arXiv subjects

T. Mueller

Publications and source records attributed to T. Mueller.

At least 19 recordsLinked to original sources

arXiv2024

SPD deformation of pearlitic, bainitic and martensitic steels

The deformation behavior of nearly fully pearlitic, bainitic and martensitic steels during severe plastic deformation is summarized in this paper. Despite their significantly different yield stresses and their microstructures, their hardening behavior during SPD is similar. Due to the enormous hardening capacity the SPD deformation is limited by the strength of the tool materials. The microstructure at the obtainable limit of strain are quite similar, which is a nanocrystalline structure in the order of 10 nm, dependent on the obtainable strain. The nanograins are partially supersaturated with carbon and the grain boundaries are stabilized by carbon. Another characteristic feature is the anisotropy in grain shape which results in an anisotropy of strength, ductility and fracture toughness. The results are important for the development of ultra-strong materials and essential for this type of steels which are frequently used for application where the behavior under rolling contact and sliding contact is important.

cond-mat.mtrl-sci↗

arXiv2023

Coherent and non-unitary errors in ZZ-generated gates

Variational algorithms such as the Quantum Approximate Optimization Algorithm have attracted attention due to their potential for solving problems using near-term quantum computers. The $ZZ$ interaction typically generates the primitive two-qubit gate in such algorithms applied for a time, typically a variational parameter, $\gamma$. Different compilation techniques exist with respect to the implementation of two-qubit gates. Due to the importance of the $ZZ$-gate, we present an error analysis comparing the continuous-angle controlled phase gate (CP) against the fixed angle controlled $Z$-gate (CZ). We analyze both techniques under the influence of coherent over-rotation and depolarizing noise. We show that CP and CZ compilation techniques achieve comparable $ZZ$-gate fidelities if the incoherent error is below $0.03 \, \%$ and the coherent error is below $0.8 \, \%$. Thus, we argue that for small coherent and incoherent error a non-parameterized two-qubit gate such as CZ in combination with virtual $Z$ decomposition for single-qubit gates could lead to a significant reduction in the calibration required and, therefore, a less error-prone quantum device. We show that above a coherent error of $0.04 \pi$ ($2 \, \%$), the CZ gate fidelity depends significantly on $\gamma$.

quant-ph↗

arXiv2023

Bridging scales with Machine Learning: From first principles statistical mechanics to continuum phase field computations to study order disorder transitions in LixCoO2

LixTMO2 (TM=Ni, Co, Mn) forms an important family of cathode materials for Li-ion batteries, whose performance is strongly governed by Li composition-dependent crystal structure and phase stability. Here, we use LixCoO2 (LCO) as a model system to benchmark a machine learning-enabled framework for bridging scales in materials physics. We focus on two scales: (a) assemblies of thousands of atoms described by density functional theory-informed statistical mechanics, and (b) continuum phase field models to study the dynamics of order-disorder transitions in LCO. Central to the scale bridging is the rigorous, quantitatively accurate, representation of the free energy density and chemical potentials of this material system by coarsegraining formation energies for specific atomic configurations. We develop active learning workflows to train recently developed integrable deep neural networks for such high-dimensional free energy density and chemical potential functions. The resulting, first principles-informed, machine learning-enabled, phase-field computations allow us to study LCO cathodes' phase evolution in terms of temperature, morphology, charge cycling and particle size.

cs.CE↗

arXiv2021

Exploring the Dust Content of Galactic Halos with Herschel. IV. NGC 3079

We present the results from an analysis of deep Herschel far-infrared observations of the edge-on disk galaxy NGC 3079. The PSF-cleaned PACS images at 100 and 160 um display a 25 kpc x 25 kpc X-shape structure centered on the nucleus that is similar in extent and orientation to that seen in Halpha, X-rays, and the far-ultraviolet. One of the dusty filaments making up this structure is detected in the SPIRE 250 um map out to ~25 kpc from the nucleus. The match between the far-infrared filaments and those detected at other wavelengths suggests that the dusty material has been lifted out of the disk by the same large-scale galactic wind that has produced the other structures in this object. A closer look at the central 10 kpc x 10 kpc region provides additional support for this scenario. The dust temperatures traced by the 100-to-160 um flux ratios in this region are enhanced within a biconical region centered on the active galactic nucleus, aligned along the minor axis of the galaxy, and coincident with the well-known double-lobed cm-wave radio structure and Halpha-X-ray nuclear superbubbles. PACS imaging spectroscopy of the inner 6-kpc region reveals broad [C II] 158 um emission line profiles and OH 79 um absorption features along the minor axis of the galaxy with widths well in excess of those expected from beam smearing of the disk rotational motion. This provides compelling evidence that the cool material traced by the [C II] and OH features directly interacts with the nuclear ionized and relativistic outflows traced by the Halpha, X-ray, and radio emission.

astro-ph.GA↗

arXiv2020

Exploring the Dust Content of Galactic Halos with Herschel III. NGC 891

We present deep far-infrared observations of the nearby edge-on galaxy NGC 891 obtained with the Herschel Space Observatory and the Spitzer Space Telescope. The maps confirm the detection of thermal emission from the inner circumgalactic medium (halo) and spatially resolve a dusty superbubble and a dust spur (filament). The dust temperature of the halo component is lower than that of the disk but increases across a region of diameter ~8.0 kpc extending at least 7.7 kpc vertically from one side of the disk, a region we call a superbubble because of its association with thermal X-ray emission and a minimum in the synchrotron scaleheight. This outflow is breaking through the thick disk and developing into a galactic wind, which is of particular interest because NGC 891 is not considered a starburst galaxy; the star formation rate surface density, 0.03 Msun/year per square kiloparsec, and gas fraction, just 10% in the inner disk, indicate the threshold for wind formation is lower than previous work has suggested. We conclude that the star formation surface density is sufficient for superbubble blowout into the halo, but the cosmic ray electrons may play a critical role in determining whether this outflow develops into a fountain or escapes from the gravitational potential. The high dust-to-gas ratio in the dust spur suggests the material was pulled out of NGC 891 through the collision of a minihalo with the disk of NGC 891. We conclude that NGC 891 offers an example of both feedback and satellite interactions transporting dust into the halo of a typical galaxy.

astro-ph.GA↗

arXiv2019

Localized inter-valley defect excitons as single-photon emitters in WSe$_2$

Single-photon emitters play a key role in present and emerging quantum technologies. Several recent measurements have established monolayer WSe$_2$ as a promising candidate for a reliable single photon source. The origin and underlying microscopic processes have remained, however, largely elusive. We present a multi-scale tight-binding simulation for the optical spectra of WSe$_2$ under non-uniform strain and in the presence of point defects employing the Bethe-Salpeter equation. Strain locally shifts excitonic energy levels into the band gap where they overlap with localized intra-gap defect states. The resulting hybridization allows for efficient filing and subsequent radiative decay of the defect states. We identify inter-valley defect excitonic states as the likely candidate for anti-bunched single-photon emission. This proposed scenario is shown to account for a large variety of experimental observations including brightness, radiative transition rates, the variation of the excitonic energy with applied magnetic and electric fields as well as the variation of the polarization of the emitted photon with the magnetic field.

cond-mat.mes-hall↗

arXiv2017

A compact broadband terahertz range quarter-wave plate

We detail the design and characterization of a terahertz range achromatic quarter-wave plate based on a stack of aligned variable thickness birefringent sapphire discs. The disc thicknesses and relative rotations of the discs are determined through a basin-hopping Monte Carlo thermal annealing routine. The basin-hopping scheme allows an improved refinement of the required thicknesses and rotations to give a predicted phase error from the ideal $\pi/2$ of only $0.5 \%$, which is a factor of approximately 6 better than previous efforts. Moreover, the large contrast between extraordinary and ordinary axes of sapphire allow us to greatly decrease the overall optical path length of our wave plate design by approximately a factor of 10 over similar designs based on quartz discs. However, this very same contrast requires very precise tolerances in the milled thicknesses of the discs and their assembly. We detail a method to compensate for differences in the thickness from their calculated ideal values. We have constructed one of our designs and found it similar in performance to other configurations, but with our much more compact geometry.

physics.ins-det↗

arXiv2017

Pseudo-Goldstone magnons in the frustrated S=3/2 Heisenberg helimagnet ZnCr2Se4 with a pyrochlore magnetic sublattice

Low-energy spin excitations in any long-range ordered magnetic system in the absence of magnetocrystalline anisotropy are gapless Goldstone modes emanating from the ordering wave vectors. In helimagnets, these modes hybridize into the so-called helimagnon excitations. Here we employ neutron spectroscopy supported by theoretical calculations to investigate the magnetic excitation spectrum of the isotropic Heisenberg helimagnet ZnCr2Se4 with a cubic spinel structure, in which spin-3/2 magnetic Cr3+ ions are arranged in a geometrically frustrated pyrochlore sublattice. Apart from the conventional Goldstone mode emanating from the (0 0 q) ordering vector, low-energy magnetic excitations in the single-domain proper-screw spiral phase show soft helimagnon modes with a small energy gap of ~0.17 meV, emerging from two orthogonal wave vectors (q 0 0) and (0 q 0) where no magnetic Bragg peaks are present. We term them pseudo-Goldstone magnons, as they appear gapless within linear spin-wave theory and only acquire a finite gap due to higher-order quantum-fluctuation corrections. Our results are likely universal for a broad class of symmetric helimagnets, opening up a new way of studying weak magnon-magnon interactions with accessible spectroscopic methods.

cond-mat.str-el↗

arXiv2017

Role of Spin Flips versus Spin Transport in Non Thermal Electrons Excited by Ultrashort Optical Pulses in Transition Metals

A joint theoretical and experimental investigation is performed to understand the underlying physics of laser-induced demagnetization in Ni and Co films. Experimentally dynamics of spins is studied by determining the time-dependent amplitude of the Voigt vector and theoretically ab-initio calculations are performed using time-dependent density functional theory. We demonstrate that overall spin-orbit induced spin-flips are the most significant contributors with super-diffusive spin transport playing very limited to no role. Our study highlights the material dependent nature of the demagnetization during the process of thermalization of non-equilibrium spins.

cond-mat.mtrl-sci↗

arXiv2015

Online Monitoring of the Osiris Reactor with the Nucifer Neutrino Detector

Originally designed as a new nuclear reactor monitoring device, the Nucifer detector has successfully detected its first neutrinos. We provide the second shortest baseline measurement of the reactor neutrino flux. The detection of electron antineutrinos emitted in the decay chains of the fission products, combined with reactor core simulations, provides an new tool to assess both the thermal power and the fissile content of the whole nuclear core and could be used by the Inter- national Agency for Atomic Energy (IAEA) to enhance the Safeguards of civil nuclear reactors. Deployed at only 7.2m away from the compact Osiris research reactor core (70MW) operating at the Saclay research centre of the French Alternative Energies and Atomic Energy Commission (CEA), the experiment also exhibits a well-suited configuration to search for a new short baseline oscillation. We report the first results of the Nucifer experiment, describing the performances of the 0.85m3 detector remotely operating at a shallow depth equivalent to 12m of water and under intense background radiation conditions. Based on 145 (106) days of data with reactor ON (OFF), leading to the detection of an estimated 40760 electron antineutrinos, the mean number of detected antineutrinos is 281 +- 7(stat) +- 18(syst) electron antineutrinos/day, in agreement with the prediction 277(23) electron antineutrinos/day. Due the the large background no conclusive results on the existence of light sterile neutrinos could be derived, however. As a first societal application we quantify how antineutrinos could be used for the Plutonium Management and Disposition Agreement.

physics.ins-det↗

arXiv2014

Herschel observations of gamma-ray burst host galaxies: implications for the topology of the dusty interstellar medium

Long-duration gamma-ray bursts (GRBs) are indisputably related to star formation, and their vast luminosity in gamma rays pin-points regions of star formation independent of galaxy mass. As such, GRBs provide a unique tool for studying star forming galaxies out to high-z independent of luminosity. Most of our understanding of the properties of GRB hosts (GRBHs) comes from optical and near-infrared (NIR) follow-up observations, and we therefore have relatively little knowledge of the fraction of dust-enshrouded star formation that resides within GRBHs. Currently ~20% of GRBs show evidence of significant amounts of dust along the line of sight to the afterglow through the host galaxy, and these GRBs tend to reside within redder and more massive galaxies than GRBs with optically bright afterglows. In this paper we present Herschel observations of five GRBHs with evidence of being dust-rich, targeted to understand the dust attenuation properties within GRBs better. Despite the sensitivity of our Herschel observations, only one galaxy in our sample was detected (GRBH 070306), for which we measure a total star formation rate (SFR) of ~100Mstar/yr, and which had a relatively high stellar mass (log[Mstar]=10.34+0.09/-0.04). Nevertheless, when considering a larger sample of GRBHs observed with Herschel, it is clear that stellar mass is not the only factor contributing to a Herschel detection, and significant dust extinction along the GRB sightline (A_{V,GRB}>1.5~mag) appears to be a considerably better tracer of GRBHs with high dust mass. This suggests that the extinguishing dust along the GRB line of sight lies predominantly within the host galaxy ISM, and thus those GRBs with A_{V,GRB}>1~mag but with no host galaxy Herschel detections are likely to have been predominantly extinguished by dust within an intervening dense cloud.

astro-ph.GA↗

arXiv2012

Charge order in LuFe2O4: an unlikely route to ferroelectricity

We present the refinement of the crystal structure of charge-ordered LuFe2O4, based on single-crystal x-ray diffraction data. The arrangement of the different Fe-valence states, determined with bond-valence-sum analysis, corresponds to a stacking of charged Fe bilayers, in contrast to the polar bilayers previously suggested. This arrangement is supported by an analysis of x-ray magnetic circular dichroism spectra, which also evidences a strong charge-spin coupling. The non-polar bilayers are inconsistent with charge order based ferroelectricity.

cond-mat.str-el↗

arXiv2011

A critical evaluation of network and pathway based classifiers for outcome prediction in breast cancer

Recently, several classifiers that combine primary tumor data, like gene expression data, and secondary data sources, such as protein-protein interaction networks, have been proposed for predicting outcome in breast cancer. In these approaches, new composite features are typically constructed by aggregating the expression levels of several genes. The secondary data sources are employed to guide this aggregation. Although many studies claim that these approaches improve classification performance over single gene classifiers, the gain in performance is difficult to assess. This stems mainly from the fact that different breast cancer data sets and validation procedures are employed to assess the performance. Here we address these issues by employing a large cohort of six breast cancer data sets as benchmark set and by performing an unbiased evaluation of the classification accuracies of the different approaches. Contrary to previous claims, we find that composite feature classifiers do not outperform simple single gene classifiers. We investigate the effect of (1) the number of selected features; (2) the specific gene set from which features are selected; (3) the size of the training set and (4) the heterogeneity of the data set on the performance of composite feature and single gene classifiers. Strikingly, we find that randomization of secondary data sources, which destroys all biological information in these sources, does not result in a deterioration in performance of composite feature classifiers. Finally, we show that when a proper correction for gene set size is performed, the stability of single gene sets is similar to the stability of composite feature sets. Based on these results there is currently no reason to prefer prognostic classifiers based on composite features over single gene classifiers for predicting outcome in breast cancer.

cs.LG↗

arXiv2010

Design of magnetic traps for neutral atoms with vortices in type-II superconducting micro-structures

We design magnetic traps for atoms based on the average magnetic field of vortices induced in a type-II superconducting thin film. This magnetic field is the critical ingredient of the demonstrated vortex-based atom traps, which operate without transport current. We use Bean's critical-state method to model the vortex field through mesoscopic supercurrents induced in the thin strip. The resulting inhomogeneous magnetic fields are studied in detail and compared to those generated by multiple normally-conducting wires with transport currents. Various vortex patterns can be obtained by programming different loading-field and transport current sequences. These variable magnetic fields are employed to make versatile trapping potentials.

physics.atom-ph↗

arXiv2010

Programmable trap geometries with superconducting atom chips

We employ the hysteretic behavior of a superconducting thin film in the remanent state to generate different traps and flexible magnetic potentials for ultra-cold atoms. The trap geometry can be programmed by externally applied fields. This new approach for atom-optics is demonstrated by three different trap types realized on a single micro-structure: a Z-type trap, a double trap and a bias field free trap. Our studies show that superconductors in the remanent state provide a new versatile platform for atom-optics and applications in ultra-cold quantum gases.

physics.atom-ph↗

arXiv2009

ATLAS Monitored Drift Tube Chambers in E = 11 MeV Neutron Background

The influence of fast neutrons on the occupancy and the single tube resolution of ATLAS muon drift detectors was investigated by exposing a chamber built out of 3 layers of 3 short standard drift tubes to neutron flux-densities of up to 16 kHz/cm2 at a neutron energy of E=11 MeV. Pulse shape capable NE213 scintillaton detectors and a calibrated BF3 neutron detector provided monitoring of the neutron flux-density and energy. The sensitivity of the drift chamber to the neutrons was measured to be 4*10-4 by comparing data sets with and without neutron background. For the investigation of tracks of cosmic muons two silicon-strip detectors above and underneath the chamber allow to compare measured drift-radii with reference tracks. Alternatively, the single tube resolution was determined using the triple-sum method. The comparison between data with and without neutron irradiation shows only a marginal effect on the resolution and little influence on the muon track reconstruction.

physics.ins-det↗

arXiv2009

The role of contacts in graphene transistors: A scanning photocurrent study

A near-field scanning optical microscope is used to locally induce photocurrent in a graphene transistor with high spatial resolution. By analyzing the spatially resolved photo-response, we find that in the n-type conduction regime a p-n-p structure forms along the graphene device due to the doping of the graphene by the metal contacts. The modification of the electronic structure is not limited only underneath the metal electrodes, but extends 0.2-0.3 um into the graphene channel. The asymmetric conduction behavior of electrons and holes that is commonly observed in graphene transistors is discussed in light of the potential profiles obtained from this photocurrent imaging approach. Furthermore, we show that photocurrent imaging can be used to probe single- / multi-layer graphene interfaces.

cond-mat.mes-hall↗

arXiv2008

Photon-Photon Entanglement with a Single Trapped Atom

An experiment is performed where a single rubidium atom trapped within a high-finesse optical cavity emits two independently triggered entangled photons. The entanglement is mediated by the atom and is characterized both by a Bell inequality violation of S=2.5, as well as full quantum-state tomography, resulting in a fidelity exceeding F=90%. The combination of cavity-QED and trapped atom techniques makes our protocol inherently deterministic - an essential step for the generation of scalable entanglement between the nodes of a distributed quantum network.

quant-ph↗