arXiv subjects

T. Kibédi

Publications and source records attributed to T. Kibédi.

17 recordsLinked to original sources

arXiv2023

Shape polarization in the tin isotopes near $N=60$ from precision $g$-factor measurements on short-lived $11/2^-$ isomers

The $g$ factors of $11/2^-$ isomers in semimagic $^{109}$Sn and $^{111}$Sn (isomeric lifetimes $τ= 2.9(3)$ ns and $τ= 14.4(7)$ ns, respectively) were measured by an extension of the Time Differential Perturbed Angular Distribution technique, which uses \LaBr detectors and the hyperfine fields of a gadolinium host to achieve precise measurements in a new regime of short-lived isomers. The results, $g(11/2^-; {^{109}\textrm{Sn}}) = -0.186(8)$ and $g(11/2^-; {^{111}\textrm{Sn}}) = -0.214(4)$, are significantly lower in magnitude than those of the $11/2^-$ isomers in the heavier isotopes and depart from the value expected for a near pure neutron $h_{11/2}$ configuration. Broken-symmetry density functional theory calculations applied to the sequence of $11/2^-$ states reproduce the magnitude and location of this deviation. The $g(11/2^-)$ values are affected by shape core polarization; the odd $0h_{11/2}$ neutron couples to $J^π=2^+,4^+,6^+...$ configurations in the weakly-deformed effective core, causing a decrease in the $g$-factor magnitudes.

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arXiv2023

Direct measurement of hexacontatetrapole, $\textbf{E6}$ γ decay from $^{\textbf{53m}}$Fe

The only proposed observation of a discrete, hexacontatetrapole ($E6$) transition in nature occurs from the T$_{1/2}$ = 2.54(2)-minute decay of $^{53m}$Fe. However, there are conflicting claims concerning its $γ$-decay branching ratio, and a rigorous interrogation of $γ$-ray sum contributions is lacking. Experiments performed at the Australian Heavy Ion Accelerator Facility were used to study the decay of $^{53m}$Fe. For the first time, sum-coincidence contributions to the weak $E6$ and $M5$ decay branches have been firmly quantified using complementary experimental and computational methods. Agreement across the different approaches confirms the existence of the real $E6$ transition; the $M5$ branching ratio and transition rate have also been revised. Shell model calculations performed in the full $pf$ model space suggest that the effective proton charge for high-multipole, $E4$ and $E6$, transitions is quenched to approximately two-thirds of the collective $E2$ value. Correlations between nucleons may offer an explanation of this unexpected phenomenon, which is in stark contrast to the collective nature of lower-multipole, electric transitions observed in atomic nuclei.

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arXiv2022

Electric monopole transition from the superdeformed band in $^{40}$Ca

The electric monopole ($E0$) transition strength $ρ^2$ for the transition connecting the third 0$^+$ level, a "superdeformed" band head, to the "spherical" 0$^+$ ground state in doubly magic $^{40}$Ca has been determined via $e^+e^-$ pair-conversion spectroscopy. The measured value, $ρ^2(E0; 0^+_3 \to 0^+_1)~=~2.3(5)\times10^{-3}$, is the smallest $ρ^2(E0; 0^+ \to 0^+)$ found in $A<50$ nuclei. In contrast, the $E0$ transition strength to the ground state observed from the second 0$^+$ state, a band head of "normal" deformation, is an order of magnitude larger, $ρ^2(E0; 0^+_2 \to 0^+_1)~=~25.9(16)\times~10^{-3}$, which shows significant mixing between these two states. Large-Scale Shell Model (LSSM) calculations were performed to understand the microscopic structure of the excited states, and the configuration mixing between them; experimental $ρ^2$ values in $^{40}$Ca and neighboring isotopes were well reproduced by the LSSM calculations. The unusually small $ρ^2(E0; 0^+_3 \to 0^+_1)$ value is due to destructive interference in the mixing of shape-coexisting structures, which are based on several different multiparticle-multihole excitations. This observation goes beyond the usual treatment of $E0$ strengths, where two-state shape mixing cannot result in destructive interference.

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arXiv2020

The radiative width of the Hoyle state from $γ$-ray spectroscopy

The cascading 3.21 MeV and 4.44 MeV electric quadrupole transitions have been observed from the Hoyle state at 7.65 MeV excitation energy in $^{12}$C, excited by the $^{12}$C(p,p$^{\prime}$) reaction at 10.7 MeV proton energy. From the proton-$γ$-$γ$ triple coincidence data, a value of ${Γ_{\rm rad}}/Γ=6.2(6) \times 10^{-4}$ was obtained for the radiative branching ratio. Using our results, together with ${Γ_π^{E0}}/Γ$ from Eriksen et al., Phys. Rev. C 102, 024320 and the currently adopted $Γ_π(E0)$ values, the radiative width of the Hoyle state is determined as $Γ_{\rm rad}=5.1(6) \times 10^{-3}$ eV. This value is about 34% higher than the currently adopted value and will impact on models of stellar evolution and nucleosynthesis.

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arXiv2020

Improved precision on the experimental E0 decay branching ratio of the Hoyle state

Stellar carbon synthesis occurs exclusively via the $3α$ process, in which three $α$ particles fuse to form $^{12}$C in the excited Hoyle state, followed by electromagnetic decay to the ground state. The Hoyle state is above the $α$ threshold, and the rate of stellar carbon production depends on the radiative width of this state. The radiative width cannot be measured directly, and must instead be deduced by combining three separately measured quantities. One of these quantities is the $E0$ decay branching ratio of the Hoyle state, and the current $10$\% uncertainty on the radiative width stems mainly from the uncertainty on this ratio. The $E0$ branching ratio was deduced from a series of pair conversion measurements of the $E0$ and $E2$ transitions depopulating the $0^+_2$ Hoyle state and $2^+_1$ state in $^{12}$C, respectively. The excited states were populated by the $^{12}$C$(p,p^\prime)$ reaction at 10.5 MeV beam energy, and the pairs were detected with the electron-positron pair spectrometer, Super-e, at the Australian National University. The deduced branching ratio required knowledge of the proton population of the two states, as well as the alignment of the $2^+_1$ state in the reaction. For this purpose, proton scattering and $γ$-ray angular distribution experiments were also performed. An $E0$ branching ratio of $Γ^{E0}_π/Γ=8.2(5)\times10^{-6}$ was deduced in the current work, and an adopted value of $Γ^{E0}_π/Γ=7.6(4)\times10^{-6}$ is recommended based on a weighted average of previous literature values and the new result. The new recommended value for the $E0$ branching ratio is about 14% larger than the previous adopted value of $Γ^{E0}_π/Γ=6.7(6)\times10^{-6}$, while the uncertainty has been reduced from 9% to 5%.

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arXiv2020

Emerging nuclear collectivity in $^{124-130}$Te

The emergence of nuclear collectivity near doubly-magic $^{132}$Sn was explored along the stable, even-even $^{124-130}$Te isotopes. Preliminary measurements of the $B(E2;4^{+}_{1}\rightarrow2^{+}_{1})$ transition strengths are reported from Coulomb excitation experiments primarily aimed at measuring the $g$ factors of the $4^{+}_{1}$ states. Isotopically enriched Te targets were excited by 198-205 MeV $^{58}$Ni beams. A comparison of transition strengths obtained is made to large-scale shell-model calculations with successes and limitations discussed.

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arXiv2019

Table of electronic factors for E0 electron and electron-positron pair conversion transitions

A new tabulation of electronic factors is reported for electron conversion for elements of Z from 5 to 126 and electronic factors for electron-positron pair conversion for elements of even Z from 4 to 100. The electronic factors for electron conversion, $Ω_{CE}$(E0), were calculated using a modified version of the CATAR program developed by Pauli and Raff with a relativistic-Hartree-Fock-Slater approach (Pauli and Raff, 1975). The electronic factors for electron-positron pair conversion, $Ω_{IPF}$(E0), were calculated using the model developed by Wilkinson (1969). The data tables presented here cover all atomic shells up to R2 and transition energies from 1 keV to 6000 keV and from 1100 keV to 8000 keV for pair conversion. A comparison with previous electronic factor tabulations is presented. Ratios of experimental Ω(E0) values for 83 E0 transitions in 8$\leq$Z$\leq$98 are compared to this tabulation. Two examples of how to use the tabulation to extract E0 strengths are also included.

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arXiv2019

First-excited state $g$ factors in the stable, even Ge and Se isotopes

Transient-field $g$-factor measurements in inverse kinematics were performed for the first-excited states of the stable, even isotopes of Ge and Se. The $g$ factors of $^{74}$Ge and $^{74}$Se were measured simultaneously using a cocktail beam, which eliminates most possible sources of systematic error in a relative $g$-factor measurement. The results are $g(^{74}{\rm Se})/g(^{74}{\rm Ge})=1.34(7)$, $g(^{70}{\rm Ge})/g(^{74}{\rm Ge}) = 1.16(15)$, $g(^{72}{\rm Ge})/g(^{74}{\rm Ge})=0.92(13)$, $g(^{76}{\rm Ge})/g(^{74}{\rm Ge})=0.88(5)$, $g(^{76}{\rm Se})/g(^{74}{\rm Se})=0.96(7)$, $g(^{78}{\rm Se})/g(^{74}{\rm Se})=0.82(5)$, $g(^{80}{\rm Se})/g(^{74}{\rm Se})=0.99(7)$ and $g(^{82}{\rm Se})/g(^{74}{\rm Se})=1.19(6)$. The measured $g$-factor ratios are in agreement with ratios from previous measurements, despite considerable variation in previous reported absolute values. The absolute values of the $g$ factors remain uncertain, however the Rutgers parametrization was used to set the transient-field strength and then compare the experimental $g$ factors with shell-model calculations based on the JUN45 and jj44b interactions. Modest agreement was found between experiment and theory for both interactions. The shell model calculations indicate that the $g(2^+_1)$ values and trends are determined largely by the balance of the spin carried by orbital motion of the protons.

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arXiv2019

Spectroscopy and excited-state $g$~factors in weakly collective ${^{111}}$Cd: confronting collective and microscopic models

The even cadmium isotopes near the neutron midshell have long been considered good examples of vibrational nuclei. However, the vibrational nature of these nuclei has been questioned based on E2 transition rates that are not consistent with vibrational excitations. In the neighbouring odd-mass nuclei, the g factors of the low-excitation collective states have been shown to be more consistent with a deformed rotational core than a vibrational core. Beyond the comparison of vibrational versus rotational models, recent advances in computational power have made shell-model calculations feasible for Cd isotopes, which may give insights into the emergence and nature of collectivity in the Cd isotopes. Collective excitations in the A ~ 100 region were studied through magnetic moments and electromagnetic transitions in 111Cd. The spectroscopy of 111Cd has been studied following Coulomb excitation. Angular correlation measurements, transient-field g-factor measurements and lifetime measurements by the Doppler-broadened line shape method were performed. The structure of the nucleus was explored in relation to particle-vibration versus particle-rotor interpretations. Large-scale shell-model calculations were performed with the SR88MHJM Hamiltonian. Excited-state g factors have been measured, spin assignments examined and lifetimes determined. Attention was given to the reported $5/2^{+}$ 753-keV and $3/2^{+}$ 755-keV states. The $3/2^{+}$ 755-keV level was not observed; evidence is presented that the reported $3/2^+$ state was a misidentification of the $5/2^{+}$ 753-keV state. It is shown that the g factors and level structure of 111Cd are not readily explained by the particle-vibration model. A particle-rotor approach has both successes and limitations. The shell-model approach successfully reproduces much of the known low-excitation structure in 111Cd.

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arXiv2018

Influence of host matrices on krypton electron binding energies and KLL Auger transition energies

The low-energy electron spectra emitted in the radioactive decay of the $^{83}$Rb and $^{83}$Sr isotopes were measured with a combined electrostatic electron spectrometer. Radioactive sources used were prepared by ion implantation of $^{83}$Sr into a high purity polycrystalline platinum foil at 30 keV and by vacuum-evaporation deposition of $^{83}$ Rb on the same type of foil. From the measured conversion electron spectra, the electron binding energies (referenced to the Fermi level) for the K, L$_1$ , L$_2$ , L$_3$ , M$_1$ , M$_2$, and M$_3$ shell/subshells of krypton in the platinum host were determined to be 14 316.4(12), 1 914.3(9), 1 720.3(9), 1 667.6(9), 281.5(9), 209.6(13), and 201.2(15) eV, respectively, and those for the evaporated layer were observed to be lower by 0.7(1) eV. For both host matrices, values of 2.3(2), 4.6(2), 1.7(2), 1.3(2), and 3.2(3) eV were obtained for the krypton K, L$_1$ , L$_2$ , L$_3$ , and M$_1$ natural atomic level widths, respectively. The absolute energies of 10 838.5(9) and 10 839.5(10) eV were measured for the KL$_2$L$_3$ ($^{1}$D$_2$) Auger transition in krypton implanted in Pt and generated in the evaporated rubidium layer, respectively. A value of 601.0(8) eV was measured for the energy difference of the KL$_2$L$_3$ ($^{1}$D$_2$) transitions in Rb and Kr in the Pt host. Multiconfiguration Dirac-Fock calculations of the krypton KLL transition energies and intensities were also performed.

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arXiv2018

Search for environmental effects on the KLL Auger spectrum of rubidium generated in radioactive decay

The KLL Auger spectrum of rubidium following the electron capture decay of $^{83}$Sr and $^{85}$Sr isotopes was experimentally studied in detail for the first time using one $^{83}$Sr source and three $^{85}$Sr sources in different host matrices. Energies, relative intensities, and natural widths of all the nine well-resolved basic spectrum components were determined and compared with both predictions and experimental data for krypton. Results of our multiconfiguration Dirac-Fock calculations demonstrated an influence of the "atomic structure effect" on absolute energies of the KLL transitions following the creation of initial vacancies by the electron capture decay. Environmental effects on the KLL Auger spectrum were distinctly observed only for the absolute transition energies.

physics.atom-ph↗

arXiv2018

Probing the $N = 14$ subshell closure: $g$ factor of the $^{26}$Mg(2$^+_1$) state

The first-excited state $g$~factor of $^{26}$Mg has been measured relative to the $g$ factor of the $^{24}$Mg($2^+_1$) state using the high-velocity transient-field technique, giving $g=+0.86\pm0.10$. This new measurement is in strong disagreement with the currently adopted value, but in agreement with the $sd$-shell model using the USDB interaction. The newly measured $g$ factor, along with $E(2^+_1)$ and $B(E2)$ systematics, signal the closure of the $νd_{5/2}$ subshell at $N=14$. The possibility that precise $g$-factor measurements may indicate the onset of neutron $pf$ admixtures in first-excited state even-even magnesium isotopes below $^{32}$Mg is discussed and the importance of precise excited-state $g$-factor measurements on $sd$~shell nuclei with $N\neq Z$ to test shell-model wavefunctions is noted.

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arXiv2018

Measurement of the intensity ratio of Auger and conversion electrons for the electron capture decay of $^{125}$I

Auger electrons emitted after nuclear decay have potential application in targeted cancer therapy. For this purpose it is important to know the Auger electron yield per nuclear decay. In this work we describe a measurement of the ratio of the number of conversion electrons (emitted as part of the nuclear decay process) to the number of Auger electrons (emitted as part of the atomic relaxation process after the nuclear decay) for the case of $^{125}$I. Results are compared with Monte-Carlo type simulations of the relaxation cascade using the BrIccEmis code. Our results indicate that for $^{125}$I the calculations based on rates from the Evaluated Atomic Data Library (EADL) underestimate the K Auger yields by 20\%.

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arXiv2018

Identification of significant $E0$ strength in the $2^+_2 \rightarrow 2^+_1$ transitions of $^{58, 60, 62}$Ni

The $E0$ transition strength in the $2^+_2 \rightarrow 2^+_1$ transitions of $^{58,60,62}$Ni have been determined for the first time following a series of measurements at the Australian National University (ANU) and the University of Kentucky (UK). The CAESAR Compton-suppressed HPGe array and the Super-e solenoid at ANU were used to measure the $δ(E2/M1)$ mixing ratio and internal conversion coefficient of each transition following inelastic proton scattering. Level half-lives, $δ(E2/M1)$ mixing ratios and $γ$-ray branching ratios were measured at UK following inelastic neutron scattering. The new spectroscopic information was used to determine the $E0$ strengths. These are the first $2^+ \rightarrow 2^+$ $E0$ transition strengths measured in nuclei with spherical ground states and the $E0$ component is found to be unexpectedly large; in fact, these are amongst the largest $E0$ transition strengths in medium and heavy nuclei reported to date.

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arXiv2018

High-spin spectroscopy and shell-model interpretation of the N < 126 radium isotopes $^{212}$Ra and $^{213}$Ra

The level structures of $^{212}$Ra and $^{213}$Ra have been established via time-correlated $γ$-ray spectroscopy following the $^{204}$Pb($^{12}$C,4$n$)$^{212}$Ra and $^{204}$Pb($^{13}$C,4$n$)$^{213}$Ra reactions. In $^{212}$Ra, levels up to $\sim 6.2$ MeV were identified and firm spin-parity assignments were achieved to a $J^π = 19^+$ isomer with a mean life of 31(3) ns. For $^{213}$Ra the corresponding values were $\sim 4.5$ MeV in excitation energy and $J^π = 33/2^+$. Two isomeric states with $J^π= 23/2^+$, $τ= 27(3)$ ns and $J^π= 33/2^+$, $τ= 50(3)$ ns were discovered in $^{213}$Ra. The experimental data were compared with semiempirical shell-model calculations, which allowed dominant configurations to be assigned to most of the observed levels.

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arXiv2011

Measured g factors and the tidal-wave description of transitional nuclei near A = 100

The transient-field technique has been used in both conventional kinematics and inverse kinematics to measure the g factors of the 2+ states in the stable even isotopes of Ru, Pd and Cd. The statistical precision of the g(2+) values has been significantly improved, allowing a critical comparison with the tidal-wave version of the cranking model recently proposed for transitional nuclei in this region.

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arXiv2011

Conversion coefficients for superheavy elements

In this paper we report on internal conversion coefficients for Z = 111 to Z = 126 superheavy elements obtained from relativistic Dirac-Fock (DF) calculations. The effect of the atomic vacancy created during the conversion process has been taken into account using the so called "Frozen Orbital" approximation. The selection of this atomic model is supported by our recent comparison of experimental and theoretical conversion coefficients across a wide range of nuclei. The atomic masses, valence shell electron configurations, and theoretical atomic binding energies required for the calculations were adopted from a critical evaluation of the published data. The new conversion coefficient data tables presented here cover all atomic shells, transition energies from 1 keV up to 6000 keV, and multipole orders of 1 to 5. A similar approach was used in our previous calculations [1] for Z = 5 - 110.

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