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T. P. O'Connor

Publications and source records attributed to T. P. O'Connor.

At least 19 recordsLinked to original sources

$β$-nuclear-recoil correlation from $^6$He decay in a laser trap

We report the first precise measurement of a $β$-recoil correlation from a radioactive noble gas ($^6{\rm He}$) confined via a magneto-optical trap. The measurement is motivated by the search for exotic tensor-type contributions to the charged weak current. Interpreted as tensor currents with right-handed neutrinos, the measurements yield: $|C_T/C_A|^2\le 0.022$ (90\% C.L.). On the other hand, for left-handed neutrinos the limits are $0.007< C_T/C_A <0.111$~(90\%\ C.L.). The sensitivity of the present measurement is mainly limited by experimental uncertainties in determining the time response properties and the distance between the atom cloud and the micro-channel plate used for recoil ion detection.

nucl-ex↗

High Resolution Spectroscopy of Neutral Yb Atoms in a Solid Ne Matrix

We present an experimental and theoretical study of the absorption and emission spectra of Yb atoms in a solid Ne matrix at a resolution of 0.025 nm. Five absorption bands were identified as due to transitions from the $4f^{14}5d^06s^2\ ^1\!S_0$ ground state configuration to $4f^{14}5d^06s6p$ and $4f^{13}5d^16s^2$ configurations. The two lowest energy bands were assigned to outer-shell transitions to $6s6p\ ^3P_1$ and $^1P_1$ atomic states and displayed the structure of a broad doublet and an asymmetric triplet, respectively. The remaining three higher-frequency bands were assigned to inner-shell transitions to distinct $J=1$ states arising from the $4f^{13}5d^16s^2$ configuration and were highly structured with narrow linewidths. A classical simulation was performed to identify the stability and symmetry of possible trapping sites in the Ne crystal. It showed that the overarching 1+2 structure of the high frequency bands could be predominantly ascribed to crystal field splitting in the axial field of a 10-atom vacancy of $C_{4v}$ symmetry. Their prominent substructures were shown to be manifestations of phonon sidebands associated with the zero-phonon lines on each crystal field state. Unprecedented for a metal-rare gas system, resolution of individual phonon states on an allowed electronic transition was possible under excitation spectroscopy which reflects the semi-quantum nature of solid Ne. In contrast to the absorption spectra, emission spectra produced by steady-state excitation into the $^1P_1$ absorption band consisted of simple, unstructured fluorescence bands.

physics.atom-ph↗

Spectroscopic Study and Lifetime Measurement of the $6d7p$ $ ^{3}F_{2}^{o}$ state of radium

We report a method for the precision measurement of the oscillator strengths and the branching ratios of the decay channels of the $6d7p$ $^3F_2$ state in $^{226}$Ra. This method exploits a set of metastable states present in Ra, allowing a measurement of the oscillator strengths that does not require knowledge of the number of atoms in the atomic beam. We measure the oscillator strengths and the branching ratios for decays to the $7s6d$ $^3D_1$, $7s6d$ $^3D_2$, and $7s6d$ $^1D_2$ states and constrain the branching ratio to the $7s6d$ $^3D_3$ state to be less than 0.4$\%$ (68$\%$ confidence limit). The lifetime of the $^3F_2$ state is determined to be $15 \pm 4$ ns.

physics.atom-ph↗

Characterizing the Optical Trapping of Rare Isotopes by Monte Carlo Simulation

Optical trapping techniques are an efficient way to probe limited quantities of rare isotopes. In order to achieve the highest possible measurement precision, it is critical to optimize the optical trapping efficiency. This work presents the development of a three-dimensional semi-classical Monte Carlo simulation of the optical trapping process and its application to optimizing the optical trapping efficiency of Radium for use in the search of the permanent electric dipole moment of $^{225}$Ra. The simulation includes an effusive-oven atomic beam source, transverse cooling and Zeeman slowing of an atomic beam, a three-dimensional magneto-optical trap, and additional processes such as collisions with residual gas molecules. We benchmark the simulation against a well-characterized $^{88}$Sr optical trap before applying it to the $^{225}$Ra optical trap. The simulation reproduces the relative gains in optical trapping efficiency measured in both the $^{88}$Sr and $^{225}$Ra optical traps. The measured and simulated values of the overall optical trapping efficiencies for $^{88}$Sr are in agreement; however, they differ by a factor of $30$ for $^{225}$Ra. Studies of several potential imperfections in the apparatus or systematic effects, such as atomic beam source misalignment and laser frequency noise, show only limited effects on the simulated trapping efficiency for $^{225}$Ra. We rule out any one systematic effect as the sole cause of the discrepancy between the simulated and measured $^{225}$Ra optical trapping efficiencies; but, we do expect that a combination of systematic effects contribute to this discrepancy. The accurate relative gains predicted by the simulation prove that it is useful for testing planned upgrades to the apparatus.

physics.atom-ph↗

Alignment of a Vector Magnetometer to an Optical Prism

A method for alignment of a vector magnetometer to a rigidly attached prism is presented. This enables optical comparison of the magnetometer axes to physical surfaces in an apparatus, and thus an absolute determination of the magnetic field direction in space. This is in contrast with more common techniques, which focus on precise determination of the relative angles between magnetometer axes, and so are more suited to measuring differences in the direction of magnetic fields. Here we demonstrate precision better than 500 $μ$rad on a fluxgate magnetometer, which also gives the coil orthogonality errors to a similar precision. The relative sensitivity of the 3 axes is also determined, with precision of about 5$\times 10^{-4}$.

physics.ins-det↗

Rapid processing of 85Kr/Kr ratios using Atom Trap Trace Analysis

We report a methodology for measuring 85Kr/Kr isotopic abundances using Atom Trap Trace Analysis (ATTA) that increases sample measurement throughput by over an order of magnitude to 6 samples per 24 hours. The noble gas isotope 85Kr (half-life = 10.7 yr) is a useful tracer for young groundwater in the age range of 5-50 years. ATTA, an efficient and selective laser-based atom counting method, has recently been applied to 85Kr/Kr isotopic abundance measurements, requiring 5-10 microliters of krypton gas at STP extracted from 50-100 L of water. Previously a single such measurement required 48 hours. Our new method demonstrates that we can measure 85Kr/Kr ratios with 3-5% relative uncertainty every 4 hours, on average, with the same sample requirements.

physics.ins-det↗

Setting a Limit on Anthropogenic Sources of Atmospheric 81Kr through Atom Trap Trace Analysis

We place a 2.5% limit on the anthropogenic contribution to the modern abundance of 81Kr/Kr in the atmosphere at the 90% confidence level. Due to its simple production and transport in the terrestrial environment, 81Kr (halflife = 230,000 yr) is an ideal tracer for old water and ice with mean residence times in the range of 10^5-10^6 years. In recent years, 81Kr-dating has been made available to the earth science community thanks to the development of Atom Trap Trace Analysis (ATTA), a laser-based atom counting technique. Further upgrades and improvements to the ATTA technique now allow us to demonstrate 81Kr/Kr measurements with relative uncertainties of 1% and place this new limit on anthropogenic 81Kr. As a result of this limit, we have removed a potential systematic constraint for 81Kr-dating.

physics.atom-ph↗

First Measurement of the Atomic Electric Dipole Moment of $^{225}$Ra

The radioactive radium-225 ($^{225}$Ra) atom is a favorable case to search for a permanent electric dipole moment (EDM). Due to its strong nuclear octupole deformation and large atomic mass, $^{225}$Ra is particularly sensitive to interactions in the nuclear medium that violate both time-reversal symmetry and parity. We have developed a cold-atom technique to study the spin precession of $^{225}$Ra atoms held in an optical dipole trap, and demonstrated the principle of this method by completing the first measurement of its atomic EDM, reaching an upper limit of $|$$d$($^{225}$Ra)$|$ $<$ $5.0\!\times\!10^{-22}$ $e \cdot$cm (95$\%$ confidence).

nucl-ex↗

Measurement of the Hyperfine Quenching Rate of the Clock Transition in $^{171}$Yb

We report the first experimental determination of the hyperfine quenching rate of the $6s^2\ ^1\!S_0\ (F=1/2) - 6s6p\ ^3\!P_0\ (F=1/2)$ transition in $^{171}$Yb with nuclear spin $I=1/2$. This rate determines the natural linewidth and the Rabi frequency of the clock transition of a Yb optical frequency standard. Our technique involves spectrally resolved fluorescence decay measurements of the lowest lying $^3\!P_{0,1}$ levels of neutral Yb atoms embedded in a solid Ne matrix. The solid Ne provides a simple way to trap a large number of atoms as well as an efficient mechanism for populating $^3\!P_0$. The decay rates in solid Ne are modified by medium effects including the index-of-refraction dependence. We find the $^3\!P_0$ hyperfine quenching rate to be $(4.42\pm0.35)\times10^{-2}\ \mathrm{s}^{-1}$ for free $^{171}$Yb, which agrees with recent ab initio calculations.

physics.atom-ph↗

Efficient, Tightly-Confined Trapping of 226Ra

We demonstrate a technique for transferring $^{226}$Ra atoms from a 3-dimensional magneto-optical-trap (MOT) into a standing wave optical dipole trap (ODT) in an adjacent chamber. The resulting small trapping volume (120 $μ$m in diameter) allows for high control of the electric and magnetic fields applied to the atoms. The atoms are first transferred to a traveling-wave optical dipole trap, which is then translated 46 cm to a science chamber. The atoms are subsequently transferred into an orthogonal standing-wave ODT by application of a 1-dimensional MOT along the traveling-wave axis. For each stage, transfer efficiencies exceeding 60% are demonstrated.

physics.atom-ph↗

Optical Excitation and Decay Dynamics of Ytterbium Atoms Embedded in a Solid Neon Matrix

Neutral ytterbium atoms embedded in solid neon qualitatively retain the structure of free atoms. Despite the atom-solid interaction, the 6s6p $^3$P$_0$ level is found to remain metastable with its lifetimes determined to be in the range of ten to hundreds of seconds. The atomic population can be almost completely transferred between the ground level and the metastable level via optical excitation and spontaneous decay. The dynamics of this process is examined, and is used to explicitly demonstrate that the transition broadening mechanism is homogeneous.

physics.atom-ph↗

Ar-39 Detection at the 10^-16 Isotopic Abundance Level with Atom Trap Trace Analysis

Atom Trap Trace Analysis (ATTA), a laser-based atom counting method, has been applied to analyze atmospheric Ar-39 (half-life = 269 yr), a cosmogenic isotope with an isotopic abundance of 8x10^-16. In addition to the superior selectivity demonstrated in this work, counting rate and efficiency of ATTA have been improved by two orders of magnitude over prior results. Significant applications of this new analytical capability lie in radioisotope dating of ice and water samples and in the development of dark matter detectors.

physics.atom-ph↗

Nuclear charge radius of $^8$He

The root-mean-square (rms) nuclear charge radius of ^8He, the most neutron-rich of all particle-stable nuclei, has been determined for the first time to be 1.93(3) fm. In addition, the rms charge radius of ^6He was measured to be 2.068(11) fm, in excellent agreement with a previous result. The significant reduction in charge radius from ^6He to ^8He is an indication of the change in the correlations of the excess neutrons and is consistent with the ^8He neutron halo structure. The experiment was based on laser spectroscopy of individual helium atoms cooled and confined in a magneto-optical trap. Charge radii were extracted from the measured isotope shifts with the help of precision atomic theory calculations.

nucl-ex↗

Laser-trapping of Ra-225 and Ra-226 with repumping by room temperature blackbody radiation

We have demonstrated Zeeman slowing and capture of neutral Ra-225 and Ra-226 atoms in a magneto-optical trap (MOT). The intercombination transition 1S0-3P1 is the only quasi-cycling transition in radium and was used for laser-cooling and trapping. Repumping along the 3D1-1P1 transition extended the lifetime of the trap from milliseconds to seconds. Room-temperature blackbody radiation was demonstrated to provide repumping from the metastable 3P0 level. We measured the isotope shift and hyperfine splittings on the 3D1-1P1 transition with the laser-cooled atoms, and set a limit on the lifetime of the 3D1 level based on the measured blackbody repumping rate. Laser-cooled and trapped radium is an attractive system for studying fundamental symmetries.

physics.atom-ph↗

A Thermal Beam of Metastable Krypton Atoms Produced by Optical Excitation

A room-temperature beam of krypton atoms in the metastable 5s[3/2]2 level is demonstrated via an optical excitation method. A Kr-discharge lamp is used to produce VUV photons at 124 nm for the first-step excitation from the ground-level 4p6 1S0 to the 5s[3/2]1 level. An 819 nm Ti:Sapphire laser is used for the second-step excitation from 5s[3/2]1 to 5p[3/2]1, followed by a spontaneous decay to the 5s[3/2]2 metastable level. A metastable atomic beam with an angular flux density of 3 x 10^14 /s/sr is achieved at the total gas flow rate of 0.01 cm^3 STP/s (or 3 x 10^17 atoms/s). The dependences of the flux on the gas flow rate, laser power, and lamp parameters are investigated.

physics.atom-ph↗

Laser Spectroscopic Determination of the 6He Nuclear Charge Radius

We have performed precision laser spectroscopy on individual 6He (t1/2 = 0.8 s) atoms confined and cooled in a magneto-optical trap, and measured the isotope shift between 6He and 4He to be 43,194.772 +/- 0.056 MHz for the 2 3S1 - 3 3P2 transition. Based on this measurement and atomic theory, the nuclear charge radius of 6He is determined, for the first time in a method independent of nuclear models, to be 2.054 +/- 0.014 fm. The result is compared with the values predicted by a number of nuclear structure calculations, and tests their ability to characterize this loosely bound, halo nucleus.

nucl-ex↗

One million year old groundwater in the Sahara revealed by krypton-81 and chlorine-36

Measurements of 81Kr/Kr in deep groundwater from the Nubian Aquifer (Egypt) were performed by a new laser-based atom-counting method. 81Kr ages range from \~2x10^5 to ~1x10^6 yr, correlate with 36Cl/Cl ratios, and are consistent with lateral flow of groundwater from a recharge area near the Uweinat Uplift in SW Egypt. Low delta-2H values of the 81Kr-dated groundwater reveal a recurrent Atlantic moisture source during Pleistocene pluvial periods. These results indicate that the 81Kr method for dating old groundwater is robust and such measurements can now be applied to a wide range of hydrologic problems.

physics.geo-ph↗

Searches for Stable Strangelets in Ordinary Matter: Overview and a Recent Example

Our knowledge on the possible existence in nature of stable exotic particles depends solely upon experimental observation. Guided by this general principle and motivated by theoretical hypotheses on the existence of stable particles of strange quark matter, a variety of experimental searches have been performed. We provide an introduction to the theoretical hypotheses, an overview of the past searches, and a more detailed description of a recent search for helium-like strangelets in the Earth's atmosphere using a sensitive laser spectroscopy method.

nucl-ex↗