arXiv subjects

T. N. Szegedi

Publications and source records attributed to T. N. Szegedi.

8 recordsLinked to original sources

arXiv2025

Gas-cell development for nuclear astrophysics motivated studies on noble gas targets and the $^3$He($α$,$γ$)$^7$Be reaction

In many astrophysical scenarios, alpha induced reactions on noble gas nuclei play a crucial role. Studying these reactions in the laboratory requires the noble gas atoms to be confined in a sufficient amount to allow the reactions. At Atomki thin-windowed gas-cell targets were developed and improved for studying alpha induced reactions on noble gases. Several stages of the gas-cell design used for activation experiments and lately a version to be used for particle scattering experiments will be presented. A new experimental study of the $^3$He($α$,$γ$)$^7$Be reaction with one of the activation gas-cell targets was performed. This reaction plays an important role both in the solar pp-chains and in big bang nucleosynthesis. The reaction cross section was measured in the past in several works, however, there are still energy regions lacking experimental data, rendering the extrapolations towards the astrophysically relevant energies uncertain. New experimental total cross section of the $^3$He($α$,$γ$)$^7$Be reaction was thus determined here in the energy range of $E_\mathrm{c.m.} = 2600-3000$ keV in about 50 keV energy steps. These results confirm the overall trend, and also the absolute scale set by the only one previous measurement in this energy range. In addition, two pilot experiments with the scattering cell were performed aiming to study the $^4$He($α$,$α$)$^4$He and $^{124}$Xe($α$,$α$)$^{124}$Xe reactions at $E_α= 18$ MeV. These studies benchmark the performance of the cell and detection system both for light and heavy noble gas targets.

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arXiv2023

Experimental determination of the $^3$He($α$,$γ$)$^7$Be reaction cross section above the $^7$Be proton separation threshold

The $^3$He($α$,$γ$)$^7$Be reaction plays a major role both in the BBN producing the majority of the primordial $^7$Li, and in the pp-chain, where it is the branching point. As a few-nucleon system, this reaction is often used to validate ab-initio theoretical calculations and/or test R-matrix theory and code implementations. For the latter, experimental data in an extended energy range is of crucial importance to test the fit and extrapolation capabilities of the different codes. The $^3$He($α$,$γ$)$^7$Be reaction cross section has been measured by several groups up to the first resonance ($E_{c.m.} \approx 3$ MeV) in the reaction. However, only one dataset exists above the $^7$Be proton separation threshold measured in a narrow energy range ($E_{c.m.} = 4.0-4.4$ MeV). In this work we extend the available experimental capture cross section database to the energy range of known $^7$Be levels. The activation method was used. The experiment was performed using a thin-window gas cell with two high-purity Al foils as entrance and exit windows. The activity of the $^7$Be nuclei implanted in the exit/catcher foil was measured by detecting the yield of the emitted $γ$~rays using shielded high-purity germanium detectors. New experimental $^3$He($α$,$γ$)$^7$Be reaction cross section data were obtained for the first time in the $E_{c.m.}=4.3-8.3$ MeV energy region. The new dataset with about 0.2 MeV step covers the energy range of known levels and particle separation thresholds. No prominent structures are observer around the $^7$Be levels. The reaction cross section is slowly increasing with increasing energy. Above the $^6$Li$+p_1$ threshold, a decrease starts in the cross section trend. The overall structure of the cross section suggest a broad resonance peaking around $E_x=7.5$ MeV $^7$Be excitation energy, with a width of 8 MeV.

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arXiv2023

Cross section measurement of the 144Sm(alpha,n)147Gd reaction for studying the alpha-nucleus optical potential at astrophysical energies

Nuclear reactions involving alpha particles play an important role in various astrophysical processes such as the gamma-process of heavy element nucleosynthesis. The poorly known low-energy alpha-nucleus optical (AOMP) potential is a key parameter to estimate the rates of these reactions. The AOMP can be tested by measuring the cross section of alpha-scattering as well as alpha-induced reactions. Low energy elastic alpha-scattering on 144Sm has recently been measured with high precision. The aim of the present work was to complement that work by measuring the (a,n) cross sections on 144Sm at low energies. The experimental data shall be used to constrain the AOMP. From this potential the 144Sm(a,g)148Gd reaction rate can be derived with reduced uncertainties. The 144Sm(a,n)147Gd reaction was studied by bombarding Sm targets with alpha-beams provided by the cyclotron accelerator of Atomki. The cross section was determined using the activation method. The gamma-radiation following the decay of the 147Gd reaction product was measured with a HPGe detector. The experimental data are analyzed within the statistical model. The cross section was measured in the alpha-energy range between 13 and 20 MeV in 1 MeV steps, i.e., from close above the (a,n) threshold. The results were compared with statistical model calculations using various approaches and parametrizations for the AOMP, and excellent agreement was obtained for two recent potentials. However, these potentials cannot reproduce literature data for the 144Sm(a,g)148Gd reaction with the same accuracy. Constraints for the AOMP were derived from an analysis of the new 144Sm(a,n)147Gd data and literature data for 144Sm(a,g)148Gd. These constraints enable a determination of the reaction rate of the 144Sm(a,g)148Gd reaction with significantly reduced uncertainties of less than a factor of two.

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arXiv2021

Low Energy measurement of the $^{96}\mathrm{Zr}(α,n)^{99}\mathrm{Mo}$ reaction cross section and its impact on weak r-process nucleosynthesis

Lighter heavy elements beyond iron and up to around silver can form in neutrino-driven ejecta in core-collapse supernovae and neutron star mergers. Slightly neutron-rich conditions favour a weak r-process that follows a path close to stability. Therefore, the beta decays are slow compared to the expansion time scales, and ($α$,n) reactions become critical to move matter towards heavier nuclei. The rates of these reactions are calculated with the statistical model and their main uncertainty, at energies relevant for the weak r-process, is the $α$+nucleus optical potential. There are several sets of parameters to calculate the $α$+nucleus optical potential leading to large deviations for the reaction rates, exceeding even one order of magnitude. Recently the $^{96}$Zr($α$,n)$^{99}$Mo reaction has been identified as a key reaction that impacts the production of elements from Ru to Cd. Here, we present the first cross section measurement of this reaction at energies (6.22 MeV $\leq$ E$_\mathrm{c.m.}$ $\leq$ 12.47 MeV) relevant for the weak r-process. The new data provide a stringent test of various model predictions which is necessary to improve the precision of the weak r-process network calculations. The strongly reduced reaction rate uncertainty leads to very well-constrained nucleosynthesis yields for $Z = 44 - 48$ isotopes under different neutrino-driven wind conditions.

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arXiv2020

High precision half-life measurement of $^{95}$Ru, $^{95}$Tc and $^{95m}$Tc with $γ$-spectroscopy

The precise knowledge of the half-life of the reaction product is of crucial importance for a nuclear reaction cross section measurement carried out with the activation technique. The cross section of the $^{92}$Mo($α$,n)$^{95}$Ru reaction was measured recently using this experimental approach. The preliminary results indicated that the literature half-life of $^{95}$Ru, derived about half a century ago, is overestimated. Therefore, the half-lives of $^{95}$Ru and its daughter isotope $^{95}$Tc and $^{95m}$Tc have been measured with high precision using $γ$-spectroscopy. The results are t$_{1/2}$=1.6033 $\pm$ 0.0044 h for $^{95}$Ru, t$_{1/2}$ = 19.258 $\pm$ 0.026 h for $^{95}$Tc and t$_{1/2}$ = 61.96 $\pm$ 0.24 d for $^{95m}$Tc. The precision of the half-life values has been increased, consequently the recently measured $^{92}$Mo($α$,n)$^{95}$Ru activation cross section will become more precise.

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arXiv2019

Cross section of $α$-induced reactions on $^{197}$Au at sub-Coulomb energies

Statistical model calculations have to be used for the determination of reaction rates in large-scale reaction networks for heavy-element nucleosynthesis. A basic ingredient of such a calculation is the a-nucleus optical model potential. Several different parameter sets are available in literature, but their predictions of a-induced reaction rates vary widely, sometimes even exceeding one order of magnitude. This paper presents the result of a-induced reaction cross-section measurements on gold which could be carried out for the first time very close to the astrophysically relevant energy region. The new experimental data are used to test statistical model predictions and to constrain the a-nucleus optical model potential. For the measurements the activation technique was used. The cross section of the (a,n) and (a,2n) reactions was determined from g-ray counting, while that of the radiative capture was determined via X-ray counting. The cross section of the reactions was measured below E$_a=20.0$~MeV. In the case of the $^{197}$Au(a,2n)$^{199}$Tl reaction down to 17.5~MeV with 0.5-MeV steps, reaching closer to the reaction threshold than ever before. The cross section of $^{197}$Au(a,n)$^{200}$Tl and $^{197}$Au(a,g)$^{201}$Tl was measured down to E$_a=13.6$ and 14.0~MeV, respectively, with 0.5-MeV steps above the (a,2n) reaction threshold and with 1.0-MeV steps below that. The new dataset is in agreement with the available values from the literature, but is more precise and extends towards lower energies. Two orders of magnitude lower cross sections were successfully measured than in previous experiments which used g-ray counting only, thus providing experimental data at lower energies than ever before. The new precision dataset allows us to find the best-fit a-nucleus optical model potential and to predict cross sections in the Gamow window with smaller uncertainties.

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arXiv2019

Cross section of $^3$He($α$,$γ$)$^7$Be around the $^7$Be proton separation threshold

The $^3$He($α$,$γ$)$^7$Be reaction is a widely studied nuclear reaction; however, it is still not understood with the required precision. It has a great importance both in Big Bang nucleosynthesis and in solar hydrogen burning. The low mass number of the reaction partners makes it also suitable for testing microscopic calculations. Despite the high number of experimental studies, none of them addresses the $^3$He($α$,$γ$)$^7$Be reaction cross sections above 3.1-MeV center-of-mass energy. Recently, a previously unobserved resonance in the $^6$Li(p,$γ$)$^7$Be reaction suggested a new level in $^7$Be, which would also have an impact on the $^3$He($α$,$γ$)$^7$Be reaction in the energy range above 4.0 MeV. The aim of the present experiment is to measure the $^3$He($α$,$γ$)$^7$Be reaction cross section in the energy range of the proposed level. For this investigation the activation technique was used. A thin window gas-cell target confining $^3$He gas was irradiated using an $α$ beam. The $^7$Be produced was implanted into the exit foil. The $^7$Be activity was determined by counting the $γ$ rays following its decay by a well-shielded high-purity germanium detector. Reaction cross sections have been determined between $E_{cm} = 4.0 - 4.4$ MeV with 0.04-MeV steps covering the energy range of the proposed nuclear level. One lower-energy cross-section point was also determined to be able to compare the results with previous studies. A constant cross section of around 10.5 $μ$barn was observed around the $^7$Be proton separation energy. An upper limit of 45 neV for the strength of a $^3$He($α$,$γ$)$^7$Be resonance is derived.

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arXiv2019

High precision half-life measurement of $^{125}$Cs and $^{125}$Xe with γ-spectroscopy

In order to provide data for the simulation of the astrophysical $γ$-process, the cross section measurement of the $^{124}$Xe(p,$γ$)$^{125}$Cs reaction is in progress at MTA Atomki using the activation technique. Precise information on the decay characteristics of the reaction products is of crucial importance for measurements carried out using this method. The half-lives of the produced $^{125}$Cs and its daughter $^{125}$Xe are published in previous works, but with large uncertainties and ambiguous values. To make these nuclear parameters more precise, the half-lives have been re-measured with high precision using $γ$-spectroscopy. The obtained new half-life values are t$_{1/2}$ = 44.35 $\pm$ 0.29 minutes for $^{125}$Cs and t$_{1/2}$ = 16.87 $\pm$ 0.08 hours for $^{125}$Xe.

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