable of disentangling the rare reaction signals from the very high background. This newly developed setup could likely be useful also to study other challenging reactions requiring the detectors to be installed directly in the neutron beam.

physics.ins-det↗

arXiv2010

Spin-Correlation Coefficients and Phase-Shift Analysis for p+$^3$He Elastic Scattering

Angular Distributions for the target spin-dependent observables A$_{0y}$, A$_{xx}$, and A$_{yy}$ have been measured using polarized proton beams at several energies between 2 and 6 MeV and a spin-exchange optical pumping polarized $^3$He target. These measurements have been included in a global phase-shift analysis following that of George and Knutson, who reported two best-fit phase-shift solutions to the previous global p+$^3$He elastic scattering database below 12 MeV. These new measurements, along with measurements of cross-section and beam-analyzing power made over a similar energy range by Fisher \textit{et al.}, allowed a single, unique solution to be obtained. The new measurements and phase-shifts are compared with theoretical calculations using realistic nucleon-nucleon potential models.

nucl-ex↗