arXiv subjects

T. Möller

Publications and source records attributed to T. Möller.

At least 37 records · Page 2Linked to original sources

arXiv2021

Herschel observations of extraordinary sources: Full Herschel/HIFI molecular line survey of Sagittarius B2(M)

We present a full analysis of a broadband spectral line survey of Sagittarius B2 (Main), one of the most chemically rich regions in the Galaxy located within the giant molecular cloud complex Sgr B2 in the Central Molecular Zone. Our goal is to derive the molecular abundances and temperatures of the high-mass star-forming region Sgr B2(M) and thus its physical and astrochemical conditions. Sgr B2(M) was observed using the Heterodyne Instrument for the Far-Infrared (HIFI) on board the Herschel Space Observatory in a spectral line survey from 480 to 1907 GHz at a spectral resolution of 1.1 MHz, which provides one of the largest spectral coverages ever obtained toward this high-mass star-forming region in the submillimeter with high spectral resolution and includes frequencies > 1 THz unobservable from the ground. We model the molecular emission from the submillimeter to the far-IR using the XCLASS program. For each molecule, a quantitative description was determined taking all emission and absorption features of that species across the entire spectral range into account. Additionally, we derive velocity resolved ortho / para ratios for those molecules for which ortho and para resolved molecular parameters are available. Finally, the temperature and velocity distributions are analyzed and the derived abundances are compared with those obtained for Sgr B2(N) from a similar HIFI survey. A total of 92 isotopologues were identified, arising from 49 different molecules, ranging from free ions to complex organic compounds and originating from a variety of environments from the cold envelope to hot and dense gas within the cores. Sulfur dioxide, methanol, and water are the dominant contributors. For the ortho / para ratios we find deviations from the high temperature values between 13 and 27 %. In total 14 % of all lines remain unidentified.

astro-ph.GA↗

arXiv2021

The physical and chemical structure of high-mass star-forming regions. Unraveling chemical complexity with the NOEMA large program "CORE"

We use sub-arcsecond resolution ($\sim$0.4$''$) observations with NOEMA at 1.37 mm to study the dust emission and molecular gas of 18 high-mass star-forming regions. We combine the derived physical and chemical properties of individual cores in these regions to estimate their ages. The temperature structure of these regions are determined by fitting H2CO and CH3CN line emission. The density profiles are inferred from the 1.37 mm continuum visibilities. The column densities of 11 different species are determined by fitting the emission lines with XCLASS. Within the 18 observed regions, we identify 22 individual cores with associated 1.37 mm continuum emission and with a radially decreasing temperature profile. We find an average temperature power-law index of q = 0.4$\pm$0.1 and an average density power-law index of p = 2.0$\pm$0.2 on scales on the order of several 1 000 au. Comparing these results with values of p derived in the literature suggest that the density profiles remain unchanged from clump to core scales. The column densities relative to N(C18O) between pairs of dense gas tracers show tight correlations. We apply the physical-chemical model MUSCLE to the derived column densities of each core and find a mean chemical age of $\sim$60 000 yrs and an age spread of 20 000-100 000 yrs. With this paper we release all data products of the CORE project available at https://www.mpia.de/core. The CORE sample reveals well constrained density and temperature power-law distributions. Furthermore, we characterize a large variety in molecular richness that can be explained by an age spread confirmed by our physical-chemical modeling. The hot molecular cores show the most emission lines, but we also find evolved cores at an evolutionary stage, in which most molecules are destroyed and thus the spectra appear line-poor again.

astro-ph.GA↗

arXiv2021

Multi-scale view of star formation in IRAS 21078+5211: From clump fragmentation to disk wind

In the massive star-forming region IRAS 21078+5211, a highly fragmented cluster (0.1~pc in size) of molecular cores is observed, located at the density peak of an elongated (1~pc in size) molecular cloud. A small (1~km/s per 0.1~pc) LSR velocity (Vlsr) gradient is detected across the axis of the molecular cloud. Assuming we are observing a mass flow from the harboring cloud to the cluster, we derive a mass infall rate of about 10^{-4}~M_{sun}~yr^{-1}. The most massive cores (labeled 1, 2, and 3) are found at the center of the cluster, and these are the only ones that present a signature of protostellar activity in terms of emission from high-excitation molecular lines or a molecular outflow. We reveal an extended (size about 0.1~pc), bipolar collimated molecular outflow emerging from core 1. We believe this is powered by a (previously discovered) compact (size <= 1000~au) radio jet, ejected by a YSO embedded in core 1 (named YSO-1), since the molecular outflow and the radio jet are almost parallel and have a comparable momentum rate. By means of high-excitation lines, we find a large (14~km/s over 500~au) Vlsr gradient at the position of YSO-1, oriented approximately perpendicular to the radio jet. Assuming this is an edge-on, rotating disk and fitting a Keplerian rotation pattern, we determine the YSO-1 mass to be 5.6+/-2.0~M_{sun}. The water masers (previously observed with VLBI) emerge within 100-300~au from YSO-1 and are unique tracers of the jet kinematics. Their three-dimensional (3D) velocity pattern reveals that the gas flows along, and rotates about, the jet axis. We show that the 3D maser velocities are fully consistent with the magneto-centrifugal disk-wind models predicting a cylindrical rotating jet. Under this hypothesis, we determine the jet radius to be about 16~au and the corresponding launching radius and terminal velocity to be about 2.2~au and 200~km/s, respectively.

astro-ph.GA↗

arXiv2020

The GUAPOS project: G31.41+0.31 Unbiased ALMA sPectral Observational Survey -- I. Isomers of C$_{2}$H$_{4}$O$_{2}$

Understanding the degree of chemical complexity that can be reached in star-forming regions, together with the identification of precursors of the building blocks of life in the interstellar medium, is one of the goals of astrochemistry. Unbiased spectral surveys with large bandwidth and high spectral resolution are thus needed, to resolve line blending in chemically rich sources and identify complex organic molecules. This kind of observations has been successfully carried out, mainly towards the Galactic Center, a region that shows peculiar environmental conditions. We present an unbiased spectral survey at 3mm of one of the most chemically rich hot molecular cores located outside the Galactic Center, in the high-mass star-forming region G31.41+0.31. In this first paper, we present the survey and discuss the detection of the 3 isomers of C$_{2}$H$_{4}$O$_{2}$: methyl formate, glycolaldehyde and acetic acid. Observations were carried out with ALMA and cover the entire Band 3 from 84 to 116 GHz with an angular resolution of $1.2^{''}$x$1.2^{''}$ and a spectral resolution of $\sim0.488$ MHz. The transitions of the 3 molecules have been analyzed with the software XCLASS. All three isomers were detected and methyl formate and acetic acid abundances in G31 are the highest detected up to now, if compared to sources in literature. The size of the emission varies among the three isomers with acetic acid showing the most compact emission while methyl formate the most extended. The comparison with chemical models suggests the necessity of grain-surface routes for the formation of methyl formate in G31, while for glycolaldehyde both scenarios could be feasible. Proposed grain-surface reaction for acetic acid is not able to reproduce the observed abundance in this work, while gas-phase scenario should be further tested due to large uncertainties.

astro-ph.SR↗

arXiv2020

Extended stellar systems in the solar neighborhood. IV. Meingast 1: the most massive stellar stream in the solar neighborhood

Nearby stellar streams carry unique information on the dynamical evolution and disruption of stellar systems in the Galaxy, the mass distribution in the disk, and provide unique targets for planet formation and evolution studies. We revisit the stream discovered in Meingast et al (2019) to search for new members, using Gaia DR2 data and a machine learning approach. We use a bagging classifier of one-class Support Vector Machines to perform a search in positions and proper motions for new stream members. We use the variable prediction frequency resulting from the multitude of classifiers to estimate a stream membership criterion which we use to select high fidelity sources. We use the HR diagram and the Cartesian velocity distribution as test and validation tools. We find about 2000 stream members with high-fidelity, or about an order of magnitude more than previously known, unveiling the stream's population across the entire stellar mass spectrum, from B-stars to M-stars, including white dwarfs. We find that, apart from being slightly more metal-poor, the HRD of the stream is indistinguishable from that of the Pleiades cluster. For the mass range at which we are mostly complete, $\sim$0.2 M$_\odot$ $ < $ M $ < $ $\sim$4 M$_\odot$, we find a normal IMF, allowing us to estimate the total mass of stream to be about 2000 M$_\odot$, making this relatively young stream by far the most massive known. In addition, we identify several white dwarfs as potential stream members. The nearby Meingast 1 stream, due to its richness, age, and distance, is a new fundamental laboratory for star and planet formation and evolution studies for the poorly studied gravitationally unbound star-formation mode. We also demonstrate that One-Class Support Vector Machines can be effectively used to unveil the full stellar populations of nearby stellar systems with Gaia data.

astro-ph.GA↗

arXiv2019

Chemical complexity in high-mass star formation: An observational and modeling case study of the AFGL 2591 VLA 3 hot core

We present a detailed observational and modeling study of the hot core VLA 3 in the high-mass star-forming region AFGL 2591, which is a target region of the NOrthern Extended Millimeter Array (NOEMA) large program CORE. Using NOEMA observations at 1.37 mm with an angular resolution of ~0."42 (1 400 au at 3.33 kpc), we derived the physical and chemical structure of the source. We modeled the observed molecular abundances with the chemical evolution code MUSCLE (MUlti Stage ChemicaL codE). Results. With the kinetic temperature tracers CH3CN and H2CO we observe a temperature distribution with a power-law index of q = 0.41+-0.08. Using the visibilities of the continuum emission we derive a density structure with a power-law index of p = 1.7+-0.1. The hot core spectra reveal high molecular abundances and a rich diversity in complex molecules. The majority of the molecules have an asymmetric spatial distribution around the forming protostar(s), which indicates a complex physical structure on scales < 1 400 au. Using MUSCLE, we are able to explain the observed molecular abundance of 10 out of 14 modeled species at an estimated hot core chemical age of ~21 100 years. In contrast to the observational analysis, our chemical modeling predicts a lower density power-law index of p < 1.4. Reasons for this discrepancy are discussed. Conclusions. Combining high spatial resolution observations with detailed chemical modeling allows us to derive a concise picture of the physical and chemical structure of the famous AFGL 2591 hot core. The next steps are to conduct a similar analysis for the whole CORE sample, and then use this analysis to constrain the chemical diversity in high-mass star formation to a much greater depth.

astro-ph.SR↗

arXiv2019

The Physical and chemical structure of Sagittarius B2 -- IV. Converging filaments in the high-mass cluster forming region Sgr B2(N)

We have used an unbiased, spectral line-survey that covers the frequency range from 211 to 275 GHz and was obtained with ALMA (angular resolution of 0.4 arcsec) to study the small-scale structure of the dense gas in Sagittarius B2 (north). Eight filaments are found converging to the central hub and extending for about 0.1 pc. The spatial structure, together with the presence of the massive central region, suggest that these filaments may be associated with accretion processes. In order to derive the kinematic properties of the gas in a chemically line-rich source like Sgr B2(N), we have developed a new tool that stacks all the detected transition lines of any molecular species. This permits to increase the signal-to-noise ratio of our observations and average out line blending effects, which are a common problem in line-rich regions. We derive velocity gradients along the filaments of about 20-100 km s$^{-1}$ pc$^{-1}$, which are 10-100 times larger than those typically found on larger scales (1 pc) in other star-forming regions. The mass accretion rates of individual filaments are about 0.05 M$_\odot$ yr$^{-1}$, which result in a total accretion rate of 0.16 M$_\odot$ yr$^{-1}$. Some filaments harbor dense cores that are likely forming stars and stellar clusters. The stellar content of these dense cores is on the order of 50% of the total mass. We conclude that the cores may merge in the center when already forming stellar clusters but still containing a significant amount of gas, resulting in a "damp" merger. The high density and mass of the central region, combined with the presence of converging filaments with high mass, high accretion rates and embedded dense cores already forming stars, suggest that Sgr B2(N) may have the potential to evolve into a super stellar cluster.

astro-ph.GA↗

arXiv2018

cellPACKexplorer: Interactive Model Building for Volumetric Data of Complex Cells

Given an algorithm the quality of the output largely depends on a proper specification of the input parameters. A lot of work has been done to analyze tasks related to using a fixed model [25] and finding a good set of inputs. In this paper we present a different scenario, model building. In contrast to model usage the underlying algorithm, i.e. the underlying model, changes and therefore the associated parameters also change. Developing a new algorithm requires a particular set of parameters that, on the one hand, give access to an expected range of outputs and, on the other hand, are still interpretable. As the model is developed and parameters are added, deleted, or changed different features of the outputs are of interest. Therefore it is important to find objective measures that quantify these features. In a model building process these features are prone to change and need to be adaptable as the model changes. We discuss these problems in the application of cellPACK, a tool that generates virtual 3D cells. Our analysis is based on an output set generated by sampling the input parameter space. Hence we also present techniques and metrics to analyze an ensemble of probabilistic volumes.

cs.GR↗

arXiv2016

eXtended CASA Line Analysis Software Suite (XCLASS)

The eXtended CASA Line Analysis Software Suite (XCLASS) is a toolbox for the Common Astronomy Software Applications package (CASA) containing new functions for modeling interferometric and single dish data. Among the tools is the myXCLASS program which calculates synthetic spectra by solving the radiative transfer equation for an isothermal object in one dimension, whereas the finite source size and dust attenuation are considered as well. Molecular data required by the myXCLASS program are taken from an embedded SQLite3 database containing entries from the Cologne Database for Molecular Spectroscopy CDMS) and JPL using the Virtual Atomic and Molecular Data Center (VAMDC) portal. Additionally, the toolbox provides an interface for the model optimizer package Modeling and Analysis Generic Interface for eXternal numerical codes (MAGIX), which helps to find the best description of observational data using myXCLASS (or another external model program), i.e., finding the parameter set that most closely reproduces the data.

astro-ph.IM↗

arXiv2014

Infrared-active phonon modes in monoclinic multiferroic MnWO4

We report on polarized infrared reflectivity measurements of multiferroic, monoclinic MnWO4 between 10K and 295K. The full dielectric tensor and the frequency dependence of the orientation of the principal axes have been determined in the frequency range of the phonons. All infrared-active phonon modes (7 A_u modes and 8 B_u modes) are unambiguously identified. In particular the strongest B_u modes have been overlooked in previous studies, in which the monoclinic symmetry was neglected in the analysis. Using a generalized Drude-Lorentz model, we determine the temperature dependence of the phonon parameters, including the orientation of the B_u modes within the ac plane. The phonon parameters and their temperature dependence have been discussed controversially in previous studies, which do not include a full polarization analysis. Our data does not confirm any of the anomalies reported above 20K. However, in the paramagnetic phase we find a drastic reduction of the spectral weights of the weakest A_u mode and of the weakest B_u mode with increasing temperature. Below 20K, the parameters of the A_u phonon modes for E||b show only subtle changes, which demonstrate a finite but weak coupling between lattice dynamics and magnetism in MnWO4. A quantitative comparison of our infrared data with the quasi-static dielectric constant epsilon_b indicates that the spectral weight of the electromagnon is tiny for E||b, in particular much smaller than the weak changes of the spectral weight of the phonons.

cond-mat.str-el↗

arXiv2013

Magnetic Moments of Chromium-Doped Gold Clusters: The Anderson Impurity Model in Finite Systems

The magnetic moment of a single impurity atom in a finite free electron gas is studied in a combined x-ray magnetic circular dichroism spectroscopy and density functional theory study of size-selected free chromium-doped gold clusters. The observed size-dependence of the local magnetic moment can essentially be understood in terms of the Anderson impurity model. Electronic shell closure in the host metal minimizes the interaction of localized impurity states with the confined free electron gas and preserves the full magnetic moment of $\unit[5]{μ_B}$ in $\mathrm{CrAu}_{2}^{+}$ and $\mathrm{CrAu}_{6}^{+}$ clusters. Even for open-shell species, large local moments are observed that scale with the energy gap of the gold cluster. This indicates that an energy gap in the free electron gas generally stabilizes the local magnetic moment of the impurity.

physics.atm-clus↗

arXiv2013

Coordination-driven magnetic-to-nonmagnetic transition in manganese doped silicon clusters

The interaction of a single manganese impurity with silicon is analyzed in a combined experimental and theoretical study of the electronic, magnetic, and structural properties of manganese-doped silicon clusters. The structural transition from exohedral to endohedral doping coincides with a quenching of high-spin states. For all geometric structures investigated, we find a similar dependence of the magnetic moment on the manganese coordination number and nearest neighbor distance. This observation can be generalized to manganese point defects in bulk silicon, whose magnetic moments fall within the observed magnetic-to-nonmagnetic transition, and which therefore react very sensitively to changes in the local geometry. The results indicate that high spin states in manganese-doped silicon could be stabilized by an appropriate lattice expansion.

physics.atm-clus↗

arXiv2012

Modeling and Analysis Generic Interface for eXternal numerical codes (MAGIX)

The modeling and analysis generic interface for external numerical codes (MAGIX) is a model optimizer developed under the framework of the coherent set of astrophysical tools for spectroscopy (CATS) project. The MAGIX package provides a framework of an easy interface between existing codes and an iterating engine that attempts to minimize deviations of the model results from available observational data, constraining the values of the model parameters and providing corresponding error estimates. Many models (and, in principle, not only astrophysical models) can be plugged into MAGIX to explore their parameter space and find the set of parameter values that best fits observational/experimental data. MAGIX complies with the data structures and reduction tools of ALMA (Atacama Large Millimeter Array), but can be used with other astronomical and with non-astronomical data.

astro-ph.IM↗

arXiv2012

Molecular line survey of the high-mass star-forming region NGC 6334I with Herschel/HIFI and the SMA

We aim at deriving the molecular abundances and temperatures of the hot molecular cores in the high-mass star-forming region NGC 6334I and consequently deriving their physical and astrochemical conditions. In the framework of the Herschel guaranteed time key program CHESS, NGC 6334I is investigated by using HIFI aboard the Herschel Space Observatory. A spectral line survey is carried out in the frequency range 480-1907 GHz, and auxiliary interferometric data from the SMA in the 230 GHz band provide spatial information for disentangling the different physical components contributing to the HIFI spectrum. The spectral lines are identified with the aid of former surveys and spectral line catalogs. The observed spectrum is then compared to a simulated synthetic spectrum with XCLASS, assuming local thermal equilibrium, and best fit parameters are derived using the model optimization package MAGIX. A total of 46 molecules are identified, with 31 isotopologues, resulting in about 4300 emission and absorption lines. High- energy levels of the dominant emitter methanol and vibrationally excited HCN are detected. The number of unidentified lines remains low with 75, or less than 2 percent of the lines detected. The modeling suggests that several spectral features need two or more components to be fitted properly. Other components could be assigned to cold foreground clouds or to outflows, most visible in the SiO emission. A chemical variation between the two embedded hot cores is found, with more N-bearing molecules identified in SMA1 and O-bearing molecules in SMA2. Spectral line surveys give powerful insights into the study of the interstellar medium. Different molecules trace different physical conditions like the inner hot core, the envelope, the outflows or the cold foreground clouds. The derived molecular abundances provide further constraints for astrochemical models.

astro-ph.GA↗

arXiv2010

Herschel observations of extra-ordinary sources: Detecting spiral arm clouds by CH absorption lines

We have observed CH absorption lines ($J=3/2, N=1 \leftarrow J=1/2, N=1$) against the continuum source Sgr~B2(M) using the \textit{Herschel}/HIFI instrument. With the high spectral resolution and wide velocity coverage provided by HIFI, 31 CH absorption features with different radial velocities and line widths are detected and identified. The narrower line width and lower column density clouds show `spiral arm' cloud characteristics, while the absorption component with the broadest line width and highest column density corresponds to the gas from the Sgr~B2 envelope. The observations show that each `spiral arm' harbors multiple velocity components, indicating that the clouds are not uniform and that they have internal structure. This line-of-sight through almost the entire Galaxy offers unique possibilities to study the basic chemistry of simple molecules in diffuse clouds, as a variety of different cloud classes are sampled simultaneously. We find that the linear relationship between CH and H$_2$ column densities found at lower $A_V$ by UV observations does not continue into the range of higher visual extinction. There, the curve flattens, which probably means that CH is depleted in the denser cores of these clouds.

astro-ph.GA↗

arXiv2008

Collective orbital excitations in orbitally ordered YVO3 and HoVO3

We study orbital excitations in the optical absorption spectra of YVO3 and HoVO3. We focus on an orbital absorption band observed at 0.4 eV for polarization E parallel c. This feature is only observed in the intermediate, monoclinic phase. By comparison with the local crystal-field excitations in VOCl and with recent theoretical predictions for the crystal-field levels we show that this absorption band cannot be interpreted in terms of a local crystal-field excitation. We discuss a microscopic model which attributes this absorption band to the exchange of two orbitals on adjacent sites, i.e., to the direct excitation of two orbitons. This model is strongly supported by the observed dependence on polarization and temperature. Moreover, the calculated spectral weight is in good agreement with the experimental result.

cond-mat.str-el↗

arXiv2008

Mott-Hubbard versus charge-transfer behavior in LaSrMnO4 studied via optical conductivity

Using spectroscopic ellipsometry, we study the optical conductivity sigma(omega) of insulating LaSrMnO4 in the energy range of 0.75-5.8 eV from 15 to 330 K. The layered structure gives rise to a pronounced anisotropy. A multipeak structure is observed in sigma_1^a(omega) (2, 3.5, 4.5, 4.9, and 5.5 eV), while only one peak is present at 5.6 eV in sigma_1^c(omega). We employ a local multiplet calculation and obtain (i) an excellent description of the optical data, (ii) a detailed peak assignment in terms of the multiplet splitting of Mott-Hubbard and charge-transfer absorption bands, and (iii) effective parameters of the electronic structure, e.g., the on-site Coulomb repulsion U_eff=2.2 eV, the in-plane charge-transfer energy Delta_a=4.5 eV, and the crystal-field parameters for the d^4 configuration (10 Dq=1.2 eV, Delta_eg=1.4 eV, and Delta_t2g=0.2 eV). The spectral weight of the lowest absorption feature (at 1-2 eV) changes by a factor of 2 as a function of temperature, which can be attributed to the change of the nearest-neighbor spin-spin correlation function across the Neel temperature. Interpreting LaSrMnO4 effectively as a Mott-Hubbard insulator naturally explains this strong temperature dependence, the relative weight of the different absorption peaks, and the pronounced anisotropy. By means of transmittance measurements, we determine the onset of the optical gap Delta^a_opt=0.4-0.45 eV at 15 K and 0.1-0.2 eV at 300 K. Our data show that the crystal-field splitting is too large to explain the anomalous temperature dependence of the c-axis lattice parameter by thermal occupation of excited crystal-field levels. Alternatively, we propose that a thermal population of the upper Hubbard band gives rise to the shrinkage of the c-axis lattice parameter.

cond-mat.str-el↗

arXiv2007

Atomic clusters of various sizes irradiated with short intense pulses of VUV radiation

Non-equilibrium processes following the irradiation of atomic clusters with short pulses of vacuum ultraviolet radiation are modelled using kinetic Boltzmann equations. The dependence of the ionization dynamics on the cluster size is investigated. The predictions on: (i) the maximal and average ion charge created, (ii) ion charge state distribution, (iii) average energy absorbed per atom, (iv) spatial charge distribution, and (v) thermalization scales are obtained for spherical xenon clusters containing: 20, 70, 2500 and 90000 atoms. These clusters were exposed to single rectangular pulses of vacuum ultraviolet radiation of various pulse intensities, I ~ 10^{12}-10^{14} W/cm^2 and durations < 50 fs, at a fixed integrated radiation flux of F=0.4 J/cm^2. The results obtained are found to be in good agreement with the available experimental data, especially the dependence on the cluster size, if it is assumed that the ions from the positively charged outer layer of the cluster constitute the dominant contribution to the experimentally measured ion charge state distribution.

physics.plasm-ph↗