arXiv subjects

T. Otsuka

Publications and source records attributed to T. Otsuka.

At least 19 recordsLinked to original sources

arXiv2026

Regularity of core coupled high-spin structure in neutron-rich $^{196-202}$Au isotopes approaching N $=126$

Excited states built upon long-lived high-spin isomers in hard-to-reach neutron-rich Au ($Z=79$) isotopes were populated using multi-nucleon transfer reactions between $^{136}$Xe and $^{198}$Pt at 7 MeV/u. These states in $^{196,\,198-202}$Au were identified for the first time using the powerful combination of the VAMOS++ spectrometer, the CATLIFE detection system, and the AGATA $γ$-ray tracking array. Their measured energies exhibit remarkable regularity as a function of neutron number and are seen to be inherited from the energies of yrast-band members in the corresponding Hg ($Z=80$) isotope. Large-scale shell-model calculations reproduce the observed regularity and show that these states arise from the unique-parity orbitals $\pi0h_{11/2}$ and $\nu0i_{13/2}$ coupled to the Hg core. This regularity is due to the dominant proton configurations of the Hg and Au isotopes, where the level energies are almost independent of different neutron-orbital occupancies. The calculated Au wave functions show significant higher-spin components of the corresponding Hg core, unlike what is expected in the conventional interpretation in terms of the weak-coupling/decoupling limits of the particle-core coupling model.

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arXiv2026

Sizeable mixing between the coexisting normal and intruder structures of $^{96}$Zr revealed through lifetime measurements

Lifetimes of excited states of the nucleus $^{96}$Zr were studied with the Doppler-shift attenuation method following the $^{94}$Zr($^{18}$O,$^{16}$O)$^{96}$Zr two-neutron transfer reaction. The obtained $B(E2;2^+_2\to0^+_2)$ and $B(E2;4^+_1\to2^+_2)$ transition strengths, amounting to $26(2)$ and $39(7)$\,W.u., respectively, firmly attribute the $2^+_2$ and $4^+_1$ states to the collective intruder band built on top of the $0^+_2$ state. The nature of this structure is discussed against predictions of the collective model using the Bohr Hamiltonian, the interacting boson model with configuration mixing, and the quasiparticle vacua shell model. The collective, interband $B(E2;4^+_1\to2^+_1)=11.2(8)$\,W.u. transition strength, refuting the previously assumed purity of both structures, is reproduced in the calculations. The quasiparticle vacua shell model predicts, in agreement with a simple two-state model based on experimental $E2$ transition strengths, considerable mixing between the normal and intruder $2^+$ states.

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arXiv2026

Triaxiality and Vibrational Modes in Strongly Deformed Nuclei

Low-energy vibrational excitations associated with the fluctuation of quadrupole deformed shapes are discussed within the framework of state-of-the-art Configuration Interaction calculations, actually performed via the Quasi-particle Vacua Shell Model version of the Monte Carlo Shell Model. Recently, low-lying $γ$ bands in heavy strongly deformed nuclei were shown to be rotational $K^P$ = 2$^+$ excitations of triaxially deformed states (see T. Otsuka {\it et al.}, Eur. Phys. J. A 61, 126 (2025)) rather than vibrational excitations as traditionally interpreted. We present additional illustrations as to how the E2 excitation strength to the gamma band changes as the triaxial deformation parameter $γ$ increases, as a systematic indicator for the evolving triaxiality. This is a part of a general formulation of E2 properties of strongly-deformed triaxial states obtained within the quantum many-body scheme. Once the triaxial picture is clarified as a whole, it is important to identify possible low-lying $γ$ and other vibrational excitations and to characterize the excitation energy at which they emerge. Focusing on two typical examples, $^{166}$Er and $^{162}$Dy, vibrational states are indeed identified above the $γ$ band using an extended version of the so-called T-plot. Notable agreement with experiment is seen for the $γ$-vibrational band in $^{166}$Er and for the $β$-vibrational band in $^{162}$Dy, regarding energy levels and $E2$ transitions. The phenomenon of shape coexistence is also shown to produce low-lying states below such vibrational band heads. These results suggest novel and rich structures in heavy deformed nuclei, opening doors to future dedicated studies.

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arXiv2026

Evolution of high-spin states in neutron-rich $^{195-202}$Au isotopes approaching the $N=126$ shell closure

\textbf{Background: } The nuclear structure in the region southwest of the doubly magic $^{208}$Pb is important to benchmark theoretical models relevant for neutron-rich heavy element formation and for the origin of the $A\approx195$ peak in the mass abundance distribution. Although neutron-rich Pb, Tl, and Hg ($Z=80-82$) isotopes are relatively well studied, experimental data for neutron-rich Au isotopes ($Z=79$) remain largely limited due to experimental challenges. \textbf{Purpose: } The purpose of this work is to investigate the evolution of the high-spin structure in neutron-rich Au isotopes near the $N=126$ shell closure and to characterize the underlying shell-model configurations, with a particular focus on the roles of the high-$j$ unique-parity $πh_{11/2}$ and $νi_{13/2}$ orbitals. \textbf{Methods: } Neutron-rich $^{195-202}$Au isotopes were produced using multi-nucleon transfer reactions of $^{198}$Pt($^{136}$Xe, $^{x}$I)$^{y}$Au at a beam energy of 7 MeV/u. %between a 7 MeV/u $^{136}$Xe beam and a $^{198}$Pt target at GANIL. Prompt and delayed $γ$-ray spectroscopy of isotopically identified reaction products was performed with a unique experimental setup combining the VAMOS++ large acceptance magnetic spectrometer, the AGATA HPGe $γ$-ray tracking array, and the CATLIFE detection system.

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arXiv2026

Electromagnetic transition strength in $^{53}$Ca: the lifetime of the $5/2^{-}$ state

High-resolution in-beam $γ$-ray spectroscopy of $^{53}$Ca was performed at the Radioactive Isotope Beam Factory (RIBF) at RIKEN. Excited states in $^{53}$Ca were populated via one-neutron and one-proton removal reactions from a $^{55}$Sc radioactive beam, and the emitted $γ$ rays were detected using the HiCARI hybrid germanium detector array. The lifetime of the first excited $5/2^{-}$ state in $^{53}$Ca was measured for the first time through an analysis of Doppler-roadened $γ$-ray line shapes arising from relativistic recoil velocities. A lifetime of $τ = 11.3_{-11.3}^{+5.3(stat)+3(sys)}$ ps was deduced, corresponding to a reduced transition probability of $B(E2;5/2^{-}{\rightarrow}1/2^{-}) > 2.6 e^{2}fm^{4}$ at the 1$σ$ level, with a best-fit value of $4.5 e^{2}fm^{4}$. The measured transition strength is compared with state-of-the-art shell-model and ab initio calculations, providing a stringent benchmark for shell-model Hamiltonians and effective charges and modern ab initio descriptions of the neutron-rich calcium isotopes approaching the potential $N$ = 40 shell closure.

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arXiv2026

Quenching of the proton $\pi0p_{3/2}$-$\pi0p_{1/2}$ spin-orbit splitting in $^{20}$O and the effect of the tensor force

We present the first direct measurement of the Z=6 shell gap in the neutron-rich 20O nucleus. The one-proton removal transfer reaction 2H(20O,3He)19N has been studied using the ACTAR TPC setup at GANIL. The use of ACTAR TPC enabled the measurement of low-cross section proton-removal reactions while preserving resolution. Eight p-hole states with l=1 were identified in 19N accounting for total strengths of 86% and 72% of the 0p3/2 and 0p1/2 single-particle orbitals, respectively. The energies and spectroscopic factors of the measured states allowed to determine the proton spin-orbit splitting 0p3/2 - 0p1/2 in 20O. The Z=6 shell gap has been established to be 5.30(14) MeV. These findings indicate a reduction of the Z=6 shell gap while adding neutrons to the sd-valence orbitals, consistent with the effects of the tensor force predicted by state-of-the-art shell model interaction SFO-tls while at variance with the emergence of a large Z=6 gap observed in other studies.

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arXiv2026

Lifetime of the $4^+_1$ state of $^{132}$Te

The evolution of the collectivity of tellurium isotopes from mid-shell towards $N=82$ is currently based mainly on properties of the first excited $2^+$ states. To extend structural information in this isotopic chain, in particular with respect to the balance of microscopic, seniority-type and collective excitations, electric quadrupole transition strengths from $4^+$ states need to be considered. An experiment was performed to determine the $4_1^+$ lifetime of $^{132}$Te via the recoil-distance Doppler-shift method at the University of Cologne tandem accelerator. The isotope of interest was populated in the two neutron-transfer reaction $^{130}$Te($^{18}$O,$^{16}$O)$^{132}$Te$^*$. The $E2$ decay transition strength has been determined to be $B(E2; 4^+_1\rightarrow 2^+_1) = 9.3(10)\, \text{W.u.}$ and compares favourably to shell model calculations.

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arXiv2025

Charge Radii Measurements of Exotic Tin Isotopes in the Proximity of $N=50$ and $N=82$

We report nuclear charge radii for the isotopes $^{104-134}$Sn, measured using two different collinear laser spectroscopy techniques at ISOLDE-CERN. These measurements clarify the arch-like trend in charge radii along the isotopic chain and reveal an odd-even staggering that is more pronounced near the $N=50$ and $N=82$ shell closures. The observed local trends are well described by both nuclear density functional theory and valence space in-medium similarity renormalization group calculations. Both theories predict appreciable contributions from beyond-mean-field correlations to the charge radii of the neutron-deficient tin isotopes. The models, however, fall short of reproducing the magnitude of the known $B(E2)$ transition probabilities, highlighting the remaining challenges in achieving a unified description of both ground-state properties and collective phenomena.

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arXiv2025

Isolated one-phonon mixed-symmetry 2+ state of the radioactive neutron-rich nuclide 132Te

The $M1$ transition strengths between excited $2^+$ states of the neutron-rich, radioactive nuclide $^{132}$Te have been studied through direct lifetime measurements using the Doppler-shift attenuation method in a two-neutron transfer reaction on a $^{130}$Te target. An unambiguous identification of the lowest-lying mixed-symmetry $2^+$ state has been achieved on the basis of the large $B(M1;2^+_2\rightarrow2^+_1$)=0.18(2) $μ_\mathrm{N}^2$ transition strength, in agreement with shell-model calculations. Results are compared to the shell model, and the analysis of both, data and calculations, unambiguously identifies the second-excited $2^+$ state of $^{132}$Te as the one-quadrupole phonon mixed-symmetry state of this isotope. A lowering of the energy and $B(M1;2^+_\mathrm{ms}\rightarrow 2^+_1)$ strength within the $N$=80 isotones toward the $Z$=50 shell closure is observed, which goes alongside with the lowering of the $E2$ collectivity approaching the magic proton shell.

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arXiv2025

Unbound neutron $\nu0d_{3/2}$ strength in $^{17}$C and the N=16 shell gap

Significant continuum strength has been observed to be populated in $^{17}$C produced in the d($^{16}$C,p) reaction at a beam energy of 17.2~MeV/nucleon. The strength appears at greater than $\sim$2~MeV above the single-neutron decay threshold and has been identified as arising from transfer into the neutron $0d_{3/2}$ orbital. Guided by shell model predictions the greater majority of the strength is associated with a 3/2$^+$ state at an excitation energy of 4.40$_{-0.14}^{+0.33}$ MeV and a much weaker 3/2$^+$ level at 5.60$_{-0.45}^{+1.35}$ MeV. The corresponding total widths were determined to be 3.45$_{-0.78}^{+1.82}$ and 1.6$_{-1.4}^{+4.6}$ MeV, respectively. From the backward angle proton differential cross sections and the branching ratios for neutron decay to the $^{16}$C(2$_{1}^{+}$) level, the corresponding spectroscopic factors to the ground state were deduced to be 0.47$\pm{10}$ and $<$0.09. Shell-model calculations employing the phenomenological SFO-tls interaction as well as Gamow Shell-Model calculations including continuum effects are in reasonable agreement with experiment, although the predicted strength lies at somewhat lower energy. The size of the N=16 shell gap ($\varepsilon_{ \nu0d_{3/2}}-\varepsilon _{ν1s_{1/2}}$) was estimated to be 5.08$_{-0.33}^{+0.43}$~MeV - some 1.3~MeV larger than found in the SFO-tls shell model calculation.

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arXiv2025

Prevailing Triaxial Shapes in Atomic Nuclei and a Quantum Theory of Rotation of Composite Objects

In the traditional view, heavy deformed nuclei are like axially-symmetric prolate ellipsoids, rotating about one of the short axes. In the present picture, their shapes may be triaxial. The triaxial shape yields complex rotations, which actually well reproduce experimental data, as confirmed by state-of-the-art Configuration Interaction calculations. Two origins are suggested for the triaxiality: (i) binding-energy gain by the symmetry restoration for triaxial shapes, and (ii) another gain by specific components of the nuclear force, like tensor force and high-multipole (e.g. hexadecupole) central force. While the origin (i) produces basic smaller triaxiality for virtually all deformed nuclei, the origin (ii) produces medium triaxiality for a certain class of nuclei. An example of the former is 154Sm, a typical showcase of axial symmetry but is now suggested to depict a modest yet finite triaxiality. The latter, medium triaxiality, is discussed from various viewpoints for some exemplified nuclei including 166Er, and experimental findings. Many-body structures of the gamma band and the double-gamma band are clarified. Regarding the general features of rotational states of deformed many-body systems including triaxial ones, the well-known J(J+1) rule of rotational excitation energies is discussed, within the quantum mechanical many-body theory, without resorting to the quantization of a rotating classical rigid body. The picture of prevailing triaxial shapes thus emerges, where the empirically known rotational-band pattern appears with good K quantum number, but the internal structure is dfferent from conventional picture a la A. Bohr. The possible relations to Davydov's rigid-triaxial-rotor model are mentioned.

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arXiv2025

Refined topology of the N = 20 island of inversion with high precision mass measurements of $^{31-33}$Na and $^{31-35}$Mg

Mass measurements of $^{31-33}$Na and $^{31-35}$Mg using the TITAN MR-TOF-MS at TRIUMF's ISAC facility are presented, with the uncertainty of the $^{33}$Na mass reduced by over two orders of magnitude. The excellent performance of the MR-TOF-MS has also allowed the discovery of a millisecond isomer in $^{32}$Na. The precision obtained shows that the binding energy of the normally closed N = 20 neutron shell reaches a minimum for $^{32}$Mg but increases significantly for $^{31}$Na, hinting at the possibility of enhanced shell strength toward the unbound $^{28}$O. We compare the results with new ab initio predictions that raise intriguing questions of nuclear structure beyond the dripline.

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arXiv2024

Giant Dipole Resonance photofission and photoneutron reactions in $^{238}$U and $^{232}$Th

New measurements of photofission and photoneutron reactions on $^{238}$U and $^{232}$Th in the Giant Dipole Resonance (GDR) energy region have been performed at the laser Compton-scattering $γ$-ray source of the NewSUBARU synchrotron radiation facility using a high-and-flat efficiency moderated $^3$He detection array. The neutron-multiplicity sorting of high-multiplicity fission neutron coincidence events has been performed using a dedicated energy dependent, multiple firing statistical treatment. The photoneutron $(γ,\,in)$ with $i$~=~1~--~3 and photofission $(γ,\,F)$ reactions have been discriminated by considering a Gaussian distribution of prompt-fission-neutron (PFN) multiplicities predicted by the theory of evaporation in sequential neutron emission from excited fission fragments. We report experimental $(γ,\,n)$, $(γ,\,2n)$, $(γ,\,3n)$ and $(γ,\,F)$ cross sections, average energies of PFNs and of $(γ,\,in)$ photoneutrons, as well as the mean number of PFNs per fission act and the width of the PFNs multiplicity distribution. Based on these primary experimental results and combined with reasonable assumptions, we extract also the first- and second-chance fission contributions. The new experimental results are compared with statistical-model calculations performed with the EMPIRE-3.2 Malta and TALYS-1.964 codes on the present data and with prompt fission emission calculations obtained with the Los Alamos model in the frame of the most probable fragmentation approach with and without sequential emission.

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arXiv2023

Level Structures of $^{56,58}$Ca Cast Doubt on a doubly magic $^{60}$Ca

Gamma decays were observed in $^{56}$Ca and $^{58}$Ca following quasi-free one-proton knockout reactions from $^{57,59}$Sc beams at $\approx 200$ MeV/nucleon. For $^{56}$Ca, a $γ$ ray transition was measured to be 1456(12) keV, while for $^{58}$Ca an indication for a transition was observed at 1115(34) keV. Both transitions were tentatively assigned as the $2^+_1 \rightarrow 0^+_{gs}$ decays, and were compared to results from ab initio and conventional shell-model approaches. A shell-model calculation in a wide model space with a marginally modified effective nucleon-nucleon interaction depicts excellent agreement with experiment for $2^+_1$ level energies, two-neutron separation energies, and reaction cross sections, corroborating the formation of a new nuclear shell above the $N$ = 34 shell. Its constituents, the $0f_{5/2}$ and $0g_{9/2}$ orbitals, are almost degenerate. This degeneracy precludes the possibility for a doubly magic $^{60}$Ca and potentially drives the dripline of Ca isotopes to $^{70}$Ca or even beyond.

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arXiv2023

Intruder configurations in $^{29}$Ne at the transition into the island of inversion: Detailed structure study of $^{28}$Ne

Detailed $γ$-ray spectroscopy of the exotic neon isotope $^{28}$Ne has been performed for the first time using the one-neutron removal reaction from $^{29}$Ne on a liquid hydrogen target at 240~MeV/nucleon. Based on an analysis of parallel momentum distributions, a level scheme with spin-parity assignments has been constructed for $^{28}$Ne and the negative-parity states are identified for the first time. The measured partial cross sections and momentum distributions reveal a significant intruder $p$-wave strength providing evidence of the breakdown of the $N=20$ and $N=28$ shell gaps. Only a weak, possible $f$-wave strength was observed to bound final states. Large-scale shell-model calculations with different effective interactions do not reproduce the large $p$-wave and small $f$-wave strength observed experimentally, indicating an ongoing challenge for a complete theoretical description of the transition into the island of inversion along the Ne isotopic chain.

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arXiv2023

Cross-shell states in $^{15}$C: a test for p-sd interactions

The low-lying structure of $^{15}$C has been investigated via the neutron-removal $^{16}$C$(d,t)$ reaction. Along with bound neutron sd-shell hole states, unbound p-shell hole states have been firmly confirmed. The excitation energies and the deduced spectroscopic factors of the cross-shell states are an important measure of the $[(p)^{-1}(sd)^{2}]$ neutron configurations in $^{15}$C. Our results show a very good agreement with shell-model calculations using the SFO-tls interaction for $^{15}$C. However, a modification of the $p$-$sd$ and $sd$-$sd$ monopole terms was applied in order to reproduce the $N=9$ isotone $^{17}$O. In addition, the excitation energies and spectroscopic factors have been compared to the first calculations of $^{15}$C with the $ab~ initio$ self-consistent Green's function method employing the NNLO$_{sat}$ interaction. The results show the sensitivity to the size of the $N=8$ shell gap and highlight the need of going beyond the current truncation scheme in the theory.

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arXiv2022

A new study of the $N=32$ and $N=34$ shell gap for Ti and V by the first high-precision MRTOF mass measurements at BigRIPS-SLOWRI

The atomic masses of $^{55}$Sc, $^{56,58}$Ti, and $^{56-59}$V have been determined using the high-precision multi-reflection time-of-flight technique. The radioisotopes have been produced at RIKEN's RIBF facility and delivered to the novel designed gas cell and multi-reflection system (ZD MRTOF), which has been recently commissioned downstream of the ZeroDegree spectrometer following the BigRIPS separator. For $^{56,58}$Ti and $^{56-59}$V the mass uncertainties have been reduced down to the order of $10\,\mathrm{keV}$, shedding new light on the $N=34$ shell effect in Ti and V isotopes by the first high-precision mass measurements of the critical species $^{58}$Ti and $^{59}$V. With the new precision achieved, we reveal the non-existence of the $N=34$ empirical two-neutron shell gaps for Ti and V, and the enhanced energy gap above the occupied $νp_{3/2}$ orbit is identified as a feature unique to Ca. We perform new Monte Carlo shell model calculations including the $νd_{5/2}$ and $νg_{9/2}$ orbits and compare the results with conventional shell model calculations, which exclude the $νg_{9/2}$ and the $νd_{5/2}$ orbits. The comparison indicates that the shell gap reduction in Ti is related to a partial occupation of the higher orbitals for the outer two valence neutrons at $N=34$.

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arXiv2022

Proton distribution radii of $^{16-24}$O: signatures of new shell closures and neutron skin

The root mean square radii of the proton density distribution in $^{16-24}$O derived from measurements of charge changing cross sections with a carbon target at $\sim$900$A$ MeV together with the matter radii portray thick neutron skin for $^{22 - 24}$O despite $^{22,24}$O being doubly magic. Imprints of the shell closures at $N$ = 14 and 16 are reflected in local minima of their proton radii that provide evidence for the tensor interaction causing them. The radii agree with it ab initio calculations employing the chiral NNLO$_{\mathrm{sat}}$ interaction, though skin thickness predictions are challenged. Shell model predictions agree well with the data.

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