arXiv subjects

T. Martinez

Publications and source records attributed to T. Martinez.

At least 19 recordsLinked to original sources

arXiv2026

Improved $^{94}$Mo neutron resonance parameters from neutron capture and transmission measurements at n_TOF and GELINA

We report high-resolution measurements of the $^{94}\mathrm{Mo}(\mathrm{n},\gamma)^{95}\mathrm{Mo}$ cross section in the neutron energy range from a few eV up to about 250 keV, performed at the n_TOF facility (CERN), and of the $^{94}\mathrm{Mo}(\mathrm{n},\mathrm{tot})$ cross section up to 32 keV, measured at GELINA (JRC Geel). A combined R-matrix analysis of capture and transmission data yields significantly improved neutron-resonance parameters for $^{94}$Mo. A total of 186 resonances were observed in this analysis of which 127 reported here for the first time. The resulting Maxwellian-averaged cross section at stellar temperatures relevant to the slow neutron-capture process (s-process) is approximately 25% lower than previous evaluations and literature values. To assess the astrophysical impact of the revised cross section, we performed s-process nucleosynthesis calculations for low-mass asymptotic giant branch stars. Despite the substantial reduction in the $^{94}\mathrm{Mo}(\mathrm{n},\gamma)^{95}\mathrm{Mo}$ rate, the final yields vary by only 3-4%. This demonstrates that the isotopic budget of $^{94}$Mo in AGB stars is primarily governed by the branching flow at $^{94}\mathrm{Nb}$ rather than by the neutron-capture destruction on $^{94}$Mo itself. The new cross section thus helps disentangle nuclear cross-section uncertainties from branching-flow effects in the s-process production of $^{94}$Mo.

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arXiv2024

A Segmented Total Energy Detector (sTED) optimized for $(n,\gamma)$ cross-section measurements at n_TOF EAR2

The neutron time-of-flight facility n_TOF at CERN is a spallation source dedicated to measurements of neutron-induced reaction cross-sections of interest in nuclear technologies, astrophysics, and other applications. Since 2014, Experimental ARea 2 (EAR2) is operational and delivers a neutron fluence of $4\times 10^7$ neutrons per nominal proton pulse, which is 50 times higher than the one of Experimental ARea 1 (EAR1) of $8\times10^5$ neutrons per pulse. The high neutron flux at EAR2 results in high counting rates in the detectors that challenged the previously existing capture detection systems. For this reason, a Segmented Total Energy Detector (sTED) has been developed to overcome the limitations in the detectors response, by reducing the active volume per module and by using a photomultiplier (PMT) optimized for high counting rates. This paper presents the main characteristics of the sTED, including energy and time resolution, response to $\gamma$-rays, and provides as well details of the use of the Pulse Height Weighting Technique (PHWT) with this detector. The sTED has been validated to perform neutron-capture cross-section measurements in EAR2 in the neutron energy range from thermal up to at least 400 keV. The detector has already been successfully used in several measurements at n_TOF EAR2.

physics.ins-det↗

arXiv2023

Fully three-dimensional sound speed-corrected multi-wavelength photoacoustic breast tomography

Photoacoustic tomography is a contrast agent-free imaging technique capable of visualizing blood vessels and tumor-associated vascularization in breast tissue. While sophisticated breast imaging systems have been recently developed, there is yet much to be gained in imaging depth, image quality and tissue characterization capability before clinical translation is possible. In response, we have developed a hybrid photoacoustic and ultrasound-transmission tomographic system PAM3. The photoacoustic component has for the first time three-dimensional multi-wavelength imaging capability, and implements substantial technical advancements in critical hardware and software sub-systems. The ultrasound component enables for the first time, a three-dimensional sound speed map of the breast to be incorporated in photoacoustic reconstruction to correct for inhomogeneities, enabling accurate target recovery. The results demonstrate the deepest photoacoustic breast imaging to date namely 48 mm, with a more uniform field of view than hitherto, and an isotropic spatial resolution that rivals that of Magnetic Resonance Imaging. The in vivo performance achieved, and the diagnostic value of interrogating angiogenesis-driven optical contrast as well as tumor mass sound speed contrast, gives confidence in the system's clinical potential.

physics.med-ph↗

arXiv2022

Total absorption $\gamma$-ray spectroscopy of the $\beta$ decays of $^{96\text{gs,m}}$Y

The $\beta$ decays of the ground state (gs) and isomeric state (m) of $^{96}$Y have been studied with the total absorption $\gamma$-ray spectroscopy technique at the Ion Guide Isotope Separator On-Line facility. The separation of the 8$^{+}$ isomeric state from the 0$^{-}$ ground state was achieved thanks to the purification capabilities of the JYFLTRAP double Penning trap system. The $\beta$-intensity distributions of both decays have been independently determined. In the analyses the de-excitation of the 1581.6 keV level in $^{96}$Zr, in which conversion electron emission competes with pair production, has been carefully considered and found to have significant impact on the $\beta$-detector efficiency, influencing the $\beta$-intensity distribution obtained. Our results for $^{96\text{gs}}$Y (0$^+$) confirm the large ground state to ground state $\beta$-intensity probability, although a slightly larger value than reported in previous studies was obtained, amounting to $96.6_{-2.1}^{+0.3}\%$ of the total $\beta$ intensity. Given that the decay of $^{96\text{gs}}$Y is the second most important contributor to the reactor antineutrino spectrum between 5 and 7 MeV, the impact of the present results on reactor antineutrino summation calculations has been evaluated. In the decay of $^{96\text{m}}$Y (8$^{+}$), previously undetected $\beta$ intensity in transitions to states above 6 MeV has been observed. This shows the importance of total absorption $\gamma$-ray spectroscopy measurements of $\beta$ decays with highly fragmented de-excitation patterns. $^{96\text{m}}$Y (8$^{+}$) is a major contributor to reactor decay heat in uranium-plutonium and thorium-uranium fuels around 10 s after fission pulses, and the newly measured average $\beta$ and $\gamma$ energies differ significantly from the previous values in evaluated databases (...)

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arXiv2020

Imaging neutron capture cross sections: i-TED proof-of-concept and future prospects based on Machine-Learning techniques

i-TED is an innovative detection system which exploits Compton imaging techniques to achieve a superior signal-to-background ratio in ($n,\gamma$) cross-section measurements using time-of-flight technique. This work presents the first experimental validation of the i-TED apparatus for high-resolution time-of-flight experiments and demonstrates for the first time the concept proposed for background rejection. To this aim both $^{197}$Au($n,\gamma$) and $^{56}$Fe($n, \gamma$) reactions were measured at CERN n\_TOF using an i-TED demonstrator based on only three position-sensitive detectors. Two \cds detectors were also used to benchmark the performance of i-TED. The i-TED prototype built for this study shows a factor of $\sim$3 higher detection sensitivity than state-of-the-art \cds detectors in the $\sim$10~keV neutron energy range of astrophysical interest. This paper explores also the perspectives of further enhancement in performance attainable with the final i-TED array consisting of twenty position-sensitive detectors and new analysis methodologies based on Machine-Learning techniques.

physics.ins-det↗

arXiv2020

Determination of Beta Decay Ground State Feeding of Nuclei of Importance for Reactor Applications

In $\beta$-decay studies the determination of the decay probability to the ground state of the daughter nucleus often suffers from large systematic errors. The difficulty of the measurement is related to the absence of associated delayed $\gamma$-ray emission. In this work we revisit the $4\pi\gamma-\beta$ method proposed by Greenwood and collaborators in the 1990s, which has the potential to overcome some of the experimental difficulties. Our interest is driven by the need to determine accurately the $\beta$-intensity distributions of fission products that contribute significantly to the reactor decay heat and to the antineutrinos emitted by reactors. A number of such decays have large ground state branches. The method is relevant for nuclear structure studies as well. Pertinent formulae are revised and extended to the special case of $\beta$-delayed neutron emitters, and the robustness of the method is demonstrated with synthetic data. We apply it to a number of measured decays that serve as test cases and discuss the features of the method. Finally, we obtain ground state feeding intensities with reduced uncertainty for four relevant decays that will allow future improvements in antineutrino spectrum and decay heat calculations using the summation method.

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arXiv2019

Total absorption $γ$-ray spectroscopy of the $β$-delayed neutron emitters $^{137}$I and $^{95}$Rb

The decays of the $β$-delayed neutron emitters $^{137}$I and $^{95}$Rb have been studied with the total absorption $γ$-ray spectroscopy technique. The purity of the beams provided by the JYFLTRAP Penning trap at the ion guide isotope separator on-line facility in Jyväskylä allowed us to carry out a campaign of isotopically pure measurements with the decay total absorption $γ$-ray spectrometer, a segmented detector composed of eighteen NaI(Tl) modules. The contamination coming from the interaction of neutrons with the spectrometer has been carefully studied, and we have tested the use of time differences between prompt $γ$-rays and delayed neutron interactions to eliminate this source of contamination. Due to the sensitivity of our spectrometer, we have found a significant amount of $β$-intensity to states above the neutron separation energy that de-excite by $γ$-rays, comparable to the neutron emission probability. The competition between $γ$ de-excitation and neutron emission has been compared with Hauser-Feshbach calculations, and it can be understood as a nuclear structure effect. In addition, we have studied the impact of the $β$-intensity distributions determined in this work on reactor decay heat and reactor antineutrino spectrum summation calculations. The robustness of our results is demonstrated by a thorough study of uncertainties, and with the reproduction of the spectra of the individual modules and the module-multiplicity gated spectra. This work represents the state-of-the-art of our analysis methodology for segmented total absorption spectrometers.

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arXiv2019

Total absorption $γ$-ray spectroscopy of niobium isomers

The $β$ intensity distributions of the decays of $^{100\text{gs},100\text{m}}$Nb and $^{102\text{gs},102\text{m}}$Nb have been determined using the Total Absorption $γ$-Ray Spectroscopy technique. The JYFLTRAP double Penning trap system was employed to disentangle the isomeric states involved, lying very close in energy, in a campaign of challenging measurements performed with the Decay Total Absorption $γ$-ray Spectrometer at the Ion Guide Isotope Separator On-Line facility in Jyväskylä. The low-spin isomeric state of each niobium case was populated through the decay of the zirconium parent, that was treated as a contaminant. We have applied a method to extract this contamination, and additionally we have obtained $β$ intensity distributions for these zirconium decays. The $β$-strength distributions evaluated with these results were compared with calculations in quasiparticle random-phase approximation, suggesting a prolate configuration for the ground states of $^{100,102}$Zr. The footprint of the Pandemonium effect was found when comparing our results for the analyses of the niobium isotopes with previous decay data. The $β$-intensities of the decay of $^{102\text{m}}$Nb were obtained for the first time. A careful evaluation of the uncertainties was carried out, and the consistency of our results was validated taking advantage of the segmentation of our spectrometer. The final results were used as input in reactor summation calculations. A large impact on antineutrino spectrum calculations was already reported and here we detail the significant impact on decay heat calculations.

nucl-ex↗

arXiv2018

Characterization and performance of the DTAS detector

DTAS is a segmented total absorption γ-ray spectrometer developed for the DESPEC experiment at FAIR. It is composed of up to eighteen NaI(Tl) crystals. In this work we study the performance of this detector with laboratory sources and also under real experimental conditions. We present a procedure to reconstruct offline the sum of the energy deposited in all the crystals of the spectrometer, which is complicated by the effect of NaI(Tl) light-yield non-proportionality. The use of a system to correct for time variations of the gain in individual detector modules, based on a light pulse generator, is demonstrated. We describe also an event-based method to evaluate the summing-pileup electronic distortion in segmented spectrometers. All of this allows a careful characterization of the detector with Monte Carlo simulations that is needed to calculate the response function for the analysis of total absorption γ-ray spectroscopy data. Special attention was paid to the interaction of neutrons with the spectrometer, since they are a source of contamination in studies of \b{eta}-delayed neutron emitting nuclei.

physics.ins-det↗

arXiv2017

Characterization of a CLYC detector for underground experiments

Large size detectors based on Cs2LiYCl6:Ce (CLYC) are capable of performing a combined $γ$-ray and neutron spectrometry and constitute a promising technology for a wide range of applications in nuclear and high energy physics. Due to their novelty, the comprehensive characterization of the performance of individual CLYC detectors is of great importance for determining their range of applicability. In this work we report on a wide series measurements performed with a commercial 2"x2" CLYC crystal. Good energy and timing resolution values of 4.7% (@ 662 keV) and 1340 ps (FWHM), respectively, were achieved, and a neutron/$γ$ separation figure of merit value of 4.2 was obtained. A dedicated measurement for investigating the intrinsic background of the detector was performed at the Laboratorio Subterráneo de Canfranc (Spain). It evidenced a sizeable contamination in the detector materials which poses limits in the use of CLYC in low background experiments. In addition, detailed Monte Carlo simulations with the GEANT4 toolkit were performed for modeling the response function of the CLYC detector to gamma-rays. An excellent agreement with the experimental data has been achieved.

physics.ins-det↗

arXiv2017

Study of the $β$-decay of $^{100}$Tc with Total Absorption $γ$-Ray Spectroscopy

The \b{eta}-decay of 100 Tc has been studied using the Total Absorption γ-Ray Spectroscopy technique at IGISOL. In this work the new DTAS spectrometer in coincidence with a cylindrical plastic \b{eta} detector has been employed. The \b{eta}-intensity to the ground state obtained from the analysis is in good agreement with previous high-resolution measurements. However, differences in the feeding to the first excited state as well as weak feeding to a new level at high excitation energy have been deduced from this experiment. Theoretical calculations performed in the quasiparticle random- phase approximation (QRPA) framework are also reported. Comparison of these calculations with our measurement serves as a benchmark for calculations of the double \b{eta}-decay of 100 Mo.

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arXiv2016

Characterization of a cylindrical plastic β-detector with Monte Carlo simulations of optical photons

In this work we report on the Monte Carlo study performed to understand and reproduce experimental measurements of a new plastic \b{eta}-detector with cylindrical geometry. Since energy deposition simulations differ from the experimental measurements for such a geometry, we show how the simulation of production and transport of optical photons does allow one to obtain the shapes of the experimental spectra. Moreover, taking into account the computational effort associated with this kind of simulation, we develop a method to convert the simulations of energy deposited into light collected, depending only on the interaction point in the detector. This method represents a useful solution when extensive simulations have to be done, as in the case of the calculation of the response function of the spectrometer in a total absorption γ-ray spectroscopy analysis.

physics.ins-det↗

arXiv2016

Total Absorption Gamma-Ray Spectroscopy of 87Br, 88Br and 94Rb Beta-Delayed Neutron Emitters

We investigate the decay of 87Br, 88Br and 94Rb using total absorption gamma-ray spectroscopy. These important fission products are beta-delayed neutron emitters. Our data show considerable gamma-intensity, so far unobserved in high-resolution gamma-ray spectroscopy, from states at high excitation energy. We also find significant differences with the beta intensity that can be deduced from existing measurements of the beta spectrum. We evaluate the impact of the present data on reactor decay heat using summation calculations. Although the effect is relatively small it helps to reduce the discrepancy between calculations and integral measurements of the photon component for 235U fission at cooling times in the range 1 to 100 s. We also use summation calculations to evaluate the impact of present data on reactor antineutrino spectra. We find a significant effect at antineutrino energies in the range of 5 to 9 MeV. In addition, we observe an unexpected strong probability for gamma emission from neutron unbound states populated in the daughter nucleus. The gamma branching is compared to Hauser-Feshbach calculations which allow one to explain the large value for bromine isotopes as due to nuclear structure. However the branching for 94Rb, although much smaller, hints of the need to increase the radiative width by one order-of-magnitude. This leads to a similar increase in the calculated (n,gamma) cross section for this very neutron-rich nucleus with a potential impact on r-process abundance calculations.

nucl-ex↗

arXiv2016

Experimental setup and procedure for the measurement of the 7Be(n,α)α reaction at n_TOF

The newly built second experimental area EAR2 of the n_TOF spallation neutron source at CERN allows to perform (n, charged particles) experiments on short-lived highly radioactive targets. This paper describes a detection apparatus and the experimental procedure for the determination of the cross-section of the 7Be(n,α) reaction, which represents one of the focal points toward the solution of the cosmological Lithium abundance problem, and whose only measurement, at thermal energy, dates back to 1963. The apparently unsurmountable experimental difficulties stemming from the huge 7Be γ-activity, along with the lack of a suitable neutron beam facility, had so far prevented further measurements. The detection system is subject to considerable radiation damage, but is capable of disentangling the rare reaction signals from the very high background. This newly developed setup could likely be useful also to study other challenging reactions requiring the detectors to be installed directly in the neutron beam.

physics.ins-det↗

arXiv2015

Total Absorption Spectroscopy Study of $^{92}$Rb Decay: A Major Contributor to Reactor Antineutrino Spectrum Shape

The antineutrino spectra measured in recent experiments at reactors are inconsistent with calculations based on the conversion of integral beta spectra recorded at the ILL reactor. $^{92}$Rb makes the dominant contribution to the reactor spectrum in the 5-8 MeV range but its decay properties are in question. We have studied $^{92}$Rb decay with total absorption spectroscopy. Previously unobserved beta feeding was seen in the 4.5-5.5 region and the GS to GS feeding was found to be 87.5(25)%. The impact on the reactor antineutrino spectra calculated with the summation method is shown and discussed.

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arXiv2015

Enhanced Gamma-Ray Emission from Neutron Unbound States Populated in Beta Decay

Total absorption spectroscopy was used to investigate the beta-decay intensity to states above the neutron separation energy followed by gamma-ray emission in 87,88Br and 94Rb. Accurate results were obtained thanks to a careful control of systematic errors. An unexpectedly large gamma intensity was observed in all three cases extending well beyond the excitation energy region where neutron penetration is hindered by low neutron energy. The gamma branching as a function of excitation energy was compared to Hauser-Feshbach model calculations. For 87Br and 88Br the gamma branching reaches 57% and 20% respectively, and could be explained as a nuclear structure effect. Some of the states populated in the daughter can only decay through the emission of a large orbital angular momentum neutron with a strongly reduced barrier penetrability. In the case of neutron-rich 94Rb the observed 4.5% branching is much larger than the calculations performed with standard nuclear statistical model parameters, even after proper correction for fluctuation effects on individual transition widths. The difference can be reconciled introducing an enhancement of one order-of-magnitude in the photon strength to neutron strength ratio. An increase in the photon strength function of such magnitude for very neutron-rich nuclei, if it proved to be correct, leads to a similar increase in the (n,gamma) cross section that would have an impact on r-process abundance calculations.

nucl-ex↗

arXiv2014

Measurement and analysis of the Am-243 neutron capture cross section at the n_TOF facility at CERN

Background:The design of new nuclear reactors and transmutation devices requires to reduce the present neutron cross section uncertainties of minor actinides. Purpose: Reduce the $^{243}$Am(n,$γ$) cross section uncertainty. Method: The $^{243}$Am(n,$γ$) cross section has been measured at the n_TOF facility at CERN with a BaF$_{2}$ Total Absorption Calorimeter, in the energy range between 0.7 eV and 2.5 keV. Results: The $^{243}$Am(n,$γ$) cross section has been successfully measured in the mentioned energy range. The resolved resonance region has been extended from 250 eV up to 400 eV. In the unresolved resonance region our results are compatible with one of the two incompatible capture data sets available below 2.5 keV. The data available in EXFOR and in the literature has been used to perform a simple analysis above 2.5 keV. Conclusions: The results of this measurement contribute to reduce the $^{243}$Am(n,$γ$) cross section uncertainty and suggest that this cross section is underestimated up to 25% in the neutron energy range between 50 eV and a few keV in the present evaluated data libraries.

nucl-ex↗

arXiv2014

$^{62}$Ni($n,γ$) and $^{63}$Ni($n,γ$) cross sections measured at n_TOF/CERN

The cross section of the $^{62}$Ni($n,γ$) reaction was measured with the time-of-flight technique at the neutron time-of-flight facility n_TOF at CERN. Capture kernels of 42 resonances were analyzed up to 200~keV neutron energy and Maxwellian averaged cross sections (MACS) from $kT=5-100$ keV were calculated. With a total uncertainty of 4.5%, the stellar cross section is in excellent agreement with the the KADoNiS compilation at $kT=30$ keV, while being systematically lower up to a factor of 1.6 at higher stellar temperatures. The cross section of the $^{63}$Ni($n,γ$) reaction was measured for the first time at n_TOF. We determined unresolved cross sections from 10 to 270 keV with a systematic uncertainty of 17%. These results provide fundamental constraints on $s$-process production of heavier species, especially the production of Cu in massive stars, which serve as the dominant source of Cu in the solar system.

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