arXiv subjects

T. Ozawa

Publications and source records attributed to T. Ozawa.

9 recordsLinked to original sources

arXiv2026

Hydrogen (deuterium) dynamics and thermal stability in ion-irradiated platinum-hydride thin films synthesized at low temperature

Hydrogen (H) and deuterium (D) interactions with transition metals play a central role in heterogeneous catalysis and hydrogen-related technologies. While H-Pt surface interactions have been extensively studied, direct investigations of hydrogen incorporation and transport in Pt remain limited due to its low solubility. Here, we study H(D) incorporation and desorption dynamics in metastable $PtH(D)_x$ thin films prepared by low-energy ion irradiation, enabling hydrogen loading far above equilibrium concentrations. Nuclear reaction analysis (NRA) reveals a nonuniform hydrogen depth profile with two accumulation regions: the subsurface and the film-substrate interface. Thermal desorption spectroscopy (TDS) exhibits two desorption peaks near 190 and 230 K, consistent with hydrogen release from these sites. Resistance relaxation measurements, analyzed within a two-parallel-channel conduction model, indicate different relaxation kinetics for subsurface and near-interface hydrogen. Arrhenius analysis reveals two thermally activated processes for $PtH_x$ with an average hydrogen concentration of $x = 0.15$, with activation energies of $130 \pm 18$ meV (subsurface) and $164 \pm 26$ meV (near interface). Above 140 K, D exhibits slower relaxation rates with activation energies of $117 \pm 8$ and $121 \pm 7$ meV for $PtD_x$ prepared under the same implantation dose. Within experimental uncertainty, the activation barriers remain comparable, while the prefactors are reduced significantly for D, indicating isotope-dependent attempt frequencies and zero-point energy effects. TDS simulations based on the Polanyi-Wigner formalism reproduce the experimental desorption spectra by resolving subsurface and near-interface contributions, in agreement with the NRA profile. These findings provide insight into hydrogen kinetics in $PtH_x$ for Pt-based catalysis, sensing, and hydrogen-metal interactions.

cond-mat.mtrl-sci↗

arXiv2021

Direct observation of photonic Landau levels and helical edge states in strained honeycomb lattices

We report the realization of a synthetic magnetic field for photons and polaritons in a honeycomb lattice of coupled semiconductor micropillars. A strong synthetic field is induced in both the s and p orbital bands by engineering a uniaxial hopping gradient in the lattice, giving rise to the formation of Landau levels at the Dirac points. We provide direct evidence of the sublattice symmetry breaking of the lowest-order Landau level wavefunction, a distinctive feature of synthetic magnetic fields. Our realization implements helical edge states in the gap between n=0 and n=1 Landau levels, experimentally demonstrating a novel way of engineering propagating edge states in photonic lattices. In light of recent advances in the enhancement of polariton-polariton nonlinearities, the Landau levels reported here are promising for the study of the interplay between pseudomagnetism and interactions in a photonic system.

cond-mat.mes-hall↗

arXiv2020

Semi-Dirac Transport and Anisotropic Localization in Polariton Honeycomb Lattices

Compression dramatically changes the transport and localization properties of graphene. This is intimately related to the change of symmetry of the Dirac cone when the particle hopping is different along different directions of the lattice. In particular, for a critical compression, a semi-Dirac cone is formed with massless and massive dispersions along perpendicular directions. Here we show direct evidence of the highly anisotropic transport of polaritons in a honeycomb lattice of coupled micropillars implementing a semi-Dirac cone. If we optically induce a vacancy-like defect in the lattice, we observe an anisotropically localized polariton distribution in a single sublattice, a consequence of the semi-Dirac dispersion. Our work opens up new horizons for the study of transport and localization in lattices with chiral symmetry and exotic Dirac dispersions.

cond-mat.mes-hall↗

arXiv2018

Tilted and type-III Dirac cones emerging from flat bands in photonic orbital graphene

The extraordinary electronic properties of Dirac materials, the two-dimensional partners of Weyl semimetals, arise from the linear crossings in their band structure. When the dispersion around the Dirac points is tilted, the emergence of intricate transport phenomena has been predicted, such as modified Klein tunnelling, intrinsic anomalous Hall effects and ferrimagnetism. However, Dirac materials are rare, particularly with tilted Dirac cones. Recently, artificial materials whose building blocks present orbital degrees of freedom have appeared as promising candidates for the engineering of exotic Dirac dispersions. Here we take advantage of the orbital structure of photonic resonators arranged in a honeycomb lattice to implement photonic lattices with semi-Dirac, tilted and, most interestingly, type-III Dirac cones that combine flat and linear dispersions. The tilted cones emerge from the touching of a flat and a parabolic band with a non-trivial topological charge. These results open the way to the synthesis of orbital Dirac matter with unconventional transport properties and, in combination with polariton nonlinearities, to the study of topological and Dirac superfluids in photonic lattices.

cond-mat.mes-hall↗

arXiv2018

Measurement of Chern numbers through center-of-mass responses

Probing the center-of-mass of an ultracold atomic cloud can be used to measure Chern numbers, the topological invariants underlying the quantum Hall effects. In this work, we show how such center-of-mass observables can have a much richer dependence on topological invariants than previously discussed. In fact, the response of the center of mass depends not only on the current density, typically measured in a solid-state system, but also on the particle density, which itself can be sensitive to the topology of the band structure. We apply a semiclassical approach, supported by numerical simulations, to highlight the key differences between center-of-mass responses and more standard conductivity measurements. We illustrate this by analyzing both the two- and the four-dimensional quantum Hall effects. These results have important implications for experiments in engineered topological systems, such as ultracold gases and photonics.

cond-mat.quant-gas↗

arXiv2017

Lasing in topological edge states of a 1D lattice

Topology describes properties that remain unaffected by smooth distortions. Its main hallmark is the emergence of edge states localized at the boundary between regions characterized by distinct topological invariants. This feature offers new opportunities for robust trapping of light in nano- and micro-meter scale systems subject to fabrication imperfections and to environmentally induced deformations. Here we show lasing in such topological edge states of a one-dimensional lattice of polariton micropillars that implements an orbital version of the Su-Schrieffer-Heeger Hamiltonian. We further demonstrate that lasing in these states persists under local deformations of the lattice. These results open the way to the implementation of chiral lasers in systems with broken time-reversal symmetry and, when combined with polariton interactions, to the study of nonlinear topological photonics.

cond-mat.mes-hall↗

arXiv2015

Edge states in polariton honeycomb lattices

The experimental study of edge states in atomically-thin layered materials remains a challenge due to the difficult control of the geometry of the sample terminations, the stability of dangling bonds and the need to measure local properties. In the case of graphene, localised edge modes have been predicted in zig-zag and bearded edges, characterised by flat dispersions connecting the Dirac points. Polaritons in semiconductor microcavities have recently emerged as an extraordinary photonic platform to emulate 1D and 2D Hamiltonians, allowing the direct visualization of the wavefunctions in both real- and momentum-space as well as of the energy dispersion of eigenstates via photoluminescence experiments. Here we report on the observation of edge states in a honeycomb lattice of coupled micropillars. The lowest two bands of this structure arise from the coupling of the lowest energy modes of the micropillars, and emulate the π and π* bands of graphene. We show the momentum space dispersion of the edge states associated to the zig-zag and bearded edges, holding unidimensional quasi-flat bands. Additionally, we evaluate polarisation effects characteristic of polaritons on the properties of these states.

cond-mat.mes-hall↗

arXiv2002

Optical Spectropolarimetry of SN 2002ap: High Velocity Asymmetric Explosion

We present spectropolarimetry of the Type Ic supernova SN 2002ap and give a preliminary analysis: the data were taken at two epochs, close to and one month later than the visual maximum (2002 February 8). In addition we present June 9 spectropolarimetry without analysis. The data show the development of linear polarization. Distinct polarization profiles were seen only in the O I λ7773 multiplet/Ca II IR triplet absorption trough at maximum light and in the Ca II IR triplet absorption trough a month later, with the latter showing a peak polarization as high as ~2 %. The intrinsic polarization shows three clear position angles: 80 degs for the February continuum, 120 degs for the February line feature, and 150 degs for the March data. We conclude that there are multiple asymmetric components in the ejecta. We suggest that the supernova has a bulk asymmetry with an axial ratio projected on the sky that is different from 1 by of order 10 %. Furthermore, we suggest very speculatively that a high velocity ejecta component moving faster than ~0.115c (e.g., a jet) contributes to polarization in the February epoch.

astro-ph↗

arXiv2002

A New High-Redshift Lyman alpha Emitter: Possible Superwind Galaxy at z = 5.69

During the course of our deep optical imaging survey for Ly alpha emitters at z approximately 5.7 in the field around the z=5.74 quasar SDSSp J104433.04-012502.2, we have found a candidate strong emission-line source. Follow-up optical spectroscopy shows that the emission line profile of this object is asymmetric, showing excess red-wing emission. These properties are consistent with an identification of Ly alpha emission at a redshift of z=5.687 +/- 0.002. The observed broad line width, Delta V_{FWHM} ~= 340 km s^{-1} and excess red-wing emission also suggest that this object hosts a galactic superwind.

astro-ph↗